We derive a number of exact relations between equilibrium and nonequilibrium quantities for spin glasses in external fields using the Jarzynski equality and gauge symmetry. For randomly-distributed longitudinal fields, a lower bound is established for the work done on the system in nonequilibrium processes, and identities are proven to relate equilibrium and nonequilibrium quantities. In the case of uniform transverse fields, identities are proven between physical quantities and exponentiated work done to the system at different parts of the phase diagram with the context of quantum annealing in mind. Additional relations are given, which relate the exponentiated work in quantum and simulated (classical) annealing. It is also suggested that the Jarzynski equality may serve as a guide to develop a method to perform quantum annealing under non-adiabatic conditions.
The applications of nonequilbrium relations such as the Jarzynski equality and the fluctuation theorem to spin glasses are considered. The spin glass is a basic platform where we consider an application of an approximate solver of combinatorial optimization problems, simulated annealing. We find a novel relationship between an average through a nonequilibrium process where the temperature changes as in simulated annealing and a thermal average in equilibrium with different amounts of quenched randomness. The results shown in the present study may serve as an alternative way to overcome critica…
The non-equilibrium dynamics of the three-dimensional Edwards-Anderson spin-glass model with different bond distributions is investigated by means of Monte Carlo simulation. A numerical method is used to determine the critical temperature and the scaling exponents of the correlation and the integrated response functions. The results obtained agree with those calculated in equilibrium simulations and suggest that the universality class does not depend on the exact form of the bond distribution.
We discuss the slow, nonequilibrium, dynamics of spin glasses in their glassy phase. We briefly review the present theoretical understanding of the spectacular phenomena observed in experiments and describe new numerical results obtained in the first large-scale simulation of the nonequilibrium dynamics of the three dimensional Heisenberg spin glass.
Motivated by short-range Ising spin glasses, we review some rigorous results and their consequences for the relation between the number/nature of equilibrium pure states and nonequilibrium dynamics. Two of the consequences for spin glass dynamics following a deep quench to a temperature with broken spin flip symmetry are: (1) Almost all initial configurations lie on the boundary between the basins of attraction of multiple pure states. (2) Unless there are uncountably many pure states with almost all pairs having zero overlap, there can be no equilibration to a pure state as time goes to infin…
In these lectures, which were presented at "Soft and Fragile Matter, Nonequilibrium Dynamics, Metastability and Flow" University of St. Andrews, 8 July - 22 July, 1999, I give an introduction to the physics of supercooled liquids and glasses and discuss some computer simulations done to investigate these systems.
We present a mean field model for spin glasses with a natural notion of distance built in, namely, the Edwards-Anderson model on the diluted D-dimensional unit hypercube in the limit of large D. We show that finite D effects are strongly dependent on the connectivity, being much smaller for a fixed coordination number. We solve the non trivial problem of generating these lattices. Afterwards, we numerically study the nonequilibrium dynamics of the mean field spin glass. Our three main findings are: (i) the dynamics is ruled by an infinite number of time-sectors, (ii) the aging dynamics consist…
We have studied numerically the dynamics of spin glasses with Ising and XY symmetry (gauge glass) in space dimensions 2, 3, and 4. The nonequilibrium spin-glass susceptibility and the nonequilibrium energy per spin of samples of large size L_b are measured as a function of anneal time t_w after a quench to temperatures T. The two observables are compared to the equilibrium spin-glass susceptibility and the equilibrium energy, respectively, measured as functions of temperature T and system size L for a range of system sizes. For any time and temperature a nonequilibrium time-dependent length sc…
We investigate spin-spin correlation functions in the low temperature phase of spin-glasses. Using the replica field theory formalism, we examine in detail their infrared (long distance) behavior. In particular we identify a longitudinal mode that behaves as massive at intermediate length scales (near-infrared region). These issues are then addressed by numerical simulation; the analysis of our data is compatible with the prediction that the longitudinal mode appears as massive, i.e., that it undergoes an exponential decay, for distances smaller than an appropriate correlation length.
Quantum annealing is a generic solver of classical optimization problems that makes full use of quantum fluctuations. We consider work statistics given by a repetition of quantum annealing processes by employing the Jarzynski equality proposed in nonequilibrium statistical physics. In particular, we analyze the distribution of the work performed by a transverse field. A special symmetry, gauge symmetry, leads to a non-trivial relationship between quantum annealing toward different targets in the theory of spin glasses. We believe that our results will be a step toward an alternative realizatio…
We introduce a set of theoretical ideas that form the basis for an analytical framework capable of describing nonequilibrium dynamics in glassy systems. We test the resulting scenario by comparing its predictions with numerical simulations of short-range spin glasses. Local fluctuations and responses are shown to be connected by a generalized local out-of-equilibrium fluctuation-dissipation relation. Scaling relationships are uncovered for the slow evolution of heterogeneities at all time scales.
The random first order transition theory of the dynamics of supercooled liquids is extended to treat aging phenomena in nonequilibrium structural glasses. A reformulation of the idea of ``entropic droplets'' in terms of libraries of local energy landscapes is introduced which treats in a uniform way the supercooled liquid (reproducing earlier results) and glassy regimes. The resulting microscopic theory of aging makes contact with the Nayaranaswamy-Moynihan-Tool nonlinear relaxation formalism and the Hodge-Scherer extrapolation of the Adam-Gibbs formula, but deviations from both approaches are…
We determine explicitly and discuss in detail the effects of the joint presence of a longitudinal and a transversal (random) magnetic field on the phases of the Random Energy Model (REM) and its hierarchical generalization, the GREM. Our results extent known results both in the classical case of vanishing transversal field and in the quantum case for vanishing longitudinal field. Following Derrida and Gardner, we argue that the longitudinal field has to be implemented hierarchically also in the Quantum GREM. We show that this ensures the shrinking of the spin glass phase in the presence of the…
We present new data on the nonequilibrium acoustic response of glasses to an applied dc electric field below 1K. When compared with the analogous dielectric response of the same material, the acoustic data show, within experimental precision, identical dependence on the perturbing field, but stronger temperature dependence. These data are difficult to reconcile with simple generalizations of the dipole gap model of two-level system (TLS) dielectric response, unless we assume that as T is decreased, interaction-based TLS collective effects increase.
We point out a possibility of the weak universality of spin-glass phase transitions in three dimensions. The Ising, the XY, and the Heisenberg models with $\pm J$ bond distributions undergo finite-temperature phase transitions with a ratio of critical exponents $γ/ν=2.4$. Evaluated critical exponents agree with corresponding experimental results. The analyses are based upon the nonequilibrium relaxation from the paramagnetic state and the finite-time scaling.
Localisation-protected quantum order extends the idea of symmetry breaking and order in ground states to individual eigenstates at arbitrary energy. Examples include many-body localised static and $π$-spin glasses in Floquet systems. Such order is inherently dynamical and difficult to detect as the order parameter typically varies randomly between different eigenstates, requiring specific superpositions of eigenstates to be targeted by the initial state. We show that two-time correlators overcome this, reflecting the presence or absence of eigenstate order even in fully-mixed, $infinite$ $temp…
The dynamic structure factor of glassy and liquid glycerol has been measured by inelastic X-ray scattering in the exchanged momentum ($Q$) region $Q$=2$÷$23 nm$^{-1}$ and in the temperature range 80$÷$570 K. Beside the propagating longitudinal excitations modes, at low temperature the spectra show a second non $Q$-dispersing peak at $\hbar Ω_T$$\approx$8.5 meV. We assign this peak to the transverse dynamics that, in topologically disordered systems, acquires a longitudinal symmetry component. This assignment is substantiated by the observation that, in the liquid, this peak vanishes when the s…
The unifying feature of glass formers (such as polymers, supercooled liquids, colloids, granulars, spin glasses, superconductors, ...) is a sluggish dynamics at low temperatures. Indeed, their dynamics is so slow that thermal equilibrium is never reached in macroscopic samples: in analogy with living beings, glasses are said to age. Here, we show how to relate experimentally relevant quantities with the experimentally unreachable low-temperature equilibrium phase. We have performed a very accurate computation of the non-equilibrium fluctuation-dissipation ratio for the three-dimensional Edward…
We have studied the nonequilibrium dynamics of spin glasses subjected to bond perturbation, which was based on the direct change in the spin-spin interaction $ΔJ$, using photo illumination in addition to temperature change $ΔT$. Differences in time-dependent magnetization are observed between that under $ΔT+ΔJ$ and $ΔT$ perturbations with the same $ΔT$. This differences shows the contribution of $ΔJ$ to spin-glass dynamics through the decrease in the overlap length. That is, the overlap length $L_{ΔT+ΔJ}$ under $ΔT+ΔJ$ perturbation is less than $L_{ΔT}$ under $ΔT$ perturbation. Furthermore, we…
We examine three-dimensional $\pm J$ Heisenberg models with and without random anisotropies in a magnetic field. We calculate both the stiffness exponent $θ_s$ at absolute zero temperature and spin-glass correlation lengths for the longitudinal and transverse spin components at finite temperatures. We suggest that, contrary to a chirality scenario predicted by Kawamura and his co-workers, a Gabay-Toulouse phase transition occurs when the anisotropies are absent, although no phase transition occurs when they are present.
Using the dedicated computer Janus, we follow the nonequilibrium dynamics of the Ising spin glass in three dimensions for eleven orders of magnitude. The use of integral estimators for the coherence and correlation lengths allows us to study dynamic heterogeneities and the presence of a replicon mode and to obtain safe bounds on the Edwards-Anderson order parameter below the critical temperature. We obtain good agreement with experimental determinations of the temperature-dependent decay exponents for the thermoremanent magnetization. This magnitude is observed to scale with the much harder to…
Sapienza University of Rome（罗马大学）；Univ. Grenoble Alpes（格勒诺布尔阿尔卑斯大学）；CNRS（法国国家科学研究中心）；Kyoto University（京都大学）；Tokyo Metropolitan University（东京都立大学）；CNR Institute of Complex Systems（意大利国家研究委员会复杂系统研究所）
A mean-field multi-spin interaction spin glass model is analyzed in the presence of a ferromagnetic coupling. The static and dynamical phase diagrams contain four phases (paramagnet, spin glass, ordinary ferromagnet and glassy ferromagnet) and exhibit reentrant behavior. The glassy ferromagnet phase has anomalous dynamical properties. The results are consistent with a nonequilibrium thermodynamics that has been proposed for glasses.
Spin-charge conversion via inverse spin Hall effect (ISHE) is essential for enabling various applications of spintronics. The spin Hall response usually follows a universal scaling relation with longitudinal electric resistivity and has mild temperature dependence because elementary excitations play only a minor role in resistivity and hence ISHE. Here we report that the ISHE of metallic glasses shows nearly two orders of magnitude enhancements with temperature increase from a threshold of 80-100 K to glass transition points. As electric resistivity changes only marginally in the temperature r…
Using inelastic neutron scattering and molecular dynamics simulations on a model Zr-Cu-Al metallic glass, we show that transverse phonons persist well into the high-frequency regime, and can be detected at large momentum transfer. Furthermore, the apparent peak width of the transverse phonons was found to follow the static structure factor. The one-to-one correspondence, which was demonstrated for both Zr-Cu-Al metallic glass and a 3-dimensional Lennard-Jones model glass, suggests a universal correlation between the phonon dynamics and the underlying disordered structure. This remarkable corre…
We present experimental evidence for the existence of a large critical transverse depinning force. These results are obtained in the weakly-pinned superconducting metal glasses Fe$_{x}$Ni$_{1-x}$Zr$_{2}$ using crossed ac and dc driving currents. We study the depinning force due to the transverse ac drive as a function of a longitudinal dc drive. The ac/dc combination allows us to separate the transverse drive from the longitudinal one. We show that the force required for depinning in the transverse direction is enhanced by a longitudinal drive, which leads to the existence of a large transvers…
We study the equilibrium and nonequilibrium properties of Boolean decision problems with competing interactions on scale-free networks in an external bias (magnetic field). Previous studies at zero field have shown a remarkable equilibrium stability of Boolean variables (Ising spins) with competing interactions (spin glasses) on scale-free networks. When the exponent that describes the power-law decay of the connectivity of the network is strictly larger than 3, the system undergoes a spin-glass transition. However, when the exponent is equal to or less than 3, the glass phase is stable for al…
Low energy excitations in a long prism geometry: testing the lower critical dimension of the Ising spin glass
Istituto per le Applicazioni del Calcolo, CNR（意大利国家研究委员会计算应用研究所）；Universidad Complutense de Madrid（马德里康普顿斯大学）；Hangzhou International Innovation Institute, Beihang University（北京航空航天大学杭州国际创新学院）；Dipartimento di Fisica, Sapienza Università di Roma（罗马大学物理系）；CNR-Nanotec, Rome Unit（意大利国家研究委员会纳米技术研究所罗马分部）；INFN, Sezione di Roma（罗马国立核物理研究所）
We test a hypothesis for the origin of dynamical heterogeneity in slowly relaxing systems, namely that it emerges from soft (Goldstone) modes associated with a broken continuous symmetry under time reparametrizations. We do this by constructing coarse grained observables and decomposing the fluctuations of these observables into transverse components, which are associated with the postulated time-fluctuation soft modes, and a longitudinal component, which represents the rest of the fluctuations. Our test is performed on data obtained in simulations of four models of structural glasses. As the …
We discuss generation of series expansions for Ising spin-glasses with a symmetric $\pm J$ (i.e. bimodal) distribution on d-dimensional hypercubic lattices using linked-cluster methods. Simplifications for the bimodal distribution allow us to go to higher order than for a general distribution. We discuss two types of problem, one classical and one quantum. The classical problem is that of the Ising spin glass in a longitudinal magnetic field, $h$, for which we obtain high temperature series expansions in variables $\tanh(J/T)$ and $\tanh(h/T)$. The quantum problem is a $T=0$ study of the Ising…
We present an ansatz for the ground states of the Quantum Sherrington-Kirkpatrick model, a paradigmatic model for quantum spin glasses. Our ansatz, based on the concept of generalized coherent states, very well captures the fundamental aspects of the model, including the ground state energy and the position of the spin glass phase transition. It further enables us to study some previously unexplored features, such as the non-vanishing longitudinal field regime and the entanglement structure of the ground states. We find that the ground state entanglement can be captured by a simple ensemble of…
We study the transition of short range Ising spin glasses in a magnetic field, within a general replica symmetric field theory, which contains three masses and eight cubic couplings, that is defined in terms of the fields representing the replicon, anomalous and longitudinal modes. We discuss the symmetry of the theory in the limit of replica number n to 0, and consider the regular case where the longitudinal and anomalous masses remain degenerate. The spin glass transitions in zero and non-zero field are analyzed in a common framework. The mean field treatment shows the usual results, that is…
The quantum critical behavior of the Ising glass in a magnetic field is investigated. We focus on the spin glass to paramagnet transition of the transverse degrees of freedom in the presence of finite longitudinal field. We use two complementary techniques, the Landau theory close to the T=0 transition and the exact diagonalization method for finite systems. This allows us to estimate the size of the critical region and characterize various crossover regimes. An unexpectedly small energy scale on the disordered side of the critical line is found, and its possible relevance to experiments on me…
We use the generic replica symmetric cubic field-theory to study the transition of short range Ising spin glasses in a magnetic field around the upper critical dimension, d=6. A novel fixed-point is found, in addition to the well-known zero magnetic field fixed-point, from the application of the renormalization group. In the spin glass limit, n going to 0, this fixed-point governs the critical behaviour of a class of systems characterised by a single cubic interaction parameter. For this universality class, the spin glass susceptibility diverges at criticality, whereas the longitudinal mode re…
