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arXiv 1402.2693cond-mat.str-el
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Thermodynamic Properties of the Quantum Spin Liquid Candidate ZnCu$_{3}$(OH)$_{6}$Cl$_{2}$ in High Magnetic Fields

Tian-Heng Han, Robin Chisnell, Craig J. Bonnoit, Danna E. Freedman, Vivien S. Zapf, Neil Harrison, Daniel G. Nocera, Yasu Takano, Young S. Lee

英文摘要:

We report measurements of the specific heat and magnetization of single crystal samples of the spin-1/2 kagome compound ZnCu$_{3}$(OH)$_{6}$Cl$_{2}$ (herbertsmithite), a promising quantum spin-liquid candidate, in high magnetic fields and at low temperatures. The magnetization was measured up to $μ_{0}H$ = 55 T at $T$ = 0.4 K, showing a saturation of the weakly interacting impurity moments in fields above $\sim10$ T. The specific heat was measured down to $T < 0.4$ K in magnetic fields up to 18 T, revealing $T$-linear and $T$-squared contributions. The $T$-linear contribution is surprisingly large and indicates the presence of gapless excitations in large applied fields. These results further highlight the unusual excitation spectrum of the spin liquid ground state of herbertsmithite.

机构、总结、中文摘要均由AI分析而来,可能存在错误,请以论文正文为准。

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