This work theoretically addresses the trapping an ionized atom with a single valence electron by means of lasers, analyzing qualitatively and quantitatively the consequences of the net charge of the particle. In our model, the coupling between the ion and the electromagnetic field includes the charge monopole and the internal dipole, within a multipolar expansion of the interaction Hamiltonian. Specifically, we perform a Power-Zienau-Woolley transformation, taking into account the motion of the center of mass. The net charge produces a correction in the atomic dipole which is of order $m_e/M$ with $m_e$ the electron mass and $M$ the total mass of the ion. With respect to neutral atoms, there is also an extra coupling to the laser field which can be approximated by that of the monopole located at the position of the center of mass. These additional effects, however, are shown to be very small compared to the dominant dipolar trapping term.
Isolating neutral and charged particles from the environment is essential in precision experiments. For decades, this has been achieved by trapping ions with radio-frequency (rf) fields and neutral particles with optical fields. Recently, trapping of ions by interaction with light has been demonstrated. This might permit combining the advantages of optical trapping and ions. For example, by superimposing optical traps to investigate ensembles of ions and atoms in absence of any radiofrequency fields, as well as to benefit from the versatile and scalable trapping geometries featured by optical …
Thorium ions exhibit unique nuclear properties with high relevance for testing symmetries of nature, and Paul traps feature an ideal experimental platform for performing high precision quantum logic spectroscopy. Loading of stable or long-lived isotopes is well-established and relies on ionization from an atomic beam. A different approach allows trapping short-lived isotopes available as alpha-decay daughters, which recoil from a thin sample of the precursor nuclide. A prominent example is the short-lived $^{229\text{m}}$Th, populated in a decay of long-lived $^{233}$U. Here, ions are provided…
Hybrid quantum systems that unite laser-cooled trapped ions and ultracold quantum gases in a single experimental setup have opened a rapidly advancing field of study, including Quantum chemistry, polaron physics, quantum information processing and quantum simulations. We present a fully developed and tested ion trap chip and propose a flat chip trap that can be placed beneath the ion trap. This design substantially addresses the difficulties specific to hybrid traps and features well-aligned chips that allow for independent adjustment of the depth of the atomic trap and the confinement and pos…
Precision optical spectroscopy of exotic ions reveals accurate information about nuclear properties such as charge radii and magnetic and quadrupole moments. Thorium ions exhibit unique nuclear properties with high relevance for testing symmetries of nature. We report loading and trapping of single $^{232}$Th$^+$ ions in a linear Paul trap, embedded into and sympathetically cooled by small crystals of trapped $^{40}$Ca$^+$ ions. Trapped Th ions are identified in a non-destructive manner from the voids in the laser-induced Ca fluorescence pattern emitted by the crystal, and alternatively, by me…
We propose a new scheme for supplying voltages to the electrodes of microfabricated ion traps, enabling access to a regime in which changes to the trapping potential are made on timescales much shorter than the period of the secular oscillation frequencies of the trapped ions. This opens up possibilities for speeding up the transport of ions in segmented ion traps and also provides access to control of multiple ions in a string faster than the Coulomb interaction between them. We perform a theoretical study of ion transport using these methods in a surface-electrode trap, characterizing the pr…
For conventional ion traps, the trapping potential is close to independent of the electronic state, providing confinement for ions dependent primarily on their charge-to-mass ratio $Q/m$. In contrast, storing ions within an optical dipole trap results in state-dependent confinement. Here we experimentally study optical dipole potentials for $^{138}\mathrm{Ba}^+$ ions stored within two distinctive traps operating at 532 nm and 1064 nm. We prepare the ions in either the $6\mathrm{S}_{\mathrm{1/2}}$ electronic ground or the $5\mathrm{D}_{\mathrm{3/2}}$/ $5\mathrm{D}_{\mathrm{5/2}}$ metastable exc…
The electronic and motional degrees of freedom of trapped ions can be controlled and coherently coupled on the level of individual quanta. Assembling complex quantum systems ion by ion while keeping this unique level of control remains a challenging task. For many applications, linear chains of ions in conventional traps are ideally suited to address this problem. However, driven motion due to the magnetic or radio-frequency electric trapping fields sometimes limits the performance in one dimension and severely affects the extension to higher dimensional systems. Here, we report on the trappin…
Rydberg atoms are remarkable tools for quantum simulation and computation. They are the focus of an intense experimental activity mainly based on low-angular-momentum Rydberg states. Unfortunately, atomic motion and levels lifetime limit the experimental time-scale to about 100$μ$s. Here, we demonstrate laser trapping of long-lived circular Rydberg states for up to 10ms. Our method is very general and opens many opportunities for quantum simulation. The 10ms trapping time corresponds to thousands of interaction cycles in a circular-state-based quantum simulator. It is also promising for quantu…
We investigate cooling mechanisms in magneto-optically and magnetically trapped erbium. We find efficient sub-Doppler cooling in our trap, which can persist even in large magnetic fields due to the near degeneracy of two Lande g factors. Furthermore, a continuously loaded magnetic trap is demonstrated where we observe temperatures below 25 microkelvin. These favorable cooling and trapping properties suggest a number of scientific possibilities for rare-earth atomic physics, including narrow linewidth laser cooling and spectroscopy, unique collision studies, and degenerate bosonic and fermionic…
For several decades, ions have been trapped by radio frequency (RF) and neutral particles by optical fields. We implement the experimental proof-of-principle for trapping an ion in an optical dipole trap. While loading, initialization and final detection are performed in a RF trap, in between, this RF trap is completely disabled and substituted by the optical trap. The measured lifetime of milliseconds allows for hundreds of oscillations within the optical potential. It is mainly limited by heating due to photon scattering. In future experiments the lifetime may be increased by further detunin…
An optical tweezer composed of a strongly focused single-spatial-mode Gaussian beam of a red-detuned 1064-nm laser can confine a single-cesium (Cs) atom at the strongest point of the light intensity. We can use this for coherent manipulation of single-quantum bits and single-photon sources. The trapping lifetime of the atoms in the optical tweezers is very short due to the impact of the background atoms, the laser intensity fluctuation of optical tweezer and the residual thermal motion of the atoms. In this paper, we analyzed the influence of the background pressure, the trap frequency of opti…
The proposal for quantum computing with rare-earth-ion qubits in inorganic crystals makes use of the inhomogeneous broadening of optical transitions in the ions to associate individual qubits with ions responding to radiation in selected frequency channels. We show that a class of Gaussian composite pulses and complex sech pulses provide accurate qubit pi-rotations, which are at the same time channel selective on a 5 MHz frequency scale and tolerant to 0.5 MHz deviations of the transition frequency of ions within a single channel. Rotations in qubit space of arbitrary angles and phases are pro…
Decoherence time has been calculated for an optical ion trap of Be atoms in a bistable potential model. Comparison has been made between decoherence time and Zeno time for double well potential as a special case. Zeno time is considered as a lower limit of decoherence time for sustainable quantum coherence. Equality of the respective timescales provides a certain transitional temperature, below which decoherence can be asymptotically minimized.
We propose a scheme for state-insensitive trapping of neutral atoms by using light with two independent wavelengths. In particular, we describe the use of trapping and control lasers to minimize the variance of the potential experienced by a trapped Rb atom in ground and excited states. We present calculated values of wavelength pairs for which the 5s and 5p_{3/2} levels have the same ac Stark shifts in the presence of two laser fields.
The wave function of a moderately cold atom in a stationary near-resonant standing light wave delocalizes very fast due to wave packet splitting. However, we show that frequency modulation of the field may suppress packet splitting for some atoms having specific velocities in a narrow range. These atoms remain localized in a small space for a long time. We propose that in a real experiment with cold atomic gas this effect may decrease the velocity distribution of atoms (the field traps the atoms with such specific velocities while all other atoms leave the field)
We perform laser spectroscopy of Yb+ ions on the 4f14 6s 2S_{1/2} - 4f13 5d 6s 3D[3/2]_{1/2} transition at 297 nm. The frequency measurements for 170Yb+, 172Yb+, 174Yb+, and 176Yb+ reveal the specific mass shift as well as the field shifts. In addition, we demonstrate laser cooling of Yb+ ions using this transition and show that light at 297 nm can be used as the second step in the photoionization of neutral Yb atoms.
We analyze evanescent fields of laser written waveguides and show that they can be used to trap atoms close to the surface of an integrated optical atom chip. In contrast to subwavelength nanofibres it is generally not possible to create a stable trapping potential using only the fundamental modes. This is why we create a stable trapping potential by using two different laser colors, such that the waveguide supports two modes for the blue detuned laser, while for the red detuned light the waveguide has only a single mode. In particular, we study such a two-color trap for Cesium atoms, and calc…
Recent advances in quantum information processing with trapped ions have demonstrated the need for new ion trap architectures capable of holding and manipulating chains of many (>10) ions. Here we present the design and detailed characterization of a new linear trap, microfabricated with scalable complementary metal-oxide-semiconductor (CMOS) techniques, that is well-suited to this challenge. Forty-four individually controlled DC electrodes provide the many degrees of freedom required to construct anharmonic potential wells, shuttle ions, merge and split ion chains, precisely tune secular mode…
We use a pulsed nitrogen laser to produce atomic ions by laser ablation, measuring the relative ion yield for several elements, including some that have only recently been proposed for use in cold trapped ion experiments. For barium, we monitor the ion yield as a function of the number of applied ablation pulses for different substrates. We also investigate the ion production as a function of the pulse energy, and the efficiency of loading an ion trap as a function of radiofrequency voltage.
Spin effects in the tunneling regime of strong field ionization of hydrogenlike highly charged ions in linearly as well as circularly polarized laser fields are investigated. The impact of the polarization of a laser field on the spin effects are analyzed. Spin-resolved differential ionization rates are calculated employing the relativistic Coulomb-corrected strong-field approximation (SFA) developed in the previous paper of the series. Analytical expressions for spin asymmetries and spin flip probability, depending on the laser's polarization, are obtained for the photoelectron momentum corre…
We report on three-dimensional optical trapping of single ions in an optical lattice formed by two counter-propagating laser beams. We characterize the trapping parameters of the standing wave using the ion as a sensor stored in a hybrid trap consisting of a radio-frequency (rf), a dc, and the optical potential. When loading ions directly from the rf into the standing-wave trap, we observe a dominant heating rate. Monte Carlo simulations confirm rf-induced parametric excitations within the deep optical lattice as the main source. We demonstrate a way around this effect by an alternative transf…
We demonstrate phase locking of two ultraviolet laser sources by modulating a fundamental infrared laser with 4th-order sidebands using an electro-optic modulator and phase locking of one sideband to a second fundamental infrared laser. Subsequent sum frequency generation and second harmonic generation successfully translates the frequency offset to the ultraviolet domain. The phase lock at 139 GHz is confirmed through stimulated Raman transitions for thermometry of $^9$Be$^+$ ions confined in a cryogenic Penning trap. This technique might be used for sideband cooling of single $^9$Be$^+$ ions…
We report on experiments with a microfabricated surface trap designed for trapping a chain of ions in a ring. Uniform ion separation over most of the ring is achieved with a rotationally symmetric design and by measuring and suppressing undesired electric fields. After minimizing these fields the ions are confined primarily by an rf trapping pseudo-potential and their mutual Coulomb repulsion. The ring-shaped crystal consists of approximately 400 Ca$^+$ ions with an estimated average separation of 9 $μm$.
Laser cooling on weak transitions is a useful technique for reaching ultracold temperatures in atoms with multiple valence electrons. However, for strongly magnetic atoms a conventional narrow-line magneto-optical trap (MOT) is destabilized by competition between optical and magnetic forces. We overcome this difficulty in Er by developing an unusual narrow-line MOT that balances optical and magnetic forces using laser light tuned to the blue side of a narrow (8 kHz) transition. The trap population is spin-polarized with temperatures reaching below 2 microkelvin. Our results constitute an alter…
We present a realization of a magneto-optical trap of mercury atoms on the intercombination line. We report on trapping of all stable mercury isotopes. We characterize the effect of laser detuning, laser intensity, and gradient field on the trapping performance of our system. The atom number for the most abundant isotope Hg-202 is 50 million atoms. Moreover, we study the difference in cooling processes for bosonic and fermionic isotopes. We observe agreement with the Doppler cooling theory for the bosonic species and show sub-Doppler cooling for the fermionic species. We reach a phase space de…
We describe a high-power, frequency-tunable, external cavity diode laser (ECDL) system near 626 nm useful for laser cooling of trapped $^9$Be$^+$ ions. A commercial single-mode laser diode with rated power output of 170 mW at 635 nm is cooled to $\approx - 31$ C, and a single longitudinal mode is selected via the Littrow configuration. In our setup, involving multiple stages of thermoelectric cooling, we are able to obtain $\approx$130 mW near 626 nm, sufficient for efficient frequency doubling to the required Doppler cooling wavelengths near 313 nm in ionized Beryllium. In order to improve no…
We present theoretical and experimental results of coherent population trapping spectra on a multi-level $^{40}$Ca$^+$-type configuration, adding a third beam to the standard two-laser $Λ$ system to avoid undesired optical pumping. We show that the extra laser can preserve the nature of the dark resonances or introduce decoherence depending on its power. Experiments are carried out using a single trapped $^{40}$Ca$^+$ ion in the $S_{1/2}-P_{1/2}-D_{3/2}$ manifold. Theoretically, the problem is solved with a Floquet-like expansion of the Liouvillian that correctly predicts all of the measured s…
We demonstrate stabilisation of an ultraviolet diode laser via Doppler free spectroscopy of Ytterbium ions in a discharge. Our technique employs polarization spectroscopy, which produces a natural dispersive lineshape whose zero-crossing is largely immune to environmental drifts, making this signal an ideal absolute frequency reference for Yb$^+$ ion trapping experiments. We stabilise an external-cavity diode laser near 369 nm for cooling Yb$^+$ ions, using amplitude-modulated polarisation spectroscopy and a commercial PID feedback system. We achieve stable, low-drift locking with a standard d…
We present a solid-state laser system that generates 750 mW of continuous-wave single-frequency output at 313 nm. Sum-frequency generation with fiber lasers at 1550 nm and 1051 nm produces up to 2 W at 626 nm. This visible light is then converted to UV by cavity-enhanced second-harmonic generation. The laser output can be tuned over a 495 GHz range, which includes the 9Be+ laser cooling and repumping transitions. This is the first report of a narrow-linewidth laser system with sufficient power to perform fault-tolerant quantum-gate operations with trapped 9Be+ ions by use of stimulated Raman t…
High-order harmonic generation (HHG) by hydrogenlike atoms/ions in the uniform periodic electric field, formed by the two linearly polarized counterpropagating laser beams of relativistic intensities, is studied. The relativistic quantum theory of HHG in such fields, at which the impeding factor of relativistic magnetic drift of a strong wave can be eliminated, is presented arising from the Dirac equation. Specifically, a scheme of HHG in underdense plasma with the copropagating ultraintense laser and fast ion beams is proposed.
A novel robust mechanism for the generation of "trapping states" is shown to exist in the coupling of a two-level system with an oscillator, which is based on nonlinearities in the laser-induced vibronic coupling. This mechanism is exemplified with an ion confined in the potential well of a trap, where the nonlinearities are due to Franck--Condon type overlap integrals of the laser waves with the ionic centre-of-mass wavefunction. In contrast to the coherent trapping mechanism known from micro-maser theory, this mechanism works also in an incoherent regime operated by noisy lasers and is there…
We propose a scalable ion trap architecture for universal quantum computation, which is composed of an array of ion traps with one ion confined in each trap. The neighboring traps are designed capable of merging into one single trap. The universal two-qubit $\sqrt{SWAP}$ gate is realized by direct collision of two neighboring ions in the merged trap, which induces an effective spin-spin interaction between two ions. We find that the collision-induced spin-spin interaction decreases with the third power of two ions' trapping distance. Even with a $200\ μm$ trapping distance between atomic ions …
We present a robust and fast laser cooling scheme suitable for trapped atoms and ions. Based on quantum interference, generated by a special laser configuration, it is able to rapidly cool the system such that the final phonon occupation vanishes to zeroth order in the Lamb-Dicke parameter in contrast to existing cooling schemes. Furthermore, it is robust under conditions of fluctuating laser intensity and frequency, thus making it a viable candidate for experimental applications.
We investigate theoretically the optical properties of an atomic gas which has been cooled by the laser cooling method velocity-selective coherent population trapping. We demonstrate that the application of a weak laser pulse gives rise to a backscattered pulse, which is a direct signal for the entanglement in the atomic system, and which leads to single-particle entanglement on the few-photon level. If the pulse is applied together with the pump lasers, it also displays the phenomenon of electromagnetically induced transparency. We suggest that the effect should be observable in a gas of Rubi…
After pumped from $5s_{1/2}$ ground state to $6p_{1/2}$ state, the population inversion between $6s_{1/2}$ and $5p_{1/2,3/2}$ will be established for Rubidium four-level active optical clock. In this paper, we calculate AC Stark shift due to lattice trapping laser which dominates the frequency shift of clock transition in lattice trapped Rubidium four-level active optical clock. Several magic wavelengths are found that can form desired optical lattice trapping potential. By choosing a proper intensity and linewidth of trapping laser, the fractional frequency uncertainty of clock transition due…
We propose a tunable phonon laser prototype with a large trapped ion array, where some of the ions are effectively pinned by optical tweezers, thus isolating a subset of ions that mimics an acoustic cavity used as a phonon lasing resonator. The cavity loss can then be controlled by the tweezer strength and the "wall thickness", the number of pinned ions for isolation. We pump the resonator by applying blue-sideband lasers, and investigate the lasing dynamics of the cavity modes such as threshold behavior, population distribution, the second-order coherence, and line-narrowed spectrum. This sch…
We present an implementation of quantum logic gates via internal state dependent displacements of ions in a linear Paul trap caused by optical dipole forces. Based on a general quantum analysis of the system dynamics we consider specific implementations with alkaline earth ions. For experimentally realistic parameters gate infidelities as low as $10^{-4}$ can be obtained.
We explore and develop the mathematics of the two multi-level ions. In particular, we describe some new features of quantum entanglement in two three-level trapped ions confined in a one-dimensional harmonic potential, allowing the instantaneous position of the center-of-mass motion of the ions to be explicitly time-dependent. By solving the exact dynamics of the system, we show how survivability of the quantum entanglement is determined by a specific choice of the initial state settings.
A scheme to implement quantum logic gates by manipulating trapped ions through interaction with monochromatic external laser field and quantized cavity field, beyond the Lamb-Dicke regime, is presented. Characteristic times, for implementing ionic state transitions using non-resont laser pulse or quantized cavity field, shows a sharp decline for large Lamb-Dicke parameter value of $η_{L}=η_{c}=0.2$, and is seen to decrease further with increase in number of initial state vibrational quanta $m$.
The Hamiltonian describing a single ion placed in a potential trap in interaction with a laser beam is studied by means of a suitable perturbative approach. It is shown, in particular, that the rotating wave approximation does not provide the correct expression, at the first perturbative order, of the evolution operator of the system.
A vital requirement for a quantum computer is the ability to locally address, with high fidelity, any of its qubits without affecting their neighbors. We propose an addressing method using composite sequences of laser pulses, which reduces dramatically the addressing error in a lattice of closely spaced atoms or ions, and at the same time significantly enhances the robustness of qubit manipulations. To this end, we design novel high-fidelity composite pulses for the most important single-qubit operations. In principle, this method allows one to beat the diffraction limit, for only atoms situat…
We study cooling of the collective vibrational motion of two 138Ba+ ions confined in an electrodynamic trap and irradiated with laser light close to the resonances S_1/2-P_1/2 (493 nm) and P_1/2-D_3/2 (650 nm). The motional state of the ions is monitored by a spatially resolving photo multiplier. Depending on detuning and intensity of the cooling lasers, macroscopically different motional states corresponding to different ion temperatures are observed. We also derive the ions' temperature from detailed analytical calculations of laser cooling taking into account the Zeeman structure of the ene…
We describe a efficient way to photoionize strontium atoms in a linear radio-frequency trap. We use a 2-photon second order process to excite the autoionization resonance (4d2 + 5p2) 1D2. A doubled pulsed Ti:Saphire laser system is used at 431nm to provide 100fsec pulses at 82Mhz. The fabrication of the laser systems for addressing the Sr+ transitions necessary for laser cooling and excitation of quantum jumps, vacuum system and ion trap structure are also described in detail. With the current setup a easy and repeatable trapping of linear ion chains is achieved at UHV pressures.
In this paper we develop a unified framework to study the coherent control of trapped ions subject to state-dependent forces. Taking different limits in our theory, we can reproduce two different designs of a two-qubit quantum gate --the pushing gate [1] and the fast gates based on laser pulses from Ref. [2]--, and propose a new design based on continuous laser beams. We demonstrate how to simulate Ising Hamiltonians in a many ions setup, and how to create highly entangled states and induce squeezing. Finally, in a detailed analysis we identify the physical limits of this technique and study t…
We present a scheme for robust and efficient projection measurement of a qubit consisting of the two magnetic sublevels in the electronic ground state of alkali earth metal ions. The scheme is based on two stimulated Raman adiabatic passages (STIRAP) involving four partially coherent laser fields. We show how the efficiency depends on experimentally relevant parameters: Rabi frequencies, pulse widths, laser linewidths, one- and two-photon detunings, residual laser power, laser polarization and ion motion.
We report a study of the axialisation and laser cooling of single ions and small clouds of ions in a Penning trap. A weak radiofrequency signal applied to a segmented ring electrode couples the magnetron motion to the cyclotron motion, which results in improved laser cooling of the magnetron motion. This allows us to approach the trapping conditions of a Paul trap, but without any micromotion. Using an ICCD camera we show that the motion of a single ion can be confined to dimensions of the order of 10 $μ$m. We have measured increased magnetron cooling rates using an rf-photon correlation techn…
The spectroscopic properties of a single, tightly trapped atom are studied, when the electronic levels are coupled by three laser fields in an $N$-shaped configuration of levels, whereby a $Λ$-type level system is weakly coupled to a metastable state. We show that depending on the laser frequencies the response can be tuned from coherent population trapping at two-photon resonance to novel behaviour at three photon resonance, where the metastable state can get almost unit occupation in a wide range of parameters. For certain parameter regimes the system switches spontaneously between dissipati…
We perform a combined theoretical and experimental investigation of the superradiance in the quantum coherent system generated by strong laser fields. The semiclassical theory of superradiance that includes the superradiant temporal profile, character duration, time delay, intensity is derived. The experimental data and theoretical predictions of 391-nm forward emission as a function of nitrogen gas pressure are compared and show good agreement. Our results not only demonstrate that the time-delayed optical amplification inside the molecular nitrogen ions is superradiance, but also reveal the …
We describe laser systems for photoionization, Doppler cooling and quantum state manipulation of beryllium ions. For photoionization of neutral beryllium, we have developed a continuous-wave 235 nm source obtained by two stages of frequency doubling from a diode laser at 940 nm. The system delivers up to 400 mW at 470 nm and 28 mW at 235 nm. For control of the beryllium ion, three laser wavelengths at 313 nm are produced by sum-frequency generation and second-harmonic generation from four infrared fiber lasers. Up to 7.2 W at 626 nm and 1.9 W at 313 nm are obtained using two pump beams at 1051…
