We investigate the effect of geometrical frustration on the $H$--$T$ phase diagrams of the classical Heisenberg antiferromagnets on triangular and kagome lattices. The phase diagrams for the two models are obtained from large scale Monte Carlo simulations. For the kagome antiferromagnet thermal fluctuations are unable to lift completely degeneracy and stabilize translationally disordered multipolar phases. We find a substantial difference in the temperature scales of the order by disorder effect related to different degeneracy of the low- and the high-field classical ground states in the kagome antiferromagnet. In the low-field regime, the Kosterlitz-Thouless transition into a spin-nematic phase is produced by unbinding of half-quantum vortices.
The $S=1/2$ kagome- and triangular-lattice Heisenberg antiferromagnets are investigated using the numerical exact diagonalization and the finite-size scaling analysis. The behaviour of the field derivative at zero magnetization is examined for both systems. The present result indicates that the spin excitation is gapless for each system.
We investigate the $S=1/2$ quantum spin antiferromagnets on the triangular and Kagome lattices in magnetic field, using the numerical exact diagonalization. Particularly we focus on an anomalous magnetization behavior of each system at 1/3 of the saturation magnetization. The critical exponent analyses suggest that it is a conventional magnetization plateau on the triangular lattice, while an unconventional phenomenon, called the magnetization ramp, on the Kagome lattice.
We discuss recently introduced numerical linked-cluster (NLC) algorithms that allow one to obtain temperature-dependent properties of quantum lattice models, in the thermodynamic limit, from exact diagonalization of finite clusters. We present studies of thermodynamic observables for spin models on square, triangular, and kagome lattices. Results for several choices of clusters and extrapolations methods, that accelerate the convergence of NLC, are presented. We also include a comparison of NLC results with those obtained from exact analytical expressions (where available), high-temperature ex…
We investigate the ground-state phase diagram of the Kondo lattice model with classical localized spins on triangular-to-kagome lattices by using a variational calculation. We identify the parameter regions where a four-sublattice noncoplanar order is stable with a finite spin scalar chirality while changing the lattice structure from triangular to kagome continuously. Although the noncoplanar spin states appear in a wide range of parameters, the spin configurations on the kagome network become coplanar as approaching the kagome lattice; eventually, the scalar chirality vanishes for the kagome…
Frustrated quantum spin systems such as the Heisenberg and Kitaev models on various lattices, have been known to exhibit various exotic properties not only at zero temperature but also for finite temperatures. Inspired by the remarkable development of the quantum frustrated spin systems in recent years, we investigate the finite-temperature properties of the $S=1/2$ Kitaev-Heisenberg models on kagome and triangular lattices by means of finite-temperature Lanczos methods with improved accuracy. In both lattices, multiple peaks are confirmed in the specific heat. To find the origin of the multip…
The effect of the quenched bond-randomness on the ordering of the $S=1/2$ antiferromagnetic Heisenberg model on the kagome lattice is investigated by means of an exact-diagonalization method. When the randomness exceeds a critical value, the ground state of the model exhibits a transition within the non-magnetic state into the randomness-relevant gapless spin-liquid state. Implications to the S=1/2 kagome-lattice antiferromagnet herbertsmithite is discussed.
A brief review is provided of earlier work on the low temperature phases of $S=1$ kagome and triangular lattice antiferromagnets in which there is sufficiently strongly single-ion anisotropy $D$ that dominates over the antiferromagnetic exchange $J$.
The spin half Heisenberg antiferromagnet on the Kagome lattice, is mapped by Contractor Renormalization to a Spin-Pseudospin Hamiltonian on the triangular superlattice. Variationally, we find a ground state with columnar dimer order. Dimer orientation fluctuations are described by an effective O(2) model at energies above an exponentially suppressed clock mass scale. Our results explain the large density of low energy singlets observed numerically, and the non magnetic T-squared specific heat observed experimentally.
Low-energy degrees of freedom of a spin-1/2 kagome antiferromagnet in the vicinity of the saturation field are mapped to a hard-hexagon model on a triangular lattice. The latter model is exactly solvable. The presented mapping allows to obtain quantitative description of the magnetothermodynamics of a quantum kagome antiferromagnet up to exponentially small corrections as well as predict the critical behavior for the transition into a magnon crystal state. Analogous mapping is presented for the sawtooth chain, which is mapped onto a model of classical hard dimers on a chain.
Using an advanced Monte Carlo algorithm and high precision spin dynamics simulation, we investigated the dynamical behavior of the Heisenberg antiferromagnet on a kagome lattice at extremely low temperatures. We demonstrate that the detection and correct identification of propagating excitations depends crucially on the choice of coordinates and we show how modes are displaced in Fourier space if a single, global Cartesian coordinate system is chosen.
The coupled spin tube system, which is equivalent to a stacked Kagome-triangular spin system, exhibits the cuboc order -- a non-coplanar spin order with a twelve-sublattice structure accompanying spontaneous breaking of the translational symmetry -- in the Kagome-triangular plane. On the basis of the spin-wave theory, we analyze spin-wave excitations of the planar Kagome-triangular spin system, where the geometric phase characteristic to the cuboc spin structure emerges. We further investigate spin-wave excitations and dynamical spin structure factors for the coupled spin tubes, assuming the s…
Classical Heisenberg antiferromagnets on two-dimensional kagome and three-dimensional hyperkagome lattices are investigated by Monte Carlo simulations. For both models the symmetry-breaking states at low temperatures are described by non-zero octupole moments or third-rank spin tensor order parameters. In the case of the two-dimensional kagome antiferromagnet, a sharp crossover into a coplanar state takes place at T_k ~ 0.004J, which we attribute to proliferation of fractional vortices. The three-dimensional model exhibits a first-order transition at T_c ~ 0.002J into a phase with critical spi…
An effective-field theory based on the single-spin cluster has been used to study of a diluted spin-$1/2$ Ising antiferromagnet on the Kagome lattice with nearest-neighbor interactions. We observe five plateaus in the magnetization curve of the diluted antiferromagnet when a magnetic field is applied which is in agreement with Monte Carlo calculation. The effect of the site-dilution on the magnetic susceptibility is also investigated and discussed. In particular, we have found that the frustrated Kagome lattice inverse susceptibility fall to zero at $0$K.
The thermal order by disorder effect in magnetic field is studied for a classical Heisenberg antiferromagnet on the kagome lattice. Using analytical arguments we predict a unique H-T phase diagram for this strongly frustrated magnet: states with a coplanar and a uniaxial triatic order parameters respectively at low and high magnetic fields and an incompressible collinear spin-liquid state at a one-third of the saturation field. We also present the Monte Carlo data which confirm existence of these phases.
When the constituent spins have an energetic preference to lie along an easy-axis, triangular and Kagome lattice antiferromagnets often develop long-range order that distinguishes the three sublattices of the underlying triangular Bravais lattice. In zero magnetic field, this three-sublattice order melts {\em either} in a two-step manner, {\em i.e.} via an intermediate phase with power-law three-sublattice order controlled by a temperature dependent exponent $η(T) \in (\frac{1}{9},\frac{1}{4})$, {\em or} via a transition in the three-state Potts universality class. Here, I predict that the uni…
Asymmetric destruction of the one-third magnetization plateau upon heating is found in the spin-1/2 kagome Heisenberg antiferromagnets using the typical pure quantum state approach. The asymmetry originates from larger density of states of low-lying excited sates of $N_{\rm s}$ spin systems with magnetization $(1/3-2/N_{\rm s})$ than that of low-lying sates with magnetization $(1/3+2/N_{\rm s})$. The enhanced specific heat and entropy that reflect the larger density of states in the lower-field side of the plateau are detectable in candidate materials of the kagome antiferromagnets. We discuss…
We discuss the ground state and the low-lying excitations of the spin-half Heisenberg antiferromagnet on the two-dimensional square-kagome lattice. This magnetic system belongs to the class of highly frustrated spin systems with an infinite non-trivial degeneracy of the classical ground state as it is known also for the Heisenberg antiferromagnet on the kagome and on the star lattice. The quantum ground state of the spin-half system is a quantum paramagnet likely with a finite spin gap and with a large number of non-magnetic excitations within this gap. The magnetization versus field curve sho…
Low energy spectrum of the S=1 kagomé Heisenberg antiferromagnet (KHAF) is studied by means of exact diagonalization and the cluster expansion. The magnitude of the energy gap of the magnetic excitation is consistent with the recent experimental observation for \mpynn. In contrast to the $S=1/2$ KHAF, the non-magnetic excitations have finite energy gap comparable to the magnetic excitation. As a physical picture of the ground state, the hexagon singlet solid state is proposed and verified by variational analysis.
The magnetization process of the S=1 and 1/2 kagome Heisenberg antiferromagnet is studied by means of the numerical exact diagonalization method. It is found that the magnetization curve at zero temperature has a plateau at 1/3 of the full magnetization. In the presence of $\sqrt{3} \times \sqrt{3}$ lattice distortion, this plateau is enhanced and eventually the ferrimagnetic state is realized. There also appear the minor plateaux above the main plateau. The physical origin of these phenomena is discussed.
The ground state phase transition in the distorted S=1 kagomé Heisenberg antiferromagnet (KHAF) is studied by means of the perturbational calculation and numerical exact diagonalization method. For strong $\sqrt{3} \times \sqrt{3}$ lattice distortion, the hexgonal singlet solid (HSS) ground state of the uniform KHAF is destroyed and new singlet state, large HSS (LHSS) state, which is globally different from the HSS state is realized. The quantum phase transition between these two singlet states is analogous to the Haldane-dimer transition in the S=1 antiferromagnetic Heisenberg chain. The pres…
In order to study the magnetic properties of frustrated metallic systems, we present Quantum Monte Carlo data on the magnetic susceptibility of the Hubbard model on triangular and Kagome lattices. We show that the underlying lattice structure is important, and determines the nature and the doping dependence of the magnetic fluctuations. In particular, in the doped Kagome case we find strong short-range magnetic correlations, which makes the metallic Kagome systems a promising field for studies of superconductivity.
We introduce a two dimensional network of corner-sharing triangles with square lattice symmetry. Properties of magnetic systems here should be similar to those on the kagome lattice. Focusing on the spin half Heisenberg quantum antiferromagnet, we generalise the spin symmetry group from SU(2) to SU(N). In the large N limit, we map the model exactly to the eight vertex model, solved by Baxter. We predict an exponential number of low-lying singlet states, a triplet gap, and a two-peak specific heat. In addition, the large N limit suggests a finite temperature phase transition into a phase with o…
The recently fabricated two-dimensional magnetic materials Cu9X2(cpa)6.xH2O (cpa=2-carboxypentonic acid; X=F,Cl,Br) have copper sites which form a triangular kagome lattice (TKL), formed by introducing small triangles (``a-trimers'') inside of each kagome triangle (``b-trimer''). We show that in the limit where spins residing on b-trimers have Ising character, quantum fluctuations of XXZ spins residing on the a-trimers can be exactly accounted for in the absence of applied field. This is accomplished through a mapping to the kagome Ising model, for which exact analytic solutions exist. We deri…
We derive exact results for close-packed dimers on the triangular kagome lattice (TKL), formed by inserting triangles into the triangles of the kagome lattice. Because the TKL is a non-bipartite lattice, dimer-dimer correlations are short-ranged, so that the ground state at the Rokhsar-Kivelson (RK) point of the corresponding quantum dimer model on the same lattice is a short-ranged spin liquid. Using the Pfaffian method, we derive an exact form for the free energy, and we find that the entropy is 1/3 ln2 per site, regardless of the weights of the bonds. The occupation probability of every bon…
We study the spin-1/2 Heisenberg model in a lattice that interpolates between the triangular and the kagome lattices. The exchange interaction along the bonds of the kagome lattice is J, and the one along the bonds connecting kagome and non-kagome sites is J', so that J'=J corresponds to the triangular limit and J'=0 to the kagome one. We use variational and exact diagonalization techniques. We analyze the behavior of the order parameter for the antiferromagnetic phase of the triangular lattice, the spin gap, and the structure of the spin excitations as functions of J'/J. Our results indicate …
We investigate the possible regular magnetic order (RMO) for the spin models with global O(3) spin rotation, based on a group theoretical approach for triangular and kagome lattices. The main reason to study these RMOs is that they are good variational candidates for the ground states of many specific models. In this work, we followed the prescription introduced by Messio et al. (L. Messio, C. Lhuillier, and G. Misguich, Phys. Rev. B, 2011, 83, 184401) for the p6m group and extended their work for different subgroups of p6m, i.e., p6, p3, p3m1, and p31m. We have listed all the possible regular…
The Kagome Heisenberg antiferromagnet is mapped onto an effective Hamiltonian on the star superlattice by Contractor Renormalization. Comparison of ground state energies on large lattices to Density Matrix Renormalization Group justifies truncation of effective interactions at range 3. Within our accuracy, magnetic and translational symmetries are not broken (i.e. a spin liquid ground state). However, we discover doublet spectral degeneracies which signal the onset of p6 - chirality symmetry breaking. This is understood by simple mean field analysis. Experimentally, the p6 chiral order paramet…
We obtain the rich phase diagrams in the Hubbard model on the triangular Kagomé lattice as a function of interaction, temperature and asymmetry, by combining the cellular dynamical mean-field theory with the continuous time quantum Monte Carlo method. The phase diagrams show the asymmetry separates the critical points in Mott transition of two sublattices on the triangular Kagomé lattice and produces two novel phases called plaquette insulator with an obvious gap and a gapless Kondo metal. When the Coulomb interaction is stronger than the critical value Uc, a short range paramagnetic insulatin…
We discuss the ground-state degeneracy of spin-$1/2$ kagome-lattice quantum antiferromagnets on magnetization plateaus by employing two complementary methods: the adiabatic flux insertion in closed boundary conditions and a 't Hooft anomaly argument on inherent symmetries in a quasi-one-dimensional limit. The flux insertion with a tilted boundary condition restricts the lower bound of the ground-state degeneracy on $1/9$, $1/3$, $5/9$, and $7/9$ magnetization plateaus under the $\mathrm{U(1)}$ spin-rotation and the translation symmetries: $3$, $1$, $3$, and $3$, respectively. This result motiv…
We determine dynamical response functions of the S=1/2 Heisenberg quantum antiferromagnet on the kagome lattice based on large-scale exact diagonalizations combined with a continued fraction technique. The dynamical spin structure factor has important spectral weight predominantly along the boundary of the extended Brillouin zone and energy scans reveal broad response extending over a range of 2 \sim 3J concomitant with pronounced intensity at lowest available energies. Dispersive features are largely absent. Dynamical singlet correlations -- which are relevant for inelastic light probes -- re…
The ground state phase transitions in the distorted S=1 kagome Heisenberg antiferromagnet (KHAF) with single-site anisotropy D are studied by the numerical exact diagonalization method. For strong easy plane anisotropy, the hexgonal singlet solid (HSS) ground state of the uniform KHAF is destroyed and large-D state is realized. The quantum phase transition between these two states is analogous to the Haldane-large-D transition in the S=1 antiferromagnetic Heisenberg chain. The combined effect of the sqrt(3) times sqrt(3) lattice distortion and single site anisotropy is also investigated. The g…
We consider a spin-$\frac{1}{2}$ kagome-like chain with competing ferro- and antiferromagnetic anisotropic exchange interactions. The ground state phase diagram of this model consists of the ferromagnetic and ferrimagnetic phases. We study the ground state and the low-temperature properties on the phase boundary between these phases. The ground state on this phase boundary is macroscopically degenerate and consists of localized magnon states. We calculate the ground state degeneracy and corresponding residual entropy. The spontaneous magnetization has a jump on the phase boundary confirming th…
Neutron diffraction studies have been carried out in the temperature(T) range between 10 K and 130 K on a single crystal of YBaCo4O7, which has the stacking of kagome and triangular lattices of CoO4 tetrahedra along the c-axis. Structural transitions have been found at two temperatures Tc1~70 K and Tc2~105 K. With decreasing T, magnetic order appears along with the transition at Tc2, but it does not grow to an ideal long-range order even at the lowest T studied (~10 K). Two groups of magnetic diffuse reflections, which originate from the Co-moments of the kagome and triangular lattices, are ob…
In spin-charge coupled systems, geometrical frustration of underlying lattice structures can give rise to nontrivial magnetic orders and electronic states. Here we explore such a possibility in the Kondo lattice model with classical localized spins on a triangular lattice by using a variational calculation and simulated annealing. We find that the system exhibits a four-sublattice collinear ferrimagnetic phase at 5/8 filling for a large Hund's-rule coupling. In this state, the system spontaneously differentiates into the up-spin kagome network and the isolated down-spin sites, which we call th…
The kagome Heisenberg antiferromagnet is a leading candidate in the search for a spin system with a quantum spin-liquid ground state. The nature of its ground state remains a matter of great debate. We conducted 17-O single crystal NMR measurements of the S=1/2 kagome lattice in herbertsmithite ZnCu$_3$(OH)$_6$Cl$_2$, which is known to exhibit a spinon continuum in the spin excitation spectrum. We demonstrate that the intrinsic local spin susceptibility $χ_{kagome}$ deduced from the 17-O NMR frequency shift asymptotes to zero below temperature T ~ 0.03 J, where J ~ 200 K is the Cu-Cu super-exc…
The flat band has attracted a lot of attention because it gives rise to many exotic phases, as recently demonstrated in magic angle twisted bilayer graphene. Here, based on first-principles calculations, we identify a metal-insulator transition in boron triangular Kagome lattice with a spin-polarized flat band at 2/3-filling. This phase transition is accompanied by the formation of a Wigner crystal, which is driven by Fermi surface nesting effect and thereby strong electron-phonon interactions, keeping ferromagnetism. Our calculation results suggest that boron triangular Kagome lattices with p…
We investigate the zero-temperature phase diagram of the nearest-neighbor kagome antiferromagnet in the presence of Dzyaloshinksii-Moriya interaction. We develop a theory for the transition between Z2 spin liquids with bosonic spinons and a phase with antiferromagnetic long-range order. Connections to recent numerical studies and experiments are discussed.
Derivation of a reduced effective model allows for a unified treatment and discussion of the $J_1$-$J_2$ Heisenberg model on a triangular and kagome lattice. Calculating thermodynamic quantities, i.e. the entropy $s(T)$ and uniform susceptibility $χ_0(T)$, numerically on systems up to effectively $N=48$ sites we show by comparing to full-model results that low-$T$ properties are well represented within the reduced model. Moreover, we find in the spin-liquid regime similar variation of $s(T)$ as well as $χ_0(T)$ in both models down to $T \ll J_1$. In particular, the spin liquid appears to be ch…
The magnetization process of the spin-S Heisenberg antiferromagnet on the kagome lattice is studied by the numerical-diagonalization method. Our numerical-diagonalization data for small finite-size clusters with S=1, 3/2, 2, and 5/2 suggest that a magnetization plateau appears at one-third of the height of the saturation in the magnetization process irrespective of S. We discuss the S dependences of the edge fields and the width of the plateau in comparison with recent results obtained by real-space perturbation theory.
The magnetization process of the isotropic Heisenberg antiferromagnet on the kagome lattice is studied. Data obtained from the numerical-diagonalization method are reexamined from the viewpoint of the derivative of the magnetization with respect to the magnetic field. We find that the behavior of the derivative at approximately one-third of the height of the magnetization saturation is markedly different from that for the cases of typical magnetization plateaux. The magnetization process of the kagome-lattice antiferromagnet reveals a new phenomenon, which we call the "magnetization ramp".
We study the system size dependence of the singlet-triplet excitation gap in the $S=1/2$ kagome-lattice Heisenberg antiferromagnet by numerical diagonalization. We successfully obtain a new result of a cluster of 42 sites. The two sequences of gaps of systems with even-number sites and that with odd-number sites are separately analyzed. Careful examination clarifies that there is no contradiction when we consider the system to be gapless.
Coupling between spin and lattice degrees of freedom are important in geometrically frustrated magnets where they can lead to degeneracy lifting and novel orders. We show that moderate spin-lattice couplings in triangular and Kagome antiferromagnets can induce complex colinear magnetic orders. When classical Heisenberg spins on the triangular lattice are coupled to Einstein phonons, a rich variety of phases emerge, including the experimentally observed four sublattice state and the five sublattice 1/5th plateau state seen in the magneto-electric material CuFeO$_2$. In addition we predict magne…
We study the ground state of a spin-half Heisenberg antiferromagnet on the stacked kagome lattice by using a spin-rotation-invariant Green's-function method. Since the pure two-dimensional kagome antiferromagnet is most likely a magnetically disordered quantum spin liquid, we investigate the question whether the coupling of kagome layers in a stacked three-dimensional system may lead to a magnetically ordered ground state. We present spin-spin correlation functions and correlation lengths. For comparison we apply also linear spin wave theory. Our results provide strong evidence that the system…
Within the t-J model, we study the electronic properties of the doped antiferromagnet on the kagome lattice based on the framework of the self-consistent mean-field theory. At the half-filling, the spin-liquid ground-state energy per site of the kagome antiferromagnet is Eg/NJ=-0.859, which is in very good agreement with the numerical estimates. Away from the half-filling, the electron photoemission spectroscopy and density of states are discussed, and the results indicate that there is a gap in the normal-state of the system.
Inspired by the recent theoretical suggestion that the random-bond $S=1/2$ antiferromagnetic Heisenberg model on the triangular and the kagome lattices might exhibit a randomness-induced quantum spin liquid (QSL) behavior when the strength of the randomness exceeds a critical value, and that this "random-singlet state" might be relevant to the QSL behaviors experimentally observed in triangular organic salts $κ{\rm -(ET)_2 Cu_2 (CN)_3}$and ${\rm EtMe_3 Sb[Pd(dmit)_2]_2}$ and in kagome herbertsmithite ${\rm CuZn_3(OH)_6Cl_2}$, we further investigate the nature of the static and the dynamical sp…
The frustration of antiferromagnetic interactions on the loosely connected kagome lattice associated to the enhancement of quantum fluctuations for S=1/2 spins was acknowledged long ago as a keypoint to stabilize novel ground states of magnetic matter. Only very recently, the model compound Herbersmithite, ZnCu3(OH)6Cl2, a structurally perfect kagome antiferromagnet, could be synthesized and enables a close comparison to theories. We review and classify various experimental results obtained over the past years and underline some of the pending issues.
Employing complementary torque magnetometry and electron spin resonance on single crystals of herbertsmithite, the closest realization to date of a quantum kagome antiferromagnet featuring a spin-liquid ground state, we provide novel insight into different contributions to its magnetism. At low temperatures, two distinct types of defects with different magnetic couplings to the kagome spins are found. Surprisingly, their magnetic response contradicts the three-fold symmetry of the ideal kagome lattice, suggesting the presence of a global structural distortion that may be related to the establi…
The recent NMR experiments on ZnCu3(OH)6Cl2 motivate our study of the effect of non- magnetic defects on the antiferromagnetic spin-1/2 kagome lattice. We use exact diagonalization methods to study the effect of two such defects on finite size systems. Our results, obtained without adjustable parameters, are in good quantitative agreement with recent Oxygen 17 NMR data. They provide support for the experimental interpretation of the presence of defects within the kagome layers due to Zn/Cu substitutions. Our results also show that disorder effects become relevant at lower temperatures, raising…
We propose a general non-perturbative scheme that quantitatively maps the low-energy sector of spin-1/2 frustrated Heisenberg antiferromagnets to effective Generalized Quantum Dimer Models. We develop the formal lattice independent frame and establish some important results on (i) the locality of the generated Hamiltonians (ii) how full resummations can be performed in this renormalization scheme. The method is then applied to the much debated kagome antiferromagnet for which a fully resummed effective Hamiltonian - shown to capture the essential properties and provide deep insights on the mic…
We prepared a powder sample of edwardsite Cd2Cu3(SO4)2(OH)6 4H2O, which is a new candidate compound for the spin-1/2 kagome antiferromagnet, and studied its magnetic properties by magnetic susceptibility and heat capacity measurements. Edwardsite has a deformed kagome lattice with an average antiferromagnetic interaction of 51 K between nearby spins and shows an antiferromagnetic order accompanied by a small ferromagnetic moment below 4.3 K. The weak ferromagnetism is likely due to spin canting caused by sizable Dzyaloshinsky-Moriya interactions, which may stabilize the long-range magnetic ord…
Herbertsmithite (ZnCu3(OH)6Cl2) is often discussed as the best realization of the highly frustrated antiferromagnetic kagome lattice known so far. We employ density functional theory calculations to determine eight exchange coupling constants of the underlying Heisenberg Hamiltonian. We find the nearest neighbour coupling J1 to exceed all other couplings by far. However, next-nearest neighbour kagome layer couplings of 0.019 J1 and interlayer couplings of up to -0.035 J1 slightly modify the perfect antiferromagnetic kagome Hamiltonian. Interestingly, the largest interlayer coupling is ferromag…
In this Letter, we identify a noncoplanar chiral spin texture on the distorted kagomé-lattice antiferromagnets induced by the presence of a magnetic field applied perpendicular to the distorted kagomé plane. The noncoplanar chiral spin texture has a nonzero scalar spin chirality similar to a chiral quantum spin liquid with broken time-reversal symmetry. In the noncoplanar regime we observe nontrivial topological magnetic excitations and thermal Hall response through the emergent field-induced scalar spin chirality in contrast to collinear ferromagnets in which the Dzyaloshinskii-Moriya (DM) sp…
We argue that the S=1/2 kagome antiferromagnet undergoes a quantum phase transition when the Dzyaloshinskii-Moriya coupling is increased. For $D<D_c$ the system is in a moment-free phase and for $D>D_c$ the system develops antiferromagnetic long-range order. The quantum critical point is found to be $D_c \simeq 0.1J$ using exact diagonalizations and finite-size scaling. This suggests that the kagome compound ZnCu$_3(OH)$_6$Cl$_3$ may be in a quantum critical region controlled by this fixed point.
We have studied the effect of the Dzyaloshinskii-Moriya interaction on kagome Heisenberg anti-ferromagnet using Schwinger boson mean field theory (SBMFT). Within SBMFT framework, Messio et al had argued that the ground state of kagome antiferromagnet is possibly a chiral topological spin liquid (Phys. Rev. Lett. 108, 207204 (2012)). Thus, we have computed zero-temperature ground state phase diagram considering the time-reversal breaking states as well as fully symmetric Ansätze. We discuss the relevance of these results in experiments and other studies. Finally, we have computed the static and…
Interplay of magnetic and thermodynamic responses in the kagome-triangular system
Key Laboratory of Multiscale Spin Physics (Ministry of Education), Beijing Normal University（北京师范大学多尺度自旋物理教育部重点实验室）；School of Physical Science and Technology, Beijing University of Posts and Telecommunications（北京邮电大学理学院）；Key Laboratory for Microstructural Material Physics of Hebei Province, School of Science, Yanshan University（燕山大学理学院河北省微观材料物理重点实验室）；Beijing Computational Science Research Center（北京计算科学研究中心）
Dynamical magnetic correlations in the geometrically frustrated Nd$\_3$Ga$\_5$SiO$\_{14}$ compound were probed by inelastic neutron scattering on a single crystal. A scattering signal with a ring shape distribution in reciprocal space and unprecedented dispersive features was discovered. Comparison with calculated static magnetic scattering from models of correlated spins suggests that the observed phase is a spin liquid inherent to an antiferromagnetic kagomé-like lattice of anisotropic Nd moments.
We investigate the connection between highly frustrated kagome based Hamiltonians and a recently synthesized family of materials containing Ti3+ S=1/2 ions. Employing a combination of all electron density functional theory and numerical diagonalization techniques, we establish the Heisenberg Hamiltonians for the distorted kagome antiferromagnets Rb2NaTi3F12, Cs2NaTi3F12 and Cs2KTi3F12. We determine magnetization curves in excellent agreement with experimental observations. Our calculations successfully clarify the relationship between the experimental observations and the magnetization-plateau…
An effective spin-orbit Hamiltonian is derived for a spin-1/2 trimerized kagome antiferromagnet in the second-order of perturbation theory in the ratio of two coupling constants. Low-energy singlet states of the obtained model are mapped to a quantum dimer model on a triangular lattice. The quantum dimer model is dominated by dimer resonances on a few shortest loops of the triangular lattice. Characteristic energy scale for the dimer model constitutes only a small fraction of the weaker exchange coupling constant.
The ground state of the S=1/2 Heisenberg antiferomagnet on kagome can be viewed as a collection of fermionic spinons bound into small, heavy singlet pairs. Low-energy magnetic excitations in this system correspond to breaking the pairs into individual spinons. We calculate the structure factor for inelastic neutron scattering from independent spinon pairs.
