Scattering induced mode splitting in active microcavities is demonstrated. Below the lasing threshold, quality factor enhancement by optical gain allows resolving, in the wavelength-scanning transmission spectrum, the resonance dips of the split modes which otherwise would not be detected in a passive resonator. In the lasing regime, mode splitting manifests itself as two lasing modes with extremely narrow linewidths. Mixing of these laser modes in a detector leads to a heterodyne beat signal whose frequency corresponds to the amount of splitting. Lasing regime not only allows ultrahigh sensitivity for mode-splitting measurements but also provides an easily accessible scheme by eliminating the need for wavelength scanning around resonant modes. Mode splitting in active microcavities has immediate impact in enhancing the sensitivity of sub-wavelength scatterer detection and in studying light-matter interactions in strong coupling regime.
We demonstrate stimulated Brillouin scattering (SBS) lasing in a strongly coupled microcavity system. By coupling two silica toroid microcavities, we achieve large mode splitting of 11 GHz, whose frequency separation matches the Brillouin frequency shift of silica. The SBS light is resonantly amplified by pumping at the higher frequency side of the supermode splitting resonance. Since the mode splitting is adjusted by changing the gap distance between the two cavities, our system does not require precise control of a mm-sized cavity diameter to match the free-spectral spacing with the Brilloui…
Nowadays, ultrasound sensors are playing an irreplaceable role in the fields of biomedical imaging and industrial nondestructive inspection. Currently, piezoelectric transducers are the most widely used ultrasound sensors, but their sensitivities drop quickly when the size becomes smaller, leading to a typical sensor size at the millimeter to centimeter scale. In order to realize both high sensitivity and spatial resolution, various optical ultrasound sensors have been developed. Among them, ultrasound sensors using high-$Q$ optical microcavities have realized unprecedented sensitivities and b…
Optical microcavities confine light spatially and temporally and find application in a wide range of fundamental and applied studies. In many areas, the microcavity figure of merit is not only determined by photon lifetime (or the equivalent quality-factor, Q), but also by simultaneous achievement of small mode volume V . Here we demonstrate ultra-high Q-factor small mode volume toroid microcavities on-a-chip, which exhibit a Q/V factor of more than $10^{6}(λ/n)^{-3}$. These values are the highest reported to date for any chip-based microcavity. A corresponding Purcell factor in excess of 200 …
We present an oxide aperture microcavity with embedded quantum dots that utilizes a three contact design to independently tune the quantum dot wavelength and birefringence of the cavity modes. A polarization splitting tuning of $\sim$5 GHz is observed. For typical microcavity polarization splittings, the method can be used to achieve perfect polarization degeneracy that is required for many polarization-based implementations of photonic quantum gates. The embedded quantum dot wavelength can be tuned into resonance with the cavity, independent of the polarization tuning.
The pseudo-spin dynamics of propagating exciton-polaritons in semiconductor microcavities are known to be strongly influenced by TE-TM splitting. As a vivid consequence, in the Rayleigh scattering regime, the TE-TM splitting gives rise to the optical spin Hall effect (OSHE). Much less is known about its role in the nonlinear optical regime in which four-wave mixing for example allows the formation of spatial patterns in the polariton density, such that hexagons and two-spot patterns are observable in the far field. Here we present a detailed analysis of spin-dependent four-wave mixing processe…
Whispering gallery mode (WGM) microcavities have been widely used for high-sensitivity ultrasound detection, due to their optical and mechanical resonances enhanced sensitivity. The ultrasound sensitivity of the cavity optomechanical system is fundamentally limited by the thermal noise. In this work, we theoretically and experimentally investigate the thermal-noise-limited sensitivity of a WGM microdisk ultrasound sensor, and optimize the sensitivity by varying the radius and thickness of the microdisk, as well as using a trench structure around the disk. Using a microdisk with a radius of 300…
Planar Bragg microcavities with monolayer WS$_2$ for strong exciton-photon coupling
School of Physics and Engineering, ITMO University（ITMO大学物理与工程学院）；Department of Physics and Astronomy, University of Sheffield（谢菲尔德大学物理与天文学系）；Experimentelle Physik 2, Technische Universität Dortmund（多特蒙德工业大学实验物理第二系）
We investigate a photonic device consisting of two coupled optical cavities possessing Rashba-Dresselhaus spin-orbit coupling, TE-TM splitting, and linear polarisation splitting that opens a tuneable energy gap at the diabolic points of the photon dispersion; giving rise to an actively addressable local Berry curvature. The proposed architecture stems from recent advancements in the design of artificial photonic gauge fields in liquid crystal cavities [K. Rechcińska et al., Science 366, 727 (2019)]. Our study opens new perspectives for topological photonics, room-temperature spinoptronics, and…
Stimulated Raman scattering (SRS) in ultra-high-Q surface-tension-induced spherical and chip-based toroid microcavities is considered both theoretically and experimentally. These microcavities are fabricated from silica, exhibit small mode volume (typically 1000 $μm^{3}$) and possess whispering-gallery type modes with long photon storage times (in the range of 100 ns), significantly reducing the threshold for stimulated nonlinear optical phenomena. Oscillation threshold levels of less than 100 $μ$% -Watts of launched fiber pump power, in microcavities with quality factors of 100 million are ob…
We study the mechanical stability of a tunable high-finesse microcavity under ambient conditions and investigate light-induced effects that can both suppress and excite mechanical fluctuations. As an enabling step, we demonstrate the ultra-precise electronic stabilization of a microcavity. We then show that photothermal mirror expansion can provide high-bandwidth feedback and improve cavity stability by almost two orders of magnitude. At high intracavity power, we observe self-oscillations of mechanical resonances of the cavity. We explain the observations by a dynamic photothermal instability…
We report the control of spontaneous emission from CdSe/ZnS core-shell quantum dots coupled to novel open-access optical microcavities. The cavities are fabricated by focused ion beam milling, and provide mode volumes less than a cubic micrometre. The quantum dot emission spectrum, spatial modes, and lifetime are all modified substantially by the presence of the cavity, and can be tuned by actively varying the cavity length. An increase in emission rate of 75% is achieved at room temperature, attributed to the Purcell effect in the 'bad emitter' regime. We demonstrate a high degree of control …
The authors study the ultrafast switching-on and -off of planar GaAs/AlAs microcavities. Up to 0.8% refractive index changes are achieved by optically exciting free carriers at 1720 nm and a pulse energy of 1.8 micro Joules. The cavity resonance is dynamically tracked by measuring reflectivity versus time delay with tunable laser pulses, and is found to shift by as much as 3.3 linewidths within a few picoseconds. The switching-off occurs with a decay time of around 50 ps. The authors derive the dynamic behavior of the carrier density and of the complex refractive index. They propose that the i…
We describe the use of monolithic, buckled-dome cavities as ultrasound sensors. Patterned delamination within a compressively stressed thin film stack produces high-finesse plano-concave optical resonators with sealed and empty cavity regions. The buckled mirror also functions as a flexible membrane, highly responsive to changes in external pressure. Owing to their efficient opto-acousto-mechanical coupling, thermal-displacement-noise limited sensitivity is achieved at low optical interrogation powers and for modest optical (Q ~ 10^3) and mechanical (Q ~ 10^2) quality factors. We predict and v…
We study rotation-induced asymmetry of far-field emission from optical microcavities, based on which a new scheme of rotation detection may be developed. It is free from the "dead zone" caused by the frequency splitting of standing-wave resonances at rest, in contrast to the Sagnac effect. A coupled-mode theory is employed to provide a quantitative explanation and guidance on the optimization of the far-field sensitivity to rotation. We estimate that a 10^4 enhancement of the minimal detectable rotation speed can be achieved by measuring the far-field asymmetry, instead of the Sagnac effect, i…
The mechanism of unidirectional emission of high Q Whispering Gallery mode in deformed circular micro- cavities is studied and firstly presented in this paper. In phase space, light in the chaotic sea leaks out the cavity through the refraction regions, whose positions are controlled by stable islands. Moreover, the positions of fixed points according to the critical line in unstable manifolds mainly determines the light leak out from which refraction region and the direction of the emission. By controlling the cavity shape, we can tune the leaky regions, as well as the positions of fixed poin…
A novel point of view on the phenomenon of self-pulsations is presented, which shows that they are a balanced state formed by two counteracting processes: beating of modes and bistable switching. A structure based on two coupled nonlinear microcavities provides a generic example of system with enhanced ability to this phenomenon. The specific design of such structure in the form of multilayered media is proposed, and the coupled mode theory is applied to describe its dynamical properties. It is emphasized that the frequency of self-pulsations is related to the frequency splitting between reson…
Owing to their dual-resonance enhanced sensitivity, cavity optomechanical systems provide an ideal platform for ultrasound sensing. In this work, we realize high sensitivity air-coupled ultrasound sensing from kilohertz (kHz) to megahertz (MHz) frequency range based on whispering gallery mode microcavities. Using a 57 um-diameter microtoroid with high optical Q factor (~10^7) and mechanical Q factor (~700), we achieve sensitivities of 46 uPa Hz^{-1/2}-10 mPa Hz^{-1/2} in a frequency range of 0.25-3.2 MHz. Thermal-noise-limited sensitivity is realized around the mechanical resonance at 2.56 MHz…
Planar microcavities allow the control and manipulation of spin-polarization, manifested in phenomena like the optical spin Hall effect due to the intrinsic polarization mode splitting. Here, we study a transparent microcavity with broken rotational symmetry, realized by aligning the optical axis of a uniaxial cavity material in the cavity plane. We demonstrate that the in-plane optical anisotropy gives rise to exceptional points in the dispersion relation, which occur pair-wise, are circularly polarized, and are cores of polarization vortices. These exceptional points are a result of the non-…
We experimentally demonstrate a technique for the generation of optical beams carrying orbital angular momentum using a planar semiconductor microcavity. Despite being isotropic systems, the transverse electric - transverse magnetic (TE-TM) polarization splitting featured by semiconductor microcavities allows for the conversion of the circular polarization of an incoming laser beam into the orbital angular momentum of the transmitted light field. The process implies the formation of topological entities, a pair of optical half-vortices, in the intracavity field.
We design, fabricate, and experimentally demonstrate a compact thermo-optic gate switch comprising a 3.78 um-long coupled L0-type photonic crystalmicrocavities on a silicon-on-insulator substrate. A nanohole is inserted in the center of each individual L0 photonic crystalmicrocavity. Coupling between identical microcavities gives rise to bonding and anti-bonding states of the coupled photonic molecules. The coupled photonic crystalmicrocavities are numerically simulated and experimentally verified with a 6 nm-wide flat-bottom resonance in its transmission spectrum, which enables wider operatio…
Integrated, ultrafast all-optical polariton transistors with sub-wavelength grating microcavities
IBM Research Europe – Zurich（IBM欧洲苏黎世研究中心）；ETH Zürich（苏黎世联邦理工学院）；AMO GmbH（AMO有限公司）；RWTH Aachen University（亚琛工业大学）；Bergische Universität Wuppertal（伍珀塔尔大学）
Optical resonances in 1D photonic crystal microcavities are investigated numerically using finite-element light scattering and eigenmode solvers. The results are validated by comparison to experimental and theoretical findings from the literature. The influence of nanometer-scale geometry variations on the resonator performance is studied. Limiting factors to ultra-high Q-factor performance are identified.
Scattering processes in an optical microcavity are investigated for the case of silicon nanocrystals embedded in an ultra-high Q toroid microcavity. Using a novel measurement technique based on the observable mode-splitting, we demonstrate that light scattering is highly preferential: more than 99.8% of the scattered photon flux is scattered into the original doubly-degenerate cavity modes. The large capture efficiency is attributed to an increased scattering rate into the cavity mode, due to the enhancement of the optical density of states over the free space value and has the same origin as …
A theoretical variation between the two distinct light-matter coupling regimes, namely weak and strong coupling, becomes uniquely feasible in open optical Fabry-Pérot microcavities with low mode volume, as discussed here. In combination with monolayers of transition-metal dichalcogenides (TMDCs) such as WS2, which exhibits a large exciton oscillator strength and binding energy, the room-temperature observation of hybrid bosonic quasiparticles, referred to as exciton-polaritons and characterized by a Rabi splitting, comes into reach. In this context, our simulations using the transfer-matrix me…
We demonstrate in open microcavities with broken chiral symmetry, quasi-degenerate pairs of co-propagating modes in a non-rotating cavity evolve to counter-propagating modes with rotation. The emission patterns change dramatically by rotation, due to distinct output directions of CW and CCW waves. By tuning the degree of spatial chirality, we maximize the sensitivity of microcavity emission to rotation. The rotation-induced change of emission is orders of magnitude larger than the Sagnac effect, pointing to a promising direction for ultrasmall optical gyroscopes.
Lithium niobate (LN) is an excellent nonlinear optical and electro-optic material that has found many applications in classical nonlinear optics, optical fiber communications and quantum photonics. Here we review the recent development of thin-film LN technology that has allowed the miniaturization of LN photonic devices and microcavities with ultrahigh quality factors. We discuss the design principle of LN devices that makes use of the largest nonlinear coefficients, various device fabrication approaches and resulting device performances, and the current and potential applications of LN micro…
Open-access microcavities are emerging as a new approach to confine and engineer light at mode volumes down to the $λ^3$ regime. They offer direct access to a highly confined electromagnetic field while maintaining tunability of the system and flexibility for coupling to a range of matter systems. This article presents a study of coupled cavities, for which the substrates are produced using Focused Ion Beam milling. Based on experimental and theoretical investigation the engineering of the coupling between two microcavities with radius of curvature of \SI{6}{\micro\meter} is demonstrated. Deta…
The simultaneous control of optical and mechanical waves has enabled a range of fundamental and technological breakthroughs, from the demonstration of ultra-stable frequency reference devices to the exploration of the quantum-classical boundaries in laser-cooling experiments. More recently, such an opto-mechanical interaction has been observed in integrated nano-waveguides and microcavities in the Brillouin regime, where short-wavelength mechanical modes scatters light at several GHz. Here we engineer coupled optical microcavities spectra to enable a low threshold excitation of mechanical trav…
Electromagnetically-induced-transparency (EIT) and Autler-Townes splitting (ATS) are two prominent examples of coherent interactions between optical fields and multilevel atoms. They have been observed in various physical systems involving atoms, molecules, meta-structures and plasmons. In recent years, there has been an increasing interest in the implementations of all-optical analogues of EIT and ATS via the interacting resonant modes of one or more optical microcavities. Despite the differences in their underlying physics, both EIT and ATS are quantified by the appearance of a transparency …
High-Q ring resonators with contacts to the waveguide core provide a versatile platform for various applications in chip-scale optomechanics, thermo- and electro-optics. We propose and demonstrate a novel approach to implement azimuthally periodic contacted ring resonators based on multi-mode Bloch matching that support contacts on both the inner and outer radius edges with small degradation to the optical Q. Radiative coupling between degenerate modes of adjacent transverse spatial order leads to imaginary frequency (Q) splitting and a scatterer avoiding high-Q "wiggler" supermode field. We e…
We study the polarization dynamics of a spatially expanding polariton condensate under nonresonant linearly polarized optical excitation. The spatially and temporally resolved polariton emission reveals the formation of non-trivial spin textures in the form of a quadruplet polarization pattern both in the linear and circular Stokes parameters, and an octuplet in the diagonal Stokes parameter. The continuous rotation of the polariton pseudospin vector through the condensate due to TE-TM splitting exhibits an ordered pattern of half-skyrmions associated with a half-integer topological number. A …
In a non-Hermitian optical system with loss and gain, an exceptional point (EP) will arise under specific parameters where the eigenvalues and eigenstates exhibit simultaneous coalescence. Here we report a dynamical switching of lasing behavior in a non-Hermitian system composed of coupled microcavities by modulating the EPs. Utilizing the effect of gain, loss and coupling on the eigenstates of coupled microcavities, the evolution path of the eigenvalues related to the laser emission characteristics can be modulated. As a result, the lasing emission property of the coupled cavities exhibits an…
We propose and design photonic crystal cavities (PCCs) in hexagonal boron nitride (hBN) for diverse photonic and quantum applications. Two dimensional (2D) hBN flakes contain quantum emitters which are ultra-bright and photostable at room temperature. To achieve optimal coupling of these emitters to optical resonators, fabrication of cavities from monolithic hBN is therefore required, to maximize the overlap between cavity optical modes and the emitters. Here, we design 2D and 1D PCCs using anisotropic indices of hBN. The influence of underlying substrates and material absorption are investiga…
Microcomb generation with simultaneous $χ^{(2)}$ and $χ^{(3)}$ nonlinearities brings new possibilities for ultra-broadband and potentially self-referenced integrated comb sources. However, the evolution of the intracavity field involving multiple nonlinear processes shows complex dynamics that is still poorly understood. Here we report on strong soliton regulation induced by fundamental-second-harmonic (FD-SH) mode coupling. The formation of solitons from chaos is extensively investigated based on coupled Lugiato-Lefever equations. The soliton generation shows more deterministic behaviors in t…
All-optical nonlinear phase modulation in open semiconductor microcavities
University of Sheffield（谢菲尔德大学）；Université Paris-Saclay（巴黎萨克雷大学）；CNRS, Centre de Nanosciences et de Nanotechnologies (C2N)（法国国家科学研究中心纳米科学与技术中心）；Department of Materials, University of Oxford（牛津大学材料系）
Exciton polaritons in semiconductor microcavities exhibit many fundamental physical effects, with some of them amenable to being controlled by external fields. The polariton transport is affected by the polaritonic spin-orbit interaction, which is caused by the splitting of transverse-electric and transverse-magnetic (TE-TM) modes. This is the basis for a polaritonic Hall effect, called optical spin Hall effect (OSHE), which is related to the formation of spin/polarization textures in momentum space, determining anisotropic ballistic transport, as well as related textures in real space. Owing …
We introduce and investigate billiard systems with an adjusted ray dynamics that accounts for modifications of the conventional reflection of rays due to universal wave effects. We show that even small modifications of the specular reflection law have dramatic consequences on the phase space of classical billiards. These include the creation of regions of non-Hamiltonian dynamics, the breakdown of symmetries, and changes in the stability and morphology of periodic orbits. Focusing on optical microcavities, we show that our adjusted dynamics provides the missing ray counterpart to previously ob…
Coherent control and manipulation of quantum degrees of freedom such as spins forms the basis of emerging quantum technologies. In this context, the robust valley degree of freedom and the associated valley pseudospin found in two-dimensional transition metal dichalcogenides is a highly attractive platform. Valley polarization and coherent superposition of valley states have been observed in these systems even up to room temperature. Control of valley coherence is an important building block for the implementation of valley qubit. Large magnetic fields or high-power lasers have been used in th…
Optical frequency combs are crucial for both fundamental science and applications demanding wide frequency spanning and ultra-precision resolutions. Recent advancements of nonlinear Kerr effect based optical frequency combs in microcavities open up new opportunities in a compact platform, however, internal cavity-enhanced nonlinearities are still unclear. Here we demonstrate transient nonlinear dynamics during optical frequency comb formation inside a Kerr microcavity. We show that gain spiking forms due to nonlinear phase modulation, causing comb lines' self-detuning nearby a cavity resonance…
Here we propose a method of the excitation of perpendicular standing spin waves (PSSWs) of different orders in an optomagnonic microcavity by ultrashort laser pulses. The microcavity is formed by a magnetic dielectric film surrounded by dielectric non-magnetic Bragg mirrors. Optical cavity modes in the magnetic layer provide concentration and strongly non-uniform distribution of the optical power over the layer thickness and therefore induce the effective field of the inverse Faraday effect also spatially non-uniform. It results in excitation of PSSWs. PSSWs whose wavevector is closest to the …
The optical spin-Hall effect results in the formation of an antisymmetric real space polarization pattern forming spin currents. In this paper, we show that the exciton-polariton parametric scattering allows us to reverse the sign of these currents. We describe the pulsed resonant excitation of a strongly coupled microcavity with a linearly polarized pump at normal incidence. The energy of the pulse is set to be close to the inflexion point of the polariton dispersion and the focusing in real space populates the reciprocal space on a ring. For pumping powers below the parametric scattering thr…
Optical microcavities are essential in numerous technologies and scientific disciplines. However, their application in many areas relies exclusively upon discrete microcavities in order to satisfy challenging combinations of ultra-low-loss performance (high cavity-Q-factor) and cavity design requirements. Indeed, finding a microfabrication bridge connecting ultra-high-Q device functions with micro and nanophotonic circuits has been a long-term priority of the microcavity field. Here, an integrated ridge resonator having a record Q factor over 200 million is presented. Its ultra-low-loss and fl…
A large body of work has accumulated over the years in the study of the optical properties of single and coupled microcavities for a variety of applications, ranging from filters to sensors and lasers. The focus has been mostly on the geometry of individual resonators and/or on their combination in arrangements often referred to as photonic molecules (PMs). Our primary concern will be the lasing properties of PMs as ideal candidates for the fabrication of integrated microlasers, photonic molecule lasers. Whereas most calculations on PM lasers have been based on cold-cavity (passive) modes, i.e…
Exceptional rings in nonlinear non-Hermitian planar optical microcavities: implementation, signal enhancement, and topology
Paderborn University（帕德博恩大学）；Wyant College of Optical Sciences, University of Arizona（亚利桑那大学怀特光学科学学院）；Department of Physics, University of Arizona（亚利桑那大学物理系）
Organic exciton-photon polariton lasers have recently been shown to be remarkable candidates for the realization of efficient sources of coherent light operating at room temperature. While their thresholds are now comparable with conventional organic photon lasers, tuning of molecular conformation and orientation as a means to further enhance their performance remains largely unexplored. Here, we first report a two-fold reduction in the threshold of a polariton laser based on a high-Q microcavity filled with an active layer of poly(9,9-dioctylfluorene) (PFO) when 15% β-phase conformation is in…
Whispering-gallery microcavities have been used to realize a variety of efficient parametric nonlinear optical processes through the enhanced light-matter interaction brought about by supporting multiple high quality factor and small modal volume resonances. Critical to such studies is the ability to control the relative frequencies of the cavity modes, so that frequency matching is achieved to satisfy energy conservation. Typically this is done by tailoring the resonator cross-section. Doing so modifies the frequencies of all of the cavity modes, that is, the global dispersion profile, which …
Solid-state microcavities combining ultra-small mode volume, wide-range resonance frequency tuning, as well as lossless coupling to a single mode fibre are integral tools for nanophotonics and quantum networks. We developed an integrated system providing all of these three indispensable properties. It consists of a nanofibre Bragg cavity (NFBC) with the mode volume of under 1 micro cubic meter and repeatable tuning capability over more than 20 nm at visible wavelengths. In order to demonstrate quantum light-matter interaction, we establish coupling of quantum dots to our tunable NFBC and achie…
We designed Si-based all-dielectric 1 $\times$ 2 TE and TM power splitters with various splitting ratios and simulated them using the inverse design of adjoint and numerical 3D finite-difference time-domain methods. The proposed devices exhibit ultra-high transmission efficiency above 98 and 99\%, and excess losses below 0.1 and 0.035 dB, for TE and TM splitters, respectively. The merits of these devices include a minor footprint of 2.2 $\times$ 2.2 $μ$m $\times$ $μ$m and a broad operating bandwidth of 200 nm with a center wavelength of $λ$ = 1.55 $μ$ m.
