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arXiv 1208.0760cond-mat.supr-concond-mat.str-el
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超导铁磁体RuSr2Gd1.4Ce 0.6Cu 2 O 10-δ的自旋动力学、短程有序和超顺磁性

Spin dynamics, short-range order and superparamagnetism in superconducting ferromagnet RuSr2Gd1.4Ce0.6Cu2O10-δ

Anuj Kumar, R. P. Tandon, V. P. S. Awana

摘要:

本文报道了超导铁磁体RuSr_2Gd_(1.4)Ce_(0.6)Cu_2 O_(10-δ)(GdRu-1222)的结构、详细的直流和线性/非线性交流、等温和热释电磁化研究。结构分析表明,GdRu-1222为四方晶系,空间群为I4/mmm。GdRu-1222是已报道的超导铁磁体,其Ru自旋在110 K附近具有磁有序性,并且在Cu-O2平面中具有低于40 K的超导性。详细的线性/非线性一次和更高次谐波的AC磁化率研究揭示了GdRu-1222的复杂磁性。在AC磁化率(χac)与T测量中观察到频率依赖性尖点。尖点位置随频率的变化符合Vogel-Fulcher定律,这是描述自旋玻璃(SG)系统的一个特征,该系统可能包含均匀/非均匀的磁相互作用/非相互作用的铁磁团簇。T = 60 K的热释光磁化(TRM)研究也支持这种解释. AC磁化结果的详细解释揭示了嵌入在自旋玻璃(SG)矩阵的不同大小的磁性(铁磁)均匀/非均匀的集群的形成。磁化与施加的磁场回路不饱和,即使在高施加的磁场(50 kOe),导致在系统中的短程磁有序,这导致在低温下冻结的集群的形成。一阶和三阶磁化率谐波的温度变化与Wohlfarth模型(WM)吻合得很好,导致超顺磁性(SPM)状态。详细的磁化(DC和AC两者)结果和它们的分析有助于解释GdRu-1222系统的温度依赖性磁性。

英文摘要:

We report structural, detailed DC and linear/non-linear AC, isothermal and thermoremanent magnetization study of the rutheno-cuprate superconducting ferromagnet RuSr2Gd1.4Ce0.6Cu2O10-δ (GdRu-1222). Structural analysis, by employing Rietveld refinement of X-ray diffraction pattern, reveals that GdRu-1222 crystallizes in tetragonal phase with I4/mmm space group. GdRu-1222 is a reported superconducting ferromagnet with Ru spins magnetic ordering at around 110 K and superconductivity below 40 K in Cu-O2 planes. Detailed linear/non-linear first and higher order harmonic of AC susceptibility studies unveiled the complex magnetism of GdRu-1222. A frequency dependent cusp is observed in AC susceptibility (χac) vs. T measurements. The change in cusp position with applied frequency followed the well known Vogel-Fulcher law, which is a feature to describe a spin-glass (SG) system with possibility of embedded homogeneous/non-homogeneous magnetically interacting/non-interacting ferromagnetic clusters. Such an interpretation is also supported by thermoremanent magnetization (TRM) study at T = 60 K. Detailed interpretation of AC magnetization results revealed the formation of magnetic (ferromagnetic) homogenous/non-homogenous clusters of different sizes embedded in spin-glass (SG) matrix. The magnetization vs. applied field loops do not saturate, even at high applied fields (50 kOe), resulting in the short-range magnetic ordering in the system, which causes the formation of clusters that freeze at low temperatures. Temperature variation of first- and third-order susceptibility harmonics show good agreement with Wohlfarth's model (WM), leading to the superparamagnetism (SPM) state. Detailed magnetization (DC and AC both) results and their analysis helped in explaining the temperature dependent magnetism of the GdRu-1222 system.

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