AC conductivity spectra of xAgI-(1-x)AgPO$_3$ fast ion conducting glasses spanning the flexible, intermediate (isostatically rigid) and stressed rigid phases are analyzed. The rescaled frequency dependent spectra are mapped into time-dependent mean square displacements out of which a typical lengthscale characterizing the spatial extent $\sqrt{\langle R^2(\infty)\rangle}$ of non-random diffusion paths is computed. The latter quantity is studied as a function of AgI composition, it is found to display a maximum in the intermediate phase, providing the first clear evidence of a typical lengthscale of a dynamical nature when a system becomes isostatically rigid and enters the intermediate phase.
Glasses prepared by physical vapour deposition have been shown to be remarkably more stable than those prepared by standard cooling protocols, with properties that appear to be similar to systems aged for extremely long times. When subjected to a rapid rise in temperature, ultrastable glasses anneal towards the liquid in a qualitatively different manner than ordinary glasses, with the seeming competition of different timescales and lengthscales. We numerically reproduce the phenomenology of ultrastable glass annealing with a kinetically constrained model, a three dimensional East model with so…
Melt homogenization and self-organization of chalcogenides glasses: evidence of sharp rigidity, stress and nanoscale phase separation transitions in the GexSe100-x binary
Muon Spin Relaxation Study of Reentrant Spin Glasses: Amorphous-Fe_{1-x}Mn_x
我们对众所周知的(Fe $_{1-x}$ Mn $_{x}$)$_{75}$ P $_{16}$ B $_6$ Al $_3$再入自旋玻璃进行了广泛的μ子自旋弛豫研究。我们发现一个强大的动态以及静态μ介子去极化率的增加在顺磁铁磁转变温度,$T_c$,并在$T_f$($T_f<T_c$),对应于强体磁不可逆性的发病。我们发现没有关键的动态签名冻结的横向$XY$自旋组件在中间温度$T_{xy}$($T_f < T_{xy} < T_c$)的额外的静态顺序没有贡献的磁化开始发展。
Elastic flexibility, fast-ion conduction, boson and floppy modes in AgPO3-AgI glasses examined in Raman scattering, IR reflectance, MDSC, ac electrical conductivity and molar volume experiments
In order to study the activated dynamics of mean-field glasses, which takes place on times of order exp(N), where N is the system size, we introduce a new model, the Correlated Random Energy Model (CREM), that allows for a smooth interpolation between the REM and the p-spin models. We study numerically and analytically the CREM in the intermediate regime between REM and p-spin. We fully characterize its energy landscape, which is like a golf-course but, at variance with the REM, has metabasins (or holes) containing several configurations. We find that an effective trap-like description for the…
We study magnetic properties of spin glass SG systems under a random field (RF), beased on the suggestion that RFs can be induced by a weak transverse field in the compound LiHo$_x$Y$_{1-x}$F$_4$. We consider a cluster spin model that allows long-range disordered interactions among clusters and short-range interactions inside the clusters, besides a local RF for each spin following a Gaussian distribution with standard deviation $Δ$. We adopt the one-step replica symmetry breaking (RSB) approach to get an exactly solvable single-cluster problem. We discuss the behavior of order parameters, spe…
The recently developed concept of spreadability, $\mathcal{S}(t)$, provides a direct link between time-dependent diffusive transport and the microstructure of two-phase media across length scales. We explicitly compute $\mathcal{S}(t)$ for well-known two-dimensional and three-dimensional model structures, including nonhyperuniform fully penetrable spheres and equilibrium hard spheres, as well as hyperuniform sphere packings derived from perfect glasses, uniformly randomized lattices (URL), disordered stealthy point processes and Bravais lattices. We further confirm that the small-, intermediat…