In the given paper the total inelastic cross-sections of the reactions of protons and deuterons on nuclear targets of enriched tin isotopes were compared. The factorization of cross-sections of reactions was discussed. Furthermore, the comparison of theoretical estimations on total inelastic cross-sections with corresponding experimental ones was made.
Thirty-eight tin isotopes have so far been observed; the discovery of these isotopes is discussed. For each isotope a brief summary of the first refereed publication, including the production and identification method, is presented.
Currently, twenty-four calcium, thirty-eight indium, thirty-eight tin and thirty-nine platinum isotopes have been observed and the discovery of these isotopes is discussed here. For each isotope a brief synopsis of the first refereed publication, including the production and identification method, is presented.
The coefficients of symmetry energy term for fragments with Z=4,11,12 measured in multifragmentation reactions initiated by proton and deuteron with energy of 3.65A GeV on enriched tin isotopes 112,118,120,124Sn are determined. The dependence of isoscaling parameter on the excitation energy, the temperature of fragmenting systems and the density ratio for heavy mass products are analised.
Experimental excitation functions for long-lived products in proton induced reactions were measured with the activation method in the 37-65 MeV energy range on natural holmium. Stacked foil irradiation technique and high resolution gamma spectrometry were used in order to measure cross-section data for the production of $^{161}$Er, $^{160}$Er and $^{159,157}$Dy. For comparison of the production routes of medically related $^{161}$Er and $^{160}$Er radioisotopes new experimental cross section data were deduced for the $^{162}$Er(p,x)$^{161,160}$Er and $^{162}$Er(d,x)$^{161,160}$Er reactions by …
Cross sections and analyzing powers for proton elastic scattering from $^{116,118,120,122,124}$Sn at 295 MeV have been measured for a momentum transfer of up to about 3.5 fm$^{-1}$ to deduce systematic changes of the neutron density distribution. We tuned the relativistic Love-Franey interaction to explain the proton elastic scattering of a nucleus whose density distribution is well known. Then, we applied this interaction to deduce the neutron density distributions of tin isotopes. The result of our analysis shows the clear systematic behavior of a gradual increase in the neutron skin thickne…
The $^{112,120}$Sn$(γ,γ')$ reactions have been studied at the S-DALINAC. Electric dipole (E1) strength distributions have been determined including contributions from unresolved strength extracted by a fluctuation analysis. Together with available data on $^{116,124}$Sn, an experimental systematics of the pygmy dipole resonance (PDR) in stable even-mass tin isotopes is established. The PDR centroid excitation energies and summed strengths are in reasonable agreement with quasiparticle-phonon model calculations based on a nonrelativistic description of the mean field but disagree with relativis…
Isospin effects in 12C ion induced reactions on enriched tin isotopes are investigated. The isoscaling parameter B is determined for different mass regions of product nuclei. It is shown that the isoscaling parameter is sensitive to the formation mechanism of products, and increases as the difference in the asymmetry is increasing. Using the exitatation energy obtained with the catcher technique temperatures, density ratio ro/ro0 for product nuclei in different mass regions and the values of symmetry energy coefficient for light mass regions of product nuclei for proton and deuteron induced re…
The isoscalar giant monopole resonance (GMR) has been investigated in a series of Sn isotopes (A=112--124) using inelstic scattering of 400-MeV alpha particles at extremely forward angles (including 0deg). The primary aim of the investigation has been to explore the role of the "symmetry-energy" term in the expression for nuclear incompressibility. It is found that the energies of the GMR in the Sn isotopes are significantly lower than those expected from the nuclear incompressibility previously extracted from the available data on the compressional-mode giant resonances.
We measure cross sections for residual nuclide formation in the mass range 6 < A < 97 caused by bombardment with protons and deuterons of 3.65 GeV/nucleon energy of enriched tin isotopes (112-Sn, 118-Sn, 120-Sn, 124-Sn). The experimental data are compared with calculations by the codes FLUKA, LAHET, CEM03, and LAQGSM03. Scaling behavior is observed for the whole mass region of residual nuclei, showing a possible multifragmentation mechanism for the formation of light products (6 < A < 31). Our analysis of the isoscaling dependence also shows a possible contribution of multifragmentation to the…
The x-ray cascade from antiprotonic atoms was studied for 106Cd, 116Cd, 112Sn, 116Sn, 120Sn, and 124Sn. Widths and shifts of the levels due to strong interaction were deduced. Isotopic effects in the Cd and Sn isotopes are clearly seen. The results are used to investigate the nucleon density in the nuclear periphery. The deduced neutron distributions are compared with the results of the previously introduced radiochemical method and with HFB calculations.
Excitation functions were measured for the natSr(d,x)88,87m,87g,86g,85gY, 87m,85g,83g,82Sr, 86g,84g,83,82m, 81gRb reactions by the stacked foil activation technique and high-resolution gamma-spectrometry up to 50 MeV. We present the first experimental activation cross section data for all investigated reactions. Our experimental data are compared with the TALYS code results as available in the TENDL-2015 on-line library. Use of deuteron induced reactions on Sr for production of medical isotopes is discussed.
A search for the various double beta decay modes of 124Sn and 112Sn has been performed on 75 kg.days of data. New half-life limits for excited states in 124Sn have been obtained including a lower limit for the decay into the first excited 2+ state of 124Te of T_half > 0.87e20 yrs (90% CL) and into the first excited 0+ state of T_half > 1.08e20 yrs (90% CL). Ground state and excited state transitions of 112Sn have also been experimentally explored. A limit for the 2 neutrino double electron capture of T_half > 1.8e19 yrs (90% CL) is obtained. The non-observation of de-excitation gammas from the…
We present a systematic configuration-interaction shell model calculation on the structure of light tin isotopes with a new global optimized effective interaction. The starting point of the calculation is the realistic CD-Bonn nucleon-nucleon potential. The unknown single-particle energies of the $1d_{3/2}$, $2s_{1/2}$ and $0h_{11/2}$ orbitals and the T=1 monopole interactions are determined by fitting to the binding energies of 157 low-lying yrast states in $^{102-132}$Sn. We apply the Hamiltonian to analyze the origin of the spin inversion between $^{101}$Sn and $^{103}$Sn that was observed …
By studying the 109Xe-->105Te-->101Sn superallowed alpha-decay chain, we observe low-lying states in 101Sn, the one-neutron system outside doubly magic 100Sn. We find that the spins of the ground state (J = 7=2) and first excited state (J = 5=2) in 101Sn are reversed with respect to the traditional level ordering postulated for 103Sn and the heavier tin isotopes. Through simple arguments and state-of-the-art shell model calculations we explain this unexpected switch in terms of a transition from the single-particle regime to the collective mode in which orbital-dependent pairing correlations, …
The dipole polarizability of stable even-mass tin isotopes 112,114,116,118,120,124 was extracted from inelastic proton scattering experiments at 295 MeV under very forward angles performed at RCNP. Predictions from energy density functionals cannot account for the present data and the polarizability of 208Pb simultaneously. The evolution of the polarizabilities in neighboring isotopes indicates a kink at 120Sn while all model results show a nearly linear increase with mass number after inclusion of pairing corrections.
We link the structure of nuclei around $^{100}$Sn, the heaviest doubly magic nucleus with equal neutron and proton numbers ($N=Z=50$), to nucleon-nucleon ($NN$) and three-nucleon ($NNN$) forces constrained by data of few-nucleon systems. Our results indicate that $^{100}$Sn is doubly magic, and we predict its quadrupole collectivity. We present precise computations of $^{101}$Sn based on three-particle--two-hole excitations of $^{100}$Sn, and reproduce the small splitting between the lowest $J^π=7/2^+$ and $5/2^+$ states. Our results are consistent with the sparse available data.
Investigations of cross-sections of deuteron induced nuclear reactions on gold were extended up to 50 MeV by using the standard stacked foil irradiation technique and high resolution gamma-ray spectrometry. New cross-sections are reported for the $^{197}$Au(d,xn)$^{197m,197g,195m,195g,193m,193g}$Hg and $^{197}$Au(d,x)$^{198m,198g,196m,196g,195,194}$Au nuclear reactions. The application for production of the medically relevant isotopes $^{198}$Au and $^{195m,195g,197m,197g}$Hg is discussed, including the comparison with other charged particle induced production routes. The possible use of the $…
The excitation of the isoscalar giant monopole resonance (ISGMR) in $^{116}$Sn and $^{208}$Pb has been investigated using small-angle (including $0^\circ$) inelastic scattering of 100 MeV/u deuteron and multipole-decomposition analysis (MDA). The extracted strength distributions agree well with those from inelastic scattering of 100 MeV/u $α$ particles. These measurements establish deuteron inelastic scattering at E$_d \sim$ 100 MeV/u as a suitable probe for extraction of the ISGMR strength with MDA, making feasible the investigation of this resonance in radioactive isotopes in inverse kinemat…
High-precision ab initio calculations of nuclear binding energies: Tin isotopes from dripline to dripline
Technische Universität Darmstadt（达姆施塔特工业大学）；ExtreMe Matter Institute EMMI, GSI Helmholtzzentrum für Schwerionenforschung GmbH（GSI重离子研究中心极端物质研究所EMMI）；KU Leuven, Instituut voor Kern- en Stralingsfysica（荷语鲁汶大学核与辐射物理研究所）；Institut d’Astronomie et d’Astrophysique, Université Libre de Bruxelles（布鲁塞尔自由大学天体物理学与天文学研究所）；Brussels Laboratory of the Universe – BLU-ULB（布鲁塞尔宇宙实验室）；IRFU, CEA, Université Paris-Saclay（巴黎萨克雷大学CEA IRFU）；Max-Planck-Institut für Kernphysik（马克斯·普朗克核物理研究所）
One-atom-thick crystals are impermeable to atoms and molecules, but hydrogen ions (thermal protons) penetrate through them. We show that monolayers of graphene and boron nitride can be used to separate hydrogen ion isotopes. Employing electrical measurements and mass spectrometry, we find that deuterons permeate through these crystals much slower than protons, resulting in a separation factor of ~10 at room temperature. The isotope effect is attributed to a difference of about 60 meV between zero-point energies of incident protons and deuterons, which translates into the equivalent difference …
We show in the Skyrme-Hartree-Fock approach that unambiguous correlations exist between observables of finite nuclei and nuclear matter properties. Using this correlation analysis to existing data on the neutron skin thickness of Sn isotopes, we find important constraints on the value E_{sym}(rho_0) and density slope L of the nuclear symmetry energy at saturation density. Combining these constraints with those from recent analyses of isospin diffusion and double neutron/proton ratio in heavy ion collisions leads to a value of L=58\pm 18 MeV approximately independent of E_{sym}(ρ_0).
The occupancies and vacancies of the valence neutron orbitals across the stable tin isotopic chain from $112\leq A\leq 124$ have been determined. These were inferred from the cross sections of neutron-adding and -removing reactions. In each case, the reactions were chosen to have good angular-momentum matching for transfer to the low- and high-$\ell$ orbitals present in this valence space. These new data are compared to older systematic studies. The effective single-neutron energies are determined by combining information from energy centroids determined from the adding and removing reactions.…
In the frame of a systematic study of activation cross sections of deuteron induced nuclear reactions on rare earths, the reactions on neodymium for production of therapeutic radionuclides were measured for the first time. The excitation functions of the natNd(d,x) 151,150,149,148m,148g,146,144,143Pm, 149,147,139mNd, 142Pr and 139gCe nuclear reactions were assessed by using the stacked foil activation technique and high resolution $γ@-spectrometry. The experimental excitation functions were compared to the theoretical predictions calculated with the modified model codes ALICE-IPPE-D and EMPIRE…
For the first time an extensive search for various double beta decay modes of 124Sn and 112Sn has been performed. A total exposure of 43.29 kg.days has been accumulated. New half-life limits of 124Sn into excited states of 124Te have been obtained; the lower half-life limit for the first excited 2+ state at 602.7keV is T_1/2 > 3.1 *10^{18}yrs (90 % CL) and for the first excited 0+ state T_1/2 > 7.7 *10^{18}yrs (90 % CL). For the very first time, ground state and excited state transitions of 112Sn have been experimentally explored. The obtained half-life limits for ECEC and beta+/EC into the fi…
The analysis results of the isotopic yields for products obtained in reactions of protons at energies 0.66, 1, 8.1GeV with separated tin isotopes are presented. The experimental data are compared in form of reactions of element cross sections for two targets of different isotope compositions. The scaling behaviour have been shown in the dependence of this ratios from neutron and proton composition at the reaction products. The discussion of scaling parameters allows to explain the mechanism of light and medium mass fragment production.
The distribution of isoscalar monopole strength in the neutron-even 112-124Sn-isotopes has been computed using a relativistic random-phase-approximation approach. The accurately-calibrated model used here (``FSUGold'') has been successful in reproducing both ground-state observables as well as collective excitations - including the giant monopole resonance (GMR) in 90Zr, 144Sm, and 208Pb. Yet this same model significantly overestimates the GMR energies in the Sn isotopes. It is argued that the question of ``Why is Tin so soft?'' becomes an important challenge to the field and one that should b…
"Why are the tin isotopes soft?" has remained, for the past decade, an open problem in nuclear structure physics: models which reproduce the isoscalar giant monopole resonance (ISGMR) in the "doubly-closed shell" nuclei, $^{90}$Zr and $^{208}$Pb, overestimate the ISGMR energies of the open-shell tin and cadmium nuclei, by as much as 1 MeV. In an effort to shed some light onto this problem, we present results of detailed studies of the ISGMR in the molybdenum nuclei, with the goal of elucidating where--and how--the softness manifests itself between $^{90}$Zr and the cadmium and tin isotopes. Th…
Deuteron elastic scattering from 15C and inelastic scattering reactions to the first excited state of 15C were studied using a radioactive beam of 15C in inverse kinematics. The scattered deuterons were measured using HELIOS. The elastic scattering differential cross sections were analyzed using the optical model. A matter deformation length δd = 1.04(11) fm has been extracted from the differential cross sections of inelastic scattering to the first excited state. The ratio of neutron and proton matrix elements Mn/Mp = 3.6(4) has been determined from this quadrupole transition. Neutron effecti…
Direct reaction techniques are powerful tools to study the single-particle nature of nuclei. Performing direct reactions on short-lived nuclei requires radioactive ion beams produced either via fragmentation or the Isotope Separation OnLine (ISOL) method. Some of the most interesting regions to study with direct reactions are close to the magic numbers where changes in shell structure can be tracked. These changes can impact the final abundances of explosive nucleosynthesis. The structure of the chain of tin isotopes is strongly influenced by the Z=50 proton shell closure, as well as the neutr…
Reactions are an important tool to study nuclear structure and for extracting reactions relevant for astrophysics. In this paper we focus on deuteron induced reactions which can provide information on neutron shell evolution as well as neutron capture cross sections. We review recent work on the systematic comparison of the continuum discretized coupled channel method, the adiabatic wave approximation and the Faddeev momentum-space approach. We also explore other aspects of the reaction mechanism and discuss in detail difficulties encountered in the calculations.
In this paper we present the first high-resolution laser spectroscopy results obtained at the GISELE laser laboratory of the GANIL-SPIRAL2 facility, in preparation for the first experiments with the S$^3$-Low Energy Branch. Studies of neutron-deficient radioactive isotopes of erbium and tin represent the first physics cases to be studied at S$^3$. The measured isotope-shift and hyperfine structure data are presented for stable isotopes of these elements. The erbium isotopes were studied using the $4f^{12}6s^2$ $^3H_6 \rightarrow 4f^{12}(^3 H)6s6p$ $J = 5$ atomic transition (415 nm) and the tin…
As a part of a thorough work of excitation functions of deuteron induced reactions, experimental cross-sections of ^{185,183m,183g,182}Os and ^{188,186,184m,184g,183}Re activation products on natRe were measured up to 40 MeV for the first time with the activation method using a stacked foil irradiation technique and high resolution γ-spectrometry. Comparison with the former results of other laboratories and with the predictions of the ALICE-IPPE and EMPIRE-3 model codes, modified for improved calculations for deuteron reactions, and with data in the TENDL-2011 library are also presented. Thick…
The ``breathing mode'' of neutron-rich nuclei is our window into the incompressibility of neutron-rich matter. After much confusion on the interpretation of the experimental data, consistency was finally reached between different models that predicted both the distribution of isoscalar monopole strength in finite nuclei and the compression modulus of infinite matter. However, a very recent experiment on the Tin isotopes at the Research Center for Nuclear Physics(RCNP) in Japan has again muddled the waters. Self-consistent models that were successful in reproducing the energy of the giant monop…
In this presentation we discuss a number of experiments on the search for proton or deuteron EDMs, which could be carried out at COSY-Juelich. Most promising is the use of an radio-frequency radial electric field flipper that would lead to the accumulation of a CP violating in-plane beam polarization by tiny spin rotations. Most crucial for storage ring searches for EDMs is the spin-coherence time, and we report on analytic evaluations which point at a much larger spin-coherence time for deuterons by about a factor of 200 compared to the one for protons, and at COSY, the spin coherence time fo…
Observation of hidden nuclear reactions on fast neutron-irradiated Lu isotopes
International Nuclear Safety Center of Ukraine of Taras Shevchenko National University of Kyiv（基辅塔拉斯舍甫琴科国立大学乌克兰国际核安全中心）；Department of Nuclear and High Energy Physics, Faculty of Physics, Taras Shevchenko National University of Kyiv（基辅塔拉斯舍甫琴科国立大学物理学院核与高能物理系）；HUN-REN Institute for Nuclear Research (HUN-REN ATOMKI)（匈牙利研究与创新网络原子核研究所）
The recoil properties of the product nuclei from the interaction of 2.2 GeV/nucleon 12-C ions from Nuclotron of the Laboratory of High Energies (LHE), Joint Institute for Nuclear Research (JINR) at Dubna with a 118-Sn target have been studied using catcher foils. The experimental data were analyzed using the mathematical formalism of the standard two-step vector model. The results for 12-C ions are compared with those for deuterons and protons. Three different Los Alamos versions of the Quark-Gluon String Model (LAQGSM) were used for comparison with our experimental data.
Purpose: Accurate new measurements of low-energy deuteron-induced reaction cross sections for natural Cr target can enhance the related database and the opportunity for an unitary and consistent account of the involved reaction mechanisms. Methods: The activation cross sections of $^{51,52,54}$Mn, $^{51}$Cr, and $^{48}$V nuclei for deuterons incident on natural Cr at energies up to 20 MeV, were measured by the stacked-foil technique and high resolution gamma spectrometry using U-120M cyclotron of the Center of Accelerators and Nuclear Analytical Methods (CANAM) of the Nuclear Physics Institute…
We present an account of the current status of the theoretical treatment of inclusive $(d,p)$ reactions in the breakup-fusion formalism, pointing to some applications and making the connection with current experimental capabilities. Three independent implementations of the reaction formalism have been recently developed, making use of different numerical strategies. The codes also originally relied on two different but equivalent representations, namely the prior (Udagawa-Tamura, UT) and the post (Ichimura-Austern-Vincent, IAV) representations. The different implementations have been benchmark…
As a part of our series of studies on deuteron induced reaction on various target materials excitation functions on natural cobalt have been measured by using stacked-foil technique. In these measurements 51Cr, 55;56;57;58Co, 51Cr, 52;54;56Mn and 56;57Ni radioisotopes have been identified. For the above isotopes the excitation functions were determined and compared with the literature data and with the results of EMPIRE and TALYS calculations taken from the TENDL 2011 library. The agreement with previous measurements was acceptable and we could also determine new cross-section data.
Results of a photon scattering experiment on 112Sn using bremsstrahlung with an endpoint energy of E_0 = 3.8 MeV are reported. A J = 1 state at E_x = 3434(1) keV has been excited. Its decay width into the ground state amounts to Gamma_0 = 151(17) meV, making it a candidate for a [2+ x 3-]1- two-phonon state. The results for 112Sn are compared with quasiparticle-phonon model calculations as well as the systematics of the lowest-lying 1- states established in other even-mass tin isotopes. Contrary to findings in the heavier stable even-mass Sn isotopes, no 2+ states between 2 and 3.5 MeV excitat…
Fragmentation of neutron-rich carbon isotopes on light targets at 27.5 MeV/nucleon
Peking University（北京大学）；Institute of Modern Physics, Chinese Academy of Sciences（中国科学院近代物理研究所）；Institute of Applied Physics and Computational Mathematics（应用物理与计算数学研究所）
From Beam to Bedside: Reinforcing Domestic Supply of $^{99}$Mo/$^{99m}$Tc using Novel High-Current D+ Cyclotrons for Compact Neutron Generation and $^{99}$Mo Production
Characterizing the nature of single-particle states outside of double shell closures is essential to a fundamental understanding of nuclear structure. This is especially true for those doubly magic nuclei that lie far from stability and where the shell closures influence nucleo-synthetic pathways. The region around $^{100}$Sn is one of the most important due to the proximity of the N=Z=50 magic numbers, the proton-drip line, and the end of the rp-process. However, owing to the low production rates, there is a lack of spectroscopic information and no firm spin-parity assignment for ground state…
The lifetimes of the low-lying excited states $2^+$ and $4^+$ have been directly measured in the neutron-deficient $^{106,108}$Sn isotopes. The nuclei were populated via a deep-inelastic reaction and the lifetime measurement was performed employing a differential plunger device. The emitted $γ$ rays were detected by the AGATA array, while the reaction products were uniquely identified by the VAMOS++ magnetic spectrometer. Large-Scale Shell-Model calculations with realistic forces indicate that, independently of the pairing content of the interaction, the quadrupole force is dominant in the $B(…
Isospin e ffects on multifragmentation properties were studied thanks to nuclear collisions between di fferent isotopes of xenon beams and tin targets. It is shown that, in central collisions leading to multifragmentation, the mean number of fragments and their mean kinetic energy increase with the neutron-richness of the total system. Comparisons with a stochastic transport model allow to attribute the multiplicity increase to the multifragmentation stage, before secondary decay. The total charge bound in fragments is proposed as an alternate variable to quantify preequilibrium emission and t…
Elastic scattering of relativistic electrons from the nucleon yields Lorentz invariant form factors that describe the fundamental distribution of charge and magnetism. The spatial dependence of the nucleon's charge and magnetism is typically interpreted in the Breit reference frame which is related by a Lorentz boost from the laboratory frame, where the nucleon is at rest. We construct a model to estimate how the Sachs electric and magnetic form factors can be corrected for the effects of relativistic recoil. When the corrections are applied, the ratio of the proton's Sachs form factors is app…
Neutron-induced background has been studied in various components of the TIN.TIN detector, which is under development for the search of Neutrinoless Double Beta Decay in $\rm^{124}Sn$. Fast neutron flux $\sim10^{6}~n~cm^{-2}s^{-1}$ covering a broad energy range ($ \sim0.1$ to $ \sim18$~MeV) was generated using $^{9}Be(p,n)^{9}B$ reaction. In addition, reactions with quasi-monoenergetic neutrons were also studied using $^{7}Li(p,n)^{7}Be$ reaction. Among the different cryogenic support structures studied, Teflon is found to be preferable compared to Torlon as there is no high energy gamma backg…
Isotopic effects observed in fragmentation reactions induced by protons, deuterons, and alpha particles of incident energies between 660 MeV and 15.3 GeV on 112-Sn and 124-Sn targets are discussed. The exponential scaling of the yield ratios with the third component of the fragment isospin (N-Z)/2 is observed in all reactions, with scaling parameters that depend on the incident energy. Breakup temperatures for these reactions are deduced from double ratios of isotopic yields and tested for their relation with the isoscaling parameters. The quantum statistical (QSM) and the statistical multifra…
The strongly isospin-dependent tensor force leads to short-range correlations (SRC) between neutron-proton (deuteron-like) pairs much stronger than those between proton-proton and neutron-neutron pairs. As a result of the short-range correlations, the single-nucleon momentum distribution develops a high-momentum tail above the Fermi surface. Because of the strongly isospin-dependent short-range correlations, in neutron-rich matter a higher fraction of protons will be depleted from its Fermi sea and populate above the Fermi surface compared to neutrons. This isospin-dependent nucleon momentum d…
