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arXiv 0912.4353cond-mat.str-elcond-mat.stat-mech
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NMR和量子蒙特卡罗模拟研究耦合梯形结构BiCu2PO6中杂质效应

Impurity effects in coupled-ladder BiCu2PO6 studied by NMR and quantum Monte Carlo simulations

L. K. Alexander, J. Bobroff, A. V. Mahajan, B. Koteswararao, N. Laflorencie, F. Alet

摘要:

我们提出了一个耦合自旋1/2梯形化合物BiCu 2 PO 6的31 P NMR研究。在纯材料中,本征磁化率和动力学显示约为的自旋间隙。非磁性Zn或磁性Ni杂质在Cu位的替代诱导交错磁化,这导致31 P NMR线加宽,而远离缺陷的磁化率不受影响。Ni对NMR谱线展宽的影响是Zn的两倍,这与量子蒙特卡罗(QMC)计算假设Ni铁磁耦合到其相邻的Cu一致。诱导力矩遵循1/T的温度依赖性,由于居里样的发展的力矩振幅,而其扩展饱和,不依赖于杂质含量或性质。这使我们能够验证杂质掺杂的一般预期的情况下,并将其扩展到磁性杂质的情况下:在反铁磁相关的低维自旋系统与反铁磁相关,任何类型的杂质诱导在低温下的交错时刻,其扩展是不与杂质的性质,但在发挥作用的内在物理在未掺杂的纯系统,从1D到2D系统。

英文摘要:

We present a 31P NMR study of the coupled spin 1/2 ladder compound BiCu2PO6. In the pure material, intrinsic susceptibility and dynamics show a spin gap of about . Substitution of non magnetic Zn or magnetic Ni impurity at Cu site induces a staggered magnetization which results in a broadening of the 31P NMR line, while susceptibility far from the defects is unaffected. The effect of Ni on the NMR line broadening is twice that of Zn, which is consistent with Quantum Monte Carlo (QMC) calculations assuming that Ni couples ferromagnetically to its adjacent Cu. The induced moment follows a 1/T temperature dependence due to the Curie-like development of the moment amplitude while its extension saturates and does not depend on impurity content or nature. This allow us to verify the generically expected scenario for impurity doping and to extend it to magnetic impurity case: in an antiferromagnetically correlated low dimensional spin system with antiferromagnetic correlations, any type of impurity induces a staggered moment at low temperature, whose extension is not linked to the impurity nature but to the intrinsic physics at play in the undoped pure system, from 1D to 2D systems.

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