In usual superconductors the carriers form Cooper pairs that have zero total momentum meaning that the superfluid density is homogeneous. We know for decades that it is a priori possible to observe at high fields the Fulde-Ferrel-Larkin-Ovchinikov (FFLO) state in which the superfluid density exhibits a field dependent modulation. The search for such inhomogeneous condensates in materials is the subject of tremendous excitement especially after the discovery of a promising high-field superconducting (HFSC) phase in CeCoIn$_5$. However, subsequent neutron and NMR experiments contradicted the FFLO picture in CeCoIn$_5$ establishing a puzzling coupling of the distinct HFSC state with a magnetic modulation. Here we show that, a novel type of exotic state is observed at high fields in CeCoIn$_5$ in which a pattern of coexisting condensates manifests. The specific pattern includes the d-wave singlet SC state, the staggered $π$-triplet SC state and Spin Density Waves (SDW). Because of particle-hole asymmetry these three condensates may either appear separately or all three together providing a new perspective on antiferromagnetic superconductors that may include high-$T_c$ cuprates and pniktides. The field induced transition to the pattern state in CeCoIn$_5$ is only a paradigm of a generic mechanism that prevents the elimination of the dominating condensate by the field via the formation of a pattern of condensates. This opens new avenues for the search of exotic states not only in electronic systems, but also in other systems where inhomogeneous condensates are actively discussed like trapped atomic fermi gases and dense quark matter.
We present nuclear magnetic resonance (NMR) measurements on the three distinct In sites of CeCoIn$_5$ with magnetic field applied in the [100] direction. We identify the microscopic nature of the long range magnetic order (LRO) stabilized at low temperatures in fields above 10.2 T while still in the superconducting (SC) state. We infer that the ordered moment is oriented along the $\hat c$-axis and map its field evolution. The study of the field dependence of the NMR shift for the different In sites indicates that the LRO likely coexists with a modulated SC phase, possibly that predicted by Fu…
Recently, Rourke et al. reported point-contact spectroscopy results on the heavy-fermion superconductor CeCoIn$_5$ [1]. They obtained conductance spectra on the c-axis surfaces of CeCoIn$_5$ single crystals. Their major claims are two-fold: CeCoIn$_5$ has i) d-wave pairing symmetry and ii) two coexisting order parameter components. In this Comment, we show that these claims are not warranted by the data presented. [1] Rourke et al., Phys. Rev. Lett. 94, 107005 (2005).
Point-contact spectroscopy was performed on single crystals of the heavy-fermion superconductor CeCoIn_5 between 150 mK and 2.5 K. A pulsed measurement technique ensured minimal Joule heating over a wide voltage range. The spectra show Andreev-reflection characteristics with multiple structures which depend on junction impedance. Spectral analysis using the generalized Blonder-Tinkham-Klapwijk formalism for d-wave pairing revealed two coexisting order parameter components, with amplitudes Delta_1 = 0.95 +/- 0.15 meV and Delta_2 = 2.4 +/- 0.3 meV, which evolve differently with temperature. Our …
The implications of the spin exciton mechanism are exposed in the context of a Spin Density Wave (SDW) instability occurring inside the superconducting phase of a layered heavy electron compound. In this model a magnetic field serves as a tuning parameter bringing the system to the point where the transverse spin correlations are enhanced due to dx2 -y2 -wave superconductivity and induces an instability to a phase with coexisting superconductivity and SDW order. The model considers electrons in a crystal with antiferromagnetic interactions and provides restrictions on the Fermi surface charact…
Recently, it has been reported that the low-temperature high-magnetic field phase in CeCoIn5 (Q-phase), has spin-density wave (SDW) order that only exists within this phase. This indicates that the SDW order is the result of the development of pair density wave (PDW) order in the superconducting phase that coexists with d-wave superconductivity. Here we develop a phenomenological theory for these coexisting orders. This provides selection rules for the PDW order and further shows that the detailed structure of this order is highly constrained. We then apply our theory to the the vortex phase. …
Thermal conductivity and specific heat were measured in the superconducting state of the heavy fermion material Ce_{1-x}La_{x}CoIn_{5}. With increasing impurity concentration x, the suppression of T_{c} is accompanied by the increase in the residual electronic specific heat expected of a d-wave superconductor, but it occurs in parallel with a decrease in residual electronic thermal conductivity. This contrasting behavior reveals the presence of uncondensed electrons coexisting with nodal quasiparticles. An extreme multiband scenario is proposed, with a d-wave superconducting gap on the heavy-e…
We have studied systematically the influence of particle-hole symmetric and asymmetric kinetic terms on the ordered phases that we may observe competing or coexisting in a tetragonal system. We show that there are precise patterns of triplets of ordered phases that are accessible (i.e. it is impossible to observe two of them without the third one). We found a systematic way to predict these patterns of states and tested it by identifying at least 16 different patterns of three order parameters that necessarily coexist in the presence of the kinetic terms. We show that there are two types of ge…
The Bardeen-Cooper-Schrieffer mechanism for superconductivity is a triumph of the theory of many-body systems. Implicit in its formulation is the existence of long-lived (quasi)particles, originating from the electronic building blocks of the materials, which interact to form Cooper pairs that move coherently in lock-step. The challenge of unconventional superconductors is that it is not only unclear what the nature of the interactions are, but whether the familiar quasi-particles that form a superconducting condensate even exist. In this work, we reveal, by the study of applied magnetic field…
Neutron scattering in strong magnetic fields is used to show the spin-resonance in superconducting CeCoIn5 (Tc=2.3 K) is a doublet. The underdamped resonance (\hbar Γ=0.069 \pm 0.019 meV) Zeeman splits into two modes at E_{\pm}=\hbar Ω_{0}\pm gμ_{B} μ_{0}H with g=0.96 \pm 0.05. A linear extrapolation of the lower peak reaches zero energy at 11.2 \pm 0.5 T, near the critical field for the incommensurate "Q-phase" indicating that the Q-phase is a bose condensate of spin excitons.
The origin of the spin resonance observed in CeCoIn5 with Inelastic Neutron Scattering is subject to debate. It has been shown recently that in this heavy electron compound at low temperature an instability to a ground state with coexisting dx2 -y2 -wave superconductivity and Spin Density Wave (SDW) order in a magnetic field is a corollary of the consideration of a collective spin excitation mode in a quasi-2D dx2 -y2 -wave Pauli-limited superconductor. This provides a natural scenario for the occurence of the puzzling high-field-low-temperature phase highlighted in CeCoIn5 . We present perspe…
It is theoretically shown that, in the four-fold symmetric d-wave superconducting phase, a paramagnetic pair-breaking (PPB) enhanced sufficiently by increasing the applied magnetic field induces not only the Fulde-Ferrell-Larkin-Ovchinnikov (FFLO) superconducting state but also an incommensurate antiferromagnetic (AFM) order with Q-vector parallel to a gap node. This AFM ordering tends to occur only below H_{c2} at low temperatures, i.e., in the presence of a nonvanishing superconducting energy gap $Δ$ rather than in the normal phase. Through a detailed study on the resulting AFM order and its…
We build a holographic superconductor model with a scalar triplet charged under an SU(2) gauge field in the bulk. In this model, the s-wave and p-wave condensates can be consistently realized. We find that there are totally four phases in this model, namely, the normal phase without any condensate, s-wave phase, p-wave phase and the s+p coexisting phase. By calculating Gibbs free energy, the s+p coexisting phase turns out to be thermodynamically favored once it can appear. The phase diagram with the dimension of the scalar operator and temperature is drawn. The temperature range for the s+p co…
One of the keys to the high-temperature superconductivity puzzle is the identification of the energy scales associated with the emergence of a coherent condensate of superconducting electron pairs. These might provide a measure of the pairing strength and of the coherence of the superfluid, and ultimately reveal the nature of the elusive pairing mechanism in the superconducting cuprates. To this end, a great deal of effort has been devoted to investigating the connection between the superconducting transition temperature Tc and the normal-state pseudogap crossover temperature T*. Here we prese…
There is a tacit assumption that multiband superconductors are essentially the same as multigap superconductors. More precisely, it is usually assumed that the number of excitation gaps in the single-particle energy spectrum of a uniform superconductor determines the number of contributing bands in the corresponding superconducting model. Here we demonstrate that contrary to this widely accepted viewpoint, the superconducting magnetic properties are sensitive to the number of contributing bands even when the corresponding excitation gaps are degenerate and cannot be distinguished. In particula…
The presence of two components in the electron fluid of high temperature superconductors and the complex charge and lattice inhomogeneity have been the hot topics of the international conference of the superstripes series, Superstripes 2015, held in Ischia in 2015. The debate on the mechanisms for reaching room temperature superconductivity has been boosted by the discovery of superconductivity with the highest critical temperature in pressurized sulfur hydride. Different complex electronic and structural landscapes showing up in superconductors which resist to the decoherence effects of high …
Spin-triplet superconductivity is a condensate of electron pairs with spin-1 and an odd-parity wavefunction. A particularly interesting manifestation of triplet pairing is a chiral p-wave state which is topologically non-trivial and a natural platform for realizing Majorana edge modes. Triplet pairing is however rare in solid state systems and so far, no unambiguous identification has been made in any bulk compound. Since pairing is most naturally mediated by ferromagnetic spin fluctuations, uranium based heavy fermion systems containing f electron elements that can harbor both strong correlat…
The condensation of an electron superfluid from a conventional metallic state at a critical temperature $T_c$ is described well by the BCS theory. In the underdoped copper-oxides, high-temperature superconductivity condenses instead from a nonconventional metallic "pseudogap" phase that exhibits a variety of non-Fermi liquid properties. Recently, it has become clear that a charge density wave (CDW) phase exists within the pseudogap regime, appearing at a temperature $T_{CDW}$ just above $T_c$. The near coincidence of $T_c$ and $T_{CDW}$, as well the coexistence and competition of CDW and super…
Free energy of a two-liquid system of charge carriers in strongly coupled electron and phonon fields and common nature of three phases in hole-doped cuprates
Large Field-Free Superconducting Diode Effect with Nonmonotonic Polarity Reversals in NbSe$_2$/CrBr$_3$ Heterostructures
Southern University of Science and Technology（南方科技大学）；International Quantum Academy, and Shenzhen Branch, Hefei National Laboratory（国际量子科学院，合肥国家实验室深圳分院）；Eastern Institute for Advanced Study, Eastern Institute of Technology（宁波东方理工大学（暂名）先进研究院）；State Key Laboratory of Optoelectronic Materials and Technologies, Sun Yat‑sen University（中山大学光电信息材料与技术国家重点实验室）
