We demonstrate experimentally a quantum memory scheme for the storage of weak coherent light pulses in an inhomogeneously broadened optical transition in a Pr^{3+}: YSO crystal at 2.1 K. Precise optical pumping using a frequency stable (about 1kHz linewidth) laser is employed to create a highly controllable Atomic Frequency Comb (AFC) structure. We report single photon storage and retrieval efficiencies of 25%, based on coherent photon echo type re-emission in the forward direction. The coherence property of the quantum memory is proved through interference between a super Gaussian pulse and the emitted echo. Backward retrieval of the photon echo emission has potential for increasing storage and recall efficiency.
Propagation of two dimensional pulses in electromagnetically induced tranparency media in the case of perpendicular storing and retrieving pulses has been analyzed. It has been shown that propagation control of the pulses in optically thick media can be used for producing interchange between pulse time-shape and intensity profile distribution. A simple obvious analytical solution for the retrieved new field has been obtained.
By solving the self-consistent system of Maxwell and density matrix equations to the first order with respect to nonadiabaticity, we obtain an analytical solution for the probe pulse propagation. The conditions for efficient storage of light are analyzed. The necessary conditions for optical propagation distance has been obtained.
We investigate the rephasing efficiency of sequences of phased pulses for spin echoes and light storage by electromagnetically induced transparency (EIT). We derive a simple theoretical model and show that the rephasing efficiency is very sensitive to the phases of the imperfect rephasing pulses. The obtained efficiency differs substantially for spin echoes and EIT light storage, which is due to the spatially retarded coherence phases after EIT light storage. Similar behavior is also expected for other light-storage protocols with spatial retardation or for rephasing of collective quantum stat…
Coherent pulse control for quantum memory is viable in the optical domain but nascent in microwave quantum circuits. We show how to realize coherent storage and on-demand pulse retrieval entirely within a superconducting circuit by exploiting and extending existing electromagnetically induced transparency technology in superconducting quantum circuits. Our scheme employs a linear array of superconducting artificial atoms coupled to a microwave transmission line.
We experimentally demonstrate optimal storage and retrieval of light pulses of arbitrary shape in atomic ensembles. By shaping auxiliary control pulses, we attain efficiencies approaching the fundamental limit and achieve precise retrieval into any predetermined temporal profile. Our techniques, demonstrated in warm Rb vapor, are applicable to a wide range of systems and protocols. As an example, we present their potential application to the creation of optical time-bin qubits and to controlled partial retrieval.
We demonstrate experimentally a procedure to obtain the maximum efficiency for the storage and retrieval of light pulses in atomic media. The procedure uses time reversal to obtain optimal input signal pulse-shapes. Experimental results in warm Rb vapor are in good agreement with theoretical predictions and demonstrate a substantial improvement of efficiency. This optimization procedure is applicable to a wide range of systems.
Photon-echo based optical quantum memory schemes often employ intermediate steps to transform optical coherences to spin coherences for longer storage times. We analyze a scheme that uses three identical chirped control pulses for coherence rephasing in an inhomogeneously broadened ensemble of three-level $Λ$-systems. The pulses induce a cyclic permutation of the atomic populations in the adiabatic regime. Optical coherences created by a signal pulse are stored as spin coherences at an intermediate time interval, and are rephased for echo emission when the ensemble is returned to the initial s…
We investigate whether it is possible to store and retrieve the intense probe pulse from a $Λ$-type homogeneous medium of cold atoms. Through numerical simulations we show that it is possible to store and retrieve the probe pulse which are not necessarily weak. As the intensity of the probe pulse increases, the retrieved pulse remains a replica of the original pulse, however there is overall broadening and loss of the intensity. These effects can be understood in terms of the dependence of absorption on the intensity of the probe. We include the dynamics of the control field, which becomes esp…
Attenuated laser pulses are often employed in place for single photons in order to test the efficiency of the elements of a quantum network. In this work we analyse theoretically the dynamics of storage of an attenuated light pulse (where the pulse intensity is at the single photon level) propagating along a transmission line and impinging on the mirror of a high finesse cavity. Storage is realised by the controlled transfer of the photonic excitations into a metastable state of an atom confined inside the cavity and occurs via a Raman transition with a suitably tailored laser pulse, which dri…
An ultralong photon storage with more than 50% retrieval efficiency is presented in the three-pulse photon echoes by using a pair of control pulses, where the control pulses play to freeze atoms dephasing process conditionally by transferring excited atoms to an auxiliary state and returning them back later. The observed photon echo decay time much longer than the spin homogeneous decay time is potential for long distance quantum communications.
We show both analytically and numerically that photons from a probe pulse are not stored in several recent experiments. Rather, they are absorbed to produce a two-photon excitation. More importantly, when an identical coupling pulse is re-injected into the medium, we show that the regenerated optical field has a pulse width that is very different from the original probe field. It is therefore, not a faithful copy of the original probe pulse.
Quantum memories for light, which allow the reversible transfer of quantum states between light and matter, are central to the development of quantum repeaters, quantum networks, and linear optics quantum computing. Significant progress has been reported in recent years, including the faithful transfer of quantum information from photons in pure and entangled qubit states. However, none of these demonstrations confirm that photons stored in and recalled from quantum memories remain suitable for two-photon interference measurements, such as C-NOT gates and Bell-state measurements, which constit…
Atomic population transfer in an inhomogeneously broadened optical medium is analyzed for on-demand photon storage-time control in both atomic frequency comb (AFC) and phase locked echoes. In AFC the photon storage mechanism belongs to the conventional three-pulse photon echoes, while the storage time control is limited by conventional two-pulse photon echoes.
We report on an experimental study of light pulse propagation and storage in a Rb atomic vapor for different pulse durations, magnetic fields, and atomic densities, and for two different isotopes. The results have been analyzed and compared with previous studies.
The three-pulse photon echo is a well-known technique to store intense light pulses in an inhomogeneously broadened atomic ensemble. This protocol is attractive because it is relatively simple and it is well suited for the storage of multiple temporal modes. Furthermore, it offers very long storage times, greater than the phase relaxation time. Here, we consider the three-pulse photon echo in both two- and three-level systems as a potential technique for the storage of light at the single-photon level. By explicit calculations, we show that the ratio between the echo signal corresponding to a …
We present experimental evidence that light storage, i.e. the controlled release of a light pulse by an atomic sample dependent on the past presence of a writing pulse, is not restricted to small group velocity media but can also occur in a negative group velocity medium. A simple physical picture applicable to both cases and previous light storage experiments is discussed.
We report experimental investigationd of optical pulse group velocity reduction and probe pulse regeneration using a Raman scheme. The new scheme which does not rely on the on-one-photon resonance electromagnetically induced transparency (EIT), has many advantages over the conventional method which critically relys on the transparency window created by an EIT process. We demonstrate significant reduction of group velocity, less probe field loss, reduced probe pulse distortion, and high probe pulse regeneration efficiency.
We demonstrate the storage of $5$ ns light pulses in a single rubidium atom coupled to a fiber-based optical resonator. Our storage protocol addresses a regime beyond the conventional adiabatic limit and approaches the theoretical bandwidth limit. We extract the optimal control laser pulse properties from a numerical simulation of our system and measure storage efficiencies of $(8.2\pm 0.6)~\%$, in close agreement with the maximum expected efficiency. Such well-controlled and high-bandwidth atom-photon interfaces are key components for future hybrid quantum networks.
Quantum memories for quantum communication need to be able to store photons for an extended time and then to release them on demand. This can be achieved in atomic frequency comb ensemble based quantum memories by control pulses that transfer the excitation to and from long-lived spin states. However, such pulses can give rise to coherent and incoherent noise due to their interaction with the memory ensemble. In this article, we experimentally demonstrate the ability to switch off the coherent noise from such control pulses during the echo emission in a spin-wave quantum memory, using the line…
We investigate the potential of atomic Bose-Einstein condensates as dynamic memory devices for coherent optical information processing. Specifically, the number of ultraslow pulses that can be simultaneously present within the storage time in the condensate has been analyzed. By modeling short-pulse propagation through the condensate, taking into account high-order dispersive properties, constraints on the information storage capacity are discussed. The roles of temperature, spatial inhomogeneity, the interatomic interactions, and the coupling laser on the pulse shape are pointed out. For a re…
It is shown theoretically that after light storing in a medium of four-level atoms it is possible to release a new pulse of a different frequency, the process being steered by another driving beam. It is also possible to store one pulse and to release two different ones, with their time separation and heights being controlled.
We demonstrate a coherent and dynamic beam splitter based on light storage in cold atoms. An input weak laser pulse is first stored in a cold atom ensemble via electromagnetically-induced transparency (EIT). A set of counter-propagating control fields, applied at a later time, retrieves the stored pulse into two output spatial modes. The high visibility interference between the two output pulses clearly demonstrates that the beam splitting process is coherent. Furthermore, by manipulating the control lasers, it is possible to dynamically control the storage time, the power splitting ratio, the…
We analyze the storage and retrieval of intense-broadband pulses with the added effects of Doppler broadening and detuning in a $Λ$ configuration. We compute analytical solutions via the inverse scattering technique and show how the signal field is transferred to a spin-wave in the atomic medium and later retrieved by the interaction of a control pulse. Due to the intensity of the pulses, the pulse area (as defined for self-induced transparency) plays a key role in the interaction, as it determines the location of the spin wave within the medium. Additionally, we compare our results to non-ide…
We have considered theoretically the feasibility of the broadband quantum memory based on the resonant tripod-type atomic configuration. In this case, the writing of a signal field is carried out simultaneously into two channels, and characterized by an excitation of two spin waves of the atomic ensemble. With simultaneous read out from both channels quantum properties of the original signal are mapped on the retrieval pulse no worse than in the case of memory based on Lambda-type atomic configuration. At the same time new possibilities are opened up for manipulation of quantum states associat…
We report on the first observation of stationary light pulses and narrowband light storage inside a hollow-core photonic crystal fiber. Laser-cooled atoms were first loaded into the fiber core providing strong light-matter coupling. Light pulses were then stored in a collective atomic excitation using a single control laser beam. By applying a second counterpropagating control beam, a light pulse could be brought to a standstill. Our work paves the way towards the creation of strongly-correlated many-body systems with photons and applications in the field of quantum information processing.
We report an experiment in which a light pulse is decelerated and trapped in a vapor of Rb atoms, stored for a controlled period of time, and then released on demand. We accomplish this storage of light by dynamically reducing the group velocity of the light pulse to zero, so that the coherent excitation of the light is reversibly mapped into a collective Zeeman (spin) coherence of the Rb vapor.
Single-photon coherent optics represents a fundamental importance for the investigation of quantum light-matter interactions. While most work has considered the interaction in the steady-state regime, here we demonstrate that a single-photon pulse shorter than any relaxation time in a medium propagates without energy loss and is consistently transformed into a zero-area pulse. A general analytical solution is found for photon passage through a cold ensemble of $Λ$-type atoms confined inside a hollow core of a single-mode photonic-crystal fiber. We use the robust far off-resonant Raman scheme t…
A long-lived quantum memory is a firm requirement for implementing a quantum repeater scheme. Recent progress in solid-state rare-earth-ion-doped systems justifies their status as very strong candidates for such systems. Nonetheless an optical memory based on spin-wave storage at the single-photon-level has not been shown in such a system to date, which is crucial for achieving the long storage times required for quantum repeaters. In this letter we show that it is possible to execute a complete atomic frequency comb (AFC) scheme, including spin-wave storage, with weak coherent pulses of $\bar…
Storage and retrieval of a squeezed vacuum was successfully demonstrated using electromagnetically induced transparency. 930ns of the squeezed vacuum pulse was incident on the laser cooled 87Rb atoms with an intense control light in a coherent state. When the squeezed vacuum pulse was slowed and spatially compressed in the cold atoms, the control light was switched off. After 3us of storage, the control light was switched on again and the squeezed vacuum was retrieved, as was confirmed using the time-domain homodyne method.
In the present manuscript, we present a high-speed method to control, manipulate and retrieve an intense vector soliton stored in the ground state coherences of a four-level atomic system. Additionally, we show the importance of the pulse area in determining the evolution of the system and present a constant in the evolution defined as the three-pulse area, a surprising extension to previously defined pulse areas.
We present a light-storage experiment in a praseodymium-doped crystal where the light is mapped onto an inhomogeneously broadened optical transition shaped into an atomic frequency comb. After absorption of the light the optical excitation is converted into a spin-wave excitation by a control pulse. A second control pulse reads the memory (on-demand) by reconverting the spin-wave excitation to an optical one, where the comb structure causes a photon-echo type rephasing of the dipole moments and directional retrieval of the light. This combination of photon echo and spin-wave storage allows us …
We report measurements of the time-dependent phases of the leak and retrieved pulses obtained in EIT storage experiments with metastable helium vapor at room temperature. In particular, we investigate the influence of the optical detuning at two-photon resonance, and provide numerical simulations of the full dynamical Maxwell-Bloch equations, which allow us to account for the experimental results.
Photon echo schemes are excellent candidates for high efficiency coherent optical memory. They are capable of high-bandwidth multi-pulse storage, pulse resequencing and have been shown theoretically to be compatible with quantum information applications. One particular photon echo scheme is the gradient echo memory (GEM). In this system, an atomic frequency gradient is induced in the direction of light propagation leading to a Fourier decomposition of the optical spectrum along the length of the storage medium. This Fourier encoding allows precision spectral manipulation of the stored light. I…
We propose a dynamical approach to quantum memories using a synchronous oscillator-cavity model, in which the coupling is shaped in time to provide the optimum interface to a symmetric input pulse. This overcomes the known difficulties of achieving high quantum input-output fidelity with storage times long compared to the input signal duration. Our generic model is applicable to any linear storage medium ranging from a superconducting device to an atomic medium. We show that with temporal modulation of coupling and/or detuning, it is possible to mode-match to time-symmetric pulses that have id…
We theoretically analyse the efficiency of a quantum memory for single photons. The photons propagate along a transmission line and impinge on one of the mirrors of a high-finesse cavity. The quantum memory is constituted by a single atom within the optical resonator. Photon storage is realised by the controlled transfer of the photonic excitation into a metastable state of the atom and occurs via a Raman transition with a suitably tailored laser pulse, which drives the atom. Our study is supported by numerical simulations, in which we include the modes of the transmission line and we use the …
Tapered optical fibers with a nanofiber waist are versatile tools for interfacing light and matter. In this context, laser-cooled atoms trapped in the evanescent field surrounding the optical nanofiber are of particular interest: They exhibit both long ground-state coherence times and efficient coupling to fiber-guided fields. Here, we demonstrate electromagnetically induced transparency, slow light, and the storage of fiber-guided optical pulses in an ensemble of cold atoms trapped in a nanofiber-based optical lattice. We measure a slow-down of light pulses to group velocities of 50 m/s. More…
We present a universal physical picture for describing storage and retrieval of photon wave packets in a Lambda-type atomic medium. This physical picture encompasses a variety of different approaches to pulse storage ranging from adiabatic reduction of the photon group velocity and pulse-propagation control via off-resonant Raman fields to photon-echo based techniques. Furthermore, we derive an optimal control strategy for storage and retrieval of a photon wave packet of any given shape. All these approaches, when optimized, yield identical maximum efficiencies, which only depend on the optica…
We report the experimental demonstration of optomechanical light storage in a silica resonator. We use writing and readout laser pulses tuned to one mechanical frequency below an optical cavity resonance to control the coupling between the mechanical displacement and the optical field at the cavity resonance. The writing pulse maps a signal pulse at the cavity resonance to a mechanical excitation. The readout pulse later converts the mechanical excitation back to an optical pulse. The light storage lifetime is determined by the relatively long damping time of the mechanical excitation.
A near perfect, storage time-extended photon echo-based quantum memory protocol has been analyzed by solving the Maxwell-Bloch equations for a backward scheme in a three-level system. The backward photon echo scheme is combined with a controlled coherence conversion process via control Rabi flopping to a third state, where the control Rabi flopping collectively shifts the phase of the ensemble coherence. The propagation direction of photon echoes is coherently determined by the phase matching condition between the data (quantum) and the control (classical) pulses. Herein we discuss the classic…
Coherent inter-conversion between an optical and a mechanical excitation in an optomechanical resonator can be used for the storage of an optical pulse as an excitation in a mechanical oscillator. This optomechanical light storage is enabled by external writing and readout pulses at one mechanical frequency below the optical resonance. In this paper, we expand an earlier experimental study [Phys. Rev. Lett. 107, 133601 (2011)] on storing an optical pulse as a radial breathing mode in a silica microsphere. We show that the heterodyne beating between a readout pulse and the corresponding retriev…
A classical logic gate connecting input and output light pulses is demonstrated. The gate operation is based on three steps: First, two incoming light pulses are stored in a Bose-Einstein condensate, second, atomic four-wave mixing generates a new matter wave, and third, the light pulses are retrieved. In the presence of the new matter wave, the retrieval generates a new optical wave. The latter will only be generated if both input light pulses are applied, thus realizing an AND gate. Finally, we show that the gate operation is phase coherent, an essential prerequisite for a quantum logic gate…
Solutions to the Maxwell-Bloch equations for a $Λ$ system are computed using the single-soliton Darboux transformation and the nonlinear superposition principle. These allow complete control of information deposited by a signal pulse (with the help of an auxiliary control pulse) in the coherence of the medium's ground states by injecting sub-sequential pulses. Additionally, we study the encoding of two signal pulses and their manipulation by a control pulse and show that multipulse storage and control are possible as long as the imprints made by encoding the signal pulses are sufficiently sepa…
We consider in this paper a two-pulse photon echo sequence as a potential quantum light storage protocol. It is widely believed that a two-pulse scheme should lead to very low efficiency and is then not relevant for this specific application. We show experimentally by using a Tm${}^{3+}$:YAG crystal that such a protocol is on contrary very efficient and even too efficient to be considered as a good quantum storage protocol. Our experimental work allows us to point out on one side the real limitations of this scheme and on the other side its benefits which can be a source of inspiration to conc…
We present a proposal for storing and retrieving a continuous-variable quadripartite polarization-entangled cluster state, using macroscopic atomic ensembles in a magnetic field. The Larmor precession of the atomic spins leads to a symmetry between the atomic canonical operators. In this scheme, each of the four spatially separated pulses passes twice through the respective ensemble in order to map the polarization-entangled cluster state onto the long-lived atomic ensembles. The stored state can then be retrieved by another four read-out pulses, each crossing the respective ensemble twice. By…
A scheme for spatial multimode quantum memory is developed such that spatial-temporal structure of a weak signal pulse can be stored and recalled via cavity-assisted off-resonant Raman interaction with a strong angular-modulated control field in an extended $Λ$-type atomic ensemble. It is shown that effective multimode storage is possible when the Raman coherence spatial grating involves wave vectors with different longitudinal components relative to the paraxial signal field. The possibilities of implementing the scheme in the solid-state materials are discussed.
We report on coherent and multi-temporal mode storage of light using the full atomic frequency comb memory scheme. The scheme involves the transfer of optical atomic excitations in Pr3+:Y2SiO5 to spin-waves in the hyperfine levels using strong single-frequency transfer pulses. Using this scheme, a total of 5 temporal modes are stored and recalled on-demand from the memory. The coherence of the storage and retrieval is characterized using a time-bin interference measurement resulting in visibilities higher than 80%, independent of the storage time. This coherent and multimode spin-wave memory i…
We consider adiabatic interaction of five-level atomic systems and their media with four short laser pulses under the condition of all two-photon detunings being zero. We derive analytical expressions for eigenvalues of the system's Hamiltonian and determine conditions of adiabaticity for both the atom and the medium. We analyse, in detail, the system's behaviour when the eigenvalue with non-vanishing energy is realized. As distinct from the usual dark state of a five-level system (corresponding to zero eigenvalue), which is a superposition of three states, in our case the superposition of fou…
We study procedures for the optimization of efficiency of light storage and retrieval based on the dynamic form of electromagnetically induced transparency (EIT) in warm Rb vapor. We present a detailed analysis of two recently demonstrated optimization protocols: a time-reversal-based iteration procedure, which finds the optimal input signal pulse shape for any given control field, and a procedure based on the calculation of an optimal control field for any given signal pulse shape. We verify that the two procedures are consistent with each other, and that they both independently achieve the m…
We propose a novel scheme to realize electrically controlled quantum memories in the opto- and electro-mechanical (OEM) cavity. Combining this OEM cavity with the mechanism of Electromagnetically Induced Transparency (EIT) we find that the quantum interference, arising from the two optical transitions of the $Λ$ type three-level atomic ensembles, can be manipulated electrically. Numerical calculations show that the probe photon state can be well stored into the atomic spin state by sending an electric current pulse and retrieved with time-reverse symmetry by sending the other current pulse wit…
A novel method of multi-bit quantum optical data storage is presented, where the storage time can be lengthened far beyond the spin phase-decay time in a reversible spin inhomogeneous system excited by consecutive resonant Raman optical data pulses. The ultralong storage time is obtained by an optical population locking mechanism of modified rephasing process. This gives potentials to quantum repeaters utilizing quantum memories for long distance quantum communications, in which ultralong storage time plays a major role.
The technological possibilities of a realistic eavesdropper are discussed. Two eavesdropping strategies taking profit of multiphoton pulses in faint laser QKD are presented. We conclude that, as long as storage of Qubits is technically impossible, faint laser QKD is not limited by this security issue, but mostly by the detector noise.
A scheme for coherent manipulation of collective atomic states is developed such that total subradiant states, in which spontaneous emission is suppressed into all directions due to destructive interference between neighbor atoms, can be created in an extended atomic ensemble. The optimal conditions for creation of such states and suitability of them for quantum storage are discussed. It is shown that in order to achieve the maximum signal-to-noise ratio the shape of a light pulse to be stored and reconstructed using a homogeneously broadened absorbtion line of an atomic system should be a tim…
It is demonstrated that the properties of light stored in a four-level atomic system can be modified by an additional control interaction present during the storage stage. By choosing the pulse area of this interaction one can in particular continuously switch between two channels into which light is released.
Stopping and regenerating a pair of single-photon pulses at adjacent locations in coherently prepared Rydberg atomic ensembles are significantly affected by their effective interaction mediated by Rydberg excitations, and the similar processes can differ notably from the one exhibiting the common Rydberg blockade as with the stationary propagation of multi-photon light beams in the same medium. Based on the complete dynamics, we reveal the detailed features in such processes by finding how the profiles of the involved quantum fields evolve in various situations. The findings help to determine …
