我们已经建立了一个气相氩离子化检测器，用于测量小的核反冲能（< 10 keVee）。在本文中，我们描述了探测器对X射线和伽马校准源的响应，包括脉冲形状分析、软件触发、气体含量优化以及信号的能量和位置依赖性。我们比较我们的实验结果与模拟使用5.9千电子伏的X射线源，以及更高能量的伽马源高达1332千电子伏。最后，我们描述的检测器，DAQ，和软件设置优化的测量气态氩中的低能核淬灭因子。这项工作是在美国能源部的主持下由劳伦斯利弗莫尔国家实验室进行的，部分根据合同W-7405-Eng-48，部分根据合同DE-AC 52 - 07 NA 27344。由整个实验室LDRD资助。LLNL-JRNL-415990-草案。
英文摘要：
We have built a gas-phase argon ionization detector to measure small nuclear recoil energies (< 10 keVee). In this paper, we describe the detector response to X-ray and gamma calibration sources, including analysis of pulse shapes, software triggers, optimization of gas content, and energy- and position-dependence of the signal. We compare our experimental results against simulation using a 5.9-keV X-ray source, as well as higher-energy gamma sources up to 1332 keV. We conclude with a description of the detector, DAQ, and software settings optimized for a measurement of the low-energy nuclear quenching factor in gaseous argon. This work was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory in part under Contract W-7405-Eng-48 and in part under Contract DE-AC52-07NA27344. Funded by Lab-wide LDRD. LLNL-JRNL-415990-DRAFT.
Xenon-doped liquid argon has been proposed as a good alternative to pure liquid argon in scintillation detectors. In this study, we report on the measurement of the time profile of scintillation light emitted from xenon-doped liquid argon with molar concentrations up to 1600 ppm. A compact setup has been developed for this study, with silicon photomultiplier (SiPM) as the photosensor and $^{210}\mathrm{Po}$ and $^{90}\mathrm{Sr}$ as scintillation sources. An effective model based on the de-excitation processes has been developed to describe the data. The results show that xenon-doped liquid ar…
The use of xenon-doped liquid argon is a promising alternative for large pure liquid-argon TPCs. Not only xenon-doped liquid argon enhances the light production, mitigating the possible suppression due to impurities, but also it increases the wavelength of the scintillation light, enlarging the effective Rayleigh scattering length and improving the detection uniformity. ProtoDUNE Dual-Phase is a 300-ton active volume LAr TPC, a prototype for the Deep Underground Neutrino Experiment (DUNE), a dual-site experiment for long-baseline neutrino oscillation studies, neutrino astrophysics and nucleon …
After a short review of previous attempts to observe and measure the near-infrared scintillation in liquid argon, we present new results obtained with NIR, a dedicated cryostat at the Fermilab Proton Assembly Building (PAB). The new results give confidence that the near-infrared light can be used as the much needed light signal in large liquid argon time projection chambers.11 pages,
ProtoDUNE-DP is a 6x6x6 m3 liquid argon time-projection-chamber (LArTPC) operated at the Neutrino Platform at CERN in 2019-2020 as a prototype of the DUNE Far Detector. DUNE is a dual-site experiment for long-baseline neutrino oscillation studies, neutrino astrophysics and nucleon decay searches. The light signal in these detectors is crucial to provide precise timing capabilities. In ProtoDUNE-DP, scintillation light produced by cosmic muons inthe LArTPC is collected by the photomultiplier tubes (PMTs) placed up to 7 m away from the point of interaction. The scintillation light production and…
In this paper we describe the performance of a light detector for Ar scintillation light made of wavelength-shifting (WLS) fibers connected to Silicon-Photomultipliers (SiPM). The setup was conceived to be used as anti-Compton veto for high purity germanium (HPGe) detectors operated directly in liquid Argon (LAr). Background suppression efficiencies for different radioactive sources were measured in a test cryostat with about 800 kg LAr. This work was part of the R\&D effort for the GERDA experiment.
We present a measurement of scintillation efficiency for a few tens of keV nuclear recoils (NR) with a liquid argon time projection chamber under electric fields ranging from $0$ to $3\ {\rm kV/cm}$. The calibration data are taken with $^{252}{\rm Cf}$ radioactive source. Observed scintillation and electroluminescence spectra are simultaneously fit with spectra derived from Geant4-based Monte Carlo simulation and an NR model. The scintillation efficiency extracted from the fit is reported as a function of recoil energy and electric field. This result can be used for designing the detector and …
A two-phase argon detector has high discrimination power between electron recoil and nuclear recoil events based on the pulse shape discrimination and the ionization/scintillation ratio (S2/S1). This character is very suitable for the dark matter search to establish the low background experiment. However, the basic properties of S2/S1 of argon are not well known, as compared with xenon. We report the evaluation of S2/S1 properties with a two-phase detector at drift-fields of 0.2-3.0 kV/cm. Finally, the discrimination power against electron recoil background of S2/S1 is discussed.
Since the 1970s it has been known that noble gases scintillate in the near infrared (NIR) region of the spectrum (0.7 $μ$m < $λ$; < 1.5$μ$m). More controversial has been the question of the NIR light yield for condensed noble gases. We first present the motivation for using the NIR scintillation in liquid argon detectors, then briefly review early as well as more recent efforts and finally show encouraging preliminary results of a test performed at Fermilab.
We have measured the properties of scintillation light in liquid argon doped with xenon concentrations from 165 ppm to 10,010 ppm using a $^{22}$Na source. The energy transfer processes in the xenon-doped liquid argon are discussed in detail, and a new waveform model is established and used to fit the average waveform. The time profile of the scintillation photon in the xenon-doped liquid argon and of the TPB emission are presented. The quantities of xenon-doped are controlled by a Mass Flow Controller which is calibrated via a Redusial Gas Analyzer to ensure that the xenon concentration is ac…
The propagation velocity of scintillation light in liquid argon $v_{g}$ at $λ\sim 128$~nm wavelength, has been measured for the first time in a dedicated experimental setup at CERN.\\ The obtained result $\frac{1}{v_{g}} = 7.46 \pm 0.08$~ns/m , is then used to derive the value of the refractive index (n) and the Rayleigh scattering length ($\mathcal{L}$) for liquid argon in the VUV region. For $λ= 128$~nm we found $n= 1.358 \pm 0.003$ and $\mathcal{L}= 99.1 \pm 2.3$~cm. The measured values are of interest for a variety of experiments searching for rare events like neutrino and dark matter inte…
Liquid argon is being employed as a detector medium in neutrino physics and Dark Matter searches. A recent push to expand the applications of scintillation light in Liquid Argon Time Projection Chamber neutrino detectors has necessitated the development of advanced methods of simulating this light. The presently available methods tend to be prohibitively slow or imprecise due to the combination of detector size and the amount of energy deposited by neutrino beam interactions. In this work we present a semi-analytical model to predict the quantity of argon scintillation light observed by a ligh…
Large volume Liquid Argon Time Projection Chambers (LAr-TPC) are used and proposed for neutrino physics and rare event search. Most of these detectors make use of the scintillation light of liquid argon for trigger purposes. Two different approaches can be adopted to provide these detectors with an effective trigger system, relying upon analog or digital processing of signal coming from photodetectors, like photomultiplier tubes or silicon photomultipliers. Each method presents advantages and drawbacks, so the implementation of a hybrid solution can benefit from both approaches. To this purpos…
The Deep Underground Neutrino Experiment (DUNE) is a leading-edge experiment for long-baseline neutrino oscillation studies, neutrino astrophysics and nucleon decay searches. ProtoDUNE-Dual Phase (DP) is a 6x6x6 m$^3$ liquid argon time-projection-chamber (LArTPC) operated at the CERN Neutrino Platform in 2019-2020 as a prototype of the DUNE Far Detector. In ProtoDUNE-DP, the scintillation and electroluminescence light produced by cosmic muons in the LArTPC is collected by photomultiplier tubes placed up to 7 m away from the ionizing track. In this paper, we present the performance of the Proto…
Liquid argon is used as active medium in a variety of neutrino and Dark Matter experiments thanks to its excellent properties of charge yield and transport and as a scintillator. Liquid argon scintillation photons are emitted in a narrow band of 10~nm centered around 127 nm and with a characteristic time profile made by two components originated by the decay of the lowest lying singlet and triplet state of the excimer Ar$_2^*$ to the dissociative ground state. A model is proposed which takes into account the quenching of the long lived triplet states through the self-interaction with other tri…
Scintillation light generated as charged particles traverse large liquid argon detectors adds valuable information to studies of weakly-interacting particles. This paper uses both laboratory measurements and cosmic ray data from the Blanche dewar facility at Fermilab to characterize the efficiency of the photon detector technology developed at Indiana University for the single phase far detector of DUNE. The efficiency of this technology was found to be 0.48% at the readout end when the detector components were characterized with laboratory measurements. A second determination of the efficienc…
Neutron veto detector based on liquid scintillator containing hydrogen atoms is an integral part of any underground experiment for dark matter search. So far, a flammable mixture of liquid hydrocarbons was used as a liquid scintillator in such detectors. A safe alternative might be a liquid scintillator based on liquid argon doped with methane. In this work, we have studied the primary scintillations in pure liquid argon and its mixtures with methane, the CH4 content varying from 100 ppm to 5%. The primary scintillations have for the first time been observed in liquid argon doped with methane,…
We have measured the scintillation and ionization yield of recoiling nuclei in liquid argon as a function of applied electric field by exposing a dual-phase liquid argon time projection chamber (LAr-TPC) to a low energy pulsed narrow band neutron beam produced at the Notre Dame Institute for Structure and Nuclear Astrophysics. Liquid scintillation counters were arranged to detect and identify neutrons scattered in the TPC and to select the energy of the recoiling nuclei. We report measurements of the scintillation yields for nuclear recoils with energies from 10.3 to 57.3 keV and for median ap…
Liquid argon (LAr) is a common choice as detection medium in particle physics and rare-event searches. Challenges of LAr scintillation light detection include its short emission wavelength, long scintillation time and short attenuation length. The addition of small amounts of xenon to LAr is known to improve the scintillation and optical properties. We present a characterization campaign on xenon-doped liquid argon (XeDLAr) with target xenon concentrations ranging from 0 to 300 ppm by mass encompassing the measurement of the photoelectron yield $Y$ , effective triplet lifetime $τ_3$ and effect…
We performed a time-resolved spectroscopic study of the VUV/UV argon scintillation as a function of pressure and electric field, by means of a wavelength sensitive detector operated with different radioactive sources. Our work conveys new evidence of distinctive features of the argon light which are in contrast with the general assumption that, for particle detection purposes, the scintillation can be considered to be largely monochromatic at 128 nm (second continuum). The wavelength and the time-resolved analysis of the photon emission reveal that the dominant component of the argon scintilla…
The scintillation yield for recoil Ar ions of 5 to 250 keV energy in liquid argon have been evaluated for direct dark matter searches. Lindhard theory is taken for estimating nuclear quenching. A theoretical model based on a biexcitonic diffusion-reaction mechanism is performed for electronic (scintillation) quenching. The electronic LET (linear energy transfer) is evaluated and used to obtain the initial track structure due to recoil Ar ions. The results are compared with experimental values reported for nuclear recoils from neutrons. The behavior of scintillation and ionization on the field …
Measuring the scintillation light in noble gases is an important detection technique in particle physics. Numerous rare event searches like neutrino beam experiments, neutrino-less double beta-decay, and dark matter searches use argon-based detectors. In liquid argon, the light yield can be enhanced by the addition of a small quantity of xenon, where $\sim 10 - 1000$ ppm are added. The general enhancement mechanism and its pathway via an energy transfer between argon and xenon excimers is well known, however the importance of absorption of argon excimer emission by atomic xenon has not been fu…
We report on a measurement of the attenuation length for the scintillation light in the tonne size liquid argon target of the ArDM dark matter experiment. The data was recorded in the first underground operation of the experiment in single-phase operational mode. The results were achieved by comparing the light yield spectra from 39-Ar and 83m-Kr to a description of the ArDM setup with a model of full light ray tracing. A relatively low value close to 0.5 m was found for the attenuation length of the liquid argon bulk to its own scintillation light. We interpret this result as a presence of op…
Experiments searching for weak interacting massive particles with noble gases such as liquid argon require very low detection thresholds for nuclear recoils. A determination of the scintillation efficiency is crucial to quantify the response of the detector at low energy. We report the results obtained with a small liquid argon cell using a monoenergetic neutron beam produced by a deuterium-deuterium fusion source. The light yield relative to electrons was measured for six argon recoil energies between 11 and 120 keV at zero electric drift field.
This paper reports the results of an experiment to directly measure the time-resolved scintillation signal from the passage of cosmic-ray muons through liquid argon. Scintillation light from these muons is of value to studies of weakly-interacting particles in neutrino experiments and dark matter searches. The experiment was carried out at the TallBo dewar facility at Fermilab using prototype light guide detectors and electronics developed for the Deep Underground Neutrino Experiment. Two models are presented for the time structure of the scintillation light, a phenomenological model and a com…
A particle detection system that exploits the scintillation light produced by ionizing particles in liquid argon (LAr) has been assembled at CERN. The system is based on 10 large-area photomultiplier tubes (PMT) immersed in a 1500-liter dewar filled with liquid argon and equipped with an extendible feed-through and mechanical support for an alpha source (241Am). The position of the source can be changed with respect to the PMT plane in vertical and horizontal directions. Arrays of silicon photomultiplier (SiPM) photodetectors, integrated in the source support, are used for the data acquisition…
Scintillation light is used in liquid argon (LAr) neutrino detectors to provide a trigger signal, veto information against cosmic rays, and absolute event timing. In this work, we discuss additional opportunities offered by detectors with enhanced sensitivity to scintillation light, that is with light collection efficiencies of about $10^{-3}$. We focus on two key detector performance indicators for neutrino oscillation physics: calorimetric neutrino energy reconstruction and neutrino/antineutrino separation in a non-magnetized detector. Our results are based on detailed simulations, with neut…
A new type of the Multi-Pixel Photon Counter (MPPC), sensitive to Vacuum Ultra-Violet (VUV) light (wavelength λ < 150 nm), is recently developed and produced by Hamamatsu Photonics K.K. The basic properties of the new MPPC are measured at cryogenic facility of Waseda university using liquid nitrogen. Temperature dependence of breakdown voltage, capacitance, and dark count rate of the MPPC are also evaluated. In addition, the absolute photon detection efficiency (PDE) for liquid argon (LAr) scintillation light (λ = 128 nm) is estimated to be about 7% with uncertainty of 2% by using 241 Am α-ray…
The possible use of a Spherical Proportional Counter for the search of neutrinoless double beta decay is investigated in the R2D2 R&D project. Dual charge and scintillation light readout may improve the detector performance. Tests were carried out with pure argon at 1.1 bar using a 6x6 mm2 silicon photomultiplier. Scintillation light was used for the first time to trigger in a spherical proportional counter. The measured drift time is in excellent agreement with the expectations from simulations. Furthermore the light signal emitted during the avalanche development exhibits features that could…
Detection of light signals is crucial to a wide range of particle detectors. In particular, efficient detection of vacuum ultraviolet (VUV) light will provide new opportunities for some novel detectors currently being developed, but is technically challenging. In this article, we characterized the performance of Hamamatsu VUV4 silicon photomultipliers (SiPMs) for detecting VUV argon scintillation light without wavelength shifting. Using a customized cryogenic amplifier design, we operated two models of VUV4 SiPMs inside liquid argon and thoroughly examined their direct sensitivities to liquid …
The spectral and temporal light emission properties of liquid argon have been studied in the context of its use in large liquid rare-gas detectors for detecting Dark Matter particles in astronomy. A table-top setup has been developed. Continuous and pulsed low energy electron beam excitation is used to stimulate light emission. A spectral range from 110 to 1000 nm in wavelength is covered by the detection system with a time resolution on the order of 1 ns.
Presented here are first tests of a Gaseous Photomultiplier based on a cascade of Thick GEM structures intended for gamma-ray position reconstruction in liquid Argon. The detector has a MgF$_2$ window, transparent to VUV light, and a CsI photocathode deposited on the first THGEM. A gain of $8\cdot10^{5}$ per photoelectron and $\sim100\%$ photoelectron collection efficiency are measured at stable operation settings. The excellent position resolution capabilities of the detector (better than 100 $μ$m) at 100 kHz readout rate, is demonstrated at room temperature. Structural integrity tests of the…
A spectroscopic study of liquid argon from the vacuum ultraviolet at 110 nm to 1000 nm is presented. Excitation was performed using continuous and pulsed 12 keV electron beams. The emission is dominated by the analogue of the so called 2nd excimer continuum. Various additional emission features were found. The time structure of the light emission has been measured for a set of well defined wavelength positions. The results help to interpret literature data in the context of liquid rare gas detectors in which the wavelength information is lost due to the use of wavelength shifters.
TetraPhenyl Butadiene is the wavelength shifter most widely used in combination with liquid Argon. The latter emits scintillation photons with a wavelength of 127 nm that need to be downshifted to be detected by photomultipliers with glass or quartz windows. TetraPhenyl Butadiene has been demonstrated to have an extremely high conversion efficiency, possibly higher than 100 % for 127 nm photons, while there is no precise information about the time dependence of its emission. It is usually assumed to be exponentially decaying with a characteristic time of the order of one ns, as an extrapolatio…
Decays of radioisotopes on inner detector surfaces can pose a major background concern for the direct detection of dark matter. While these backgrounds are conventionally mitigated with position cuts, these cuts reduce the exposure of the detector by decreasing the sensitive mass, and uncertainty in position determination may make it impossible to adequately remove such events in certain detectors. In this paper, we provide a new technique for substantially reducing these surface backgrounds in liquid argon (LAr) detectors, independent of position cuts. These detectors typically use a coating …
LArGe is a GERDA low-background test facility to study novel background suppression methods in a low-background environment, for future application in the GERDA experiment. Similar to GERDA, LArGe operates bare germanium detectors submersed into liquid argon (1 m$^3$, 1.4 tons), which in addition is instrumented with photomultipliers to detect argon scintillation light. The scintillation signals are used in anti-coincidence with the germanium detectors to effectively suppress background events that deposit energy in the liquid argon. The background suppression efficiency was studied in combina…
A liquid argon time projection chamber, constructed for the Argon Response to Ionization and Scintillation (ARIS) experiment, has been exposed to the highly collimated and quasi-monoenergetic LICORNE neutron beam at the Institute de Physique Nuclaire Orsay in order to study the scintillation response to nuclear and electronic recoils. An array of liquid scintillator detectors, arranged around the apparatus, tag scattered neutrons and select nuclear recoil energies in the [7, 120] keV energy range. The relative scintillation efficiency of nuclear recoils was measured to high precision at null f…
We measure the liquid argon scintillation response to electronic recoils in the energy range of $2.82$ to $1274.6~{\rm keV}$ at null electric field. The single-phase detector with a large optical coverage used in this measurement yields $12.8 \pm 0.3 ~ (11.2 \pm 0.3)~{\rm photoelectron/keV}$ for $511.0$-${\rm keV}$ $γ$-ray events based on a photomultiplier tube single photoelectron response modeling with a Gaussian plus an additional exponential term (with only a Gaussian term). It is exposed to a variety of calibration sources such as $^{22}{\rm Na}$ and $^{241}{\rm Am}$ $γ$-ray emitters, and…
The GERDA experiment searches for the neutrinoless double beta ($0νββ$) decay in $^{76}$Ge in order to probe whether the neutrino is a Majorana particle and to shed light on the neutrino mass ordering. For investigating such a rare decay it is necessary to minimize the background of the experiment. In Phase II of the GERDA experiment the scintillation light of liquid argon (LAr) is used as an additional background veto. In order to estimate the efficiency of such a LAr veto it has to be known how far the scintillation light, which peaks at 128 nm, can travel within the LAr. A dedicated setup w…
Large liquid argon detectors have become widely used in low rate experiments, including dark matter and neutrino research. However, the optical properties of liquid argon are not well understood at the large scales relevant for current and near-future detectors.The index of refraction of liquid argon at the scin- tillation wavelength has not been measured, and current Rayleigh scattering length calculations disagree with measurements. Furthermore, the Rayleigh scattering length and index of refraction of solid argon and solid xenon at their scintillation wavelengths have not been previously me…
In this investigation the response to the scintillation light generated by through-going cosmic muons in liquid argon (LAr) was measured by two light guide technologies and two readout technologies after five weeks of running in the TallBo dewar at Fermilab. The response was remeasured after the dewar was drained of LAr, refilled, and then run again for an additional four weeks. After the dewar was refilled, there was clear evidence that the scintillation signal had dropped significantly. The two light guide technologies were developed at Indiana University and MIT/Fermilab. The two readout te…
