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arXiv 1406.7344cond-mat.mes-hallphysics.optics
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扭曲双层石墨烯中鞍点激子的光学声子共振

Optical-phonon resonances with saddle-point excitons in twisted-bilayer graphene

Ado Jorio, Mark Kasperczyk, Nick Clark, Elke Neu, Patrick Maletinsky, Aravind Vijayaraghavan, Lukas Novotny

摘要:

扭曲双层石墨烯(tBLG)在态密度中表现出范霍夫奇异性,其可以通过改变扭曲角$θ$来调节。一个$θ$定义的tBLG已被生产和其特征在于与光学反射率和共振拉曼散射。的$θ$工程的光学响应被证明是一致的持久鞍点激子。由于二维鞍点激子的锐度,可以实现与斯托克斯和反斯托克斯拉曼散射分量的单独共振,类似于先前对一维碳纳米管观察到的。斯托克斯和反斯托克斯发射的激发功率依赖性表明这两个过程是相关的,并且它们共享相同的声子。

英文摘要:

Twisted-bilayer graphene (tBLG) exhibits van Hove singularities in the density of states that can be tuned by changing the twisting angle $θ$. A $θ$-defined tBLG has been produced and characterized with optical reflectivity and resonance Raman scattering. The $θ$-engineered optical response is shown to be consistent with persistent saddle-point excitons. Separate resonances with Stokes and anti-Stokes Raman scattering components can be achieved due to the sharpness of the two-dimensional saddle-point excitons, similar to what has been previously observed for one-dimensional carbon nanotubes. The excitation power dependence for the Stokes and anti-Stokes emissions indicate that the two processes are correlated and that they share the same phonon.

机构、总结、中文摘要均由AI分析而来,可能存在错误,请以论文正文为准。

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