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arXiv 1402.1609cond-mat.str-el
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巡游铁磁体CeCrGe3中的重费米子和近藤晶格行为

Heavy fermion and Kondo lattice behavior in the itinerant ferromagnet CeCrGe3

Debarchan Das, T. Gruner, H. Pfau, U. B. Paramanik, U. Burkhardt, C. Geibel, Z. Hossain

摘要:

用X射线吸收光谱、磁化率$χ(T)$、等温磁化强度M(H)、电阻率$ρ(T)$、比热C($T$)和热电势S($T$)测量研究了多晶CeCrGe $_{3}$和LaCrGe $_{3}$的物理性质。发现这些化合物以六方钙钛矿结构(空间群\textit{P6$_{3}$/mmc})结晶,如先前报道的。$ρ(T)$、$χ(T)$和C($T$)数据证实了$T_{C}$分别为90 K和70 K的LaCrGe $_{3}$和CeCrGe $_{3}$中巡游Cr矩的体铁磁有序。此外,在CeCrGe $_{3}$的C($T$)数据中,在3 K附近也观察到一个弱的异常.由比热测量得到的$ρ$和索末菲系数$γ$的有限值的T依赖性证实了这两种化合物都具有金属性质。此外,CeCrGe $_{3}$的$ρ$的$T$依赖性反映了近藤晶格行为。130 mJ/mol的增强的$γ$,K $^{2}$与从$ρ(T)$推断的近藤晶格行为一起建立CeCrGe $_{3}$作为具有$\sim$ 45的准粒子质量重整化因子的中等重费米子化合物。

英文摘要:

Physical properties of polycrystalline CeCrGe$_{3}$ and LaCrGe$_{3}$ have been investigated by x-ray absorption spectroscopy, magnetic susceptibility $χ(T)$, isothermal magnetization M(H), electrical resistivity $ρ(T)$, specific heat C($T$) and thermoelectric power S($T$) measurements. These compounds are found to crystallize in the hexagonal perovskite structure (space group \textit{P6$_{3}$/mmc}), as previously reported. The $ρ(T)$, $χ(T)$ and C($T$) data confirm the bulk ferromagnetic ordering of itinerant Cr moments in LaCrGe$_{3}$ and CeCrGe$_{3}$ with $T_{C}$ = 90 K and 70 K respectively. In addition a weak anomaly is also observed near 3 K in the C($T$) data of CeCrGe$_{3}$. The T dependences of $ρ$ and finite values of Sommerfeld coefficient $γ$ obtained from the specific heat measurements confirm that both the compounds are of metallic character. Further, the $T$ dependence of $ρ$ of CeCrGe$_{3}$ reflects a Kondo lattice behavior. An enhanced $γ$ of 130 mJ/mol\,K$^{2}$ together with the Kondo lattice behavior inferred from the $ρ(T)$ establish CeCrGe$_{3}$ as a moderate heavy fermion compound with a quasi-particle mass renormalization factor of $\sim$ 45.

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