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arXiv 0904.4613cond-mat.supr-concond-mat.mtrl-sci
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空穴掺杂超导体Pr1-xSrxFeAsO的结构研究

Structural study on hole-doped superconductors Pr1-xSrxFeAsO

J Ju, Z Li, G Mu, H-H Wen, K Sato, M Watahiki, G Li, K Tanigaki

摘要:

利用同步辐射X射线衍射数据分析了Pr_(1-x)Sr_xFeAsO(1111)超导体系的结构细节,研究了随着Sr浓度的增加,体系从非超导向空穴掺杂超导转变过程中的结构参数。当Sr掺杂量达到0.221时,出现超导性。晶格常数的线性增加证明Sr被成功地引入到体系中,并且其浓度可以通过电子密度分析准确地确定。Pr_(1-x)Sr_xFeAsO超导体的结构参数随Sr浓度的变化以及它们与其他铁基超导体的结构参数的比较表明,在空穴掺杂的(1111)超导体中,导电As-Fe-As层和绝缘Pr-O-Pr层之间的层间空间对提高Tc有重要作用,这似乎不同于电子掺杂的系统。

英文摘要:

The structural details in Pr1-xSrxFeAsO (1111) superconducting system are analyzed using data obtained from synchrotron X-ray diffraction and the structural parameters are carefully studied as the system is moving from non-superconducting to hole-doped superconducting with the Sr concentration. Superconductivity emerges when the Sr doping amount reaches 0.221. The linear increase of the lattice constants proves that Sr is successfully introduced into the system and its concentration can accurately be determined by the electron density analyses. The evolution of structural parameters with Sr concentration in Pr1-xSrxFeAsO and their comparison to other similar structural parameters of the related Fe-based superconductors suggest that the interlayer space between the conducting As-Fe-As layer and the insulating Pr-O-Pr layer is important for improving Tc in the hole-doped (1111) superconductors, which seems to be different from electron-doped systems.

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