At zero temperature and strong applied magnetic fields the ground sate of an anisotropic antiferromagnet is a saturated paramagnet with fully aligned spins. We study the quantum phase transition as the field is reduced below an upper critical $H_{c2}$ and the system enters a XY-antiferromagnetic phase. Using a bond operator representation we consider a model spin-1 Heisenberg antiferromagnetic with single-ion anisotropy in hyper-cubic lattices under strong magnetic fields. We show that the transition at $H_{c2}$ can be interpreted as a Bose-Einstein condensation (BEC) of magnons. The theoretical results are used to analyze our magnetization versus field data in the organic compound $NiCl_2$-$4SC(NH_2)_2$ (DTN) at very low temperatures. This is the ideal BEC system to study this transition since $H_{c2}$ is sufficiently low to be reached with static magnetic fields (as opposed to pulsed fields). The scaling of the magnetization as a function of field and temperature close to $H_{c2}$ shows excellent agreement with the theoretical predictions. It allows to obtain the quantum critical exponents and confirm the BEC nature of the transition at $H_{c2}$.
Based on a realistic spin Hamiltonian for a frustrated quasi-two dimensional spin-1/2 antiferromagnet Cs$_{2}$CuCl$_{4}$, a three-dimensional spin ordering in the applied magnetic field $B$ near the saturation value $B_{c}$ is studied within the magnon Bose-Einstein condensation (BEC) scenario. With the use of a hard-core boson formulation of the spin model, a strongly anysotropic magnon dispersion in Cs$_{2}$CuCl$_{4}$ is calculated. In the dilute magnon limit near $B_{c}$, the hard-core boson constraint is resulted in an effective magnon interaction which is treated in the Hartree-Fock appro…
Bose-Einstein condensation (BEC) of triplet excitations triggered by a magnetic field, sometimes called magnon BEC, in dimerized antiferromagnets gives rise to a long-range antiferromagnetic order in the plane perpendicular to the applied magnetic field. To explore the effects of spin-orbit coupling on magnon condensation, we study a spin model on a distorted honeycomb lattice with dimerized Heisenberg exchange ($J$ terms) and uniform off-diagonal exchange ($Γ'$ terms) interactions. Via variational Monte Carlo calculations and spin-wave theory, we find that an out-of-plane magnetic field can i…
In this work, we investigate the evolution and settling of magnon condensation in the spin-1/2 dimer system Sr$_{3}$Cr$_{2}$O$_{8}$ using a combination of magnetostriction in pulsed fields and inelastic neutron scattering in a continuous magnetic field. The magnetic structure in the Bose-Einstein condensation (BEC) phase was probed by neutron diffraction in pulsed magnetic fields up to 39~T. The magnetic structure in this phase was confirmed to be an XY-antiferromagnetic structure validated by irreducible representational analysis. The magnetic phase diagram as a function of an applied magneti…
Magnetization, magnetic torque, neutron diffraction and NMR experiments are used to map out the $H$$-$$T$ phase diagram of the prototypical quasi-two-dimensional ferro-antiferromagnet Pb$_2$VO(PO$_4$)$_2$ in magnetic fields up to 27 T. When the field is applied perpendicular to the axis of magnetic anisotropy, a new magnetic state emerges through a discontinuous transition and persists in a narrow field range just below saturation. The measured NMR spectra suggest a complex and possibly incommensurate magnetic order in that regime.
Single crystal elastic and inelastic neutron scattering experiments are performed on the frustrated ferro-antiferromagnet SrZnVO(PO4)2 in high magnetic fields. The fully polarized state, the presaturation phase and the columnar-antiferromagnetic phase just bellow the presaturation phase were investigated. The observed renormalization of spin wave bandwidths, re-distribution of intensities between different branches and non-linearities in the magnetization curve are all indicative of strong deviations from classical spin wave theory. The previously observed presaturation transition is attribute…
We consider 2D Heisenberg antiferromagnets on a triangular lattice with spatially anisotropic interactions in a high magnetic field close to the saturation. We show that this system possess rich phase diagram in field/anisotropy plane due to competition between classical and quantum orders: an incommensurate non-coplanar spiral state, which is favored classically, and a commensurate co-planar state, which is stabilized by quantum fluctuations. We show that the transformation between these two states is highly non-trivial and involves two intermediate phases -- the phase with co-planar incommen…
Motivated by recent observation of a new high field phase near saturation in chromium spinels $A$Cr$_2$O$_4$ ($A=$ Zn, Cd, Hg), we study the $S = 3/2$ pyrochlore Heisenberg antiferromagnet with biquadratic interactions. Magnon instability analysis at the saturation field reveals that a very small biquadratic interaction can induce magnon pairing in pyrochlore antiferromagnets, which leads to the emergence of a ferro-quadrupolar phase, or equivalently a spin nematic phase, below the saturation field. We present the magnetic phase diagram in an applied field, studying both $S=3/2$ and $S=1$ spin…
We investigate the field-induced insulator-to-superfluid transition of bosonic quasiparticles in $S=1/2$ weakly-coupled dimer antiferromagnets. In presence of realistic disorder due to site dilution of the magnetic lattice, we show that the system displays an extended Bose-glass phase characterized by the localization of the hard-core quasiparticles.
We study the effects of spin-orbit coupling (SOC) on the large-U Hubbard model on anisotropic triangular lattice at half-filling using the Schwinger-boson method. We find that the SOC will in general lead to a zero temperature condensation of the Schwinger bosons with a single condensation momentum. As a consequence, the spin-spin correlation vanishes along the z-axis but develops in the $x$-$y$ plane, with the ordering wave vector being dramatically dependent on the SOC. Moreover, the phase boundary of the magnetic ordered state extends to the region of large spatial anisotropy with increased…
We performed a comprehensive electron spin resonance, magnetization and heat capacity study on the field-induced magnetic phase transitions in the kagome antiferromagnet $α-Cu_3Mg(OH)_6Br_2$. With the successful preparation of single crystals, we mapped out the magnetic phase diagrams under the $c$-axis and $ab$-plane directional magnetic fields $B$. For $B\|c$, the three-dimensional (3D) magnon Bose-Einstein condensation (BEC) is evidenced by the power law scaling of the transition temperature, $T_c\propto (B_c-B)^{2/3}$. For $B\|ab$, the transition from the canted antiferromagetic (CAFM) sta…
We study the effects of quantum fluctuations in magnetic properties of quantum frustrated ferromagnets in a magnetic field. It is shown that a non-classical phase or a phase separation appears due to quantum fluctuations below the saturation field in a parameter range close to the classical zero-field phase boundary between ferromagnetic and antiferromagnetic phases, for the case that the classical antiferromagnetic state is not an eigenstate of the quantum model. As an example to which this argument is applicable, we study the S=1/2 J1-J2 Heisenberg model with ferromagnetic J1 (J1<0) on the b…
Saturation field entropies of antiferromagnetic Ising models on quasi one-dimensional lattices (ladders) and the kagome lattice are calculated. The former is evaluated exactly by constructing the corresponding transfer matrices, while the latter calculation uses Binder's algorithm for efficiently and exactly computing the partition function of over 1300 spins to give, in Boltzmann's units, S = 0.393589(6). We comment on the relation of the kagome lattice to the experimental situation in the spin-ice compound dysprosium titanium oxide.
The structure of K2Ni2(MoO4)3 consists of S=1 tetramers formed by Ni^{2+} ions. The magnetic susceptibility chi(T) and specific heat Cp(T) data on a single crystal show a broad maximum due to the low-dimensionality of the system with short-range spin correlations. A sharp peak is seen in chi(T) and Cp(T) at about 1.13 K, well below the broad maximum. This is an indication of magnetic long-range order i.e., the absence of spin-gap in the ground state. Interestingly, the application of a small magnetic field (H>0.1 T) induces magnetic behavior akin to Bose-Einstein condensation (BEC) of triplon …
We study the low-temperature thermodynamic properties of a number of frustrated quantum antiferromagnets which support localized magnon states in the vicinity of the saturation field. For this purpose we use 1) a mapping of the low-energy degrees of freedom of spin systems onto the hard-core object lattice gases and 2) an exact diagonalization of finite spin systems of up to N=30 sites. The considered spin systems exhibit universal behavior which is determined by a specific hard-core object lattice gas representing the independent localized magnon states. We test the lattice gas description by…
Magnetization processes of spin-1/2 Heisenberg ladders are studied using strong-coupling expansions, numerical diagonalization of finite systems and a bosonization approach. We find that the magnetization exhibits plateaux as a function of the applied field at certain rational fractions of the saturation value. Our main focus are ladders with 3 legs where plateaux with magnetization one third of the saturation value are shown to exist.
We study the high magnetic field regime of the antiferromagnetic insulator Cs$_2$CuCl$_4$ by expressing the spin-1/2 operators in the relevant Heisenberg model in terms of hard-core bosons and implementing the hard-core constraint via an infinite on-site interaction. We focus on the case where the external magnetic field exceeds the saturation field $B_{c}\approx8.5\;\mathrm{T}$ and is oriented along the crystallographic $a$ axis perpendicular to the lattice plane. Because in this case the excited states are separated by an energy gap from the ground state, we may use the self-consistent ladde…
Quantum phase transition at the saturation field is studied for a class of frustrated quantum antiferromagnets. The considered models include (i) the $J_1$-$J_2$ frustrated square-lattice antiferromagnet with $J_2={1/2}J_1$ and (ii) the nearest-neighbor Heisenberg antiferromagnet on a face centered cubic lattice. In the fully saturated phase the magnon spectra for the two models have lines of degenerate minima. Transition into partially magnetized state is treated via a mapping to a dilute gas of hard core bosons and by complementary spin-wave calculations. Momentum dependence of the exact fou…
Low-temperature specific-heat measurements on YbRh2Si2 at the second order antiferromagnetic (AF) phase transition reveal a sharp peak at T_N=72 mK. The corresponding critical exponent alpha turns out to be alpha=0.38, which differs significantly from that obtained within the framework of the fluctuation theory of second order phase transitions based on the scale invariance, where alpha=0.1. We show that under the application of magnetic field the curve of the second order AF phase transitions passes into a curve of the first order ones at the tricritical point leading to a violation of the cr…
This work reports the synthesis, structure and magnetic properties of the single crystal of a facile spin 1/2 one dimensional Heisenberg antiferromagnet bis(4-aminopyridinium) bis(oxalato)cuprate(II) dihydrate, (C 5 H 7 N 2 ) 2 [Cu(C 2 O 4 ) 2 ].2H 2 O. Single crystals of large sizes of the title compound were obtained using the technique of liquid-liquid diffusion or layer diffusion with 100 % yield. Single crystal X-ray diffraction measurements revealed a very good quality of the grown single crystals with small value of goodness of fit R obtained at 1.058. The structure comprises corner-sha…
The elementary excitations in antiferromagnets are magnons, quasiparticles with integer spin and Bose statistics. In an experiment their density is controlled efficiently by an applied magnetic field and can be made finite to cause the formation of a Bose-Einstein condensate (BEC). Studies of magnon condensation in a growing number of magnetic materials provide a unique window into an exciting world of quantum phase transitions (QPT) and exotic quantum states.
We study the role of long range dipolar interactions on antiferromagnetic spin chains, from the classical $S\to \infty$ limit to the deep quantum case $S=1/2$, including a transverse magnetic field. To this end, we combine different techniques such as classical energy minima, classical Monte Carlo, linear spin waves, bosonization and DMRG. We find a phase transition from the already reported dipolar ferromagnetic region to an antiferromagnetic region for high enough antiferromagnetic exchange. Thermal and quantum fluctuations destabilize the classical order before reaching magnetic saturation …
Unconventional features of the magnetization curve at zero temperature such as plateaus or jumps are a hallmark of frustrated spin systems. Very little is known about their behavior at non-zero temperatures. Here we investigate the temperature dependence of the magnetization curve of the kagome lattice antiferromagnet in particular at 1/3 of the saturation magnetization for large lattice sizes of up to N=48 spins. We discuss the phenomenon of asymmetric melting and trace it back to a combined effect of unbalanced magnetization steps on either side of the investigated plateau as well as on the …
We calculate the angular resolved photoemission spectra (ARPES) of a spin-1/2 Heisenberg antiferromagnet as a function of magnetic fields using both the exact diagonalization method and self-consistent Born approximation. Below the saturation field $B_C$, strong scattering between spin waves and a hole, created by photoemission of an electron, significantly narrows the quasiparticle band that is characterized by the lowering of the quasiparticle energy at $(π,π)$ with increasing field. Accordingly, in ARPES the quasiparticle peak gets shaper near $(π,π)$ and broader elsewhere. Furthermore, we …
We study the spin 1/2 triangular-lattice $J_1$-$J_2$-$J_3$ antiferromagnet close to the saturation field using the dilute Bose gas theory, where the magnetic structure is determined by the condensation of magnons. We focus on the case of ferromagnetic $J_1$ and antiferromagnetic $J_2,J_3$, that is particularly rich because frustration effects allow the single-magnon energy dispersion to have six-fold degenerate minima at incommensurate momenta. Our calculation also includes an interlayer coupling $J_0$, which covers both antiferromagnetic and ferromagnetic cases including negligibly small regi…
The magnetization process of the S=1/2 Heisenberg antiferromagnet on the kagome lattice is studied by the numerical-diagonalization method. We successfully obtain a new result of the magnetization process of a 42-site cluster in the entire range. Our analysis clarifies that the critical behavior around one-third of the height of the saturation is different from the typical behavior of the well-known magnetization plateau in two-dimensional systems. We also examine the effect of the $\sqrt{3}\times\sqrt{3}$-type distortion added to the kagome lattice. We find at one-third of the height of the s…
The critical exponent of the phase boundary has been examined on the three-dimensional incommensurate ordering phase in the spin-1/2 ferromagnetic-leg ladder 3-Br-4-F-V [=3-(3-bromo-4-fluorophenyl)-1,5-diphenylverdazyl]. Using the temperature-window fitting technique, we obtained the critical exponents which agreed with the three-dimensional (3D) Bose-Einstein condensation (BEC) universality class at both sides of the lower critical field and the saturation field. 3-Br-4-F-V thus becomes a new member of the quantum magnets which prove the universality of the 3D BEC exponent.
We discuss the magnetization process slightly below the saturation field in frustrated magnets. A condensation of bound magnons on the spin-polarized state induces either a spin nematic phase or a state with phase separation. The (effective) interaction between the bound magnon pairs not only is crucial to the stability of the nematic phase, but also determines the slope of the magnetization curve near saturation. We generally derive the expression of this interaction by using the perturbative scattering theory. By applying the method to coupled zigzag chains LiCuVO4, we find the positive pair…
We present a study of the dynamic structure factor of the antiferromagnetic spin-1/2 Heisenberg chain at finite temperatures and finite magnetic fields. Using Quantum-Monte-Carlo based on the stochastic series expansion and Maximum-Entropy methods we evaluate the longitudinal and the transverse dynamic structure factor from vanishing magnetic fields up to and above the threshold $B_c$ for ferromagnetic saturation, as well as for high and for intermediate temperatures. We study the field-induced redistribution of spectral weight contrasting longitudinal versus transverse excitations. At finite …
Quantum criticality of the spin-1/2 ferromagnetic-leg ladder 3-I-V [=3-(3-iodophenyl)-1,5-diphenylverdazyl] has been examined with respect to the antiferromagnetic to paramagnetic phase transition near the saturation field $H_{c}$. The phase boundary $T_{c}(H)$ follows the power-law $T_{c}(H)\propto H_{c}-H$ for a wide temperature range. This characteristic behavior is discussed as a quasi-one-dimensional (quasi-1D) Bose-Einstein condensation, which is predicted theoretically for weakly coupled quasi-1D ferromagnets. Thus, 3-I-V provides the first promising candidate for this attractive predic…
Excitonic insulators are usually considered to form via the condensation of a soft charge mode of bound electron-hole pairs. This, however, presumes that the soft exciton is of spin-singlet character. Early theoretical considerations have also predicted a very distinct scenario, in which the condensation of magnetic excitons results in an antiferromagnetic excitonic insulator state. Here we report resonant inelastic x-ray scattering (RIXS) measurements of Sr3Ir2O7. By isolating the longitudinal component of the spectra, we identify a magnetic mode that is well-defined at the magnetic and struc…
We report $^{133}$Cs nuclear magnetic resonance (NMR) measurements on the 2D frustrated Heisenberg antiferromagnet Cs$_2$CuCl$_4$ down to 2 K and up to 15 T. We show that $^{133}$Cs NMR is a good probe of the magnetic degrees of freedom in this material. Cu spin degrees of freedom are sensed through a strong anisotropic hyperfine coupling. The spin excitation gap opens above the critical saturation field. The gap value was determined from the activation energy of the nuclear spin-lattice relaxation rate in a magnetic field applied parallel to the Cu chains (b axis). The values of the g-factor …
The emergence of a finite staggered magnetization in quantum Heisenberg antiferromagnets subject to a uniform magnetic field can be viewed as Bose-Einstein condensation of magnons. Using non-perturbative results for the infrared behavior of the interacting Bose gas, we present exact results for the staggered spin-spin correlation functions of quantum antiferromagnets in a magnetic field at zero temperature. In particular, we show that in dimensions 1 < D <= 3 the longitudinal dynamic structure factor S_parallel(q,omega) describing staggered spin fluctuations in the direction of the staggered m…
We study the three-dimensional bosonic t-J model, i.e., the t-J model of "bosonic electrons" at finite temperatures. This model describes a system of cold bosonic atoms with two species in an optical lattice. The model is derived from the Hubbard model for very large on-site repulsive interaction between bosons of same species (hard-core nature) and also strong correlations between different species. The operator B_{xσ} for an atom at the site x with a two-component (pseudo-) spin σ(=1,2) is treated as a hard-core boson operator, and represented by a composite of two slave particles; a spinon …
We investigate the thermodynamic properties of the frustrated bilayer quantum Heisenberg antiferromagnet at low temperatures in the vicinity of the saturation magnetic field. The low-energy degrees of freedom of the spin model are mapped onto a hard-square gas on a square lattice. We use exact diagonalization data for finite spin systems to check the validity of such a description. Using a classical Monte Carlo method we give a quantitative description of the thermodynamics of the spin model at low temperatures around the saturation field. The main peculiarity of the considered two-dimensional…
We predict that spin-waves in an ordered quantum antiferromagnet (AFM) in a strong magnetic field become unstable with respect to spontaneous two-magnon decays. At zero temperature, the instability occurs between the threshold field $H^*$ and the saturation field $H_c$. As an example, we investigate the high-field dynamics of a Heisenberg antiferromagnet on a square lattice and show that the single-magnon branch of the spectrum disappears in the most part of the Brillouin zone.
Field-tuned incommensurate fan phase in an Ising-like triangular antiferromagnet
University of Oxford（牛津大学）；Institute for Solid State Physics, University of Tokyo（东京大学固体物理研究所）；Rutherford Appleton Laboratory（鲁瑟福阿普尔顿实验室）；University of Tennessee（田纳西大学）
Based on the slave-boson theory of the two-dimensional $t-t'-J$ model, we calculate the superconducting condensation energy for optimally doped and overdoped high $T_{c}$ cuprates at finite temperatures using a renormalized random phase approximation. The contributions come from the mean-field part and the antiferromagnetic spin fluctuations. In the presence of neutron resonance peak at $(π,π)$, the latter is shown to have similar temperature and doping dependences as the difference in antiferromagnetic (AF) exchange energy between the normal and the superconducting state. This difference has …
We report the results of magnetization and specific heat measurements of Ba$_2$CoTeO$_6$ composed of two subsystems A and B, which are magnetically described as an $S\,{=}\,1/2$ triangular-lattice Heisenberg-like antiferromagnet and a $J_1-J_2$ honeycomb-lattice Ising-like antiferromagnet, respectively. These two subsystems were found to be approximately decoupled. Ba$_2$CoTeO$_6$ undergoes magnetic phase transitions at $T_{\rm N1}\,{=}\,12.0$ K and $T_{\rm N2}\,{=}\,3.0$ K, which can be interpreted as the orderings of subsystems B and A, respectively. Subsystem A exhibits a magnetization plat…
Structural and magnetic properties of a quasi-one-dimensional spin-$1/2$ compound NaVOPO$_4$ are explored by x-ray diffraction, magnetic susceptibility, high-field magnetization, specific heat, electron spin resonance, and $^{31}$P nuclear magnetic resonance measurements, as well as complementary \textit{ab initio} calculations. Whereas magnetic susceptibility of NaVOPO$_4$ may be compatible with the gapless uniform spin chain model, detailed examination of the crystal structure reveals a weak alternation of the exchange couplings with the alternation ratio $α\simeq 0.98$ and the ensuing zero-…
We investigate the critical properties of the $S=1/2$ bond-alternating spin chain with a next-nearest-neighbor interaction in magnetic fields. By the numerical calculation and the exact solution based on the effective Hamiltonian, we show that there is a parameter region where the longitudinal incommensurate spin correlation becomes dominant around the half-magnetization of the saturation. Possible interpretations of our results are discussed. We next investigate the effects of the interchain interaction ($J^{\prime}$). The staggered susceptibility and the uniform magnetization are calculated …
We study the interplay between disorder and interactions for emergent bosonic degrees of freedom induced by an external magnetic field in the Br-doped spin-gapped antiferromagnetic material Ni(Cl$_{1-x}$Br$_x$)$_2$-4SC(NH$_2$)$_2$ (DTNX). Building on nuclear magnetic resonance experiments at high magnetic field [A. Orlova et al., Phys. Rev. Lett. 118, 067203 (2017)], we describe the localization of isolated impurity states, providing a realistic theoretical modeling for DTNX. Going beyond single impurity localization we use quantum Monte Carlo simulations to explore many-body effects from whic…
We predict that an external field can induce a spin order in highly frustrated classical Heisenberg magnets. We find analytically stabilization of collinear states by thermal fluctuations at a one-third of the saturation field for kagome and garnet lattices and at a half of the saturation field for pyrochlore and frustrated square lattices. This effect is studied numerically for the frustrated square-lattice antiferromagnet by Monte Carlo simulations for classical spins and by exact diagonalization for $S=1/2$. The field induced collinear states have a spin gap and produce magnetization platea…
Motivated by recent experimental processes, we systemically investigate strongly correlated spin-1 ultracold bosons trapped in a three-dimensional optical lattice in the presence of an external magnetic field. Based on a recently developed bosonic dynamical mean-field theory (BDMFT), we map out complete phase diagrams of the system for both antiferromagnetic and ferromagnetic interactions, where various phases are found as a result of the interplay of spin-dependent interaction and quadratic Zeeman energy. For antiferromagnetic interactions, the system demonstrates competing magnetic orders, i…
We clarify the existence of several magnetization plateaux for the kagome $S=1/2$ antiferromagnetic Heisenberg model in a magnetic field. Using approximate or exact localized magnon eigenstates, we are able to describe in a similar manner the plateau states that occur for magnetization per site $m=1/3$, $5/9$, and $7/9$ of the saturation value. These results are confirmed using large-scale Exact Diagonalization on lattices up to 63 sites.
We discuss theoretically a frustrated Heisenberg antiferromagnet in magnetic field close to the saturation one. It is demonstrated that a small biaxial anisotropy and/or the magnetic dipolar interaction produce a delicate balance between phases with a commensurate canted, incommensurate helical (conical), and fan spin orderings. As a result, different sequences of phase transitions are realized depending on values of these small anisotropic interactions. We derive analytical expressions for critical fields and ground-state energies of the phases which are in a quantitative agreement with our a…
Motivated by the low temperature magnetization curves of several spinel chromites, we theoretically study classical mechanisms of degeneracy lifting in pyrochlore antiferromagnets. Our main focus is on the coupling of spin exchange to lattice distortions. Prior work by Penc et al. (Phys. Rev. Lett. 93, 197203 (2004)) has demonstrated that such coupling leads to a robust magnetization plateau at half the saturation moment per spin, in agreement with experiment. We show that a simple Einstein model incorporating local site distortions generates a ``universal'' magnetic order on the plateau, and …
The magnetization process of an S=1/2 antiferromagnet on the kagome lattice, [Cu_3(titmb)_2(OCOCH_3)_6]H_2O {titmb= 1,3,5-tris(imidazol-1-ylmethyl)-2,4,6 trimethylbenzene} has been measured at very low temperatures in both pulsed and steady fields. We have found a new dynamical behavior in the magnetization process: a plateau at one third of the saturation magnetization appears in the pulsed field experiments for intermediate sweep rates of the magnetic field and disappears in the steady field experiments. A theoretical analysis using exact diagonalization yields J_1=-19K and J_2=6K, for the n…
Motivated by recent experiments on low-dimensional quantum magnets in applied magnetic fields, we present a theoretical analysis of their properties based on the nonlinear sigma model. The spin stiffness and a 1/N expansion are used to map the regimes of spin-gap behavior, predominantly linear magnetization, and spin saturation. A two-parameter renormalization-group study gives the characteristic properties over the entire parameter range. The model is relevant to many systems exhibiting Haldane physics, and is applied here to the two-chain spin ladder compound CuHpCl.
Ba3Mn2O8 is a spin-dimer compound based on pairs of S = 1, 3d2, Mn5+ ions arranged on a triangular lattice. Antiferromagnetic intradimer exchange leads to a singlet ground state in zero-field, with excited triplet and quintuplet states at higher energy. High field thermodynamic measurements are used to establish the phase diagram, revealing a substantial asymmetry of the quintuplet condensate. This striking effect, all but absent for the triplet condensate, is due to a fundamental asymmetry in quantum fluctuations of the paramagnetic phases near the various critical fields.
Magnon Bose condensation (BC)in the symmetry breaking magnetic field is a result of unusual form of the Zeeman energy, which has terms linear in the spin-wave operators and terms mixing excitations differ in the Wave-vector of the magnetic structure. The following examples are considered: simple easy-plane tetragonal antiferromagnets (AF), frustrated AF family$R_2Cu O_4$ where $R=Pr,Nd$ etc. and cubic magnets with the Dzyaloshinskii-Moriya interaction ($Mn Si$ etc.). In all cases the BC becomes important when the magnetic field becomes comparable with the spin-wave gap. The theory is illustrat…
We report the results of magnetization and specific heat measurements on Ba$_3$NiSb$_2$O$_9$, which is a quasi-two-dimensional spin-1 triangular-lattice antiferromagnet. We observed a nonclassical magnetization plateau at one-third of the saturation magnetization that is driven by spin frustration and quantum fluctuation. Exact diagonalization for a 21-site rhombic cluster was performed to analyze the magnetization process. Experimental and calculated results agree well.
We investigate the nature of the magnetic excitations of a bilayer single-orbital Hubbard model in the intermediate-coupling regime. This model exhibits a quantum phase transition (QPT) between a paramagnetic (PM) and an insulating antiferromagnetic (AFM) phase at a critical value of the coupling strength. By using the random phase approximation, we show that the QPT is continuous when the PM state is a band insulator and that the corresponding quantum critical point (QCP) arises from the condensation of preformed excitons. These low-energy excitons reemerge on the other side of the QCP as the…
We present the zero temperature phase diagram of a Heisenberg antiferromagnet on a frustrated triangular lattice with nearest neighbor ($J_1$) and next nearest neighbor ($J_2$) interactions, in a magnetic field. We show that the classical model has an accidental degeneracy for all $J_2/J_1$ and all fields, but the degeneracy is lifted by quantum fluctuations. We show that at large $S$, for $J_2/J_1 <1/8$, quantum fluctuations select the same sequence of three sublattice co-planar states in a field as for $J_2 =0$, and for $1/8<J_2/J_1 <1$ they select the canted stripe state for all non-zero fi…
We study the ground state properties of a quantum antiferromagnet in the kagome lattice in the presence of a magnetic field, paying particular attention to the stability of the plateau at magnetization 1/3 of saturation. While the plateau is reinforced by certain deformations of the lattice, like the introduction of structural defect lines and against an Ising anisotropy, ground state correlations are seen to be quite different and the undistorted SU(2) case appears to be rather special.
