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arXiv 0811.3457cond-mat.supr-con
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定向弱铁磁超导体RuSr $_2$ RCu $_2$ O $_8$(R =稀土)的各向异性磁性和超导性质

Anisotropic magnetic and superconducting properties of aligned weak-ferromagnetic superconductor RuSr$_2$RCu$_2$O$_8$ (R = rare earths)

B. C. Chang, C. H. Hsu, M. F. Tai, H. C. Ku, Y. Y. Hsu

摘要:

用粉末取向法研究了RuSr_2RCu_2O_8(R = Pr,Nd,Sm,Eu,Gd,Gd_(0.5)Dy_(0.5))弱铁磁超导体的各向异性物理性质。RuSr 2GdCu 2 O 8铜酸盐是一种弱铁磁超导体,在TN(Ru)= 131 K时具有Ru磁矩的磁序,在Tc = 56 K时CuO 2层发生超导转变,在TN(Gd)= 2.5K时具有低温Gd反铁磁序。由于该四元体系的弱磁各向异性,只有当R = Eu和Gd时,才能通过场旋转粉末取向方法在环氧树脂中获得高度c轴取向的微晶粉末(直径约1-10 $μ$ m),其中c轴垂直于取向的磁场Ba = 0.9 T,并平行于旋转轴。对于较小的稀土化合物R = Gd 0.5 Dy 0.5,可以使用简单场粉末排列方法实现粉末排列,其中c轴沿着排列的磁场部分排列。磁化率的各向异性温度依赖性的c轴取向的粉末表现出弱各向异性与$χ_{c} > χ_{ab}$在室温下由于各向异性稀土,Eu和Gd,贡献和交叉$χ_{c} < χ_{ab}$低于190 K,其中强Ru各向异性短程交换相互作用超过了稀土的贡献。由于晶粒尺寸小,在低于39 K的涡旋晶格熔化温度下,在1-G场中,定向微晶RuSr 2GdCu 2 O 8粉末/环氧树脂的各向异性抗磁超导晶内屏蔽信号比晶间多晶块体样品的信号弱得多(d ~ 1-10 $μ$ m)、长穿透深度($λ_{ab}$ ~ 0.55 $μ$ m,$λ_{c}$ ~ 0.66 $μ$ m)和CuO 2层的二维(2D)特征。

英文摘要:

The powder alignment method is used to investigate the anisotropic physical properties of the weak-ferromagnetic superconductor system RuSr2RCu2O8 (R = Pr, Nd, Sm, Eu, Gd, Gd0.5Dy0.5). The RuSr2GdCu2O8 cuprate is a weak-ferromagnetic superconductor with a magnetic ordering of Ru moments at TN(Ru) = 131 K, a superconducting transition in the CuO2 layers at Tc = 56 K, and a low temperature Gd antiferromagnetic ordering at TN(Gd) = 2.5 K. Due to weak magnetic anisotropy of this tetragonal system, highly c-axis aligned microcrystalline powder (diameter ~ 1-10 $μ$m) in epoxy can be obtained only for R = Eu and Gd through the field-rotation powder alignment method where c-axis is perpendicular to the aligned magnetic field Ba = 0.9 T and parallel to the rotation axis. For smaller rare earth compound R = Gd0.5Dy0.5, powder alignment can be achieved using the simple field powder alignment method where c-axis is partially aligned along the aligned magnetic field. The anisotropic temperature dependence of magnetic susceptibility for the c-axis aligned powders exhibit weak anisotropy with $χ_{c} > χ_{ab}$ at room temperature due to anisotropic rare earth, Eu and Gd, contribution and crossover to $χ_{c} < χ_{ab}$ below 190 K where strong Ru anisotropic short-range exchange interaction overtakes the rare earth contribution. Anisotropic diamagnetic superconducting intragrain shielding signal of aligned microcrystalline RuSr2GdCu2O8 powder-in-epoxy below vortex lattice melting temperature at 39 K in 1-G field is much weaker than the intergrain polycrystalline bulk sample signal due to the small grain size (d ~ 1-10 $μ$m), long penetration depth ($λ_{ab}$ ~ 0.55 $μ$m, $λ_{c}$ ~ 0.66 $μ$m) and the two-dimensional (2D) character of CuO2 layers.

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