Magnetic metamaterials consist of magnetic resonators smaller in size than their excitation wavelengths. Their unique electromagnetic properties were characterized by the effective media theory at the early stage. However, the effective media model does not take into account the interactions between magnetic elements; thus, the effective properties of bulk metamaterials are the result of the "averaged effect" of many uncoupled resonators. In recent years, it has been shown that the interaction between magnetic resonators could lead to some novel phenomena and interesting applications that do not exist in conventional uncoupled metamaterials. In this paper, we will give a review of recent developments in magnetic plasmonics arising from the coupling effect in metamaterials. For the system composed of several identical magnetic resonators, the coupling between these units produces multiple discrete resonance modes due to hybridization. In the case of a system comprising an infinite number of magnetic elements, these multiple discrete resonances can be extended to form a continuous frequency band by strong coupling. This kind of broadband and tunable magnetic metamaterial may have interesting applications. Many novel metamaterials and nanophotonic devices could be developed from coupled resonator systems in the future.
Using interplay between surface plasmons and metamaterials, we propose a new technique for novel metamaterial designs. We show that surface plasmons existing on thin metal surfaces can be used to "drive" non-resonant structures in their vicinity to provide new types of electric and magnetic resonators. These resonators strictly adhere to surface plasmon dispersion of the host metal film. The operating frequency of the resultant metamaterials can be scaled to extremely high frequencies, otherwise not possible with conventional split-ring-resonator-based designs. Our approach opens new possibili…
We demonstrate polarization controlled absorption in plasmonic bimetallic metamaterials. We fabricate and experimentally characterize Au/Ni ring resonator arrays, where by varying the wavelength and polarization of the incident wave, local electromagnetic fields and dissipation can be suppressed or enhanced in the Au and Ni areas of the rings.
A terahertz metamaterial consisting of radiative slot antennas and subradiant complementary split-ring resonators exhibits plasmon induced opacity in a narrow spectral range due to the destructive interference between the bright and dark modes of the coupled oscillators. Femtosecond optical excitations instantly quench the mode coupling and plasmon oscillations, injecting photocarriers into the metamaterial. The plasmon resonances in the coupled metamaterial are transiently restored by intense terahertz pulses. The strong terahertz fields induce intervalley scattering and interband tunneling o…
We report that hybridizing semiconductor quantum dots with plasmonic metamaterial leads to a multi-fold intensity increase and narrowing of their photoluminescence spectrum. The luminescence enhancement is a clear manifestation of the cavity quantum electrodynamics Purcell effect that can be controlled by the metamaterial's design. This observation is an essential step towards understanding loss compensation in metamaterials with gain media and for developing metamaterial-enhanced gain media.
We theoretically investigate the optical properties of parity-time (PT)-symmetric three dimensional metamaterials composed of strongly-coupled planar plasmonic waveguides. By tuning the loss-gain balance, we show how the initially isotropic material becomes both asymmetric and unidirectional. The highly tunable optical dispersion of PT -symmetric metamaterials provides a foundation for designing an entirely new class of three-dimensional bulk synthetic media, with applications ranging from sub-diffraction-limited optical lenses to non-reciprocal nanophotonic devices.
We consider the plasmon polaritons along a layer of hyperbolic metamaterial propagating in the plane of the anisotropy axis with an arbitrary its orientation. As a layer material, we use periodic plane-layered artificial medium or hyperbolic metamaterial of thin metal and dielectric layers and produce its homogenization. The conditions for the existence of fast, slow, leakage, gliding flowing, forward and backward plasmon-polaritons are found. The Fresnel formulas for the diffraction of a plane wave of arbitrary polarization on such a structure are obtained. The dispersion of plasmon-polariton…
Strongly anisotropic media with hyperbolic dispersion can be used for claddings of plasmonic waveguides. In order to analyze the fundamental properties of such waveguides, we analytically study 1D waveguides arranged of a hyperbolic metamaterial (HMM) in a HMM-Insulator-HMM (HIH) structure. We show that hyperbolic metamaterial claddings give flexibility in designing the properties of HIH waveguides. Our comparative study on 1D plasmonic waveguides reveals that HIH-type waveguides can have a higher performance than MIM or IMI waveguides.
We analyze surface electromagnetic waves with hyperbolic dispersion supported at the interface between a semi-infinite isotropic medium and an effective uniaxial material. Apart from known types plasmons with hyperbolic dispersion curve, sometimes referred to as Dyakonov plasmons [Z. Jacob and E. E. Narimanov, APL 93, 221109 (2008)], we classify two new types of surface waves with hyperbolic dispersion. One type of such waves, in contrary to Dyakonov plasmons, does not require hyperbolic metamaterials to be involved. These hybrid-polarized plasmon modes with both TE and TM electromagnetic comp…
Near perfect infrared light absorption at multi-spectral wavelengths has been experimentally demonstrated by using multiplexed metal square plasmon resonance structures. Optical power absorption over 95% has been observed in dual-band metamaterial absorbers at two separate wavelengths and optical power absorption over 92.5% has been observed in triple-band metamaterial absorbers at three separate wavelengths. The peak absorption wavelengths are primarily determined by the sizes of the metal squares in the multiplexed structures. Electrical field distributions in the middle of the dielectric sp…
We show that a metallic plate with fractal-shaped slits can be homogenitized as a plasmonic metamaterial with plasmon frequency dictated by the fractal geometry. Owing to the all-dimensional subwavelength nature of the fractal pattern, our system supports both transverse-electric and transverse-magnetic surface plasmons. As a result, this structure can be employed to focus light sources with all-dimensional subwavelength resolutions and enhanced field strengths. Microwave experiments reveal that the best achievable resolution is only, and simulations demonstrate that similar effects can be rea…
We theoretically study the propagation of large-wavevector waves (volume plasmon polaritons) in multilayer hyperbolic metamaterials with two levels of structuring. We show that when the parameters of a subwavelength metal-dielectric multilayer ("substructure") are modulated ("superstructured") on a larger, wavelength scale, the propagation of volume plasmon polaritons in the resulting multiscale hyperbolic metamaterials is subject to photonic band gap phenomena. A great degree of control over such plasmons can be exerted by varying the superstructure geometry. When this geometry is periodic, s…
Studying basic physical effects sustained in metamaterials characterized by specific constitutive relation is a research topic with a long standing tradition. Besides intellectual curiosity, it derives its importance from the ability to predict observable phenomena that are, if found with an actual metamaterial, a clear indication on its properties. Here, we consider a nonlocal (strong spatial dispersion), lossy, and isotropic metamaterial and study the impact of the nonlocality on the dispersion relation of surface plasmon polaritons sustained at an interface between vacuum and such metamater…
We derive general coupled-mode equations describing the nonlinear interaction of electromagnetic modes in media with loss and gain. Our approach is rigorously based on the Lorentz reciprocity theorem, and it can be applied to a broad range of metal-dielectric photonic structures, including plasmonic waveguides and metamaterials. We verify that our general results agree with the previous analysis of particular cases, and predict novel effects on self- and cross-phase modulation in multi-layer nonlinear fishnet metamaterials.
Plasmon induced transparency (PIT) effect in a terahertz graphene metamaterial is numerically and theoretically analyzed. The proposed metamaterial comprises of a pair of graphene split ring resonators placed alternately on both sides of a graphene strip of nanometer scale. The PIT effect in the graphene metamaterial is studied for different vertical and horizontal configurations. Our results reveal that there is no PIT effect in the graphene metamaterial when the centers of both the split ring resonators and the graphene strip are collinear to each other. This is a noteworthy feature, as the …
We present how to physically realize the auxiliary source described in the recently introduced active plasmon injection loss compensation scheme for enhanced near-field superlensing. Particularly, we show that the characteristics of the auxiliary source described in the active plasmon injection scheme including tunable narrow-band and selective amplification via convolution can be realized by using a hyperbolic metamaterial functioning as a near-field spatial filter. Besides loss compensation, the proposed near-field spatial filter can be useful for real-time high resolution edge detection.
All-optical active plasmonic devices are of fundamental importance for designing efficient nanophotonic circuits. We theoretically propose and numerically investigate an active plasmonic device made up of a nonlinear epsilon-near-zero metamaterial slab of thickness smaller than 100 nanometers lying on a linear epsilon-near-zero metamaterial substrate. We predict that, in free-space coupling configuration, the device, operating at low-intensity, would display plasmon mediated hysteresis behavior since the phase difference between the reflected and the incident optical waves turns out to be mult…
By embedding four-rod resonators inside double-split ring resonators superlattice, a planar composite metamaterial possessing tripod plasmonic resonances is fabricated. Double Fano resonances are observed where a common subradiant driven oscillator is coupled with two superradiant oscillators. As a classical analogue of four-level tripod atomic system, the transmission spectrum of the composite metamaterial exhibits a double Fano-based coherent effect. Transfer of absorbed power between two superradiant oscillators is controlled by manipulating two coupling strengths conjugated through the pol…
The use of metamaterial as a way to mitigate the negative effects of absorption in metals on the Purcell effect in metal-dielectric structures is investigated. A layered metal-dielectric structure is considered as an anisotropic medium in the long-wavelength limit. The dispersion of the surface plasmon appearing at the boundary between such a structure and a different dielectric material, as well as the position of the peak in the local density of states are studied for various combinations of materials and filling factors of the periodic structure. The calculated frequency dependence of the P…
We consider an array of the meta-atom consisting of two cut-wires and a split-ring resonator interacting with an electromagnetic field with two polarization components. We prove that such metamaterial system can be taken as a classical analogue of an atomic medium with a double- $Λ$-type four-level configuration coupled with four laser fields, exhibits an effect of plasmon induced transparency (PIT), and displays a similar behavior of atomic four-wave mixing (FWM). We demonstrate that when nonlinear varactors are mounted onto the gaps of the split-ring resonators the system can acquire giant s…
We consider a simple configuration for realizing one-dimensional slow-light metamaterials with large bandwidth-delay products using stub-shaped Fabry-Perot resonators as building blocks. Each metaatom gives rise to large group indices due to a classical analog of the dressed-state picture of electromagnetically-induced transparency. By connecting up to eight metaatoms, we find bandwidth-delay products over unity and group indices approaching 100. Our approach is quite general and can be applied to any type of Fabry-Perot resonators and tuned to different operating wavelengths.
We demonstrate that surface plasmons of a thin metal film interacting with a periodic array of nano-structures around it can be utilized to make bulk negative index metamaterials at visible spectrum with simultaneously negative permittivity and permeability. These surface plasmon driven metamaterials have high figure of merit and can be tuned arbitrarily to operate at any wavelength in the visible spectrum and possibly at ultraviolet spectrum. We numerically demonstrate the idea by a metamaterial structure which exhibits a strong magnetic response resulting in a negative index of refraction in…
Metamaterials have introduced a whole new world of unusual materials with functionalities that cannot be attained in naturally occurring material systems by mimicking and controlling the natural phenomena at subwavelength scales. However, the inherent absorption losses pose fundamental challenge to the most fascinating applications of metamaterials. Based on a novel plasmon injection (PI or Π) scheme, we propose a coherent optical amplification technique to compensate losses in metamaterials. Although the proof of concept device here operates under normal incidence only, our proposed scheme ca…
Photoelectric properties of metamaterials containing non-centrosymmetric, similarly oriented metallic nanoparticles embedded in a homogeneous semiconductor matrix are theoretically studied. Due to the asymmetric shape of the nanoparticle boundary, photoelectron emission acquires a preferred direction, resulting in a photocurrent flow in that direction when nanoparticles are uniformly illuminated by a homogeneous plane wave. This effect is a direct analogy of the photogalvanic (or bulk photovoltaic) effect known to exist in media with non-centrosymmetric crystal structure, such as doped lithium…
Surface plasmon polaritons (SPPs) lasing requires population inversion, it is inefficient and possesses poor spectral properties. We develop an inversion-less concept for a quantum plasmonic waveguide that exploits unidirectional superradiant SPP emission of radiation to produce intense coherent surface plasmon beams. Our scheme includes a resonantly driven cold atomic medium in a lossless dielectric situated above an ultra-low loss negative index metamaterial~(NIMM) layer. We propose generating unidirectional superradiant radiation of the plasmonic field within an atomic medium and a NIMM lay…
Metamaterials with artificial optical properties have attracted significant research interest. In particular, artificial magnetic resonances in non-unity permeability tensor at optical frequencies in metamaterials have been reported. However, only non-unity diagonal elements of the permeability tensor have been demonstrated to date. A gyromagnetic permeability tensor with non-zero off-diagonal elements has not been observed at the optical frequencies. Here we report the observation of gyromagnetic properties in the near-infrared wavelength range in a magneto-plasmonic metamaterial. The non-zer…
A hybrid metal-graphene metamaterial (MM) is reported to achieve the active control of the broadband plasmon-induced transparency (PIT) in THz region. The unit cell consists of one cut wire (CW), four U-shape resonators (USRs) and monolayer graphene sheets under the USRs. Via near-field coupling, broadband PIT can be produced through the interference between different modes. Based on different arrangements of graphene positions, not only can we achieve electrically switching the amplitude of broadband PIT, but also can realize modulating the bandwidth of the transparent window. Simultaneously,…
The second harmonic generation is one of the most important applications of nonlinear effect, which has attracted great interests in nonlinear optics and microwave in the past decades. To the best of our knowledge, however, generating the second harmonics of surface plasmon polaritons (SPPs) has not been reported. Here, we propose to generate the second harmonics of spoof SPPs with high efficiency at microwave frequencies using subwavelength-scale nonlinear active device integrated on specially designed plasmonic waveguides, which are composed of two ultrathin corrugated metallic strips printe…
We theoretically study fishnet metamaterials at optical frequencies. In contrast to earlier works, we provide a microscopic description by tracking the transversal and longitudinal flows of energy through the fishnet mesh composed of intersecting subwavelength plasmonic waveguides. The analysis is supported by a semi-analytical model based on surface-plasmon coupled-mode equations, which provides accurate formulas for the fishnet refractive index, including the real-negative and imaginary parts. The model simply explains how the surface plasmons couple at the waveguide intersections and it shi…
The interaction of light with matter has triggered the interest of scientists for long time. The area of plasmonics emerges in this context through the interaction of light with valence electrons in metals. The random phase approximation in the long wavelength limit is used for analytical investigation of plasmons in three-dimensional metals, in a two-dimensional electron gas and finally in the most famous two-dimensional semi-metal, namely graphene. We show that plasmons in bulk metals as well as in a two-dimensional electron gas originate from classical laws, whereas, quantum effects appear …
We develop a general theoretical framework of integrated paired photon-plasmon generation through spontaneous wave mixing in nonlinear plasmonic and metamaterial nanostructures, rigorously accounting for material dispersion and losses in quantum regime through the electromagnetic Green function. We identify photon-plasmon correlations in layered metal-dielectric structures with 70% internal heralding quantum efficiency, and reveal novel mechanism of broadband generation enhancement due to topological transition in hyperbolic metamaterials.
Dispersion properties of metals and propagation of quantum bulk plasmon in the high photon energy regime are studied. The nonlocal dielectric permittivity of a metal is determined by the quantum plasma effects and is calculated by applying the Wigner equation in the kinetic theory and taking into account the electron lattice collisions. The properties of epsilon near zero material are investigated in a thin gold film. The spectrum and the damping rate of the quantum bulk plasmon are obtained for a wide range of energies, and the electron wave function is analytically calculated in both classic…
Plasmonic metamaterials support the localized surface plasmon resonance (LSPR), which is sensitive to the change in the dielectric environment and highly desirable for ultrasensitive biochemical sensing. In this work, a novel design of supercell metamaterials of four mutually rotating split ring resonators (SRRs) is proposed, where simultaneous excitations of odd (N=1 and N = 3) and even (N=2) resonance modes are realized due to additional asymmetry from the rotation and show insensitivity to two orthogonal polarizations. The full utilization of these three resonance dips show bright prospects…
We investigate the optical properties of sub-wavelength layered metal/dielectric structures, also known as hyperbolic metamaterials (HMMs), using exact analytical Kronig Penney (KP) model. We show that hyperbolic isofrequency surfaces exist for all combinations of layer permittivities and thicknesses, and the largest Purcell enhancements (PE) of spontaneous radiation are achieved away from the nominally hyperbolic region. Detailed comparison of field distributions, dispersion curves, and Purcell factors (PF) between the HMMs and Surface Plasmon Polaritons (SPPs) guided modes in metal/dielectri…
We observe unique absorption resonances in silver/silica multilayer-based epsilon-near-zero (ENZ) metamaterials that are related to radiative bulk plasmon-polariton states of thin-films originally studied by Ferrell (1958) and Berreman (1963). In the local effective medium, metamaterial descrip- tion, the unique effect of the excitation of these microscopic modes is counterintuitive and captured within the complex propagation constant, not the effective dielectric permittivities. Theoretical anal- ysis of the band structure for our metamaterials shows the existence of multiple Ferrell-Berreman…
Metamaterial approach is capable of drastically increasing the critical temperature, Tc, of composite metal-dielectric superconductors. Tripling of Tc was observed in bulk Al-Al2O3 core-shell metamaterials. A theoretical model based on the Maxwell-Garnett approximation provides a microscopic explanation of this effect in terms of electron-electron pairing mediated by a hybrid plasmon-phonon excitation. We report the first observation of this excitation in Al-Al2O3 core-shell metamaterials using inelastic neutron scattering. This result provides support for this novel mechanism of superconducti…
By using an elegant response function theory, which does not require matching of the messy boundary conditions, we investigate the surface plasmon excitations in the multicoaxial cylindrical cables made up of negative-index metamaterials. The multicoaxial cables with {\em dispersive} metamaterial components exhibit rather richer (and complex) plasmon spectrum with each interface supporting two modes: one TM and the other TE for (the integer order of the Bessel function) $m \ne 0$. The cables with {\em nondispersive} metamaterial components bear a different tale: they do not support simultaneou…
We present an analytical description of the nonlocal optical response of plasmonic nanowire metamaterials that enable negative refraction, subwavelength light manipulation, and emission lifetime engineering. We show that dispersion of optical waves propagating in nanowire media results from coupling of transverse and longitudinal electromagnetic modes supported by the composite and derive the nonlocal effective medium approximation for this dispersion. We derive the profiles of electric field across the unit cell, and use these expressions to solve the long-standing problem of additional bound…
Harnessing artificial optical magnetism requires rather complex two- and three-dimensional structures, examples include split-ring and fishnet metamaterials and nanoparticles with non-trivial magnetic properties. By contrast, dielectric properties can be tailored even in planar and pattern-free, one-dimensional (1D) arrangements, for example metal/dielectric multilayer metamaterials. These systems are extensively investigated due to their hyperbolic and plasmonic response, which, however, is considered to be limited to TM polarization, based on the general consensus that they do not possess in…
We demonstrate that both linear and nonlinear Fano resonances can be realized on two dimensional magnetic metamaterials. The Fano resonance comes from the interference between localized magnetic plasmon resonance and propagating surface plasmon polaritons. When studying the linear optical response of the metamaterial structure, this interference phenomenon was observed in the ellipsometric spectrum. By finely tailoring the geometrical parameters of the magnetic metamaterial device, the nonlinear Fano response was tuned to a near-infrared wavelength (1.61-1.8 μm) of femtosecond pump laser, and …
We theoretically investigate general existence conditions for broadband bulk large-wavevector (high-k) propagating waves (such as volume plasmon polaritons in hyperbolic metamaterials) in subwavelength periodic multilayer structures. Describing the elementary excitation in the unit cell of the structure by a generalized resonance pole of a reflection coefficient, and using Bloch's theorem, we derive analytical expressions for the band of large-wavevector propagating solutions. We apply our formalism to determine the high-k band existence in two important cases: the well-known metal-dielectric,…
We demonstrate that the trapped magnetic resonance mode can be induced in an asymmetric double-bar structure for electromagnetic waves normally incident onto the double-bar plane, which mode otherwise cannot be excited if the double bars are equal in length. By adjusting the structural geometry, the trapped magnetic resonance becomes transparent with little resonance absorption when it happens in the dipolar resonance regime, a phenomenon so-called plasmonic analogue of electromagnetically induced transparency. Accordingly, the additional magnetic resonance by introducing asymmetry is explaine…
Photonic metamaterials allow for a range of exciting applications unattainable with ordinary dielectrics. However, the metallic nature of their meta-atoms may result in increased optical losses. Gain-enhanced metamaterials are a potential solution to this problem, but the conception of realistic, three-dimensional designs is a challenging task. Starting from fundamental electrodynamic and quantum-mechanical equations we establish and deploy a rigorous theoretical model for the spatial and temporal interaction of lightwaves with free and bound electrons inside and around metallic (nano-) struct…
Ultrafast excitation of Bloch plasmon polaritons in hyperbolic metamaterials with an extreme ultra-violet transient grating
Umeå University（于默奥大学）；Elettra Sincrotrone Trieste（的里雅斯特同步辐射中心）；CIC nanoGUNE BRTA（nanoGUNE研究中心）；Ikerbasque, Basque Foundation for Science（伊卡巴斯克，巴斯克科学基金会）；Università degli Studi di Modena e Reggio Emilia（摩德纳和雷焦艾米利亚大学）；Wallenberg Initiative Materials Science for Sustainability（瓦伦堡可持续材料科学倡议）
We identify a route towards achieving a negative index of refraction at optical frequencies based on coupling between plasmonic waveguides that support backwards waves. We show how modal symmetry can be exploited in metal-dielectric waveguide pairs to achieve negative refraction of both phase and energy. By properly controlling coupling between adjacent waveguides, a metamaterial consisting of a one-dimensional multilayer stack exhibiting an isotropic index of -1 can be achieved at a free-space wavelength of 400 nm. The general concepts developed here may inspire new low-loss metamaterial desi…
We study the dispersion relation of a metamaterial composed of metallic disks and bars arranged to have kagome symmetry and find that a plasmonic flat band is formed by the topological nature of the kagome lattice. To confirm the flat-band formation, we fabricate the metamaterial and make transmission measurements in the terahertz regime. Two bands formed by transmission minima that depend on the polarization of the incident terahertz beams are observed. One of the bands corresponds to the flat band, as confirmed by the fact that the resonant frequency is almost independent of the incident ang…
We consider a simple cubic array of metallic nanoparticles supporting extended collective plasmons that arise from the near-field dipolar interaction between localized surface plasmons in each nanoparticle. We develop a fully analytical quantum theory of the strong-coupling regime between these collective plasmons and photons resulting in plasmon polaritons in the nanoparticle array. Remarkably, we show that the polaritonic band gap and the dielectric function of the metamaterial can be significantly modulated by the polarization of light. We unveil how such an anisotropic behavior in the plas…
To efficiently integrate cutting-edge terahertz technology into compact devices, the highly confined terahertz plasmons are attracting intensive attentions. Compared to plasmons at visible frequencies in metals, terahertz plasmons, typically in lightly doped semiconductors or graphene, are sensitive to carrier density (n) and thus have an easy tunability, which, however, leads to unstable or imprecise terahertz spectra. By deriving a simplified but universal form of plasmon frequencies, here we reveal a unified mechanism for generating unusual n-independent plasmons (DIPs) in all topological s…
We demonstrate on-demand control of localized surface plasmons in metamaterials by means of incident light polarization. An asymmetric mode, selectively excited by s-polarized light, interfere destructively with a bright element, thereby allowing the incident light to propagate at a fairly low loss, corresponding to electromagnetically induced transparency (EIT) in an atomic system. In contrast, a symmetric mode, excited by p-polarized light, directly couples with the incident light, which is analogous to the switch-off of EIT. The light polarization-dependent excitation of asymmetric and symm…
A film-coupled metamaterial structure is numerically investigated for enhancing the light absorption in an ultrathin photovoltaic layer of crystalline gallium arsenide (GaAs). The top subwavelength concave grating and the bottom metallic film could not only effectively trap light with the help of wave interference and magnetic resonance effects excited above the bandgap, but also practically serve as electrical contacts for photon-generated charge collection. The energy absorbed by the active layer is greatly enhanced in the film-coupled metamaterial structure, resulting in significant enhance…
In this work, we report the design of a wavelength-tunable infrared metamaterial by exciting magnetic resonance with phase transition of vanadium dioxide (VO2). Numerical simulation shows a broad absorption peak at the wavelength of 10.9 um when VO2 is a metal, but it shifts to 15.1 um when VO2 changes to dielectric phase below its phase transition temperature of 68degC. The large tunability of 38.5% in the resonance wavelength stems from the different excitation conditions of magnetic resonance assisted by plasmon in metallic VO2 but optical phonons in dielectric VO2. The physical mechanism i…
