A decade ago, Budakian and Putterman (Phys. Rev. Lett., {\bf 85}, 1000 (2000)) ascribed friction to the formation of bonds arising from contact charging when a gold tip of a surface force apparatus was dragged on polymethylmethacrylate surface. We propose a stick-slip model that captures the observed correlation between stick-slip events and charge transfer, and the lack of dependence of the scale factor connecting the force jumps and charge transfer on normal load. Here, stick-slip dynamics arises as a competition between the visco-elastic and plastic deformation time scales and that due to the pull speed with contact charging playing a minor role. Our model provides an alternate basis for explaining most experimental results without ascribing friction to contact charging.
How friction affects adhesion is addressed. The problem is considered in the context of a very stiff sphere adhering to a compliant, isotropic, linear elastic substrate, and experiencing adhesion and frictional slip relative to each other. The adhesion is considered to be driven by very large attractive tractions between the sphere and the substrate that can act only at very small distances between them. As a consequence, the adhesion behavior can be represented by the Johnson-Kendall-Roberts model, and this is assumed to prevail also when frictional slip is occurring. Frictional slip is consi…
We develop the theory for stick-slip motion in ultra-thin liquid films confined between two moving atomically-flat surfaces. Our model is based on hydrodynamic equation for the flow coupled to the dynamic order parameter field describing the ``shear melting and freezing'' of the confined fluid. This model successfully accounts for observed phenomenology of friction in ultra-thin films, including periodic and chaotic sequences of slips, transitions from stick-slip motion to steady sliding.
Even the most regular stick-slip frictional sliding is always stochastic, with irregularity in both the intervals between slip events and the sizes of the associated stress drops. Applying small-amplitude oscillations to the shear force, we show, experimentally and theoretically, that the stick-slip periods synchronize. We further show that this phase-locking is related to the inhibition of slow rupture modes which forces a transition to fast rupture, providing a possible mechanism for observed remote triggering of earthquakes. Such manipulation of collective modes may be generally relevant to…
Conventional slippery surfaces show isotropic drop mobility in all directions, but many applications require directional drop motion along a particular path only. In previous studies, researchers used topographic substrates, together with different external stimuli, to demonstrate anisotropic drop motion, which is not very efficient and cost-effective. Herein, we report a novel approach to smartly control drop motion on lubricating fluid coated chemically heterogeneous surfaces composed of alternating hydrophobic and hydrophilic stripes. Upon depositing an aqueous drop on such a surface, the u…
This paper is concerned with the quasi-static rheology of packings of glass spheres of diameter d (d=0.2mm, 0.7mm or 3mm). Stick-slip behaviour is observed on small spheres, i.e d=0.2mm & 0.7mm ; one observes also in this case a weakening of the rheology as the rate of deformation increases, and the larger the rate the larger the weakening; this generates macroscopic instabilities and stick-slip. Statistics of stick-slip events have been determined, which show that the larger the sample the more regular (i.e. "periodic") the sick-slip, the faster the strain rate the less periodic the events. O…
We study the onset of friction for rough contacting blocks whose interface is coated with a thin lubrication layer. High speed measurements of the real contact area and stress fields near the interface reveal that propagating shear cracks mediate lubricated frictional motion. While lubricants reduce interface resistances, surprisingly, they significantly increase energy dissipated, $Γ$, during rupture. Moreover, lubricant viscosity affects the onset of friction but has no effect on $Γ$. Fracture mechanics provide a new way to view the otherwise hidden complex dynamics of the lubrication layer.
When a frictional interface is subject to a localized shear load, it is often (experimentally) observed that local slip events initiate at the stress concentration and propagate over parts of the interface by arresting naturally before reaching the edge. We develop a theoretical model based on linear elastic fracture mechanics to describe the propagation of such precursory slip. The model's prediction of precursor lengths as a function of external load is in good quantitative agreement with laboratory experiments as well as with dynamic simulations, and provides thereby evidence to recognize f…
The effect of random surface roughness on hydrodynamics of viscous incompressible liquid is discussed. Roughness-driven contributions to hydrodynamic flows, energy dissipation, and friction force are calculated in a wide range of parameters. When the hydrodynamic decay length (the viscous wave penetration depth) is larger than the size of random surface inhomogeneities, it is possible to replace a random rough surface by effective stick-slip boundary conditions on a flat surface with two constants: the stick-slip length and the renormalization of viscosity near the boundary. The stick-slip len…
Using a high-speed camera, we follow the propagation of the detachment front during the peeling of an adhesive tape from a flat surface. In a given range of peeling velocity, this front displays a multiscale unstable dynamics, entangling two well-separated spatiotemporal scales, which correspond to microscopic and macroscopic dynamical stick-slip instabilities. While the periodic release of the stretch energy of the whole peeled ribbon drives the classical macro-stick-slip, we show that the micro-stick-slip, due to the regular propagation of transverse dynamic fractures discovered by Thoroddse…
A prominent spatiotemporal failure mode of frictional systems is self-healing slip pulses, which are propagating solitonic structures that feature a characteristic length. Here, we numerically derive a family of steady state slip pulse solutions along generic and realistic rate-and-state dependent frictional interfaces, separating large deformable bodies in contact. Such nonlinear interfaces feature a non-monotonic frictional strength as a function of the slip velocity, with a local minimum. The solutions exhibit a diverging length and strongly inertial propagation velocities, when the driving…
Stick-slip, manifest as intermittent tangential motion between two solids, is a well-known friction instability that occurs in a number of natural and engineering systems. In the context of adhesive polymer interfaces, this phenomenon has often been solely associated with Schallamach waves, which are termed slow waves due to their low propagation speeds. We study the dynamics of a model polymer interface using coupled force measurements and high speed \emph{in situ} imaging, to explore the occurrence of stick-slip linked to other slow wave phenomena. Two new waves---slip pulse and separation p…
We study the possibility for a semi-infinite block of linear viscoelastic material, in homogeneous frictional contact with a non-deformable one, to slide under shear via a periodic set of ``self-healing pulses'', i.e. a set of drifting slip regions separated by stick ones. We show that, contrary to existing experimental indications, such a mode of frictional sliding is impossible for an interface obeying a simple local Coulomb law of solid friction. We then discuss possible physical improvements of the friction model which might open the possibility of such dynamics, among which slip weakening…
We study the effect of atomic scale surface-lubricant interactions on nanoscale boundary-lubricated friction, by considering two example surfaces - hydrophilic mica and hydrophobic graphene - confining thin layers of water in molecular dynamics simulations. We observe stick-slip dynamics for thin water films confined by mica sheets, involving periodic breaking-reforming transitions of atomic scale capillary water bridges formed around the potassium ions of mica. However, only smooth sliding without stick-slip events is observed for water confined by graphene, as well as for thicker water layer…
We discuss the stick-slip motion of an elastic block sliding along a rigid substrate. We argue that for a given external shear stress this system shows a discontinuous nonequilibrium transition from a uniform stick state to uniform sliding at some critical stress which is nothing but the Griffith threshold for crack propagation. An inhomogeneous mode of sliding occurs, when the driving velocity is prescribed instead of the external stress. A transition to homogeneous sliding occurs at a critical velocity, which is related to the critical stress. We solve the elastic problem for a steady-state …
Using a high speed camera, we study the peeling dynamics of an adhesive tape under a constant load with a special focus on the so-called stick-slip regime of the peeling. It is the first time that the very fast motion of the peeling point is imaged. The speed of the camera, up to 16000 fps, allows us to observe and quantify the details of the peeling point motion during the stick and slip phases: stick and slip velocities, durations and amplitudes. First, in contrast with previous observations, the stick-slip regime appears to be only transient in the force controlled peeling. Additionally, we…
Intermittent motion, called stick--slip, is a friction instability that commonly occurs during relative sliding of two elastic solids. In adhesive polymer contacts, where elasticity and interface adhesion are strongly coupled, stick--slip results from the propagation of slow detachment waves at the interface. Using \emph{in situ} imaging experiments at an adhesive contact, we show the occurrence of two distinct detachment waves moving parallel (Schallamach wave) and anti-parallel (separation wave) to the applied remote sliding. Both waves cause slip in the same direction and travel at speeds m…
We study experimentally the fracture dynamics during the peeling at a constant velocity of a roller adhesive tape mounted on a freely rotating pulley. Thanks to a high speed camera, we measure, in an intermediate range of peeling velocities, high frequency oscillations between phases of slow and rapid propagation of the peeling fracture. This so-called stick-slip regime is well known as the consequence of a decreasing fracture energy of the adhesive in a certain range of peeling velocity coupled to the elasticity of the peeled tape. Simultaneously with stick-slip, we observe low frequency osci…
By means of atomistic simulations, we demonstrate that a dislocation core exhibits intermittent quasistatic restructuring during incremental shear within the same Peierls valley. This can be regarded as a stick-slip transition, which is also reproduced for a one-dimensional Frenkel-Kontorova chain under rigid boundary conditions. This occurs due to a discontinuous jump in an order parameter of the system, which signifies the extent of region forbidden for the presence of particles in the chain. The stick-slip phenomenon observed in the dislocation core is also shown to be reflected after dimen…
The spontaneous nucleation of accelerating slip along slowly driven frictional interfaces is central to a broad range of geophysical, physical and engineering systems, with particularly far-reaching implications for earthquake physics. A common approach to this problem associates nucleation with an instability of an expanding creep patch upon surpassing a critical length $L_c$. The critical nucleation length $L_c$ is conventionally obtained from a spring-block linear stability analysis extended to interfaces separating elastically-deformable bodies using model-dependent fracture mechanics esti…
Nanodot deposition on a side surface of a rectangular sample and digital image correlation are used to quantify the in-plane strain fields associated with the propagation of a shear band in a PdNiP bulk metallic glass,induced by rolling. Within the resolution of the method related to an average inter-dot distance of 100 nm, deformation is found to be highly localized at the shear bands, while alternating areas with a size of 100 - 400 nm with opposite local shear strains are found. This phenomenon substantiates a local stick-slip nature of shear band propagation during the metallic glass defor…
Powders and grains exhibit unpredictable jamming-to-flow transitions that manifest themselves on geophysical scales in catastrophic slip events such as landslides and earthquakes, and on laboratory/industrial scales in profound processing difficulties. Over the past few years, insight into these transitions has been provided by new evidence that slip events may accompanied, or even preceded, by electrical effects. In the present work, we quantify the correlation between slip and the separation of electrical charges, using an archetypal granular material: photoelastic polymers. We measure a str…
It is now known that the equations of motion for the contact point during peeling of an adhesive tape mounted on a roll introduced earlier are singular and do not support dynamical jumps across the two stable branches of the peel force function. By including the kinetic energy of the tape in the Lagrangian, we derive equations of motion that support stick-slip jumps as a natural consequence of the inherent dynamics. In the low mass limit, these equations reproduce solutions obtained using a differential-algebraic algorithm introduced for the earlier equations. Our analysis also shows that mass…
We have devised an original laboratory experiment where we investigate the frictional behaviour of a single crystal salt slider over a large number of deformation cycles. Because of its physical properties, salt, a surrogate for natural faults, allows for friction and plastic deformation and pressure solution creep to be efficient on the same timescale. During the same experiment, we observe a continuous change of the frictional behaviour of the slider under constant conditions of stiffness, temperature and loading velocity. The stick-slip regime is progressively vanishing, eventually reaching…
We perform real-time measurements of the net contact area between two blocks of like material at the onset of frictional slip. We show that the process of interface detachment, which immediately precedes the inception of frictional sliding, is governed by three different types of detachment fronts. These crack-like detachment fronts differ by both their propagation velocities and by the amount of net contact surface reduction caused by their passage. The most rapid fronts propagate at intersonic velocities but generate a negligible reduction in contact area across the interface. Sub-Rayleigh f…
This paper presents the stability analysis of a system sliding at low velocities ($< 100 μ$m.s$^{-1}$) under a periodically modulated normal load, preserving interfacial contact. Experiments clearly evidence that normal vibrations generally stabilize the system against stick-slip oscillations, at least for a modulation frequency much larger than the stick-slip one. The mechanical model of Bureau {\it et al.} (2000), validated on the steady-state response of the system, is used to map its stability diagram. The model takes explicitly into account the finite shear stiffness of the load-bearing a…
An adiabatic approach is developed for the problem of boundary friction between two atomically smooth and incommensurate solid surfaces, separated by a monolayer of lubricant atoms. This method permits to consider very slow macroscopic motion of the parts in contact, separately from fast thermic motions of individual atoms. A characteristic ''stick-slip'' behavior of the tangential force on the contact is obtained within a simple 1D model, relevant for the tip and sample system in friction force microscopy (FFM). This behavior reflects the specific mechanism of stress energy accumulation, thro…
University of Oslo（奥斯陆大学）；Lanzhou Institute of Chemical Physics, Chinese Academy of Sciences（中国科学院兰州化学物理研究所）；Forschungszentrum Jülich（于利希研究中心）；MultiscaleConsulting
We describe benchmark experiments to evaluate the frictional properties of laser patterned low-density polyethylene as a function of sliding velocity, normal force and humidity. The pattern is a square lattice of square cavities with sub-mm spacing. We find that dynamic friction decreases compared to non-patterned surfaces, since stress concentrations lead to anticipated detachment, and that stick-slip behavior is also affected. Friction increases with humidity, and the onset of stick-slip events occurs in the high humidity regime. Experimental results are compared with numerical simulations o…
The stress profile and reorientation of grains, in response to a point force applied to a preloaded two dimensional granular system, are calculated in the context of a continuum theory that incorporates the texture of the packing. When high friction prevents slip at the inter-grain contacts, an anisotropic packing propagates stress along two peaks which amalgamate into a single peak as the packing is disordered into a less anisotropic structure; this single peak may be wider or narrower than in the isotropic case, depending on the preparation of the packing. At lower frictions, an effective tr…
A tribological system consisting of two contacting blocks has been considered. One of them is arranged between two springs, the other is driven periodically. The kinetics of the system has been studied in the boundary friction mode, when an ultrathin lubricant film is contained between the atomically smooth surfaces. In order to describe the film state, the expression for the free energy density is used in the form of an expansion in a power series in the order parameter, the latter being reduced to the shear modulus of a lubricant. The stick-slip mode is shown to be realized in a wide range o…
We investigate the dynamics of peeling of an adhesive tape subjected to a constant pull speed. We derive the equations of motion for the angular speed of the roller tape, the peel angle and the pull force used in earlier investigations using a Lagrangian. Due to the constraint between the pull force, peel angle and the peel force, it falls into the category of differential-algebraic equations requiring an appropriate algorithm for its numerical solution. Using such a scheme, we show that stick-slip jumps emerge in a purely dynamical manner. Our detailed numerical study shows that these set of …
We determined frictional figures of merit for a pair of layered honeycomb nanostructures, such as graphane, fluorographene, MoS$_2$ and WO$_2$ moving over each other, by carrying out ab-initio calculations of interlayer interaction under constant loading force. Using Prandtl-Tomlinson model we derived critical stiffness required to avoid stick-slip behavior. We showed that these layered structures have low critical stiffness even under high loading forces due to their charged surfaces repelling each other. The intrinsic stiffness of these materials exceed critical stiffness and thereby avoid t…
We discuss crack propagation along the interface between two dissimilar materials. The crack edge separates two states of the interface, ``stick'' and ``slip''. In the slip region we assume that the shear stress is proportional to the sliding velocity, i.e. the linear viscous friction law. In this picture the static friction appears as the Griffith threshold for crack propagation. We calculate the crack velocity as a function of the applied shear stress and find that the main dissipation comes from the macroscopic region and is mainly due to the friction at the interface. The relevance of our …
Recent experiments indicate that frictional sliding occurs by the nucleation of detachment fronts at the contact interface that may appear well before the onset of global sliding. This intriguing precursory activity is not accounted for by traditional friction theories but is extremely important for friction dominated geophysical phenomena such as earthquakes, landslides or avalanches. Here we simulate the onset of slip of a three dimensional elastic body resting on a surface and show that experimentally observed frictional precursors depend in a complex non-universal way on the sample geometr…
Experimental measurements have reported ultra-fast and radius-dependent water transport in carbon nanotubes which are absent in boron nitride nanotubes. Despite considerable effort, the origin of this contrasting (and fascinating) behaviour is not understood. Here, with the aid of machine learning-based molecular dynamics simulations that deliver first-principles accuracy, we investigate water transport in single-wall carbon and boron nitride nanotubes. Our simulations reveal a large, radius-dependent hydrodynamic slippage on both materials with water experiencing indeed a $\approx 5$ times lo…
Sliding along frictional interfaces separating dissimilar elastic materials is qualitatively different from sliding along interfaces separating identical materials due to the existence of an elastodynamic coupling between interfacial slip and normal stress perturbations in the former case. This bimaterial coupling has important implications for the dynamics of frictional interfaces, including their stability and rupture propagation along them. We show that while this bimaterial coupling is a monotonically increasing function of the bimaterial contrast, when it is coupled to interfacial shear s…
The onset of frictional instabilities, e.g. earthquakes nucleation, is intimately related to velocity-weakening friction, in which the frictional resistance of interfaces decreases with increasing slip velocity. While this frictional response has been studied extensively, less attention has been given to steady-state velocity-strengthening friction, in spite of its potential importance for various aspects of frictional phenomena such as the propagation speed of interfacial rupture fronts and the amount of stored energy released by them. In this note we suggest that a crossover from steady-stat…
The surface of a crystal made of roughly spherical molecules exposes, above its bulk rotational phase transition at T= T$_r$, a carpet of freely rotating molecules, possibly functioning as "nanobearings" in sliding friction. We explored by extensive molecular dynamics simulations the frictional and adhesion changes experienced by a sliding C$_{60}$ flake on the surface of the prototype system C$_{60}$ fullerite. At fixed flake orientation both quantities exhibit only a modest frictional drop of order 20% across the transition. However, adhesion and friction drop by a factor of $\sim$ 2 as the …
The transition from stick to slip at a dry frictional interface occurs through the breaking of the junctions between the two contacting surfaces. Typically, interactions between the junctions through the bulk lead to rupture fronts propagating from weak and/or highly stressed regions, whose junctions break first. Experiments find rupture fronts ranging from quasi-static fronts with speeds proportional to external loading rates, via fronts much slower than the Rayleigh wave speed, and fronts that propagate near the Rayleigh wave speed, to fronts that travel faster than the shear wave speed. The…
The current understanding of the earthquake interevent times distribution (ITD) is incomplete. The Weibull distribution is often used to model the earthquake ITD. We link the earthquake ITD on single faults with the Earth's crustal shear strength distribution by means of a phenomenological stick - slip model. We obtain Weibull ITD for power-law stress accumulation, i.e., $σ(t) = αt^β$, where $β>0$ for single faults or systems with homogeneous strength statistics. We show that logarithmic stress accumulation leads to the log-Weibull ITD. For the Weibull ITD, we prove that (i) $m= βm_s$, where $…
We investigate atomic scale friction between clean graphite surfaces by using molecular dynamics. The simulation reproduces atomic scale stick-slip motion and low frictional coefficient, both of which are observed in experiments using frictional force microscope. It is made clear that the microscopic origin of low frictional coefficients of graphite lies on the honeycomb structure in each layer, not only on the weak interlayer interaction as believed so far.
We describe the results of atomic-level stick-slip friction measurements performed on chemically-modified graphite, using atomic force microscopy (AFM). Through detailed molecular dynamics simulations, coarse-grained simulations, and theoretical arguments, we report on complex indentation profiles during AFM scans involving local reversible exfoliation of the top layer of graphene from the underlying graphite sample and its effect on the measured friction force during retraction of the scanning tip. In particular, we report nearly constant lateral stick-slip magnitudes at decreasing loads, whi…
The rupture of the interface joining two materials under frictional contact controls their macroscopic sliding. Interface rupture dynamics depend markedly on the mechanical properties of the bulk materials that bound the frictional interface. When the materials are similar, recent experimental and theoretical work has shown that shear cracks described by Linear Elastic Fracture Mechanics (LEFM) quantitatively describe the rupture of frictional interfaces. When the elastic properties of the two materials are dissimilar, many new effects take place that result from bimaterial coupling: the norma…
