We determine the complete set of generalized spin squeezing inequalities, given in terms of the collective angular momentum components, for particles with an arbitrary spin. They can be used for the experimental detection of entanglement in an ensemble in which the particles cannot be individually addressed. We also present a large set of criteria involving collective observables different from the angular momentum coordinates. We show that some of the inequalities can be used to detect k-particle entanglement and bound entanglement.
By identifying non-local effects in systems of identical Bosonic qubits through correlations of their commuting observables, we show that entanglement is not necessary to violate certain squeezing inequalities that hold for distinguishable qubits and that spin squeezing may not be necessary to achieve sub-shot noise accuracies in ultra-cold atom interferometry.
A complete set of generalized spin-squeezing inequalities is derived for an ensemble of particles with an arbitrary spin. Our conditions are formulated with the first and second moments of the collective angular momentum coordinates. A method for mapping the spin-squeezing inequalities for spin-1/2 particles to entanglement conditions for spin-j particles is also presented. We apply our mapping to obtain a generalization of the original spin-squeezing inequality to higher spins. We show that, for large particle numbers, a spin-squeezing parameter for entanglement detection based on one of our …
We derive spin squeezing inequalities that generalize the concept of the spin squeezing parameter and provide necessary and sufficient conditions for genuine 2-, or 3- qubit entanglement for symmetric states, and sufficient condition for general states of $N$ qubits. Our inequalities have a clear physical interpretation as entanglement witnesses, can be relatively easy measured, and are given by complex, but {\it elementary} expressions.
Particle number fluctuations, no matter how small, are present in experimental set-ups. One should rigorously take these fluctuations into account, especially, for entanglement detection. In this context, we generalize the spin squeezing inequalities introduced by Tóth et al. in Phys. Rev. Lett. 99, 250405 (2007). These new inequalities are fulfilled by all separable states even when the number of particle is not constant, and may present quantum fluctuations. These inequalities are useful for detecting entanglement in many-body systems when the super-selection rule does not apply, or when onl…
Spin squeezing inequalities (SSI) represent a major tool to probe quantum entanglement among a collection of few-level atoms, and are based on collective spin measurements and their fluctuations. Yet, for atomic ensembles of spin-$j$ atoms and ultracold spinor gases, many experiments can image the populations in all Zeeman sublevels $s=-j, -j+1, \dots, j$, potentially revealing finer features of quantum entanglement not captured by SSI. Here we present a systematic approach which exploits Zeeman-sublevel population measurements in order to construct novel entanglement criteria, and illustrate …
We present detailed derivations, various improvements and application to concrete experimental data of spin squeezing inequalities formulated recently by some of us [Phys. Rev. Lett. {\bf 95}, 120502 (2005)]. These inequalities generalize the concept of the spin squeezing parameter, and provide necessary and sufficient conditions for genuine 2-, or 3- qubit entanglement for symmetric states, and sufficient entanglement condition for general $N$-qubit states. We apply our method to theoretical study of Dicke states, and, in particular, to $W$-states of $N$ qubits. Then, we analyze the recently …
We determine the complete set of generalized spin squeezing inequalities. These are entanglement criteria that can be used for the experimental detection of entanglement in a system of spin-1/2 particles in which the spins cannot be individually addressed. They can also be used to show the presence of bound entanglement in the thermal states of several spin models.
What is the relation between spin squeezing and entanglement? To clarify this, we derive the full set of generalized spin squeezing inequalities for the detection of entanglement. These are inequalities for the mean values and variances of the collective angular momentum components J_k. They can be used for the experimental detection of entanglement in a system of spin-1/2 particles in which the spins cannot be individually addressed. We present various sets of inequalities that can detect all entangled states that can be detected based on the knowledge of: (i) the mean values and variances of…
We propose a method to infer the single-particle entropy of bosonic atoms in an optical lattice and to study the local evolution of entropy, spin squeezing, and entropic inequalities for entanglement detection in such systems. This method is based on experimentally feasible measurements of non-nearest-neighbour coherences. We study a specific example of dynamically controlling atom tunneling between selected sites and show that this could potentially also improve the metrologically relevant spin squeezing.
In analogy with the spin-squeezing inequality of Wang and Sanders [Physical Review A 68, 012101 (2003)], we find inequalities describing macroscopic polarization correlations that are obeyed by all classical fields, and whose violation implies entanglement of the photons that make up the optical beam. We consider a realistic and exactly-solvable experimental scenario employing polarization- squeezed light from an optical parametric oscillator (OPO) and find that any two photons separated by less than the OPO coherence time are polarization entangled. The polarization entanglement is robust aga…
Bell's inequality for continuous-variable bipartite systems is studied. The inequality is expressed in terms of pseudo-spin operators and quantum expectation values are calculated for generic two-mode squeezed states characterized by a squeezing parameter $r$ and a squeezing angle $φ$. Allowing for generic values of the squeezing angle is especially relevant when $φ$ is not under experimental control, such as in cosmic inflation, where small quantum fluctuations in the early Universe are responsible for structures formation. Compared to previous studies restricted to $φ=0$ and to a fixed orien…
We establish a connection between quantum inequalities (known from quantum field theory on curved spacetimes) and the degree of squeezing in quantum-optical experiments. We prove an inequality which binds the reduction of the electric-field fluctuations to their duration. The bigger the level of fluctuations-suppression the shorter its duration. As an example of the application of this inequality in the case of squeezed light whose phase is controlled with 1% accuracy we derive a limit of -15dB on the allowed degree of squeezing.
We extend the criteria for $k$-particle entanglement from the spin squeezing parameter presented in [A.S. Sørensen and K. Mølmer, Phys. Rev. Lett. {\bf 86}, 4431 (2001)] to systems with a fluctating number of particles. We also discuss how other spin squeezing inequalities can be generalized to this situation. Further, we give an operational meaning to the bounds for cases where the individual particles cannot be addressed. As a by-product, this allows us to show that in spin squeezing experiments with cold gases the particles are typically distinguishable in practise. Our results justify the …
Quantum electronic noise, the random current fluctuations generated by electrons crossing a quantum conductor, has been thoroughly studied from the electron point of view. Recent experiments have shown that such noise may have striking properties in terms of the quantum electromagnetic field it generates. Both the existence of vacuum squeezing \cite{PAN_squeezing} and generation of correlated photon pairs \cite{C4quantique} have been observed. Here we demonstrate that this electromagnetic field also violates Bell-like inequalities, thereby proving its true quantum nature. This is achieved by t…
In spin-1 collective atomic systems, the spin and nematic-tensor operators constitute the su(3) Lie algebra whose su(2) subalgebras are shown to give two distinct classes of squeezing which are unitarily equivalent to spin squeezing and spin-nematic squeezing. We explicitly construct a unitary operator that generates an arbitrary squeezed spin-nematic state from an arbitrary Fock state. In particular, we demonstrate that squeezed spin states can be generated from a polar state and that squeezed spin-nematic sates can be generated from a fully spin-polarized state.
The explicit dynamics of the moments for the GKSL equation is obtained. In our case the GKSL equation corresponds to Poisson stochastic processes which lead to unitary jumps. We consider squeeze operators as the unitary jumps.
We propose a new spin squeezing criterion for arbitrary multi-qubit states that is invariant under local unitary operations. We find that, for arbitrary pure two-qubit states, spin squeezing is equivalent to entanglement, and multi-qubit states are entangled if this new spin squeezing parameter is less than 1.
Temporal Bell inequalities, or Leggett-Garg Inequalities (LGI), are studied for continuous-variable systems placed in a squeezed state. The importance of those systems lies in their broad applicability which allows the description of many different physical settings in various branches of physics, ranging from cosmology to condensed matter physics and from optics to quantum information theory. LGI violations are explored and systematically mapped in squeezing parameter space. Configurations for which LGI violation occurs are found but it is shown that no violation can be obtained if all squeez…
Three-outcome multipartite Bell inequalities: applications to dimension witnessing and spin-nematic squeezing in many-body systems
ICFO-Institut de Ciencies Fotoniques, The Barcelona Institute of Science and Technology（ICFO-光子科学研究所，巴塞罗那科学技术研究所）；Institute for Quantum Optics and Quantum Information, Austrian Academy of Sciences（奥地利科学院量子光学与量子信息研究所）；Vienna Center for Quantum Science and Technology (VCQ), Faculty of Physics, University of Vienna（维也纳大学物理学院量子科学与技术维也纳中心）；ICREA（加泰罗尼亚高级研究局）；Department of Physics, ETH Zürich（苏黎世联邦理工学院物理系）；Instituut-Lorentz, Universiteit Leiden（莱顿大学洛伦兹研究所）
We propose an implementation of the parametric amplification of an arbitrary radiation-field state previously prepared in a high-Q cavity. This nonlinear process is accomplished through the dispersive interactions of a single three-level atom (fundamental |g>, intermediate |i>, and excited |e> levels) simultaneously with i) a classical driving field and ii) a previously prepared cavity mode whose state we wish to squeeze. We show that, in the adiabatic approximantion, the preparation of the initial atomic state in the intermediate level |i> becomes crucial for obtaing the degenerated parametri…
As the generation of squeezed states of light has become a standard technique in laboratories, attention is increasingly directed towards adapting the optical parameters of squeezed beams to the specific requirements of individual applications. It is known that imaging, metrology, and quantum information may benefit from using squeezed light with a tailored transverse spatial mode. However, experiments have so far been limited to generating only a few squeezed spatial modes within a given setup. Here, we present the generation of single-mode squeezing in Laguerre-Gauss and Bessel-Gauss modes, …
We extend the definition of generalized coherent states to include the case of time-dependent dispersion. We introduce a suitable operator providing displacement and dynamical rescaling from an arbitrary ground state. As a consequence, squeezing is naturally embedded in this framework, and its dynamics is ruled by the evolution equation for the dispersion. Our construction provides a displacement-operator method to obtain the squeezed states of arbitrary systems.
We examine transfer of particle entanglement and spin squeezing between atomic and photonic subsystems in optical cavities coupled by two-photon exchange. Each cavity contains a single atom, interacting with cavity photons with a two-photon cascade transition. Particle entanglement is characterized by evaluating optimal spin squeezing inequalities, for the cases of initially separable and entangled two-photon states. It is found that particle entanglement is first generated among the photons in separate cavities and then transferred to the atoms. The underlying mechanism is recognized as an in…
We have developed a quantum memory technique that is completely compatible with current quantum information processing for continuous variables of light, where arbitrary frequency sidebands of a squeezed vacuum can be stored and retrieved using bichromatic electromagnetic induced transparency. 2MHz sidebands of squeezed vacuum pulses with temporal widths of 470ns and a squeezing level of -1.78 +- 0.02dB were stored for 3us in the laser-cooled 87Rb atoms. -0.44 +- 0.02dB of squeezing was retrieved, which is the highest squeezing ever reported for a retrieved pulse.
We consider a way to generate operational inequalities to test nonclassicality (or quantumness) of multimode (or multiparty) bosonic fields that unifies the derivation of many known inequalities and allows to propose new ones. The nonclassicality criteria are based on Vogel's criterion corresponding to analyzing the positivity of multimode P functions or, equivalently, the positivity of matrices of expectation values of, e.g., creation and annihilation operators. We analyze not only monomials, but also polynomial functions of such moments, which can sometimes enable simpler derivations of phys…
We demonstrate two simple theorems about squeezing induced by bilinear spin-spin interactions that conserve spin parity -- including a vast majority of quantum spin models implemented by state-of-the-art quantum simulators. In particular we show that squeezing captures the first form of quantum correlations which are produced: 1) at equilibrium, by adiabatically turning on the spin-spin interactions starting from a factorized state aligned with an external, arbitrary field; 2) away from equilibrium, by evolving unitarily the same state with the interacting Hamiltonian.
Planar squeezed states, i.e. quantum states which are squeezed in two orthogonal spin components, have recently attracted attention due to their applications in atomic interferometry and quantum information [Q. Y. He et al, New J. Phys. 14, 093012 (2012)]. While canonical variables such as quadratures of the radiation field can be squeezed in at most one component, simultaneous squeezing in two orthogonal spin components can be achieved due to the angular momentum commutation relations. We present a novel scheme for planar squeezing via quantum non-demolition (QND) measurements in spin-1 syste…
The concept of entangled quantum states is considered in the context of systems of identical particles, based on the requirement that in order to represent physical states both for the overall system and the sub-systems which may be entangled, the density operators must satisfy the symmetrisation principle and global and local super-selection rules that prohibit states in which there are coherences between differing particle numbers. These requirements and their justification are fully discussed. In the second quantisation approach used, both the system and the sub-systems are modes (or sets o…
Phenomena such as state-swap, quadrature squeezing, entanglement and violation of entanglement inequalities are frequently reported to occur in quantum systems only. It is shown here that these effects can also occur in cholesteric liquid crystals in the presence of an applied magnetic field. The nature of these effects as well as the conditions for their observation are analysed.
We present generic Bell inequalities for multipartite multi-dimensional systems. The inequalities that any local realistic theories must obey are violated by quantum mechanics for even-dimensional multipartite systems. A large set of variants are shown to naturally emerge from the generic Bell inequalities. We discuss particular variants of Bell inequalities, that are violated for all the systems including odd-dimensional systems.
There is currently much interest in the two-axis countertwisting spin squeezing Hamiltonian suggested originally by Kitagawa and Ueda, since it is useful for interferometry and metrology. No analytical solution valid for arbitrary spin values seems to be available. In this article we systematically consider the issue of the analytical solvability of this Hamiltonian for various specific spin values. We show that the spin squeezing dynamics can be considered to be analytically solved for angular momentum values upto $21/2$, i.e. for $21$ spin half particles. We also identify the properties of t…
Theoretical models of spins coupled to bosons provide a simple setting for studying a broad range of important phenomena in many-body physics, from virtually mediated interactions to decoherence and thermalization. In many atomic, molecular, and optical systems, such models also underlie the most successful attempts to engineer strong, long-ranged interactions for the purpose of entanglement generation. Especially when the coupling between the spins and bosons is strong---such that it cannot be treated perturbatively---the properties of such models are extremely challenging to calculate theore…
Based on the generators of $SU(n)$ we present inequalities for detecting quantum entanglement for $2 \otimes d$ and $M \otimes N$ systems. These inequalities provide a sufficient condition of entanglement for bipartite mixed states and give rise to an experimental way of entanglement detection.
We show that an ensemble of identical d-level atoms can be efficiently described by d-1 collective oscillator degrees of freedom in the vicinity of a product state with all atoms in the same, but otherwise arbitrary single-particle state. We apply our description to two different kinds of spin squeezing: (i) when each spin-F atom is individually squeezed without creating interatomic entanglement and (ii) when a particular collective atomic oscillator mode is squeezed via quantum non-demolition (QND) measurement and feedback. When combined in sequence, the order of the two methods is relevant i…
We provide a generalization for the polygamy constraint of multiparty entanglement in arbitrary dimensional quantum systems. By using the $β$th-power of entanglement of assistance for $0\leq β\leq1$ and the Hamming weight of the binary vector related with the distribution of subsystems, we establish a class of weighted polygamy inequalities of multiparty entanglement in arbitrary dimensional quantum systems. We further show that our class of weighted polygamy inequalities can even be improved to be tighter inequalities with some conditions on the assisted entanglement of bipartite subsystems.
We show that spin squeezing implies pairwise entanglement for arbitrary symmetric multiqubit states. If the squeezing parameter is less than or equal to 1, we demonstrate a quantitative relation between the squeezing parameter and the concurrence for the even and odd states. We prove that the even states generated from the initial state with all qubits being spin down, via the one-axis twisting Hamiltonian, are spin squeezed if and only if they are pairwise entangled. For the states generated via the one-axis twisting Hamiltonian with an external transverse field for any number of qubits great…
We investigate polygamy relations of multipartite entanglement in arbitrary-dimensional quantum systems. By improving an inequality and using the $β$th ($0\leqβ\leq1$) power of entanglement of assistance, we provide a new class of weighted polygamy inequalities of multipartite entanglement in arbitrary-dimensional quantum systems. We show that these new polygamy relations are tighter than the ones given in [Phys. Rev. A 97, 042332 (2018)].
We investigate the exact dynamics of a system of two independent harmonic oscillators coupled through their angular momentum. The exact analytic solution of the equations of motion for the field operators is derived, and the conditions for dynamical stability are obtained. As application, we examine the emergence of squeezing and mode entanglement for an arbitrary separable coherent initial state. It is shown that close to instability, the system develops considerable entanglement, which is accompanied with simultaneous squeezing in the coordinate of one oscillator and the momentum of the othe…
We derive a Bell-type inequality for observables with arbitrary spectra. For the case of continuous variable systems we propose a possible experimental violation of this inequality, by using squeezed light and homodyne detection together with methods of quantum-state reconstruction. It is shown that the violation is also possible for realistic detection efficiencies.
Robust spin-squeezing with random interaction graphs: the lesson from universality
Max Planck Institute for the Physics of Complex Systems（马克斯·普朗克复杂系统物理研究所）；CNR-INO（国家研究委员会光学研究所）；LENS（欧洲非线性科学实验室）；Institute for Quantum Optics and Quantum Information of the Austrian Academy of Sciences（奥地利科学院量子光学与量子信息研究所）；Institute for Theoretical Physics, University of Innsbruck（因斯布鲁克大学理论物理研究所）；Institut für Theoretische Physik, ETH Zürich（苏黎世联邦理工学院理论物理研究所）；CNR-INO, Area Science Park, Basovizza（国家研究委员会光学研究所，巴斯维察科学园区）
We propose a generalized structure of Bell inequalities for arbitrary d-dimensional bipartite systems, which includes the existing two types of Bell inequalities introduced by Collins-Gisin-Linden-Massar-Popescu [Phys. Rev. Lett. 88, 040404 (2002)] and Son-Lee-Kim [Phys. Rev. Lett. 96, 060406 (2006)]. We analyze Bell inequalities in terms of correlation functions and joint probabilities, and show that the coefficients of correlation functions and those of joint probabilities are in Fourier transform relations. We finally show that the coefficients in the generalized structure determine the cha…
Pairwise entanglement properties of a symmetric multi-qubit system are analyzed through a complete set of two-qubit local invariants. Collective features of entanglement, such as spin squeezing, are expressed in terms of invariants and a classifcation scheme for pairwise entanglement is proposed. The invariant criteria given here are shown to be related to the recently proposed (Phys. Rev. Lett. 95, 120502 (2005)) generalized spin squeezing inequalities for pairwise entanglement in symmetric multi-qubit states.
We introduce an entanglement-depth criterion optimized for planar quantum squeezed (PQS) states. It is connected with the sensitivity of such states for estimating an arbitrary, not necessarily small phase. We compare numerically our criterion with the well-known extreme spin squeezing condition of Sørensen and Mølmer [Phys. Rev. Lett. 86, 4431 (2001)] and show that our condition detects a higher depth of entanglement when both planar spin variances are squeezed below the standard quantum limit. We employ our theory to monitor the entanglement dynamics in a PQS state produced via quantum non-d…
In an ensemble of two-level atoms that can be described in terms of a collective spin, entangled states can be used to enhance the sensitivity of interferometric precision measurements. While non-Gaussian spin states can produce larger quantum enhancements than spin-squeezed Gaussian states, their use requires the measurement of observables that are nonlinear functions of the three components of the collective spin. In this paper we develop strategies that achieve the optimal quantum enhancements using non-Gaussian states produced by a nonlinear one-axis-twisting Hamiltonian, and show that mea…
In contrast to the canonically conjugate variates $q$,$p$ representing the position and momentum of a particle in the phase space distributions, the three Cartesian components, $J_{x}$,$J_{y}$, $J_{z}$ of a spin-$j$ system constitute the mutually non-commuting variates in the quasi-probabilistic spin distributions. It can be shown that a univariate spin distribution is never squeezed and one needs to look into either bivariate or trivariate distributions for signatures of squeezing. Several such distributions result if one considers different characteristic functions or moments based on variou…
Bell inequalities bound the strength of classical correlations between observers measuring on a shared physical system. However, studies of physical correlations can be considered beyond the standard Bell scenario by networks of observers sharing some configuration of many independent physical systems. Here, we show how to construct Bell-type inequalities for correlations arising in any tree-structured network i.e. networks without cycles. This is achieved by an iteration procedure that in each step allows one to add a branch to the tree-structured network and construct a corresponding Bell-ty…
We present a set of Bell inequalities which are sufficient and necessary for separability of general pure multipartite quantum states in arbitrary dimensions. The relations between Bell inequalities and distillability are also studied. We show that any quantum states that violate one of these Bell inequalities are distillable.
Characterizing trade-offs between simultaneous violations of multiple Bell inequalities in a large network of qubits is computationally demanding. We propose a graph-theoretic approach to efficiently produce Bell monogamy relations in arbitrary arrangements of qubits. All the relations obtained for bipartite Bell inequalities are tight and leverage only a single Bell monogamy relation. This feature is unique to bipartite Bell inequalities, as we show that there is no finite set of such elementary monogamy relations for multipartite inequalities. Nevertheless, many tight monogamy relations for …
In device-independent quantum information processing Bell inequalities are not only used as detectors of nonlocality, but also as certificates of relevant quantum properties. In order for these certificates to work, one very often needs Bell inequalities that are maximally violated by specific quantum states. Recently, in [A. Salavrakos et al., Phys. Rev. Lett. 119, 040402 (2017)] a general class of Bell inequalities, with arbitrary numbers of measurements and outcomes, has been designed, which are maximally violated by the maximally entangled states of two quantum systems of arbitrary dimensi…
We examine how non-destructive measurements generate spin squeezing in an atomic Bose-Einstein condensate confined in a double-well trap. The condensate in each well is monitored using coherent light beams in a Mach-Zehnder configuration that interacts with the atoms through a quantum nondemolition Hamiltonian. We solve the dynamics of the light-atom system using an exact wavefunction approach, in the presence of dephasing noise, which allows us to examine arbitrary interaction times and a general initial state. We find that monitoring the condensate at zero detection current and with identica…
We study the generation of planar quantum squeezed (PQS) states by quantum non-demolition (QND) measurement of a cold ensemble of $^{87}$Rb atoms. Precise calibration of the QND measurement allows us to infer the conditional covariance matrix describing the $F_y$ and $F_z$ components of the PQS, revealing the dual squeezing characteristic of PQS. PQS states have been proposed for single-shot phase estimation without prior knowledge of the likely values of the phase. We show that for an arbitrary phase, the generated PQS gives a metrological advantage of at least 3.1 dB relative to classical st…
