In this work we present a platform for testing the device performance of a cavity-emitter system, using an ensemble of emitters and a tapered optical fiber. This method provides high-contrast spectra of the cavity modes, selective detection of emitters coupled to the cavity, and an estimate of the device performance in the single- emitter case. Using nitrogen-vacancy (NV) centers in diamond and a GaP optical microcavity, we are able to tune the cavity onto the NV resonance at 10 K, couple the cavity-coupled emission to a tapered fiber, and measure the fiber-coupled NV spontaneous emission decay. Theoretically we show that the fiber-coupled average Purcell factor is 2-3 times greater than that of free-space collection; although due to ensemble averaging it is still a factor of 3 less than the Purcell factor of a single, ideally placed center.
A technique is demonstrated which efficiently transfers light between a tapered standard single-mode optical fiber and a resonant mode of a high-Q photonic crystal cavity with mode volume less than a cubic wavelength in size. Cavity mode quality factors of 4.7 x 10^4 are measured, and a total fiber-to-cavity coupling efficiency of 44% is demonstrated.
We present the design of two-dimensional photonic crystal microcavities in thin diamond membranes well suited for coupling of color centers in diamond. By comparing simulated and ideal field distributions in Fourier and real space and by according modification of air hole positions and size, we optimize the cavity structure yielding high quality factors up to Q = 320000 with a modal volume of V = 0.35 (lambda/n)^3. Using the very same approach we also improve previous designs of a small modal volume microcavity in silicon, gaining a factor of 3 in cavity Q. In view of practical realization of …
Optical coupling of nitrogen vacancy centers in single-crystal diamond to an on-chip microcavity is demonstrated. The microcavity is fabricated from a hybrid gallium phosphide and diamond material system, and supports whispering gallery mode resonances with spectrometer resolution limited Q > 25000.
Diamond cavity optomechanical devices hold great promise for quantum technology based on coherent coupling between photons, phonons and spins. These devices benefit from the exceptional physical properties of diamond, including its low mechanical dissipation and optical absorption. However the nanoscale dimensions and mechanical isolation of these devices can make them susceptible to thermo-optic instability when operating at the high intracavity field strengths needed to realize coherent photon--phonon coupling. In this work, we overcome these effects through engineering of the device geometr…
We have produced high transmission sub-wavelength tapered optical fibers for the purpose of whispering gallery mode coupling in fused silica microcavities at 780 nm. A detailed analysis of the fiber transmittance evolution during tapering is demonstrated to reflect precisely the mode coupling and cutoff in the fiber. This allows to control the final size, the number of guided modes and their effective index. These results are checked by evanescent wave mapping measurements on the resulting taper.
Hybrid quantum gates hold great promise for quantum information processing since they preserve the advantages of different quantum systems. Here we present compact quantum circuits to deterministically implement controlled-NOT, Toffoli, and Fredkin gates between a flying photon qubit and diamond nitrogen-vacancy (NV) centers assisted by microcavities. The target qubits of these universal quantum gates are encoded on the spins of the electrons associated with the diamond NV centers and they have long coherence time for storing information, and the control qubit is encoded on the polarizations o…
We design extremely flexible ultrahigh-Q diamond-based double-heterostructure photonic crystal slab cavities by modifying the refractive index of the diamond. The refractive index changes needed for ultrahigh-Q cavities with $Q ~ 10^7$, are well within what can be achieved ($Δn \sim 0.02$). The cavity modes have relatively small volumes $V<2 (λ/n)^3$, making them ideal for cavity quantum electro-dynamic applications. Importantly for realistic fabrication, our design is flexible because the range of parameters, cavity length and the index changes, that enables an ultrahigh-Q is quite broad. Fur…
We cooled ultrathin tapered fibers to cryogenic temperatures and controllably coupled them with high-Q microsphere resonators at a wavelength close to the optical transition of diamond nitrogen vacancy centers. The 310-nm-diameter tapered fibers were stably nanopositioned close to the microspheres with a positioning stability of approximately 10 nm over a temperature range of 7-28 K. A cavity-induced phase shift was observed in this temperature range, demonstrating a discrete transition from undercoupling to overcoupling.
Defect centers in diamond are promising building blocks for quantum networks thanks to a long-lived spin state and bright spin-photon interface. However, their low fraction of emission into a desired optical mode limits the entangling success probability. The key to overcoming this is through Purcell enhancement of the emission. Open Fabry-Perot cavities with an embedded diamond membrane allow for such enhancement while retaining good emitter properties. To guide the focus for design improvements it is essential to understand the influence of different types of losses and geometry choices. In …
We demonstrated a simple and reliable technique of coupling diamond nanocrystal containing NV center to tapered optical fiber. We carefully studied fluorescence of the fiber itself and were able to suppress it to the level lower than single photon emission from the NV center. Single photon statistics was demonstrated at the fiber end as well as up to 3 times improvement in collection efficiency with respect to our confocal microscope
Open Fabry-Perot microcavities represent a promising route for achieving a quantum electrodynamics (cavity-QED) platform with diamond-based emitters. In particular, they offer the opportunity to introduce high purity, minimally fabricated material into a tunable, high quality factor optical resonator. Here, we demonstrate a fiber-based microcavity incorporating a thick (> 10 μm) diamond membrane with a finesse of 17,000, corresponding to a quality factor Q ~ $10^6$. Such minimally fabricated, thick samples can contain optically stable emitters similar to those found in bulk diamond. We observe…
We report cavity-enhanced Raman scattering from a single-crystal diamond membrane embedded in a highly miniaturized fully-tunable Fabry-Pérot cavity. The Raman intensity is enhanced 58.8-fold compared to the corresponding confocal measurement. The strong signal amplification results from the Purcell effect. We show that the cavity-enhanced Raman scattering can be harnessed as a narrowband, high-intensity, internal light-source. The Raman process can be triggered in a simple way by using an optical excitation frequency outside the cavity stopband and is independent of the lateral positioning of…
We propose a method of generating entanglement using single photons and electron spins in the regime of resonance scattering. The technique involves matching the spontaneous emission rate of the spin dipole transition in bulk dielectric to the modified rate of spontaneous emission of the dipole coupled to the fundamental mode of an optical microcavity. We call this regime resonance scattering where interference between the input photons and those scattered by the resonantly coupled dipole transition result in a reflectivity of zero. The contrast between this and the unit reflectivity when the …
We succeeded in measuring phase shift spectra of a microsphere cavity coupled with a tapered fiber using a weak coherent probe light at the single photon level. We utilized a tapered fiber with almost no depolarization and constructed a very stable phase shift measurement scheme based on polarization analysis using photon counting. Using a very weak probe light (\bar{n} = 0:41), we succeeded in observing the transition in the phase shift spectrum between undercoupling and overcoupling (at gap distances of 500 and 100 nm, respectively).We also used quantum state tomography to obtain a 'purity s…
High-cooperativity coupling and spin-resolved extinction of tin-vacancy centers in a diamond-like microcavity
Karlsruhe Institute of Technology (KIT)（卡尔斯鲁厄理工学院）；University of Kassel（卡塞尔大学）；University of Stuttgart（斯图加特大学）；Ulm University（乌尔姆大学）；University of Leipzig（莱比锡大学）；Ferdinand-Braun-Institut (FBH)（费迪南德·布劳恩研究所）；Humboldt-Universität zu Berlin（柏林洪堡大学）；Fraunhofer Institute for Applied Solid State Physics（弗劳恩霍夫应用固态物理研究所）
Motivated by developments in quantum information science, much recent effort has been directed toward coupling individual quantum emitters to optical microcavities. Such systems can be used to produce single photons on demand, enable nonlinear optical switching at a single photon level, and implement functional nodes of a quantum network, where the emitters serve as processing nodes and photons are used for long-distance quantum communication. For many of these practical applications, it is important to develop techniques that allow one to generate outgoing single photons of desired frequency …
