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arXiv 1208.4690cond-mat.supr-con
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$^{63}$ Cu和$^{199}$ Hg NMR $_{2}$ CuO $_{4+δ}$单晶的研究

$^{63}$Cu and $^{199}$Hg NMR study of HgBa$_{2}$CuO$_{4+δ}$ single crystals

Damian Rybicki, Jürgen Haase, Marc Lux, Michael Jurkutat, Martin Greven, Guichuan Yu, Yuan Li, Xudong Zhao

摘要:

我们报告的$^{63}$铜和$^{199}$汞NMR磁位移和线宽的温度依赖性的最佳掺杂和欠掺杂的HgBa $_{2}$ CuO $_{4+δ}$单晶,以及四极分裂和其分布的$^{63}$铜。从$^{63}$ Cu和$^{199}$ Hg \textit{magnetic shifts},我们最近得出结论,存在两个自旋分量,它们具有不同的温度依赖性[J. Haase,D.里比茨基角P. Slichter,M.格雷文湾Yu,Y. Li和X. Zhao,Phys. Rev. B 85,104517(2012)]。在这里,我们给出了一个全面的帐户的所有数据,并专注于线宽和四极分裂。虽然$^{63}$铜四极耦合和它的分布是由和大的温度无关,我们确定了三个区域的温度,其中的磁宽度显着不同:在最低温度的磁力线宽度是由刚性磁通量晶格,似乎已经消失以上约60 K。在中温区,从60 K以上开始,磁力线宽度由赝能隙自旋分量引起的磁位移的空间分布决定,并随总位移线性增长,直到约\textit{$\sim$} 170-230 K,这取决于样品和核。高于这个温度,第三个区域开始突然变窄,第二个,费米液体般的自旋分量变得均匀。我们表明,所有的线宽,四极以及磁性,以上的磁通量占主导地位的区域可以理解一个简单的模型,假设一个相干的电荷密度的变化与伴随的两个自旋分量的变化。此外,我们发现一个温度无关的自旋为基础的扩大在这两个样品是不相干的与其他扩大的欠掺杂晶体,但成为相干的最佳掺杂晶体。

英文摘要:

We report on the temperature dependence of $^{63}$Cu and $^{199}$Hg NMR magnetic shifts and linewidths for an optimally doped and an underdoped HgBa$_{2}$CuO$_{4+δ}$ single crystal, as well as the quadrupole splitting and its distribution for $^{63}$Cu. From the $^{63}$Cu and $^{199}$Hg \textit{magnetic shifts} we have recently concluded on the existence of two spin components with different temperature dependencies [J. Haase, D. Rybicki, C. P. Slichter, M. Greven, G. Yu, Y. Li, and X. Zhao, Phys. Rev. B 85, 104517 (2012)]. Here we give a comprehensive account of all data and focus on the linewidths and quadrupole splittings. While the $^{63}$Cu quadrupole coupling and its distribution are by and large temperature independent, we identify three regions in temperature for which the magnetic widths differ significantly: at the lowest temperatures the magnetic linewidths are dominated by the rigid fluxoid lattice that seems to have disappeared above about 60 K. In the intermediate temperature region, starting above 60 K, the magnetic linewidth is dominated by the spatial distribution of the magnetic shift due to the pseudogap spin component, and grows linearly with the total shift up to about \textit{$\sim$}170-230 K, depending on sample and nucleus. Above this temperature the third region begins with an sudden narrowing where the second, Fermi-liquid-like spin component becomes homogeneous. We show that all linewidths, quadrupolar as well as magnetic, above the fluxoid dominated region can be understood with a simple model that assumes a coherent charge density variation with concomitant variations of the two spin components. In addition, we find a temperature independent spin based broadening in both samples that is incoherent with the other broadening for the underdoped crystal, but becomes coherent for the optimally doped crystal.

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