We show that a crystal of mesoscopic Fe8 single molecule magnets is an experimental realization of the Quantum Ising Phase Transition (QIPT) model in a transverse field, with dipolar interactions. Quantum annealing has enabled us to explore the QIPT at thermodynamical equilibrium. The phase diagram and critical exponents we obtain are compared to expectations for the mean-field QIPT Universality class.
Theory of Two-Step Magnetic Ordering Phenomena in a Geometrically Frustrated Heisenberg Pyrochlore Antiferromagnet with Long Range Dipolar Interactions
利用平均场论研究了具有交换作用和偶极-偶极相互作用的烧绿石晶格上的海森堡反铁磁体模型。在处理偶极通过使用埃瓦尔德方法，一个软（临界）模式与一个独特的有序波矢量被选择为所有强度的偶极偶极耦合。对于弱偶极子，选择部分有序的三个子晶格自旋结构（P态），其中q_{ord} =（1/2 1/2 1/2）。一个完全有序的四个子晶格自旋结构（F态），q =（000），与P态竞争，并随着温度的降低而成为稳定的结构。我们的结果进行了比较，对其他的理论计算和连接到最近的实验结果Gd 2 Ti 2 O 7进行了讨论。
The kinetic mechanisms underlying bottom-up assembly of colloidal particles have been widely investigated in efforts to control crystallization pathways and to direct growth into targeted superstructures for applications including photonic crystals. Current work builds on recent progress in the development of kinetic theories for crystal growth of body-centered-cubic crystals in systems with short-range inter-particle interactions, accounting for a greater diversity of crystal structures and the role of the longer-ranged interactions and orientational degrees of freedom arising in polar system…
We study the ground state and magnetic hysteresis properties of 2$d$ arrays ($L^{}_x\times L^{}_y$) of dipolar interacting magnetic nanoparticles (MNPs) by performing micromagnetic simulations. Our primary interest is to understand the effect of sample shape, $Θ$- the ratio of the dipolar strength to the anisotropy strength, and the direction of the applied field $\vec{H} = H_{o}\hat{e}^{}_H$ on the ground state and the magnetic hysteresis in an array of MNPs. To study the effect of shape of the sample, we have varied the aspect ratio $A^{}_r=L^{}_y/L^{}_x$ which in turn, is found to induce sh…
Hybrid Improper Ferroelectricity (HIF) allows the generation of an electrical polarization in the AA'BB'O$_6$ double perovskite materials thanks to the combination of two non-polar octahedral distortions. Nevertheless, for selected combination of the A/A' cations a non-polar incommensurate phase is observed with average symmetry $C2/m$. Thanks to a detailed crystallographic description of the incommensurate phase, based on electron, neutron and x-ray diffraction data, we show that the incommensurate modulation is related to an abrupt change of the out-of-phase tilting along the a- and c-axis w…
We study near-neighbour and dipolar Ising models on a lattice of corner-sharing octahedra. In an extended parameter range of both models, frustration between antiferromagnetism and a spin-ice-like three-in-three-out rule stabilises a Coulomb phase with correlated dipolar and quadrupolar spin textures, both yielding distinctive neutron-scattering signatures. Strong further-neighbour perturbations cause the two components to order independently, resulting in unusual multi-$k$ orders. We propose experimental realisations of our model in rare-earth antiperovskites.
We report an interesting case where magnetic phenomena can transcend mesoscopic scales. Our system consists of tubes created by assembly of dipolar spheres. The cylindrical topology results in the breakup of degeneracy observed in the planar square and triangular packings. As far as the ground state is concerned, tubes switch from circular to axial magnetization with increasing tube length. All magnetostatic properties found in magnetic nanotubes, in which the dipolar interaction is comparable or dominate over the exchange interaction, are reproduced by the dipolar tubes including an intermedi…
Chiral magnetism has gained enormous interest in recent years because of the anticipated wealth of applications in nanoelectronics. The demonstrated stabilization of chiral magnetic domain walls and skyrmions has been attributed to the actively investigated Dzyaloshinskii-Moriya interaction. Recently, however, predictions were made that suggest dipolar interactions can also stabilize chiral domain walls and skyrmions, but direct experimental evidence has been lacking. Here we show that dipolar interactions can indeed stabilize chiral domain walls by directly imaging the magnetic domain walls u…
We present a comprehensive study of static and dynamic magnetic properties in the Ising-like dipolar antiferromagnet (AFM) DyScO$_3$\ by means of DC and AC magnetization measurements supported by classical Monte-Carlo calculations. Our AC-susceptibility data show that the magnetic dynamics exhibit a clear crossover from an Arrhenius-like regime to quantum tunneling of magnetization (QTM) at $T^* = 10$ K. Below $T_{\mathrm{N}} = 3.2$ K DyScO$_3$ orders in an antiferromagnetic $GxAy$-type magnetic structure and the magnetization dynamics slow down to the minute timescale. The low-temperature mag…
The dipolar interaction is known to substantially affect the properties of magnetic nanoparticles. This is particularly important when the particles are kept in a fluid suspension or packed inside nano-carriers. In addition to its usual long-range nature, in these cases the dipolar interaction may also induce the formation of clusters of particles, thereby strongly modifying their magnetic anisotropies. In this paper we show how AC susceptibility may be used to obtain important information regarding the influence of the dipolar interaction in a sample. We develop a model which includes both as…
Using the two-level approximation of the energy barrier, we perform extensive kinetic Monte Carlo simulations to probe the relaxation characteristics in a two-dimensional ($L^{}_x\times L^{}_y$) array of magnetic nanoparticle as a function of dipolar interaction strength $h^{}_d$, aspect ratio $A^{}_r=L^{}_y/L^{}_x$, and temperature $T$. In the case of weak dipolar interaction ($h^{}_d\approx0$) and substantial temperature, the magnetic relaxation follows the Néel Brown model as expected. Interestingly, the dipolar interaction of enough strength is found to induce antiferromagnetic coupling in…
Magnetic skyrmions are localized particle-like nontrivial swirls that are promising in building high-performance topological spintronic devices. The read-out functions in skyrmionic devices require the translation of magnetic skyrmions to electrical signals. Here, we report combined real-space magnetic imaging and anisotropic magnetoresistance studies on dipolar skyrmions. A single skyrmion chain and single skyrmion are observed using Lorentz transmission electron microscopy imaging. Meanwhile, the field, helicity, and skyrmion count dependence of anisotropic magnetoresistance of the Fe3Sn2 na…
The results of extensive Monte Carlo simulations of classical spins on the two-dimensional kagome lattice with only dipolar interactions are presented. In addition to revealing the six-fold degenerate ground state, the nature of the finite-temperature phase transition to long-range magnetic order is discussed. Low temperature states consisting of mixtures of degenerate ground state configurations separated by domain walls can be explained as a result of competing exchange-like and shape anisotropy-like terms in the dipolar coupling. Fluctuations between pairs of degenerate spin configurations …
We combine the anisotropy of magnetic interactions and the point symmetry of finite solids in the study of dipolar clusters as new basic units for multiferroics metamaterials. The hamiltonian of magnetic dipoles with an easy axis at the vertices of polygons and polyhedra, maps exactly into a hamiltonian with symmetric and antisymmetric exchange couplings. The last one gives rise to a Dzyaloshinskii-Moriya contribution responsible for the magnetic modes of the systems and their symmetry groups, which coincide with those of a particle in a crystal field with spin-orbit interaction. We find that …
Numerical study of spin-dependent transition rates within pairs of dipolar and strongly exchange coupled spins with (s=1/2) during magnetic resonant excitation
We study spin wave excitations in a three-dimensional nanocomposite magnet of exchange coupled hard (SmCo$_5$) and soft (FeCo) phases. The dipolar interaction splits the spin wave energies into the upper and lower branches of the spin wave manifold. When the amount of the soft phase is increased the energy of low-lying spin excitations is considerably softened due to two reasons: (i) the low- lying mode locked into the soft phase region with a spin wave gap at ${\bf k}= 0$ which scales approximately proportional to the anisotropy constant of the soft phase and (ii) the internal dipolar field w…
A phase transition is often accompanied by the appearance of an order parameter and symmetry breaking. Certain magnetic materials exhibit exotic hidden-order phases, in which the order parameters are not directly accessible to conventional magnetic measurements. Thus, experimental identification and theoretical understanding of a hidden order are difficult. Here we combine neutron scattering and thermodynamic probes to study the newly discovered rare-earth triangular-lattice magnet TmMgGaO$_4$. Clear magnetic Bragg peaks at K points are observed in the elastic neutron diffraction measurements.…
Magneto-dielectric spectra of La0.95Ca0.05CoO3 covering the crossover of spin states reveals strong coupling of its spin and dipolar degrees of freedom. Signature of spin-state transition at 30K clearly manifests in magnetization, supported by Co L_3,2-edge XAS data on the doped-specimen as consistent with its suppressed T_SST vs. ~150K for pure LaCoO3. Dispersive activation-step Δε'(T_ω)~O(10^2) and relaxation-peak ε"(T_ω) reflect the allied influence of coexistent spin-states on the dielectric character. Dipolar relaxation in the LS regime below T_SST is partly segmental (VFT kinetics) featu…
The magnetoelectric effect predicted in topological insulators makes heterostructures that combine magnetic materials and such insulators promising candidates for spintronics applications. Here, we theoretically consider a setup that exhibits two well-separated interfaces between a topological insulator and a ferromagnetic insulator. We show that there is a topological magnetic dipole-dipole interaction stemming from long-range Coulomb interactions. We analytically derive the magnetization dynamics at the two interfaces and discuss how the long-range coupling can be applied to non-locally indu…
We address the issue of inter-particle dipolar interactions in the context of magnetic hyperthermia. More precisely, the main question dealt with here is concerned with the conditions under which the specific absorption rate is enhanced or reduced by dipolar interactions. For this purpose, we propose a theory for the calculation of the AC susceptibility, and thereby the specific absorption rate, for a monodisperse two-dimensional assembly of nanoparticles with oriented anisotropy, in the presence of a DC magnetic field, in addition to the AC magnetic field. We also study the competition betwee…
Using first-principle calculations and kinetic Monte Carlo simulation, we study the local and averaged hysteresis in tiny clusters of k magnetic nanoparticles (MNPs) or k-mers. We also analyze the variation of local dipolar field acting on the constituent nanoparticles as a function of the external magnetic field. The dipolar interaction is found to promote chain-like arrangement in such a cluster. Irrespective of cluster size, the local hysteresis response depends strongly on the corresponding dipolar field acted on a nanoparticle. In a small k-mer, there is a wide variation in local hysteres…
Magnetoelastic Waves in Ferromagnetic Thin Films Mediated by Dipolar Interactions
Institute of Science Tokyo（东京科学大学）；The University of Tokyo（东京大学）；NTT, Inc.（日本电报电话公司）；Japan Atomic Energy Agency（日本原子能研究开发机构）；RIKEN（理化学研究所）；Hiroshima University（广岛大学）
Materials that have a hysteretic response to an external field are essential in modern information storage and processing technologies. The magnetization curves of several natural and artificial materials have previously been measured and explained in terms of the Neel model, Preisach phenomenological model, the creation, propagation, and annihilation of topological defects, or by resonant quantum tunnelling of the magnetization in single molecule magnets. However, a simple way to design the magnetic response of a material is missing. Here, we propose and experimentally realize an elementary m…
Effective theory of quantum phases in the dipolar planar rotor chain
University of Waterloo（滑铁卢大学）；Institute For Quantum Computing, University of Waterloo（滑铁卢大学量子计算研究所）；Perimeter Institute for Theoretical Physics（理论物理前沿研究所）
