We have observed the evolution of phase diagram and vortex pinning using a single ferromagnet/superconductor bilayer of [Co/Pt]8/Nb through a special demagnetization procedure. It induces a continuous and reversible change of the domain width with equal positive/negative domains enabling the observation of the predicted tunable phase diagram. The tunable domain pattern also systematically affects vortex pinning. We have determined the dependence of the activation energy of vortex pinning on domain width, temperature, and magnetic field.
Materials with reduced dimensionality often exhibit exceptional properties that are different from their bulk counterparts. Here we report the emergence of a commensurate 2 $\times$ 2 charge density wave (CDW) in monolayer and bilayer SnSe$_2$ films by scanning tunneling microscope. The visualized spatial modulation of CDW phase becomes prominent near the Fermi level, which is pinned inside the semiconductor band gap of SnSe$_2$. We show that both CDW and Fermi level pinning are intimately correlated with band bending and virtual induced gap states at the semiconductor heterointerface. Through…
Vortex pinning in a type-II superconducting Pb film covering a Co/Pt multilayer with perpendicular magnetic anisotropy is investigated. Different stable magnetic domain patterns like band and bubble domains can be created in the Co/Pt multilayer, clearly influencing the vortex pinning in the superconducting Pb layer. Most effective pinning is observed for the bubble domain state. We demonstrate that the pinning properties of the superconductor/ferromagnet bilayer can be controlled by tuning the size, density and magnetization direction of the bubbles.
We use local and global magnetometry measurements to study the influence of magnetic domain width w on the domain-induced vortex pinning in superconducting/ferromagnetic bilayers, built of a Nb film and a ferromagnetic Co/Pt multilayer with perpendicular magnetic anisotropy, with an insulating layer to eliminate proximity effect. The quasi-periodic domain patterns with different and systematically adjustable width w, as acquired by a special demagnetization procedure, exert tunable vortex pinning on a superconducting layer. The largest enhancement of vortex pinning, by a factor of more than 10…
We investigated the pinning of flux lines in a superconducting film by a regular array of magnetic antidots. The sample consists of a Co/Pt multilayer with perpendicular magnetic anisotropy in which a regular pattern of submicron holes is introduced and which is covered by a type-II superconducting Pb film. The resulting ferromagnetic/superconducting heterostructure shows a pronounced asymmetric magnetization curve with respect to the field polarity. This asymmetry clearly demonstrates that the magnetic contribution dominates the pinning potential imposed by the magnetic antidots on the superc…
This paper reports the observation of hysteresis in the vortex pinning in a superconductor / ferromagnetic epitaxial nanocomposite consisting of fcc Gd particles incorporated in a Nb matrix. We show that this hysteretic pinning is associated with magnetic reversal losses in the Gd particles and is fundamentally different in origin to pinning interactions previously observed for ferromagnetic particles or other microstructural features.
We study a high-TC superconducting (YBa2Cu3O7-d) / ferromagnetic (Co/Pt multilayer) hybrid which exhibits resistance switching driven by the magnetic history: depending on the direction of the external field, a pronounced decrease or increase of the mixed-state resistance is observed as magnetization reversal occurs within the Co/Pt multilayer. We demonstrate that stray magnetic fields cause these effects via i) creation of vortices/antivortices and ii) magnetostatic pinning of vortices that are induced by the external field.
The continuum theory of domain structures in ferromagnetic/superconducting bilayers fails when the equilibrium domain size becomes comparable with effective penetration depth $Λ$. Instead, a lattice of discrete vortices must be considered. Here, we report our results on the discrete vortex lattices in stripe domain structures of ferromagnetic/superconducting bilayers. The vortices are assumed to be situated periodically on chains in stripe domains. We study the configurations containing up to three chains per domain, and calculate their equilibrium energies, equilibrium domain size and vortex …
We have studied the local critical current density, jc, in the superconductor thin film of bilayer structures consisting of YBa2Cu3O7 and the ferromagnets La2/3Ca1/3MnO3 and SrRuO3, respectively, by means of quantitative magneto-optics. A pronounced hysteresis of jc was observed which is ascribed to the magnetization state of the ferromagnetic layer. The results are discussed within the frame of magnetic vortex - wall interactions.
The discrete vortex lattices in a ferromagnet/superconductor bilayer are studied when the ferromagnet has periodic stripe domains with an out-of-plane magnetization. The vortices are assumed to be situated periodically on chains in the stripe domains. Only up to two vortex chains per domain configurations are considered. When the domain period is fixed, the threshold magnetization is calculated at which the transition from the Meissner state to the mixed state occurs. When the domain period is not fixed, the equilibrium domain size and vortex positions are calculated, depending on the domain's…
We performed magnetization measurements in a single crystal of the anisotropic bilayer pnictide superconductor KCa$_2$Fe$_4$As$_4$F$_2$, with $T_c$ $\simeq$ 34 K, for $H$$\parallel$$c$-axis and $H$$\parallel$$ab$-planes. A second magnetization peak (SMP) was observed in the isothermal $M(H)$ curves measured below 16 K for $H$$\parallel$$ab$-planes. A peak in the temperature variation of the critical current density, $J_{c}$($T$), at 16 K, strongly suggests the emergence of Josephson vortices at lower temperatures, which leads to the SMP in the sample. In addition, it is noticed that the appear…
Superconductor/Ferromagnet (S/F) hybrid systems show interesting magneto-transport behaviors that result from the transfer of properties between both constituents. For instance, magnetic memory can be transferred from the F into the S through the pinning of superconducting vortices by the ferromagnetic textures. The ability to tailor this type of induced behavior is important to broaden its range of applications. Here we show that engineering the F magnetization reversal allows tuning the strength of the vortex pinning (and memory) effects, as well as the field range in which they appear. This…
This is an analytical study of pinning and spontaneous vortex phase is a system consisting of a superconducting thin film pierced by a long ferromagnetic columnar defect of finite radius $R$. The magnetic fields, screening currents, energy and pinning forces for this system are calculated. The interaction between the magnetic field of vortices and the magnetization outside the plane of the film and its close proximity enhances vortex pinning significantly. Spontaneous vortex phase appears when the magnetization of the columnar defect is increased above a critical value. Transitions between pha…
The pinning properties of type-II superconductors can be efficiently controlled by using laterally nanostructured ferromagnet / superconductor bilayers. This will be illustrated by studying the flux pinning in thin superconducting Pb films which are deposited on top of two types of magnetic nanostructures with out-of-plane magnetisation: (i) an array of dots, and (ii) an array of antidots, both made from a Co/Pt multilayer. The magnetisation curves of the Pb film are extremely asymmetric with respect to the polarity of the magnetic field when the magnetic moments in the Co/Pt multilayer were a…
Extraordinary Hall effect (EHE) in bilayer F/S(N) was investigated theoretically. The conductivity tensor $σ_{αβ}$ is calculated in the Kubo formalism with Green functions found as the solutions of the Gorkov equations. We considered diffuse transport in the ferromagnetic layer, taking into account as a main mechanism of electron resistivity s-d scattering. In this model Gorkov equations for s-electrons in the ferromagnetic layer remain linear and are solved easily. It is shown that Hall field $E^H$ for both F/S and F/N contacts are step-functions of the coordinate perpendicular to the planes …
We report on the first observation of a pronounced re-entrant superconductivity phenomenon in superconductor/ferromagnetic layered systems. The results were obtained using a superconductor/ferromagnetic-alloy bilayer of Nb/Cu(1-x)Ni(x). The superconducting transition temperature T_{c} drops sharply with increasing thickness d_{CuNi} of the ferromagnetic layer, until complete suppression of superconductivity is observed at d_{CuNi}= 4 nm. Increasing the Cu(1-x)Ni(x) layer thickness further, superconductivity reappears at d_{CuNi}=13 nm. Our experiments give evidence for the pairing function osc…
Strong pinning of superconducting flux quanta by a square array of 1 $μ$m-sized ferromagnetic dots in a magnetic-vortex state was visualized by low-temperature magnetic force microscopy (LT-MFM). A direct correlation of the superconducting flux lines with the positions of the dots was derived. The force that the MFM tip exerts on the individual vortex in the depinning process was used to estimate the spatial modulation of the pinning potential. It was found, that the superconducting vortices which are preferably located on top of the Py dots experience about 15 times stronger pinning forces as…
Vortex motion in ferromagnetic-superconducting bilayers constituted by thin YBa$_2$Cu$_3$O$_{7-δ}$ film deposited on the top of thin manganite La$_{0.67}$Sr$_{0.33}$MnO$_3$ film has been investigated. Both films were deposited on uniformly twinned single-crystalline substrates and patterned into strips directed at different angles to the twin lines pattern. These conditions lead to the guided vortex motion at different angles to the periodic pinning potential. It has been established that critical current and flux flow resistance in such an anisotropic pinning landscape-scale follow the ellipt…
Scanning tunneling spectroscopy measurements conducted on epitaxially grown bilayers of half-metallic ferromagnetic La2/3Ca1/3MnO3 (LCMO) on superconducting (SC) (100)YBa2Cu3O7-delta (YBCO) reveal long-range penetration of superconducting order into the LCMO. This anomalous proximity effect manifests itself in the tunneling spectra measured on the LCMO layer as gaps and zero bias conductance peaks. Remarkably, these proximity-induced spectral features were observed for bilayers with LCMO thickness of up to 30 nm, an order of magnitude larger than the expected ferromagnetic coherence length in …
We realized point contact spectroscopy experiment on ferromagnet/superconductor bilayers. Differential conductance curves show several features that we explained within Bogoliubov-de Gennes formalism considering the presence of two interfaces in the normal-metal-tip/ferromagnet/superconductor device. We demonstrate that such configuration is suitable as local probe of the spin polarization and thickness of ferromagnetic layer, directly on bilayer areas. This is due to the high sensitivity of the Andreev surface states to the physical properties of the ferromagnetic interlayer.
We study theoretically the magnetic screening properties of thin, diffusive superconductor/ferromagnet bilayers subject to a perpendicular magnetic field. We find that the effective penetration depth characterizing the magnetic response oscillates with the thickness of the ferromagnetic layer on the scale of the ferromagnetic coherence length.
Scanning tunneling spectroscopy measurements on thin epitaxial SrRuO3/(100)YBCO ferromagnet/superconductor bilayers, reveal localized regions in which the superconductor order parameter penetrates the ferromagnet to more than 26 nm, an order of magnitude larger than the coherence length in the ferromagnetic layer. These regions consist of narrow (< 10 nm) and long strips, separated by at least 200 nm, consistent with the known magnetic domain wall structure in SrRuO3. We attributed this behavior to Crossed Andreev Reflections, taking place in the vicinity of the magnetic domain walls.
The excitation spectrum of clean ferromagnet-superconductor bilayers is calculated within the framework of the self-consistent Bogoliubov-de Gennes theory. Because of the proximity effect, the superconductor induces a gap in the ferromagnet spectrum, for thin ferromagnetic layers. The effect depends strongly on the exchange field in the ferromagnet. We find that as the thickness of the ferromagnetic layer increases, the gap disappears, and that its destruction arises from those quasiparticle excitations with wavevectors mainly along the interface. We discuss the influence that the interface qu…
Scanning tunneling spectroscopy of thin epitaxial $SrRuO_{3}/(110)YBa_2Cu_3O_{7-δ}$ ferromagnet/superconductor bilayers, reveal a clear penetration of the Andreev bound states into the ferromagnetic layer. The penetration is manifested in the density of states of the ferromagnet as a split zero bias conductance peak with an imbalance between peak heights. Our data indicate that the splitting occurs at the superconductor side as a consequence of induced magnetization, confirming recent theoretical predictions. The imbalance is attributed to the spin polarization in the ferromagnet.
We investigate ferromagnetic resonance (FMR) modulation in $d$-wave superconductor (SC)/ferromagnetic insulator (FI) bilayer systems theoretically. The modulation of the Gilbert damping in these systems reflects the existence of nodes in the $d$-wave SC and shows power-law decay characteristics within the low-temperature and low-frequency limit. Our results indicate the effectiveness of use of spin pumping as a probe technique to determine the symmetry of unconventional SCs with high sensitivity for nanoscale thin films.
Using scanning tunneling microscopy and Ginzburg-Landau simulations we explore vortex configurations in magnetically coupled NbSe$_2$-Permalloy superconductor-ferromagnet bilayer. The Permalloy film with stripe domain structure induces periodic local magnetic induction in the superconductor creating a series of pinning-antipinning channels for externally added magnetic flux quanta. Such laterally confined Abrikosov vortices form quasi-1D arrays (chains). The transitions between multichain states occur through propagation of kinks at the intermediate fields. At high fields we show that the syst…
We study the transport properties of vortex matter in a superconducting thin film separated by a thin insulator layer from a ferromagnetic layer. We assume an alternating stripe structure for both FM and SC layers as found in [7]. We calculate the periodic pinning force in the stripe structure resulting from a highly inhomogeneous distribution of the vortices and antivortices. We show that the transport properties in FM-SC bilayer are highly anisotropic. In the absence of random pinning it displays a finite resistance for the current perpendicular to stripes and is superconducting for the curr…
We analyze the enhancement of the superconducting critical temperature of superconducting/ferromagnetic bilayers due to the appearance of localized superconducting states in the vicinity of magnetic domain walls in the ferromagnet. We consider the case when the main mechanism of the superconductivity destruction via the proximity effect is the exchange field. We demonstrate that the influence of the domain walls on the superconducting properties of the bilayer may be quite strong if the domain wall thickness is of the order of superconducting coherence length.
The theoretical description of the Fulde-Ferrell-Larkin-Ovchinnikov like state establishing in nanostructered bilayers of ferromagnetic (F) and superconducting (S) material leads to critical temperature oscillations and reentrant superconductivity as the F-layer thickness gradually increases. The experimental realization of these phenomena is an important prerequisite for the fabrication of the Ferromagnet/Superconductor/Ferromagnet core structure of the superconducting spin-valve. A switching of the spin-valve is only expected if such non-monotonic critical temperature behavior is observed in…
Superconductor/ferromagnet bilayers are known to exhibit nontrivial dependence of the critical temperature T_c on the thickness d_f of the ferromagnetic layer. We develop a general method for investigation of T_c as a function of the bilayer's parameters. It is shown that interference of quasiparticles makes T_c(d_f) a nonmonotonic function. The results are in good agreement with experiment. Our method also applies to multilayered structures.
We report the first measurements of the effective superfluid density n_S(T) \propto λ^{-2}(T) of Superconductor-Ferromagnet (SC/FM) bilayers, where λis the effective magnetic field penetration depth. Thin Nb/Ni bilayers were sputtered in ultrahigh vacuum in quick succession onto oxidized Si substrates. Nb layers are 102 A thick for all samples, while Ni thicknesses vary from 0 to 100 A. T_C determined from λ^{-2}(T) decreases rapidly as Ni thickness d_Ni increases from zero to 15 A, then it has a shallow minimum at d_Ni \approx 25 A. λ^{-2}(0) behaves similarly, but has a minimum several times…
Measurements of the polar Kerr effect using a zero-area-loop Sagnac magnetometer on Pb/Ni and Al/(Co-Pd) proximity-effect bilayers show unambiguous evidence for the "inverse proximity effect," in which the ferromagnet (F) induces a finite magnetization in the superconducting (S) layer. To avoid probing the magnetic effects in the ferromagnet, the superconducting layer was prepared much thicker than the light's optical penetration depth. The sign and size of the effect, as well as its temperature dependence agree with recent predictions by Bergeret et al..
We study the elasticity, fluctuations and pinning of a putative spontaneous vortex solid in ferromagnetic superconductors. Using a rigorous thermodynamic argument, we show that in the idealized case of vanishing crystalline pinning anisotropy the long-wavelength tilt modulus of such a vortex solid vanishes identically, as guaranteed by the underlying rotational invariance. The vanishing of the tilt modulus means that, to lowest order, the associated tension elasticity is replaced by the softer, curvature elasticity. The effect of this is to make the spontaneous vortex solid qualitatively more …
Superconducting spintronics in hybrid superconductor/ferromagnet (S-F) heterostructures provides an exciting potential new class of device. The prototypical super-spintronic device is the superconducting spin-valve, where the critical temperature, $T_c$, of the S-layer can be controlled by the relative orientation of two (or more) F-layers. Here, we show that such control is also possible in a simple S/F bilayer. Using field history to set the remanent magnetic state of a thin Er layer, we demonstrate for a Nb/Er bilayer a high level of control of both $T_c$ and the shape of the resistive tran…
We study the electronic instabilities of doped bilayer silicene using the random phase approximation. In contrast to the singlet $d+id'$ superconductivity at the low doping region, we find that the system is an itinerant ferromagnet in the narrow doping regions around the Van Hove singularities, and a triplet $p+ip'$ superconductor in the vicinity of these regions. Adding a weak Kane-Mele spin-orbit coupling to the system further singles out the time-reversal invariant equal-spin helical $p+ip'$ pairing as the leading instability. The triplet pairing identified here is driven by the ferromagne…
We have made an experimental study of the tunneling density of states (DOS) in strong ferromagnetic thin films (CoFe) in proximity with a thick superconducting film (Nb) as a function of $d_F$, the ferromagnetic thickness. Remarkably, we find that as $d_F$ increases, the superconducting DOS exhibits a scaling behavior in which the deviations from the normal-state conductance have a universal shape that decreases exponentially in amplitude with characteristic length $d^*\approx 0.4$ nm. We do not see oscillations in the DOS as a function of $d_F$, as expected from predictions based on the Usade…
In bilayers consisting of ferromagnetic and superconducting films, the ferromagnetic film in its domain state induces inhomogeneous distribution of magnetic fields in the superconducting film. When the ferromagnetic film has bubble magnetic domains in a labyrinth structure, it has been found that the pinning of the vortices increases; hence, the critical current of the superconducting film becomes larger. Here we study the effect of parallel ferromagnetic domain structure in Nb/SrRuO3 on the critical current of Nb with current flowing perpendicularly to the domains and find that in this case t…
We demonstrate that Josephson devices with nontrivial phase difference $% 0<φ_g <π$ in the ground state can be realized in structures composed from longitudinally oriented normal metal (N) and ferromagnet (F) films in the weak link region. Oscillatory coupling across F-layer makes the first harmonic in the current-phase relation relatively small, while coupling across N-layer provides negative sign of the second harmonic. To derive quantitative criteria for a $φ$-junction, we have solved two-dimensional boundary-value problem in the frame of Usadel equations for overlap and ramp geometries of …
We investigate superconducting phase transition in superconductor(S)/ferromagnet(F) bilayer with Rasba spin-orbit interaction at S/F interface. This spin-orbit coupling produces spontaneous supercurrents flowing inside the atomic-thickness region near the interface, which are compensated by the screening Meissner currents [S. Mironov and A. Buzdin, Phys. Rev. Lett \textbf{118}, 077001 (2017)]. In the case of thin superconducting film the emergence of the spontaneous surface currents causes the increase of the superconducting critical temperature and we calculate the actual value of the critica…
The existence of coherent magnetic correlations in the normal phase of cuprate high-temperature superconductors has proven difficult to measure directly. Here we report on a study of ferromagnetic-superconductor bilayers of La2/3Ca1/3MnO3/YBa2Cu3O7 (LCMO/YBCO) with varying YBCO layer thicknesses. Using x-ray magnetic circular dichroism, we demonstrate that the ferromagnetic layer induces a Cu magnetic moment in the adjacent high-temperature superconductor. For thin samples, this moment exists at all temperatures below the Curie temperature of the LCMO layer. However, for a YBCO layer thicker t…
Thermally induced magnetization dynamics is currently a flourishing field of research due to its potential application in information technology. We study the paradigmatic system of a magnetic domain wall in a thermal gradient which is interacting with an adjacent superconductor. The spin-transfer torques arising in this system due to the combined action of the giant thermoelectric effect and the creation of equal-spin pairs in the superconductor are large enough to give rise to high domain wall velocities $10^3$ times larger than previously predicted.
A resonant enhancement of the neutron standing waves is proposed to use in order to increase the magnetic neutron scattering from a "superconductor/ferromagnet"(S/F) bilayer. The model calculations show that usage of this effect allows to increase the magnetic scattering intensity by factor of hundreds. Aspects related to the growth procedure (order of deposition, roughness of the layers etc) as well as experimental conditions (resolution, polarization of the neutron beam, background etc) are also discussed. Collected experimental data for the S/F heterostructure Cu(32nm)/V(40nm)/Fe(1nm)/MgO c…
We study theoretically the influence of spin accumulation on superconductivity in a superconductor/ferromagnet bilayer. It is well-known that the superconductivity in S/F bilayers is suppressed by the proximity to a ferromagnet. The spin accumulation by itself is also a depairing factor. But here we show that creation of the spin accumulation on top of effective exchange depairing, caused by the proximity to a ferromagnet, can lead to an opposite result. The superconductivity can be partially recovered by spin-dependent quasiparticle distribution. The systems with realistic parameters are cons…
We demonstrate that the hybrid structures consisting of a superconducting layer with an adjacent spin-textured ferromagnet demonstrate the variety of equilibrium magnetoelectric effects originating from coupling between the conduction electron spin and superconducting current. By deriving and solving the generalized Usadel equation which takes into account the spin-filtering effect we find that a supercurrent generates spin polarization in the superconducting film which is non-coplanar with the local ferromagnetic moment. The inverse magnetoelectric effect in such structures is shown to result…
