Early onset of ground-state deformation in the neutron-deficient polonium isotopes
T. E. Cocolios, W. Dexters, M. D. Seliverstov, A. N. Andreyev, S. Antalic, A. E. Barzakh, B. Bastin, J. Buscher, I. G. Darby, D. V. Fedorov, V. N. Fedosseyev, K… 展开作者
T. E. Cocolios, W. Dexters, M. D. Seliverstov, A. N. Andreyev, S. Antalic, A. E. Barzakh, B. Bastin, J. Buscher, I. G. Darby, D. V. Fedorov, V. N. Fedosseyev, K. T. Flanagan, S. Franchoo, S. Fritzsche, G. Huber, M. Huyse, M. Keupers, U. Koster, Yu. Kudryavtsev, E. Mane, B. A. Marsh, P. L. Molkanov, R. D. Page, A. M. Sjoedin, I. Stefan, J. Van de Walle, P. Van Duppen, M. Venhart, S. G. Zemlyanoy, M. Bender, P. -H. Heenen
In-source resonant ionization laser spectroscopy of the even-$A$ polonium isotopes $^{192-210,216,218}$Po has been performed using the $6p^37s$ $^5S_2$ to $6p^37p$ $^5P_2$ ($λ=843.38$ nm) transition in the polonium atom (Po-I) at the CERN ISOLDE facility. The comparison of the measured isotope shifts in $^{200-210}$Po with a previous data set allows to test for the first time recent large-scale atomic calculations that are essential to extract the changes in the mean-square charge radius of the atomic nucleus. When going to lighter masses, a surprisingly large and early departure from sphericity is observed, which is only partly reproduced by Beyond Mean Field calculations.
Currently, forty-two thallium, forty-two lead, forty-one bismuth, and forty-two polonium isotopes have so far been observed; the discovery of these isotopes is discussed. For each isotope a brief summary of the first refereed publication, including the production and identification method, is presented.
The newly developed multi-quasiparticle triaxial projected shell-model approach is employed to study the high-spin band structures in neutron-deficient even-even Ce- and Nd-isotopes. It is observed that gamma-bands are built on each intrinsic configuration of the triaxial mean-field deformation. Due to the fact that a triaxial configuration is a superposition of several K-states, the projection from these states results in several low-lying bands originating from the same intrinsic configuration. This generalizes the well-known concept of the surface gamma-oscillation in deformed nuclei based …
The evolution of quadrupole and octupole collectivity in neutron-deficient Xe, Ba, Ce, and Nd nuclei near the "octupole magic" neutron number $N=56$ is investigated within the mapped $sdf$-IBM framework. Microscopic input is obtained via quadrupole and octupole constrained Hartree-Fock-Bogoliubov calculations, based on the parametrization D1M of the Gogny energy density functional. Octupole-deformed mean-field ground states are predicted for Ba and Ce isotopes near $N=56$. Excitation energies of positive- and negative-parity states as well as electric transition rates are computed with wave fu…
The electromagnetic decay of $^{250m}$No and the stability of neutron deficient Rf isotopes
IJCLab, CNRS/IN2P3 and Université Paris Saclay（法国萨克雷大学）；IPHC, CNRS/IN2P3 and Université de Strasbourg（斯特拉斯堡大学）；FLNR, JINR（杜布纳联合核研究所）；Dubna State Univerity（杜布纳国立大学）
Velocity distributions of heavy residues (A_Res > A_Tar), produced in irradiations of Au-197 and Ho-165 with Ne-20 at bombarding energies of E = 208 MeV, have been measured at the velocity filter SHIP. While for the products from Ne-20 + Ho-165 just a mean value of v/v_CN = 0.91+-0.01 was obtained, individual residues, attributed to isotopes of astatine and polonium with mass numbers ranging from A=195 to A=203 could be identified by means of alpha - spectroscopy in the bombardments Au-197. A linear increase of the mean velocity from v/v_CN = 0.85 to v/v_CN = 0.93 with decreasing residue mass …
Neutron-deficient krypton isotopes are of particular interest due to the coexistence of oblate and prolate shapes in low-lying states and the transition of ground-state from one dominate shape to another as a function of neutron number. A detailed interpretation of these phenomena in neutron-deficient Kr isotopes requires the use of a method going beyond a mean-field approach that permits to determine spectra and transition probabilities. The aim of this work is to provide a systematic calculation of low-lying state in the even-even 68-86Kr isotopes and to understand the shape coexistence phen…
The discovery of naturally occurring long-lived isomeric states (t_1/2 > 10^8 yr) in the neutron-deficient isotopes 211,213,217,218Th [A. Marinov et al., Phys. Rev. C 76, 021303(R) (2007)] was reexamined using accelerator mass spectrometry (AMS). Because AMS does not suffer from molecular isobaric background in the detection system, it is an extremely sensitive technique. Despite our up to two orders of magnitude higher sensitivity we cannot confirm the discoveries of neutron-deficient thorium isotopes and provide upper limits for their abundances.
Evidence for the existence of long-lived neutron-deficient isotopes has been found in a study of naturally-occurring Th using iductively coupled plasma-sector field mass spectrometry. They are interpreted as belonging to the recently discovered class of long-lived high spin super- and hyperdeformed isomers.
Production cross sections and excitation functions of neutron deficient isotopes of U, Pa and Th have been measured in the reaction of 22Ne + 208Pb. The comparison of experimental production cross sections of uranium isotopes with the neutron number 126 <= N <= 134 to the values calculated using statistical model of nuclear deexcitation has been carried out. There is shown, that none of the commonly used methods of introduction of shell effect influence on the production cross sections of evaporations residues allows to reproduce unambigiously used set of experimental data. Simple semiempirica…
The masses of the exotic isotopes $^{210-214}$Ac and $^{210-214}$Ra have been measured with a multi-reflection time-of-flight mass spectrograph. These isotopes were obtained in flight as fusion-evaporation products behind the gas-filled recoil ion separator GARIS-II at RIKEN. The new direct mass measurements serve as an independent and direct benchmark for existing $α$-$γ$ spectroscopy data in this mass region. Further, new mass anchor points are set for U and Np nuclei close to the $N=126$ shell closure for a future benchmark of the $Z=92$ sub-shell for neutron-deficient heavy isotopes. Our m…
In an experiment with the BigRIPS separator at the RIKEN Nishina Center, the fragmentation of a $^{78}$Kr beam allowed the observation of new neutron-deficient isotopes at the proton drip-line. Clean identification spectra could be produced and $^{63}$Se, $^{67}$Kr, and $^{68}$Kr were identified for the first time. In addition, $^{59}$Ge was also observed. Three of these isotopes, $^{59}$Ge, $^{63}$Se, and $^{67}$Kr, are potential candidates for ground-state two-proton radioactivity. In addition, the isotopes $^{58}$Ge, $^{62}$Se, and $^{66}$Kr were also sought but without success. The present…
The neutron-deficient mercury isotopes, $^{184,186}$Hg, were studied with the Recoil Distance Doppler Shift (RDDS) method using the Gammasphere array and the Köln Plunger device. The Differential Decay Curve Method (DDCM) was employed to determine the lifetimes of the yrast states in $^{184,186}$Hg. An improvement on previously measured values of yrast states up to $8^{+}$ is presented as well as first values for the $9_{3}$ state in $^{184}$Hg and $10^{+}$ state in $^{186}$Hg. $B(E2)$ values are calculated and compared to a two-state mixing model which utilizes the variable moment of inertia …
The masses of ten proton-rich nuclides, including the N=Z+1 nuclides 85-Mo and 87-Tc, were measured with the Penning trap mass spectrometer SHIPTRAP. Compared to the Atomic Mass Evaluation 2003 a systematic shift of the mass surface by up to 1.6 MeV is observed causing significant abundance changes of the ashes of astrophysical X-ray bursts. Surprisingly low alpha-separation energies for neutron-deficient Mo and Tc are found, making the formation of a ZrNb cycle in the rp process possible. Such a cycle would impose an upper temperature limit for the synthesis of elements beyond Nb in the rp pr…
The neutron-deficient Ca isotopes continue to attract attention due to their importance for testing isospin symmetry and their relevance in capture reactions of interest for nova nucleosynthesis and the shape of light curves in Type I X-ray bursts. To date, spectroscopic information on 38,39 Ca is largely limited to data on lower-spin excited states. Here, we report in-beam γ-ray spectroscopy of complementary higher-spin, complex-structure states in 39 Ca populated in fast-beam-induced, momentum-dissipative processes leading to neutron pickup onto excited configurations of the projectile, 9 Be…
This paper reports on the hyperfine-structure and radioactive-decay studies of the neutron-deficient francium isotopes $^{202-206}$Fr performed with the Collinear Resonance Ionization Spectroscopy (CRIS) experiment at the ISOLDE facility, CERN. The high resolution innate to collinear laser spectroscopy is combined with the high efficiency of ion detection to provide a highly-sensitive technique to probe the hyperfine structure of exotic isotopes. The technique of decay-assisted laser spectroscopy is presented, whereby the isomeric ion beam is deflected to a decay spectroscopy station for alpha…
We present systematic calculations on the spectroscopy and transition properties of even-even Te isotopes by using the large-scale configuration interaction shell model approach with a realistic interaction. These nuclei are of particular interest since their yrast spectra show a vibrational-like equally-spaced pattern but the few known E2 transitions show anomalous rotational-like behavior, which cannot be reproduced by collective models. Our calculations reproduce well the equally-spaced spectra of those isotopes as well as the constant behavior of the $B(E2)$ values in $^{114}$Te. The calcu…
Using isochronous mass spectrometry at the experimental storage ring CSRe in Lanzhou, the masses of $^{82}$Zr and $^{84}$Nb were measured for the first time with an uncertainty of $\sim 10$ keV, and the masses of $^{79}$Y, $^{81}$Zr, and $^{83}$Nb were re-determined with a higher precision. %The latter differ significantly from their literature values. The latter are significantly less bound than their literature values. Our new and accurate masses remove the irregularities of the mass surface in this region of the nuclear chart. Our results do not support the predicted island of pronounced lo…
The new neutron-deficient isotope $^{249}$No was synthesized for the first time in the fusion-evaporation reaction $^{204}$Pb($^{48}$Ca,3n)$^{249}$No. After separation, using the kinematic separator SHELS, the new isotope was identified with the GABRIELA detection system through genetic correlations with the known daughter and granddaughter nuclei $^{245}$Fm and $^{241}$Cf. The alpha-decay activity of $^{249}$No has an energy of 9129(22)$~$keV and half-life 38.3(2.8) ms. An upper limit of 0.2\% was measured for the fission branch of $^{249}$No. Based on the present data and recent information …
Shape coexistence in the $Z \approx 82$ region has been established in mercury, lead and polonium isotopes. Even-even mercury isotopes with $100 \leq N \leq 106$ present multiple fingerprints of this phenomenon, which seems to be no longer present for $N \geq 110$. According to a number of theoretical calculations, shape coexistence is predicted in the $^{188}$Hg isotope. The $^{188}$Hg nucleus was populated using two different fusion-evaporation reactions with two targets, $^{158}$Gd and $^{160}$Gd, and a beam of $^{34}$S, provided by the Tandem-ALPI accelerators complex at the Laboratori Naz…
An analysis of recent experimental data [J. Khuyagbaatar et al., Phys. Rev. C 104, L031303 (2021)] has established the existence of two fissioning states in $^{253}$Rf: the ground state and a low-lying isomeric state, most likely involving the same neutron single-particle configurations as in the lighter isotone $^{251}$No. The ratio of fission half-lives measured in $^{253}$Rf was used to predict the fission properties of the 1/2$^{+}$ isomeric state in $^{251}$No and draw conclusions as to the stability against fission of even lighter Rf systems. This paper focusses again on the fission prop…
Large-scale shell-model calculations are carried out in the model space including neutron-hole orbitals $2p_{1/2}$, $1f_{5/2}$, $2p_{3/2}$, $0i_{13/2}$, $1f_{7/2}$ and $0h_{9/2}$ to study the structure and electromagnetic properties of neutron deficient Pb isotopes. An optimized effective interaction is used. Good agreement between full shell-model calculations and experimental data is obtained for the spherical states in isotopes $^{194-206}$Pb. The lighter isotopes are calculated with an importance-truncation approach constructed based on the monopole Hamiltonian. The full shell-model result…
Exploring the statistical properties of the neutron-deficient $^{109}$In isotope with the Oslo method
University of Oslo（奥斯陆大学）；Norwegian Nuclear Research Centre（挪威核研究中心）；Technische Universität Darmstadt（达姆施塔特工业大学）；Western Michigan University（西密歇根大学）；GANIL, CEA/DRF-CNRS/IN2P3（法国国家重离子加速器和实验室（GANIL））；Université Libre de Bruxelles（布鲁塞尔自由大学）；University of California, Berkeley（加州大学伯克利分校）
Direct mass measurements of the low-spin $3/2^{(-)}$ and high-spin $13/2^{(+)}$ states in the neutron-deficient isotopes $^{195}$Po, $^{197}$Po, and high-spin $13/2^{(+)}$ state in $^{199}$Po were performed with the Penning-trap mass spectrometer ISOLTRAP at ISOLDE-CERN. These measurements allow the determination of the excitation energy of the isomeric state arising from the $ν$i$_{13/2}$ orbital in $^{195,197}$Po. Additionally, the excitation energy of isomeric states of lead, radon, and radium isotopes in this region were obtained from $α$-decay chains. The new excitation energies complete …
We have studied via in-beam $γ$-ray spectroscopy $^{196}$Po and $^{198}$Po, which are the first neutron-deficient Po isotopes to exhibit a collective low-lying structure. The ratios of yrast state energies and the E2 branching ratios of transitions from non-yrast to yrast states are indicative of a low-lying vibrational structure. The onset of collective motion in these isotopes can be attributed to the opening of the neutron i$_{13/2}$ orbital at N$\approx$112 and the resulting large overlap between the two valence protons in the h$_{9/2}$ orbital and the valence neutrons in the i$_{13/2}$ or…
The evolution and coexistence of the nuclear shapes as well as the corresponding low-lying collective states and electromagnetic transition rates are investigated along the Krypton isotopic chain within the framework of the interacting boson model (IBM). The IBM Hamiltonian is determined through mean-field calculations based on the several parametrizations of the Gogny energy density functional and the relativistic mean-field Lagrangian. The mean-field energy surfaces, as functions of the axial $β$ and triaxial $γ$ quadrupole deformations, are mapped onto the expectation value of the interacti…
Nuclei located in the neutron-deficient Pb region have a complex structure, rapidly evolving as a function of neutron and proton numbers. The most famous example is $^{186}$Pb where the three lowest levels are $0^+$ states, the two excited $0^+$ ones being located at low excitation energy around 600 keV. Coexisting structures with different properties are found in the neighboring nuclei. Many experiments have been performed over the last few years in which in-band and out-of-band $γ$ transition probabilities have been measured. A detailed interpretation of experimental data requires the use of…
High-precision ab initio calculations of nuclear binding energies: Tin isotopes from dripline to dripline
Technische Universität Darmstadt（达姆施塔特工业大学）；ExtreMe Matter Institute EMMI, GSI Helmholtzzentrum für Schwerionenforschung GmbH（GSI重离子研究中心极端物质研究所EMMI）；KU Leuven, Instituut voor Kern- en Stralingsfysica（荷语鲁汶大学核与辐射物理研究所）；Institut d’Astronomie et d’Astrophysique, Université Libre de Bruxelles（布鲁塞尔自由大学天体物理学与天文学研究所）；Brussels Laboratory of the Universe – BLU-ULB（布鲁塞尔宇宙实验室）；IRFU, CEA, Université Paris-Saclay（巴黎萨克雷大学CEA IRFU）；Max-Planck-Institut für Kernphysik（马克斯·普朗克核物理研究所）
Background: Thick-target-induced nucleon-adding transfer reactions onto energetic rare-isotope beams are an emerging spectroscopic tool. Their sensitivity to single-particle structure complements one-nucleon removal reaction capabilities in the quest to reveal the evolution of nuclear shell structure in very exotic nuclei. Purpose: To add intermediate-energy, carbon-target-induced one-proton pickup reactions to the arsenal of $γ$-ray tagged direct reactions applicable in the regime of low beam intensities and to apply these for the first time to $fp$-shell nuclei. Methods: Inclusive and partia…
Rare isotope beams of neutron-deficient $^{106,108,110}$Sn nuclei from the fragmentation of $^{124}$Xe were employed in an intermediate-energy Coulomb excitation experiment yielding $B(E2, 0^+_1 \to 2^+_1)$ transition strengths. The results indicate that these $B(E2,0^+_1 \to 2^+_1)$ values are much larger than predicted by current state-of-the-art shell model calculations. This discrepancy can be explained if protons from within the Z = 50 shell are contributing to the structure of low-energy excited states in this region. Such contributions imply a breaking of the doubly-magic $^{100}$Sn cor…
Neutron-deficient $^{177-185}$Hg isotopes were studied using in-source laser resonance-ionization spectroscopy at the CERN-ISOLDE radioactive ion-beam facility, in an experiment combining different detection methods tailored to the studied isotopes. These include either alpha-decay tagging or Multi-reflection Time-of-Flight gating to identify the isotopes of interest. The endpoint of the odd-even nuclear shape staggering in mercury was observed directly by measuring for the first time the isotope shifts and hyperfine structures of $^{177-180}$Hg. Changes in the mean-square charge radii for all…
In explosive stellar environments like supernovae, the temperatures are high enough for the production of heavy neutron-deficient nuclei, the socalled p-nuclei. Up to now, the knowledge of the reaction rates of p-nuclei is based on theoretical parameterizations using statistical model calculations. At the bremsstrahlung facility of the superconducting electron accelerator ELBE of FZ Dresden-Rossendorf, we aim to measure the photodisintegration rates of heavy nuclei experimentally. Photoactivation measurements on the astrophysically relevant p-nuclei 92Mo and 144Sm have been performed with brem…
Lifetimes of $2^+_1$ and $4^+_1$ states, as well as some negative-parity and non-yrast states, in $^{188-200}$Hg were measured using $γ-γ$ electronic fast timing techniques with the LaBr$_3$(Ce) detector array of the GRIFFIN spectrometer. The excited states were populated in the $ε/β^+$-decay of $J^π=7^+/2^-$ $^{188-200}$Tl produced at the TRIUMF-ISAC facility. The deduced B(E2) values are compared to different interacting boson model predictions. The precision achieved in this work over previous ones allows for a meaningful comparison with the different theoretical models of these transitiona…
The available data for E2 transition strengths in the region between neutron-deficient Hf and Pt isotopes are far from complete. More and precise data are needed to enhance the picture of structure evolution in this region and to test state-of-the-art nuclear models. In a simple model, the maximum collectivity is expected at the middle of the major shell. However, for actual nuclei, this picture may no longer be the case, and one should use a more realistic nuclear-structure model. We address this point by studying the spectroscopy of Hf. We remeasure the 2^+_1 half-lives of 172,174,176Hf, for…
Fragment energy spectra of neutron deficient isotopes are significantly more energetic than those of neutron rich isotopes of the same element. This trend is well beyond what can be expected for the bulk multi-fragmentation of an equilibrated system. It can be explained, however, if some of these fragments are emitted earlier through the surface of the system while it is expanding and cooling.
Enhanced octupole collectivity is expected in the neutron-deficient Ge, Se and Kr isotopes with neutron number $N \approx 40$ and has indeed been observed for $^{70,72}$Ge. Shape coexistence and configuration mixing are, however, a notorious challenge for theoretical models trying to reliably predict octupole collectivity in this mass region, which is known to feature rapid shape changes with changing nucleon number and spin of the system. To further investigate the microscopic configurations causing the prolate-oblate-triaxial shape transition at $A \approx 72$ and their influence on octupole…
Direct reaction techniques are powerful tools to study the single-particle nature of nuclei. Performing direct reactions on short-lived nuclei requires radioactive ion beams produced either via fragmentation or the Isotope Separation OnLine (ISOL) method. Some of the most interesting regions to study with direct reactions are close to the magic numbers where changes in shell structure can be tracked. These changes can impact the final abundances of explosive nucleosynthesis. The structure of the chain of tin isotopes is strongly influenced by the Z=50 proton shell closure, as well as the neutr…
In this paper we present the first high-resolution laser spectroscopy results obtained at the GISELE laser laboratory of the GANIL-SPIRAL2 facility, in preparation for the first experiments with the S$^3$-Low Energy Branch. Studies of neutron-deficient radioactive isotopes of erbium and tin represent the first physics cases to be studied at S$^3$. The measured isotope-shift and hyperfine structure data are presented for stable isotopes of these elements. The erbium isotopes were studied using the $4f^{12}6s^2$ $^3H_6 \rightarrow 4f^{12}(^3 H)6s6p$ $J = 5$ atomic transition (415 nm) and the tin…
Laser Spectroscopy of Thulium Isotopes Near the $N=82$ Shell Closure: Nuclear Moment and Charge Radius of ${}^{152\mathrm{m}}\mathrm{Tm}$
GSI Helmholtzzentrum für Schwerionenforschung GmbH（GSI亥姆霍兹重离子研究中心有限公司）；Helmholtz-Institut Mainz（美因茨亥姆霍兹研究所）；Johannes Gutenberg-Universität Mainz（约翰内斯·古腾堡大学美因茨分校）；Technische Universität Darmstadt（达姆施塔特工业大学）；KU Leuven（鲁汶大学）；Grand Accelerateur National d’Ions Lourds（法国国家大型重离子加速器研究所）
In-gas-cell laser ionization spectroscopy studies on the neutron deficient 97-101Ag isotopes have been performed with the LISOL setup. Magnetic dipole moments and mean-square charge radii have been determined for the first time with the exception of 101Ag, which was found in good agreement with previous experimental values. The reported results allow tentatively assigning the spin of 97,99Ag to 9/2 and confirming the presence of an isomeric state in these two isotopes, whose collapsed hyperfine structure suggests a spin of 1/2 . The effect of the N=50 shell closure is not only manifested in th…
If the mass excess of neutron-deficient nuclei and their neutron-rich mirror partners are both known, it can be shown that deviations of the Isobaric Mass Multiplet Equation (IMME) in the form of a cubic term can be probed. Such a cubic term was probed by using the atomic mass of neutron-rich magnesium isotopes measured using the TITAN Penning trap and the recently measured proton-separation energies of $^{29}$Cl and $^{30}$Ar. The atomic mass of $^{27}$Mg was found to be within 1.6$σ$ of the value stated in the Atomic Mass Evaluation. The atomic masses of $^{28,29}$Mg were measured to be both…
We report here the results of a study of the $β$ decay of the proton-rich Ge isotopes, $^{60}$Ge and $^{62}$Ge, produced in an experiment at the RIKEN Nishina Center. We have improved our knowledge of the half-lives of $^{62}$Ge (73.5(1) ms), $^{60}$Ge (25.0(3) ms) and its daughter nucleus, $^{60}$Ga (69.4(2) ms). We measured individual $β$-delayed proton and $γ$ emissions and their related branching ratios. Decay schemes and absolute Fermi and Gamow-Teller transition strengths have been determined. The mass excesses of the nuclei under study have been deduced. A total $β$-delayed proton-emiss…
The structure of the neutron-deficient 9C isotope was studied via elastic scattering of radioactive 8B on protons. An excitation function for resonance elastic scattering was measured in the energy range from 0.5 to 3.2 MeV in the center-of-momentum system. A new excited state in 9C was observed at an excitation energy of 3.6 MeV. An R-matrix analysis indicates spin-parity 5/2- for the new state. The results of this experiment are compared with Continuum Shell Model calculations.
The lifetimes of the low-lying excited states $2^+$ and $4^+$ have been directly measured in the neutron-deficient $^{106,108}$Sn isotopes. The nuclei were populated via a deep-inelastic reaction and the lifetime measurement was performed employing a differential plunger device. The emitted $γ$ rays were detected by the AGATA array, while the reaction products were uniquely identified by the VAMOS++ magnetic spectrometer. Large-Scale Shell-Model calculations with realistic forces indicate that, independently of the pairing content of the interaction, the quadrupole force is dominant in the $B(…
Decay studies of very neutron-deficient nuclei ranging from 39Ti to 49Ni have been performed during a projectile fragmentation experiment at the GANIL/LISE3 separator. For all nuclei studied in this work, 39,40Ti, 42,43Cr, 46Mn, 45,46,47Fe and 49Ni, half-lives and decay spectra have been measured. In a few cases, gamma coincidence measurements helped to successfully identify the initial and final states of transitions. In these cases, partial decay scheme are proposed. For the most exotic isotopes, 39Ti, 42Cr, 45Fe and 49Ni, which are candidates for two-proton radioactivity from the ground sta…
High-spin states of neutron deficient Trans-Lead nucleus $^{204}$At were populated up to $\sim 8\,{\rm MeV}$ excitation through the $^{12}$C + $^{197}$Au fusion evaporation reaction. Decay of the associated levels through prompt and delayed $γ$-ray emissions were studied to evaluate the underlying nuclear structure. The level scheme, which was partly known, was extended further. An isomeric $16^+$ level with observed lifetime $τ=52 \pm 5\, {\rm ns}$, was established from our measurements. Attempts were made to interpret the excited states based on multi quasiparticle and hole structures involv…
Accurate atomic mass measurements of neutron-deficient and neutron-rich nuclides around the doubly-magic 208Pb and of neutron-rich cesium isotopes were performed with the Penning trap mass spectrometer ISOLTRAP at ISOLDE/CERN. The masses of 145,147Cs, 181,183Tl, 186Tlm, 187Tl, 196Tlm, 205Tl, 197Pbm, 208Pb, 190 to 197Bi, 209,215,216Bi, 203,205,229Fr, and 214,229,230Ra were determined. The obtained relative mass uncertainty in the range of $2 \cdot 10^{-7}$ to $2 \cdot 10^{-8}$ is not only required for safe identification of isomeric states but also allows mapping the detailed structure of the m…
The lifetimes of the first 2$^{+}$ states in the neutron-deficient $^{76,78}$Sr isotopes were measured using a unique combination of the $γ$-ray line-shape method and two-step nucleon exchange reactions at intermediate energies. The transition rates for the 2$^{+}$ states were determined to be $B$(E2;2$^{+}$$\to 0^{+}$) = 2220(270) e$^{2}$fm$^{4}$ for $^{76}$Sr and 1800(250) e$^{2}$fm$^{4}$ for $^{78}$Sr, corresponding to large deformation of $β_2$ = 0.45(3) for $^{76}$Sr and 0.40(3) for $^{78}$Sr. The present data provide experimental evidence for mutually enhanced collectivity that occurs at…
