We consider a monolayer of particles floating at a horizontal liquid-gas interface -- a particle raft. Upon compressing the monolayer in a Langmuir trough, the particles at first pack but ultimately the monolayer buckles out of the plane. We measure the stress profile within the raft at the onset of buckling and show for the first time that such systems exhibit a Janssen effect: the stress decays exponentially away from the compressing barriers over a length scale that depends on the width of the trough. We find quantitative agreement between the rate of decay and the simple theory presented by Janssen and others. This demonstrates that floating particle rafts have a granular, as well as elastic, character, which is neglected by current models. Finally, we suggest that our experimental setup may be suitable for exploring granular effects in two dimensions without the complications of gravity and basal friction.
We investigate a model system for the rotational dynamics of inertial many-particle clustering, in which sub-millimeter objects are acoustically levitated in air. Driven by scattered sound, levitated grains self-assemble into a monolayer of particles, forming mesoscopic granular rafts with both an acoustic binding energy and a bending rigidity. Detuning the acoustic trap can give rise to stochastic forces and torques that impart angular momentum to levitated objects. As the angular momentum of a quasi-two-dimensional granular raft is increased, the raft deforms from a disk to an ellipse, event…
We investigate the mechanical response of a compressed monolayer of large and dense particles at a liquid-fluid interface: a granular raft. Upon compression, rafts first wrinkle; then, as the confinement increases, the deformation localizes in a unique fold. This characteristic buckling pattern is usually associated to floating elastic sheets and as a result, particle laden interfaces are often modeled as such. Here, we push this analogy to its limits by comparing the first quantitative measurements of the raft morphology to a theoretical continuous elastic model of the interface. We show that…
Confined two-dimensional assemblies of floating particles, known as granular rafts, are prone to develop a highly nonlinear response under compression. Here we investigate the transition to the friction-dominated jammed state and map the gradual development of the internal stress profile with flexible pressure sensors distributed along the raft surface. Surprisingly, we observe that the surface stress screening builds up much more slowly than previously thought and that the typical screening distance later dramatically decreases. We explain this behavior in terms of progressive friction mobili…
Tunable mechanical properties and air-based lubrication in an acoustically levitated granular material
James Franck Institute, University of Chicago（詹姆斯·弗兰克研究所，芝加哥大学）；Department of Physics, University of Chicago（芝加哥大学物理系）；Department of Physics, Drexel University（德雷塞尔大学物理系）；Department of Chemistry, Stanford University（斯坦福大学化学系）；Department of Radiology, Stanford University（斯坦福大学放射学系）；Department of Chemical Engineering, Stanford University（斯坦福大学化学工程系）
Quasi-static tensile experiments were performed for a model disordered solid consisting of a two-dimensional raft of polydisperse floating granular particles with capillary attractions. The ductility is tuned by controlling the capillary interaction range, which varies with the particle size. During the tensile tests, after an initial period of elastic deformation, strain localization occurs and leads to the formation of a shear band at which the pillar later fails. In this process, small particles with long-ranged interactions can endure large plastic deformations without forming significant …
The acoustic levitation of small particles provides a versatile platform to investigate the collective dynamical properties of self-assembled many-body systems in the presence of hydrodynamic coupling. However, acoustic scattering forces can only generate attractive interactions at close range in the levitation plane, limiting self-assembly to rafts where particles come into direct, dissipative, contact. Here, we overcome this limitation by using particles small enough that the viscosity of air establishes a repulsive streaming flow at close range. By tuning the size of particles relative to t…
We study the collective behaviour of a close packed monolayer of non-Brownian particles at a fluid-liquid interface. Such a particle raft forms a two-dimensional elastic solid and can support anisotropic stresses and strains, e.g. it buckles in uniaxial compression and cracks in tension. We characterise this solid in terms of a Young's modulus and Poisson ratio derived from simple theoretical considerations and show the validity of these estimates by using an experimental buckling assay to deduce the Young's modulus.
According to the lipid raft hypothesis, biological lipid membranes are laterally heterogeneous and filled with nanoscale ordered "raft" domains, which are believed to play an important role for the organization of proteins in membranes. However, the mechanisms stabilizing such small rafts are not clear, and even their existence is sometimes questioned. Here we report the observation of raft-like structures in a coarse-grained molecular model for multicomponent lipid bilayers. On small scales, our membranes demix into a liquid ordered (lo) and a liquid disordered (ld) phase. On large scales, ph…
Experimental measurements of the response of a two dimensional system of plastic beads subjected to steady shear are reported. The beads float at the surface of a fluid substrate and are subjected to a slow, steady-shear in a Couette geometry. The flow consists of irregular intervals of solid-like, jammed behavior, followed by stress relaxations. We report on statistics that characterize the stress fluctuations as a function of several parameters including shear-rate and packing density. Over a range of densities between the onset of flow to the onset of buckling (overpacking) of the system, t…
The University of Tokyo（东京大学）；Central University of Rajasthan（拉贾斯坦中央大学）；Université de Lille（里尔大学）；ESPCI Paris（巴黎高等物理化工国立工程学院）；Aoyama Gakuin University（青山学院大学）
We use the first Betti number of a complex to characterize the morphological structure of granular samples in mechanical equilibrium. We analyze two-dimensional granular packings after a tapping process by means of both simulations and experiments. States with equal packing fraction obtained with different tapping intensities are distinguished after the introduction of a filtration parameter which determines the particles (nodes in the network) that are joined by an edge. We first use numerical simulations to characterize the effect of the precision in the particles localization by artificiall…
We have experimentally investigated the bouncing behavior and damping performance of a container partially filled with granular chains, namely a chain-filled damper. The motion of the chain-filled damper, recorded by a particle tracing technology, demonstrates that the granular chains can efficiently absorb the collisional energy of the damper. We extract both the restitution coefficient of the first collision and the total flight time to characterize the dissipation ability of the damper. Two containers and three types of granular chains, different in size, stiffness and restitution coefficie…
The behaviour of a vertically vibrated granular bed is reminiscent of a liquid in that it exhibits many phenomena such as convection and Faraday-like surface waves. However, when the lateral dimensions of the bed are confined such that a quasi-one-dimensional geometry is formed, the only phenomena that remain are bouncing bed and the granular Leidenfrost effect. This permits the observation of the granular Leidenfrost state for a wide range of energy injection parameters, and more specifically allows for a thorough characterisation of the low-frequency oscillation (LFO) that is present in this…
We investigate the dynamics of granular columns of point particles that interact via long-range hydrodynamic interactions and fall under the action of gravity. We investigate the influence of inertia using the Green's function for the Oseen equation. The initial conditions (density and aspect ratio) are systematically varied. Our results suggest that universal self-similar laws may be sufficient to characterize the temporal and structural evolution of the granular columns. A characteristic time above which an instability is triggered (which may enable the formation of clusters) is also retriev…
The particle-scale dynamics of granular materials have commonly been characterized by the self-diffusion coefficient $D$. However, this measure discards the collective and topological information known to be an important characteristic of particle trajectories in dense systems. Direct measurement of the entanglement of particle space-time trajectories can be obtained via the topological braid entropy $\Sbraid$, which has previously been used to quantify mixing efficiency in fluid systems. Here, we investigate the utility of $\Sbraid$ in characterizing the dynamics of a dense, driven granular m…
Granular simulations are used to probe the particle scale dynamics at short, intermediate, and long time scales for gravity driven, dense granular flows down an inclined plane. On approach to the angle of repose, where motion ceases, the dynamics become intermittent over intermediate times, with strong temporal correlations between particle motions -- temporally heterogeneous dynamics. This intermittency is characterised through large scale structural events whereby the contact network periodically spans the system. A characteristic time scale associated with these processes increases as the s…
This paper describes methods to measure flow rate and jamming onset of granules discharged through a flat-bottom cylindrical hopper with a circular orifice. The intrinsic jamming onset for ideal particles (spherical, monodisperse, smooth) is experimentally measured by two independent methods, with good agreement. For non-ideal particles, the normalized jamming onset increases with elongated granule shape, broadened size distribution and increased friction as measured by the drained angle of repose. An empirical model of the jamming onset is introduced to quantify these effects over the range o…
The theory of homogeneously driven granular gases of hard particles predicts that the stationary state is characterized by a velocity distribution function with overpopulated high-energy tails as compared to the exponential decay valid for molecular gases. While this fundamental theoretical result was confirmed by numerous numerical simulations, an experimental confirmation is still missing. Using self-rotating active granular particles, we find a power-law decay of the velocity distribution whose exponent agrees well with the theoretic prediction.
We develop and fully characterize a meshfree Lagrangian (particle) model for continuum-based numerical modeling of dry and submerged granular flows. The multiphase system of the granular material and the ambient fluid is treated as a multi-density multi-viscosity system in which the viscous behaviour of the granular phase is predicted using a regularized viscoplastic rheological model with a pressure-dependent yield criterion. The numerical technique is based on the Weakly-Compressible Moving Particle Semi-implicit (WC-MPS) method. The required algorithms for approximation of the effective vis…
We investigate experimentally the collective behavior of a wet granular monolayer under vertical vibrations. The spherical particles are partially wet such that there are short-ranged attractive interactions between adjacent particles. As the vibration strength increases, clustering, reorganizing and melting regimes are identified subsequently through a characterization with the bond-orientational order parameters and the mean kinetic energy of the particles. The melting transition is found to be a continuous process starting from the defects inside the crystal.
Fingering instabilities akin to the Rayleigh-Taylor (RT) instability in fluids have been observed in a binary granular system consisting of dense and small particles layered on top of lighter and larger particles, when the system is subjected to vertical vibration and fluidizing gas flow. Using observations from experiments and numerical modelling we explore whether the theory developed to describe the Rayleigh-Taylor (RT) instability in fluids is also applicable to binary granular systems. Our results confirm the applicability of the classic RT instability theory for binary granular systems d…
Diverging correlation lengths on either side of the jamming transition are used to formulate a rheological model of granular shear flow, based on the propagation of stress through force chain networks. The model predicts three distinct flow regimes, characterized by the shear rate dependence of the stress tensor, that have been observed in both simulations and experiments. The boundaries separating the flow regimes are quantitatively determined and testable. In the limit of jammed granular solids, the model predicts the observed anomalous scaling of the shear modulus and a new relation for the…
The transition between shear-flowing and shear-arrested states of frictional granular matter is studied using constant-stress discrete element simulations. By subjecting a dilute system of frictional grains to a constant external shear stress and pressure, friction-dependent critical shear stress and density are clearly identified with both exhibiting a crossover between low and high friction. The critical shear stress bifurcates two nonequilibrium steady states: (i) steady state shear flow characterized by a constant deformation rate, and (ii) shear arrest characterized by temporally decaying…
Scattering methods are widespread used to characterize the structure and constituents of matter on small length scales. This motivates this introductory text on identifying prospective approaches to scattering-based methods for granular media. A survey to light scattering by particles and particle ensembles is given. It is elaborated why the established scattering methods using X-rays and visible light cannot in general be transferred to granular media. Spectroscopic measurements using Terahertz radiation are highlighted as they to probe the scattering properties of granular media, which are s…
We describe experiments on monodisperse spherical particles in an annular cell geometry, vibrated from below and sheared from above. This system shows a freezing/melting transition such that under sufficient vibration a crystallized state is observed, which can be melted by sufficient shear. We characterize the hysteretic transition between these two states, and observe features reminiscent of both a jamming transition and critical phenomena.
Liquid has a significant effect on the flow of wet granular assemblies. We explore the effects of liquid induced cohesion on the flow characteristics of wet granular materials. We propose a cohesion-scaling approach that enables invariant flow characteristics for different particles sizes in rotating drums. The strength of capillary forces between the particles is significantly reduced by making the glass beads hydrophobic via chemical silanization. Main results of rotating drum experiments are that liquid-induced cohesion decreases both the width of the flowing region and the velocity of the …
Recent numerical work has shown that high-speed confined granular flows down inclines exhibit a rich variety of flow patterns, including dense unidirectional flows, flows with longitudinal vortices and supported flows characterized by a dense core surrounded by a dilute hot granular gas (Brodu et al, JFM 2015). Here, we revisit the results obtained by Brodu et al. (JFM, 2015) and present new features characterizing these flows. In particular, we provide vertical and transverse profiles for the packing fraction, velocity and granular temperature.We also characterize carefully the transition bet…
Flowing granular materials often abruptly arrest if not driven by sufficient applied stresses. Such abrupt cessation of motion can be economically expensive in industrial materials handling and processing, and is significantly consequential in intermittent geophysical phenomena such as landslides and earthquakes. Using discrete element simulations, we calculate states of steady flow and arrest for granular materials under the conditions of constant applied pressure and shear stress, which are also most relevant in practice. Here the material can dilate or compact, and flow or arrest, in respon…
The critical rheology of sheared frictional granular materials near jamming transition is numer- ically investigated. It is confirmed that there exist a true critical density which characterizes the onset of the yield stress, and two fictitious critical densities which characterize the scaling laws of rheological properties. We find the existence of a hysteresis loop between two of the critical densities for each friction coefficient. It is noteworthy that the critical scaling law for frictionless jamming transition seems to be still valid even for frictional jamming despite using fictitious c…
We analyze particle velocity fluctuations in a simulated granular system subjected to homogeneous quasistatic shearing. We show that these fluctuations share the following scaling characteristics of fluid turbulence in spite of their different physical origins: 1) Scale-dependent probability distribution with non-Guassian broadening at small time scales; 2) Power-law spectrum, reflecting long-range correlations and the self-affine nature of the fluctuations; 3) Superdiffusion with respect to the mean background flow.
By detailed Molecular Dynamics and Monte Carlo simulations %of a realistic model we show that granular materials at rest can be described as thermodynamics systems. First we show that granular packs can be characterized by few parameters, as much as fluids or solids. Then, in a second independent step, we demonstrate that these states can be described in terms of equilibrium distributions which coincide with the Statistical Mechanics of powders first proposed by Edwards. We also derive the system equation of state as a function of the ``configurational temperature'', its new intensive thermody…
We perform three dimensional molecular dynamics simulations of cohesive granular particles under a plane shear. From the simulations, we found that the granular temperature of the system abruptly decreases to zero after reaching the critical temperature, where the characteristic time $t_{\rm cl}$ is approximately represented by $t_{\rm cl} \propto (ζ-ζ_{\rm cr})^{-β}$ with the dissipation rate $ζ$, the critical dissipation rate $ζ_{\rm cr}$ and the exponent $β\simeq 0.8$. We also found that there exist a variety types of clusters depending on the initial density and the dissipation rate.
We investigate theoretically how the stress propagation characteristics of granular materials evolve as they are subjected to increasing pressures, comparing the results of a two-dimensional scalar lattice model to those of a molecular dynamics simulation of slightly polydisperse discs. We characterize the statistical properties of the forces using the force histogram and a two-point spatial correlation function of the forces. For the lattice model, in the granular limit the force histogram has an exponential tail at large forces, while in the elastic regime the force histogram is much narrowe…
We present experimental evidence for a first-order freezing/melting phase transition in a nonequilibrium system -- an oscillated two-dimensional isobaric granular fluid. The steady-state transition occurs between a gas and a crystal and is characterized by a discontinuous change in both density and temperature. It is suppressed if the number of particles is incommensurate with the cell size, shows rate-dependent hysteresis, and obeys the Lindemann criterion for melting. Further, the measured equation of state both above and below the phase transition compares well with theory.
Base roughness plays an important role to the dynamics of granular flows but is yet poorly understood due to the difficulty of its quantification. For a bumpy base made by spheres, at least two factors should be considered to characterize its geometric roughness, namely the size ratio of base- to flow-particles and the packing of base particles. In this paper, we propose a definition of base roughness, Ra, which is a function of both the size ratio and the packing arrangement of base particles. The function is generalized for random and regular packing of multi-layered spheres, where the range…
According to the acoustic fluidization hypothesis, elastic waves at a characteristic frequency form inside seismic faults even in the absence of an external perturbation. These waves are able to generate a normal stress which contrasts the confining pressure and promotes failure. Here, we study the mechanisms responsible for this wave activation via numerical simulations of a granular fault model. We observe the particles belonging to the percolating backbone, which sustains the stress, to perform synchronized oscillations over ellipticlike trajectories in the fault plane. These oscillations o…
