We study the heat transfer between elastic solids with randomly rough surfaces. We include both the heat transfer from the area of real contact, and the heat transfer between the surfaces in the noncontact regions. We apply a recently developed contact mechanics theory, which accounts for the hierarchical nature of the contact between solids with roughness on many different length scales. For elastic contact, at the highest (atomic) resolution the area of real contact typically consists of atomic (nanometer) sized regions, and we discuss the implications of this for the heat transfer. For solids with very smooth surfaces, as is typical in many modern engineering applications, the interfacial separation in the non-contact regions will be very small, and for this case we show the importance of the radiative heat transfer associated with the evanescent electromagnetic waves which exist outside of all bodies.
When two elastic solids with randomly rough surfaces are brought in contact, a very inhomogeneous stress distribution sigma(x) will occur at the interface. Here I study the elastic energy and the correlation function <sigma(q)sigma(-q)>, where sigma(q) is the Fourier transform of sigma(x) and where <...> stands for ensemble average. I relate <sigma(q})sigma(-q)> to the elastic energy stored at the interface, and I show that for self affine fractal surfaces, quite generally <sigma(q)sigma(-q)> \sim q^{-(1+H)}, where H is the Hurst exponent of the self-affine fractal surface.
We study the average separation between an elastic solid and a hard solid with a nominal flat but randomly rough surface, as a function of the squeezing pressure. We present experimental results for a silicon rubber (PDMS) block with a flat surface squeezed against an asphalt road surface. The theory shows that an effective repulse pressure act between the surfaces of the form p proportional to exp(-u/u0), where u is the average separation between the surfaces and u0 a constant of order the root-mean-square roughness, in good agreement with the experimental results.
I show how flexoelectricity result in a fluctuating surface electric potential when elastic solids with random roughness are squeezed into contact. The flexoelectric potential may induce surface charge distributions and hence contribute to triboelectricity. Using the developed theory I analyze the Kelvin Force Microscopy data of Baytekin et al for the electric potential above a polydimethylsiloxane (PDMS) surface after it was peeled away from another PDMS surface
We study the distribution of interfacial separations P(u) at the contact region between two elastic solids with randomly rough surfaces. An analytical expression is derived for P(u) using Persson's theory of contact mechanics, and is compared to numerical solutions obtained using (a) a half-space method based on the Boussinesq equation, (b) a Green's function molecular dynamics technique and (c) smart-block classical molecular dynamics. Overall, we find good agreement between all the different approaches.
We present exact numerical results for the friction force and the contact area for a viscoelastic solid (rubber) in sliding contact with hard, randomly rough substrates. The rough surfaces are self-affine fractal with roughness over several decades in length scales. We calculate the contribution to the friction from the pulsating deformations induced by the substrate asperities. We also calculate how the area of real contact, $A(v,p) $, depends on the sliding speed $v$ and on the nominal contact pressure $p$, and we show how the contact area for any sliding speed can be obtained from a univers…
In this paper we investigate the loading and unloading behavior of soft solids in adhesive contact with randomly rough profiles. The roughness is assumed to be described by a self-affine fractal on a limited range of wave-vectors. A spectral method is exploited to generate such randomly rough surfaces. The results are statistically averaged, and the calculated contact area and applied load are shown as a function of the penetration, for loading and unloading conditions. We found that the combination of adhesion forces and roughness leads to a hysteresis loading-unloading loop. This shows that …
In this work, we numerically study the elastic contact between isotropic and anisotropic, rigid, randomly rough surfaces and linearly elastic counterfaces as well as the subsequent Reynolds flow through the gap between the two contacting solids. We find the percolation threshold to depend on the fluid-flow direction when the Peklenik number indicates anisotropy unless the system size clearly exceeds the roll-off wave length parallel to the easy flow direction. A critical contact area near 0.415 is confirmed. Heuristically corrected effective-medium treatments satisfactorily provide Reynolds fl…
The wetting properties of solid substrates with customary (i.e., macroscopic) random roughness are considered as a function of the microscopic contact angle of the wetting liquid and its partial pressure in the surrounding gas phase. Analytic expressions are derived which allow for any given lateral correlation function and height distribution of the roughness to calculate the wetting phase diagram, the adsorption isotherms, and to locate the percolation transition in the adsorbed liquid film. Most features turn out to depend only on a few key parameters of the roughness, which can be clearly …
I study fluid flow at the interface between elastic solids with randomly rough surfaces. I use the contact mechanics model of Persson to take into account the elastic interaction between the solid walls and the Bruggeman effective medium theory to account for the influence of the disorder on the fluid flow. I calculate the flow tensor which determines the pressure flow factor and, e.g., the leak-rate of static seals. I show how the perturbation treatment of Tripp can be extended to arbitrary order in the ratio between the root-mean-square roughness amplitude and the average interfacial surface…
We generalize the Persson contact mechanics and rubber friction theory to the case where both surfaces have surface roughness. The solids can be rigid, elastic or viscoelastic, and can be homogeneous or layered. We calculate the contact area, the viscoelastic contribution to the friction force, and the average interfacial separation as a function of the sliding speed and the nominal contact pressure. We illustrate the theory with numerical results for a rubber block sliding on a road surface. We find that with increasing sliding speed, the influence of the roughness on the rubber block decreas…
The viscous dissipation between rigid, randomly rough indenters and linearly elastic counter bodies sliding past them is investigated using Green's function molecular dynamics. The study encompasses a variety of models differing in the height spectra properties of the rigid indenter, in the viscoelasticity of the elastomer, and in their interaction. All systems reveal the expected damping linear in sliding velocity $v$ at small $v$ and a pronounced maximum at intermediate $v$. Persson's theory of rubber friction, which is adopted to the studied model systems, reflects all observed trends. Howe…
We derive a very simple and effective stickiness criterion for solids having random roughness using a new asymptotic theory, which we validate with that of Persson and Scaraggi and independent numerical experiments. Previous claims that stickiness may depend on small scale quantities such as rms slopes and/or curvatures, obtained by making oversimplified assumptions on the contact area geometry, are largely incorrect, as the truncation of the PSD spectrum of roughness at short wavelengths is irrelevant. We find stickiness is destroyed typically at roughness amplitudes up to three orders of mag…
I study how the contact area and the work of adhesion, between two elastic solids with randomly rough surfaces, depend on the relative humidity. The surfaces are assumed to be hydrophilic, and capillary bridges form at the interface between the solids. For elastically hard solids with relative smooth surfaces, the area of real contact and therefore also the sliding friction, are maximal when there is just enough liquid to fill out the interfacial space between the solids, which typically occurs for $d_{\rm K} \approx 3 h_{\rm rms}$, where $d_{\rm K}$ is the height of the capillary bridge and $…
The adhesive contact between elastic solids with randomly rough, self affine fractal surfaces is studied by molecular dynamics (MD) simulations. The interfacial binding energy obtained from the simulations of nominally flat and curved surfaces is compared with the predictions of the contact mechanics theory by Persson. Theoretical and simulation results agree rather well, and most of the differences observed can be attributed to finite size effects and to the long-range nature of the interaction between the atoms in the block and the substrate in the MD model, as compared to the analytical the…
In this supplementary materials section, we provide (i) additional information on the numerical simulations of the main work, (ii) the derivation of all prefactors in the analytical theory, and (iii) unpublished experiments of the contact stiffness of a polymer pressed against a rough substrate.
We report on measurements of the local friction law at a multi-contact interface formed between a smooth rubber and statistically rough glass lenses, under steady state friction. Using contact imaging, surface displacements are measured, and inverted to extract both distributions of frictional shear stress and contact pressure with a spatial resolution of about 10~$μ$m. For a glass surface whose topography is self-affine with a Gaussian height asperity distribution, the local frictional shear stress is found to vary strongly sub-linearly with the local contact pressure over the whole investiga…
We study the sliding of elastic solids in adhesive contact with flat and rough interfaces. We consider the dependence of the sliding friction on the elastic modulus of the solids. For elastically hard solids with planar surfaces with incommensurate surface structures we observe extremely low friction (superlubricity), which very abruptly increases as the elastic modulus decreases. We show that even a relatively small surface roughness may completely kill the superlubricity state.
Contact force--indentation depth measurements in contact experiments involving compliant materials, such as polymers and gels, show a hysteresis loop whose size depends on the maximum indentation depth. This depth-dependent hysteresis (DDH) is not explained by classical contact mechanics theories and was believed to be due to effects such as material viscoelasticity, plasticity, surface polymer interdigitation, and moisture, etc. It has been observed that the DDH energy loss initially increases and then decreases with roughness. A mechanics model based on the occurrence of adhesion and roughne…
We study frictionless and non-adhesive contact between elastic half-spaces with self-affine surfaces. Using a recently suggested corrective technique, we ensure an unprecedented accuracy in computation of the true contact area evolution under increasing pressure. This accuracy enables us to draw conclusions on the role of the surface's spectrum breadth (Nayak parameter) in the contact area evolution. We show that for a given normalized pressure, the contact area decreases logarithmically with the Nayak parameter. By linking the Nayak parameter with the Hurst exponent (or fractal dimension), we…
We study the sliding of elastic solids in adhesive contact with flat and rough interfaces. We consider the dependence of the sliding friction on the elastic modulus of the solids. For elastically hard solids with planar surfaces with incommensurate surface structures we observe extremely low friction (superlubricity), which very abruptly increases as the elastic modulus decreases. We show that even a relatively small surface roughness or a low concentration of adsorbates may completely kill the superlubricity state.
The total elastic stiffness of two contacting bodies with a microscopically rough interface has an interfacial contribution K that is entirely attributable to surface roughness. A quantitative understanding of K is important because it can dominate the total mechanical response and because it is proportional to the interfacial contributions to electrical and thermal conductivity in continuum theory. Numerical simulations of the dependence of K on the applied squeezing pressure p are presented for nominally flat elastic solids with a range of surface roughnesses. Over a wide range of p, K rises…
When two solids are squeezed together they will in general not make atomic contact everywhere within the nominal (or apparent) contact area. This fact has huge practical implications and must be considered in many technological applications. In this paper I briefly review basic theories of contact mechanics. I consider in detail a recently developed contact mechanics theory. I derive boundary conditions for the stress probability distribution function for elastic, elastoplastic and adhesive contact between solids and present numerical results illustrating some aspects of the theory. I analyze …
Friction in static and sliding contact of rough surfaces is important in numerous physical phenomena. We seek to understand macroscopically observed static and sliding contact behavior as the collective response of a large number of microscopic asperities. We develop an efficient numerical framework that can be used to investigate how the macroscopic response of multiple frictional contacts depends on long-range elastic interactions, different constitutive assumptions about the deforming contacts and their local shear resistance, and surface roughness. We approximate the contact between two ro…
We study experimentally and theoretically the equilibrium adhesive contact between a smooth glass lens and a rough rubber surface textured with spherical microasperities with controlled height and spatial distributions. Measurements of the real contact area $A$ versus load $P$ are performed under compression by imaging the light transmitted at the microcontacts. $A(P)$ is found to be non-linear and to strongly depend on the standard deviation of the asperity height distribution. Experimental results are discussed in the light of a discrete version of Fuller and Tabor's (FT) original model (\te…
When adhesive elastomeric materials slide over hard rough surfaces at low velocities, there are two primary dissipative mechanisms that control how friction changes with sliding velocity: viscoelastic dissipation and adhesive dissipation. To distinguish the contribution of these dissipative mechanisms we have measured frictional shear stresses for crosslinked polydimethylsiloxane (PDMS) on three different rough surfaces of similar surface chemistry across nearly six decades of sliding velocity. The results show that the observed friction is dominated by adhesive dissipation, rather than viscoe…
Field-theoretical approach to estimate mean gap and gap distribution in randomly rough surface contact mechanics
Yangzhou University（扬州大学）；Institute of Mechanics, Chinese Academy of Sciences（中国科学院力学研究所）；University of Chinese Academy of Sciences（中国科学院大学）；Hefei University of Technology（合肥工业大学）
Flash temperature in sliding contacts: comparing theory with experiments
Peter Grünberg Institute (PGI-1), Forschungszentrum Jülich（于利希研究中心）；State Key Laboratory of Solid Lubrication, Lanzhou Institute of Chemical Physics, Chinese Academy of Sciences（中国科学院兰州化学物理研究所固体润滑国家重点实验室）；MultiscaleConsulting（多尺度咨询公司）
We study the influence of surface roughness on the adhesion of elastic solids. Most real surfaces have roughness on many different length scales, and this fact is taken into account in our analysis. We consider in detail the case when the surface roughness can be described as a self affine fractal, and show that when the fractal dimension D_f >2.5, the adhesion force may vanish, or be at least strongly reduced. We consider the block-substrate pull-off force as a function of roughness, and find a partial detachment transition preceding a full detachment one. The theory is in good qualitative ag…
The dynamic of contact formation between soft materials immersed in a fluid is accompanied by fluid drainage and elastic deformation. As a result, controlling the coupling between lubrication pressure and elasticity provides strategies to design materials with reversible and dynamic adhesion to wet or flooded surfaces. We characterize the elastic deformation of a soft coating with nanometer-scale roughness as it approaches and contacts a rigid surface in a fluid environment. The lubrication pressure during the approach causes elastic deformation and prevents contact formation. We observe defor…
We systematically check explicit and implicit assumptions of Persson's contact mechanics theory. It casts the evolution of the pressure distribution ${\rm Pr}(p)$ with increasing resolution of surface roughness as a diffusive process, in which resolution plays the role of time. The tested key assumptions of the theory are: (a) the diffusion coefficient is independent of pressure $p$, (b) the diffusion process is drift-free at any value of $p$, (c) the point $p=0$ acts as an absorbing barrier, i.e., once a point falls out of contact, it never reenters again, (d) the Fourier component of the ela…
We discuss how surface roughness influence the adhesion between elastic solids. We introduce a Tabor number which depends on the length scale or magnification, and which gives information about the nature of the adhesion at different length scales. We consider two limiting cases relevant for (a) elastically hard solids with weak adhesive interaction (DMT-limit) and (b) elastically soft solids or strong adhesive interaction (JKR-limit). For the former cases we study the nature of the adhesion using different adhesive force laws ($F\sim u^{-n}$, $n=1.5-4$, where $u$ is the wall-wall separation).…
We study the fluid squeeze-out from the interface between an elastic solid with a flat surface and a rigid solid with a randomly rough surface. As an application we discuss fluid squeeze-out between a tire tread block and a road surface. Some implications for the leakage of seals are discussed, and experimental data are presented to test the theory.
The description of elastic, nonadhesive contacts between solids with self-affine surface roughness seems to necessitate knowledge of a large number of parameters. However, few parameters suffice to determine many important interfacial properties as we show by combining dimensional analysis with numerical simulations. This insight is used to deduce the pressure dependence of the relative contact area and the mean interfacial separation $Δ\bar{u}$ and to present the results in a compact form. Given a proper unit choice for pressure $p$, i.e., effective modulus $E^*$ times the root-mean-square gr…
The effect of rough walls on the phase behaviour of a confined liquid crystal (LC) fluid is studied using constant pressure Monte Carlo simulations. The LC is modelled as a fluid of soft ellipsoidal molecules and the rough walls are represented as a hard wall with a number of molecules randomly embedded in them. It is found that the isotropic-nematic (IN) transition is shifted to higher pressures for rougher walls.
Adhesion hysteresis can be caused by elastic instabilities that are triggered by surface roughness or chemical heterogeneity. However, the role of these instabilities in adhesion hysteresis remains poorly understood because we lack theoretical and numerical models accounting for realistic roughness. Our work focuses on the adhesion of soft elastic spheres with low roughness or weak heterogeneity, where the indentation process can be described as a Griffith-like propagation of a nearly circular external crack. We discuss how to describe the contact of spheres with chemical heterogeneity that le…
The detachment of material in an adhesive wear process is driven by a fracture mechanism which is controlled by a critical length-scale. Previous efforts in multi-asperity wear modeling have applied this microscopic process to rough elastic contact. However, experimental data shows that the assumption of purely elastic deformation at rough contact interfaces is unrealistic, and that asperities in contact must deform plastically to accommodate the large contact stresses. We therefore investigate the consequences of plastic deformation on the macro-scale wear response using novel elastoplastic c…
We report on normal contact and friction measurements of model multicontact interfaces formed between smooth surfaces and substrates textured with a statistical distribution of spherical micro-asperities. Contacts are either formed between a rigid textured lens and a smooth rubber, or a flat textured rubber and a smooth rigid lens. Measurements of the real area of contact $A$ versus normal load $P$ are performed by imaging the light transmitted at the microcontacts. For both interfaces, $A(P)$ is found to be sub-linear with a power law behavior. Comparison to two multi-asperity contact models,…
Nematic liquid crystals at rough and fluctuating interfaces are analyzed within the Frank elastic theory and the Landau-de Gennes theory. We study specifically interfaces that locally favor planar anchoring. In the first part we reconsider the phenomenon of Berreman anchoring on fixed rough surfaces, and derive new simple expressions for the corresponding azimuthal anchoring energy. Surprisingly, we find that for strongly aligning surfaces, it depends only on the geometrical surface anisotropy and the bulk elastic constants, and not on the precise values of the chemical surface parameters. In …
We present a numerical model for the prediction of the rough contact mechanics of a viscoelastic block, with graded rheology, in steady sliding contact with a randomly rough rigid surface. In particular, we derive the effective surface response of a stepwise or continuously-graded block in the Fourier domain, which is then embedded in a Fourier-based residuals molecular dynamic formulation of the contact mechanics. Finally we discuss on the role of small-scale wavelengths on rubber friction and contact area, and we demonstrate that the rough contact mechanics exhibits effective interface prope…
Adhesive peeling of a thin elastic film from a substrate is a classic problem in mechanics. However, many of the investigations on this topic to date have focused on peeling from substrates with flat surfaces. In this paper, we study the problem of peeling an elastic thin film from a rigid substrate that has periodic surface undulations. We allow for contact between the detached part of the film with the substrate. We give analytical results for computing the equilibrium force given the true peeling angle, which is the angle at which the detached part of the film leaves the substrate. When the…
We study the time dependency of the (average) interfacial separation between an elastic solid with a flat surface and a rigid solid with a randomly rough surface, squeezed together in a fluid. We use an analytical theory describing the fluid flow factors, based on the Persson contact mechanics theory and the Bruggeman effective medium theory, to calculate the removal of the fluid from the contacting interface of the two solids. In order to test this approach, we have performed simple squeeze-out experiments. The experimental results are compared to the theory predictions.
We study the frictional behavior of both elastic and viscoelastic thin coatings bonded to a seemingly rigid substrate and sliding against a rough profile in the presence of Coulomb friction at the interface. The aim is to explore the effect of the coupling between the normal and tangential displacement fields arising from the finiteness of the material thickness and to quantify the contribution this can have on energy losses. We found that, due to normal-tangential coupling, asymmetric contacts and consequently additional friction are observed even for purely elastic layers, indeed associated …
The spontaneous formation of double helices for filaments under torsion is common and significant. For example, the research on the supercoiling of DNA is helpful for understanding the replication and transcription of DNA. Similar double helices can appear in polymer chains, carbon nanotube yarns, cables, telephone wires and so forth. We noticed that non-uniform double helices can be produced due to the surface friction induced by the self-contact. Therefore an ideal model was presented to investigate the formation of double helices for elastic rods under torque. A general equilibrium conditio…
On the flash temperature in sliding rubber contacts
Peter Grünberg Institute (PGI-1), Forschungszentrum Jülich（于利希研究中心）；Lanzhou Institute of Chemical Physics, Chinese Academy of Sciences（中国科学院兰州化学物理研究所）；MultiscaleConsulting（多尺度咨询公司）
Contact mechanics-based models for the friction of nominally flat rough surfaces have not been able to adequately capture certain key experimentally observed phenomenona, such as the transition from a static friction peak to a lower level of sliding friction and the shear-induced contact area reduction that has been observed in the pre-sliding regime especially for soft materials. Here, we propose a statistical model based on physically-rooted contact mechanics laws describing the micromechanics of individual junctions. The model considers the quasi-static tangential loading, up to full slidin…
I discuss fluid flow at the interface between solids with anisotropic roughness. I show that for randomly rough surfaces with anisotropic roughness, the contact area percolate at the same relative contact area as for isotropic roughness, and that the Bruggeman effective medium theory and the critical junction theory give nearly the same results for the fluid flow conductivity. This shows that, in most cases, the surface roughness observed at high magnification is irrelevant for fluid flow problems such as the leakage of static seals, and fluid squeeze-out.
We report on the elastic contact between a spherical lens and a patterned substrate, composed of an hexagonal lattice of cylindrical pillars. The stress field and the size of the contact area are obtained by means of numerical methods (discrete Green's function superposition and iterative bisection-like methods). For small indentations, a transition from a Hertzian to a Boussinesq-Cerruti-like behavior is observed when the surface fraction of the substrate that is covered by pillars is increased. In particular, we present a master curve defined by two dimensionless parameters, which allows to …
We study fluid flow at the interfaces between elastic solids with randomly rough, self-affine surfaces. We show by numerical simulation that elastic deformation lowers the relative contact area at which contact patches percolate in comparison to traditional approaches to seals. Elastic deformation also suppresses leakage through contacts even far away from the percolation threshold. Reliable estimates for leakage can be obtained by combining Persson's contact mechanics theory with a slightly modified version of Bruggeman's effective-medium solution of the Reynolds equation.
We have employed a numerical procedure to analyze the adhesive contact between a soft elastic layer and a rough rigid substrate. The solution of the problem is obtained by calculating the Green's function which links the pressure distribution to the normal displacements at the interface. The problem is then formulated in the form of a Fredholm integral equation of the first kind with a logarithmic kernel, and the boundaries of the contact area are calculated by requiring that the energy of the system is stationary. The methodology has been employed to study the adhesive contact between an elas…
A numerical analysis of mechanical frictionless contact between rough self-affine elastic manifolds was carried out. It is shown that the lower cutoff wavenumber in surface spectra is a key parameter controlling the representativity of the numerical model. Using this notion we demonstrate that for representative surfaces the evolution of the real contact area with load is universal and independent of the Hurst roughness exponent. By introducing a universal law containing three constants, we extend the study of this evolution beyond the limit of infinitesimal area fractions.
We report results of investigations of a high-speed drainage of thin aqueous films squeezed between randomly nanorough surfaces. A significant decrease in hydrodynamic resistance force as compared with predicted by Taylor's equation is observed. However, this reduction in force does not represents the slippage. The measured force is exactly the same as that between equivalent smooth surfaces obeying no-slip boundary conditions, but located at the intermediate position between peaks and valleys of asperities. The shift in hydrodynamic thickness is shown to be independent on the separation and/o…
We study the nominal (ensemble averaged) contact pressure $p(x)$ acting on a cylinder squeezed in contact with an elastic half-space with random surface roughness. The contact pressure is Hertzian-like for $α< 0.01$ and Gaussian-like for $α> 10$, where the dimensionless parameter $α= h_{\rm rms}/δ$ is the ratio between the root-mean-square roughness amplitude and the penetration for the smooth surfaces case (Hertz contact).
We report results of lattice Boltzmann simulations of a high-speed drainage of liquid films squeezed between a smooth sphere and a randomly rough plane. A significant decrease in the hydrodynamic resistance force as compared with that predicted for two smooth surfaces is observed. However, this force reduction does not represent slippage. The computed force is exactly the same as that between equivalent smooth surfaces obeying no-slip boundary conditions, but located at an intermediate position between peaks and valleys of asperities. The shift in hydrodynamic thickness is shown to depend on t…
