Features of rheological laws applied to solid-like granular materials are recalled and confronted to microscopic approaches via discrete numerical simulations. We give examples of model systems with very similar equilibrium stress transport properties -- the much-studied force chains and force distribution -- but qualitatively different strain responses to stress increments. Results on the stability of elastoplastic contact networks lead to the definition of two different rheological regimes, according to whether a macroscopic fragility property (propensity to rearrange under arbitrary small stress increments in the thermodynamic limit) applies. Possible consequences are discussed.
The recoverable strain is shown to correlate to the temporal evolution of microstructure via time-resolved small-angle neutron scattering (SANS) and dynamic shear rheology. Investigating two distinct polymeric materials of wormlike micelles and fibrin network, we demonstrate that, in addition to the nonlinear structure-property relationships, the shear and normal stress evolution is dictated by the recoverable strain. A distinct sequence of physical processes under large amplitude oscillatory shear (LAOS) is identified that clearly contains information regarding both the steady-state flow curv…
The similarity in atomic structure between liquids and glasses has stimulated a long-standing hypothesis that the nature of glasses may be more fluid like, rather than an apparent solid. In principle, the nature of glasses can be characterized by measuring the dynamic response of rheology to shear strain rate in the glass state. However, limited by the brittleness of glasses and current experimental techniques, the dynamic behaviors of glasses were mainly assessed in the supercooled liquid state or in the glass state within a narrow rate range. Therefore, the nature of glasses has not been wel…
We study strain-controlled plastic deformation of crystalline solids via two-dimensional discrete dislocation dynamics simulations. To this end, we characterize the average stress-strain curves as well as the statistical properties of strain bursts and the related stress drops as a function of the imposed strain rate and the stiffness of the specimen-machine system. The dislocation system exhibits strain rate sensitivity such that a larger imposed strain rate results in a higher average stress at a given strain. In the limit of small strain rate and driving spring stiffness, the sizes and dura…
Spatially heterogeneous relaxational dynamics and the evolution of recoverable strain following flow cessation of a ductile nanocolloidal glass
Johns Hopkins University(约翰斯·霍普金斯大学);University of Illinois Urbana-Champaign(伊利诺伊大学厄巴纳-香槟分校);Argonne National Laboratory(阿贡国家实验室);University of Ottawa(渥太华大学)