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arXiv 1004.4685cond-mat.str-el
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对ARPES中观察到的铜氧化物高能异常的认识

Insights on the cuprate high energy anomaly observed in ARPES

B. Moritz, S. Johnston, T. P. Devereaux

摘要:

最近,角分辨光电子能谱已被用来突出在高结合能的铜氧化物超导体的一个令人不安的大带重整化:高能量“瀑布”或高能量异常(HEA)。异常是目前的空穴和电子掺杂的铜氧化物,以及半填充的母绝缘体与不同的能量尺度上产生的相图的两侧。虽然光电发射矩阵元素在改变能带色散的美学外观(即创建“瀑布”状外观)方面显然起作用,但它们对导致HEA的强能带重整化的物理基础提供了不充分的描述。模型计算的单带哈伯德哈密顿展示了相关性在HEA的形成中所发挥的作用,并揭示了空穴和电子掺杂的铜酸盐的HEA能量尺度的显着差异。此外,这种方法适当地捕获光谱权重的转移伴随着掺杂在相关的材料,并提供了一个统一的描述的HEA跨越两侧的铜酸盐相图。我们发现,异常划分的过渡,或交叉,从准粒子带在低结合能附近的费米能级到价带在较高的结合能,假设是强氧字符。

英文摘要:

Recently, angle-resolved photoemission spectroscopy has been used to highlight an anomalously large band renormalization at high binding energies in cuprate superconductors: the high energy "waterfall" or high energy anomaly (HEA). The anomaly is present for both hole- and electron-doped cuprates as well as the half-filled parent insulators with different energy scales arising on either side of the phase diagram. While photoemission matrix elements clearly play a role in changing the aesthetic appearance of the band dispersion, i.e. creating a "waterfall"-like appearance, they provide an inadequate description for the physics that underlies the strong band renormalization giving rise to the HEA. Model calculations of the single-band Hubbard Hamiltonian showcase the role played by correlations in the formation of the HEA and uncover significant differences in the HEA energy scale for hole- and electron-doped cuprates. In addition, this approach properly captures the transfer of spectral weight accompanying doping in a correlated material and provides a unifying description of the HEA across both sides of the cuprate phase diagram. We find that the anomaly demarcates a transition, or cross-over, from a quasiparticle band at low binding energies near the Fermi level to valence bands at higher binding energy, assumed to be of strong oxygen character.

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