具有单个宽带相位成形laser脉冲的多维光谱学
Multidimensional spectroscopy with a single broadband phase-shaped laser pulse
摘要：
本文计算了四阶相位整形可见光脉冲在外场中的频散非线性传输信号。两个相位分布，相位阶跃和相位脉冲，被认为是。本文给出了一个三电子带模型系统，通过改变检测频率和相位参数得到的二维信号。我们演示了如何双光子和受激拉曼共振可以操纵的相位分布和符号，并选择量子路径可以被抑制。
英文摘要：
We calculate the frequency-dispersed nonlinear transmission signal of a phase-shaped visible pulse to fourth order in the field. Two phase profiles, a phase-step and phase-pulse, are considered. Two dimensional signals obtained by varying the detected frequency and phase parameters are presented for a three electronic band model system. We demonstrate how two-photon and stimulated Raman resonances can be manipulated by the phase profile and sign, and selected quantum pathways can be suppressed.
机构、总结、中文摘要均由AI分析而来，可能存在错误，请以论文正文为准。
