arXivDaily arXiv每日学术速递 周一至周五更新
arXiv 1207.0102cond-mat.str-elcond-mat.mes-hall
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纳米罗盘-海森堡平面团簇的磁性

Magnetic properties of nanoscale compass-Heisenberg planar clusters

F. Trousselet, A. M. Oles, P. Horsch

摘要:

我们研究了正方形晶格上自旋为1/2的模型,通过增加最近邻之间的扰动海森堡相互作用来推广量子罗盘模型,并研究了它的相图和磁激发。这个模型的动机既来自于轨道简并的强关联系统领域,也来自于为量子计算提出的基于固态的器件领域。我们发现,Compass模型的高简并基态是脆弱的,对于任何有限振幅的海森堡耦合,都将变为双重简并基态。通过计算有限集团的自旋结构因子与Lanczos对角化,我们证明了丰富的各种相位特征的Z2对称性,这是铁磁,C型反铁磁,或Neel型,并分析量子涨落的影响相边界。在有序相中,罗盘相互作用的各向异性导致自旋波的有限激发间隙。我们发现,对于小的纳米级团簇与大的各向异性间隙的最低激发列翻转激发,出现由于海森堡扰动的指南针模型的简并基态的流形。我们导出了一个有效的一维XYZ模型,它忠实地再现了这些激发态的精确结构,并阐明了它们的微观起源。低能量列翻转或罗盘型激发对于退相干过程是鲁棒的,因此被很好地设计用于在量子计算中存储信息。我们还指出,氮空位中心之间的偶极相互作用,形成一个矩形晶格的金刚石矩阵可能允许固态实现的各向异性指南针海森堡模型。

英文摘要:

We study a model of spins 1/2 on a square lattice, generalizing the quantum compass model via the addition of perturbing Heisenberg interactions between nearest neighbors, and investigate its phase diagram and magnetic excitations. This model has motivations both from the field of strongly correlated systems with orbital degeneracy and from that of solid-state based devices proposed for quantum computing. We find that the high degeneracy of ground states of the compass model is fragile and changes into twofold degenerate ground states for any finite amplitude of Heisenberg coupling. By computing the spin structure factors of finite clusters with Lanczos diagonalization, we evidence a rich variety of phases characterized by Z2 symmetry, that are either ferromagnetic, C-type antiferromagnetic, or of Neel type, and analyze the effects of quantum fluctuations on phase boundaries. In the ordered phases the anisotropy of compass interactions leads to a finite excitation gap to spin waves. We show that for small nanoscale clusters with large anisotropy gap the lowest excitations are column-flip excitations that emerge due to Heisenberg perturbations from the manifold of degenerate ground states of the compass model. We derive an effective one-dimensional XYZ model which faithfully reproduces the exact structure of these excited states and elucidates their microscopic origin. The low energy column-flip or compass-type excitations are robust against decoherence processes and are therefore well designed for storing information in quantum computing. We also point out that the dipolar interactions between nitrogen-vacancy centers forming a rectangular lattice in a diamond matrix may permit a solid-state realization of the anisotropic compass-Heisenberg model.

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