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arXiv 1111.5017cond-mat.str-el
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自旋1各向异性反铁磁体$NiCl_2-4SC(NH_2)_2$的磁激发

Magnetic excitations in the spin-1 anisotropic antiferromagnet $NiCl_2-4SC(NH_2)_2$

C. Psaroudaki, S. A. Zvyagin, J. Krzystek, A. Paduan-Filho, X. Zotos, N. Papanicolaou

摘要:

自旋为1的各向异性反铁磁体NiCl_2-4SC(NH_2)_2表现出类似于玻色-爱因斯坦凝聚的场诱导量子相变.在这里,我们提出了系统的高场电子自旋共振(ESR)的实验和理论研究的结果,这种化合物,特别强调单离子两磁振子束缚态。为了澄清理论和实验之间的一些剩余的差异,在这种材料中的磁激励的频率场依赖性进行了重新分析。特别是,一个更全面的解释单离子两磁振子束缚态的实验签名与理论结果完全一致。我们还澄清了所谓的中间相的ESR谱的结构。

英文摘要:

The spin-1 anisotropic antiferromagnet NiCl_2-4SC(NH2)_2 exhibits a field-induced quantum phase transition that is formally analogous to Bose-Einstein condensation. Here we present results of systematic high-field electron spin resonance (ESR) experimental and theoretical studies of this compound with a special emphasis on single-ion two-magnon bound states. In order to clarify some remaining discrepancies between theory and experiment, the frequency-field dependence of magnetic excitations in this material is reanalyzed. In particular, a more comprehensive interpretation of the experimental signature of single-ion two-magnon bound states is shown to be fully consistent with theoretical results. We also clarify the structure of the ESR spectrum in the so-called intermediate phase.

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