Recent experiments on bismuth have uncovered remarkably rich magnetization structure at fields well beyond the regime in which all carriers are expected to reside in the lowest Landau level. Motivated by these findings, we start from a microscopic tight-binding model and derive a low-energy Hamiltonian for the holes and three Dirac electrons pockets in bismuth. We find that an unconventional electron Zeeman effect, overlooked previously, suppresses the quantum limit for the electrons dramatically, giving rise to the observed anomalous magnetization structure. We further study interaction effects near fields at which the 2nd Landau level for one electron pocket empties, where magnetization hysteresis was observed. Here we find instabilities towards both charge density wave and Wigner crystal phases, and propose that hysteresis arises from a first-order transition out of the latter.
We have investigated the Se isotope effect in layered bismuth chalcogenide (BiCh2-based) superconductor LaO0.6F0.4Bi(S,Se)2 with 76Se and 80Se. For all examined samples, the Se concentration, which is linked to the superconducting properties, is successfully controlled within x = 1.09-1.14 in LaO0.6F0.4BiS2-xSex. From the magnetization and electrical resistivity measurements, changes in Tc are not observed for the LaO0.6F0.4Bi(S,Se)2 samples with 76Se and 80Se isotopes. Our results suggest that pairing in the BiCh2-based superconductors is not mediated by phonons, and unconventional supercondu…
We study the phase diagram of a two-dimensional ultracold Fermi gas with the synthetic spin-orbit coupling (SOC) that has recently been realized at NIST. Due to the coexistence of anisotropic SOC and effective Zeeman fields in the NIST scheme, the system shows rich structure of phase separation involving exotic gapless superfluid and Fulde-Ferrell-Larkin-Ovchinnikov (FFLO) pairing states with different center-of-mass momentum. In particular, we characterize the stability region of FFLO states and demonstrate their unique features under SOC. We then show that the effective transverse Zeeman fie…
Electrons in a metal subject to magnetic field commonly exhibit oscillatory behavior as the field strength varies, with a period set by the area of quantized electronic orbits. Recent experiments on elemental bismuth have revealed oscillations for fields above 9 tesla that do not follow this simple dependence and have been interpreted as a signature of electron fractionalization in the bulk. We argue instead that a simple explanation in terms of the surface states of bismuth exists when additional features of the experiment are included. These surface electrons are known to have significant sp…
We find that a model Hamiltonian of s-wave superconductors in the presence of spin-orbit interactions and a Zeeman field is exactly solvable. Most intriguingly, based on the exact solutions, an unconventional type of Fulde-Ferrel-Larkin-Ovchinnikov (FFLO) ground state is rigorously revealed, in which the center-of-mass momentum of the fermion pair is proportional to the Zeeman field. We also elaborate on the drifting effect of the Zeeman field on the spin-orbit-coupled Bose-Einstein condensate.
As shown in former papers, the nonadiabatic Heisenberg model presents a novel mechanism of Cooper pair formation generated by the strongly correlated atomic-like motion of the electrons in narrow, roughly half-filled "superconducting bands". These are energy bands represented by optimally localized spin-dependent Wannier functions adapted to the symmetry of the material under consideration. The formation of Cooper pairs is not the result of an attractive electron-electron interaction but can be described in terms of quantum mechanical constraining forces constraining the electrons to form Coop…
We derive the Ginzburg-Landau theory of unconventional singlet superconductors in the presence of a Zeeman field and impurities, in order to examine the resulting Fulde-Ferrell-Larkin-Ovchinnikov (FFLO) phases. We show that the behavior of the FFLO phases in unconventional superconductors in the presence of impurities is qualitatively different from that found for s-wave superconductors.
Chiral symmetry breaking of phonons plays an essential role in emergent quantum phenomena owing to its strong coupling to spin degree of freedom. However, direct experimental evidence of the chiral phonon-spin coupling is lacking. In this study, we report a chiral phonon-mediated interlayer exchange interaction in atomically controlled ferromagnetic metal (SrRuO3)-nonmagnetic insulator (SrTiO3) heterostructures. Owing to the unconventional interlayer exchange interaction, we have observed rotation of magnetic moments as a function of nonmagnetic insulating spacer thickness, resulting in a spin…
We develop a theory of the coexistence of superconductivity (SC) and antiferromagnetism (AFM) in CeCoIn5. We show that in Pauli-limited nodal superconductors the nesting of the quasi-particle pockets induced by Zeeman pair-breaking leads to incommensurate AFM with the moment normal to the field. We compute the phase diagram and find a first order transition to the normal state at low temperatures, absence of normal state AFM, and coexistence of SC and AFM at high fields, in agreement with experiments. We also predict the existence of a new double-Q magnetic phase.
Chains of magnetic atoms, placed on the surface of s-wave superconductors, have been established as a laboratory for the study of Majorana bound states. In such systems, the breaking of time reversal due to magnetic moments gives rise to the formation of in-gap states, which hybridize to form one-dimensional topological superconductors. However, in unconventional superconductors even non-magnetic impurities induce in-gap states since scattering of Cooper pairs changes their momentum but not their phase. Here, we propose a path for creating topological superconductivity, which is based on an un…
We report the observation of the fractional quantum Hall effect in the lowest Landau level of a two-dimensional electron system (2DES), residing in the diluted magnetic semiconductor Cd(1-x)Mn(x)Te. The presence of magnetic impurities results in a giant Zeeman splitting leading to an unusual ordering of composite fermion Landau levels. In experiment, this results in an unconventional opening and closing of fractional gaps around filling factor v = 3/2 as a function of an in-plane magnetic field, i.e. of the Zeeman energy. By including the s-d exchange energy into the composite Landau level spe…
The paper is devoted to a study of superconducting properties of population-imbalanced fermionic mixtures in quasi-one dimensional optical lattices. The system can be effectively described by the attractive Hubbard model with the Zeeman magnetic field term. We investigated the ground state phase diagram of the model as a function of the chemical potential and the magnetic field. The ground state of the system exhibits the conventional BCS-type superconductivity as well as the unconventional so-called Fulde-Ferrell-Larkin-Ovchinnikov state, in which the total momentum of Cooper pairs is non-zer…
Two-dimensional magnetic materials have recently attracted great interest due to their unique functions as the electric field control of a magnetic phase and the anomalous spin Hall effect. For such remarkable functions, a spin-orbit coupling (SOC) serves as an essential ingredient. Here we report a giant positive magnetoresistance in a layered magnetic semiconductor AgCrSe2, which is a manifestation of the subtle combination of the SOC and Zeeman-type spin splitting. When the carrier concentration approaches the critical value of 2.5\times10^18 cm^-3, a sizable positive magnetoresistance of ~…
We investigated the magnetism under a magnetic field in the quasi-two-dimensional organic Mott insulator $κ$-(BEDT-TTF)$_{2}$Cu[N(CN)$_{2}$]Cl through magnetization and $^{13}$C-NMR measurements. We found that in the nominally paramagnetic phase (i.e., above Néel temperature) the field-induced local moments have a staggered component perpendicular to the applied field. As a result, the antiferromagnetic transition well defined at a zero field becomes crossover under a finite field. This unconventional behavior is qualitatively reproduced by the molecular-field calculation for Hamiltonian inclu…
Numerical studies by Wójs, Yi and Quinn have suggested that an unconventional fractional quantum Hall effect is plausible at filling factors $ν=$ 1/3 and 1/5, provided the interparticle interaction has an unusual form for which the energy of two fermions in the relative angular momentum three channel dominates. The interaction between composite fermions in the second $Λ$ level (composite fermion analog of the electronic Landau level) satisfies this property, and recent studies have supported unconventional fractional quantum Hall effect of composite fermions at $ν^*=$ 4/3 and 5/3, which manife…
We study superconducting properties of population-imbalanced ultracold Fermi mixtures in the honeycomb lattice that can be effectively described by the spin-imbalanced attractive Hubbard model in the presence of a Zeeman magnetic field. We use the mean-field theory approach to obtain ground state phase diagrams including some unconventional superconducting phases such as the Fulde--Ferrell--Larkin--Ovchinnikov (FFLO) phase. We show that this phase is characterized by atypical behaviour of the Cooper pairs total momentum in the external magnetic field. We show that the momentum changes its valu…
The $J_1$-$J_2$ quantum spin sawtooth chain is a paradigmatic one-dimensional frustrated quantum spin system exhibiting unconventional ground-state and finite-temperature properties. In particular, it exhibits a flat energy band of one-magnon excitations accompanied by an enhanced magnetocaloric effect for two singular ratios of the basal interactions $J_1$ and the zigzag interactions $J_2$. In our paper, we demonstrate that one can drive the spin system into a flat-band scenario by applying an appropriate electric field, thus overcoming the restriction of fine-tuned exchange couplings $J_1$ a…
It is shown that unconventional nature of superconducting state of PrOs_4Sb_12, a Pr-based heavy electron compound with the filled-Skutterudite structure, can be explained in a unified way by taking into account the structure of the crystalline-electric-field (CEF) level, the shape of the Fermi surface determined by the band structure calculation, and a picture of the quasiparticles in f$^{2}$-configuration with magnetically singlet CEF ground state. Possible types of pairing are narrowed down by consulting recent experimental results. In particular, the chiral "p"-wave states such as p_x+ip_y…
Recently, the interplay between the Dirac/Weyl fermion and various bulk properties, such as magnetism, has attracted considerable attention, since unconventional transport and optical phenomena were discovered. However, the design principles for such materials have not been established well. Here, we propose that the layered material $A$Mn$X_2$ ($A$: alkaline and rare-earth ions, $X$: Sb, Bi) is a promising platform for systematically exploring strongly correlated Dirac metals, which consists of the alternative stack of the $X^-$ square net layer hosting a 2D Dirac fermion and the $A^{2+}$-Mn$…
Topological states of matter are, generally, quantum liquids of conserved topological defects. We establish this by constructing and analyzing topological field theories which describe the dynamics of field singularities using gauge fields. Homotopy groups are utilized to identify topologically protected singularities, and the conservation of their protected number is captured by a topological action term that unambiguously obtains from the given set of symmetries. Stable phases of these theories include quantum liquids with emergent massless Abelian and non-Abelian gauge fields, as well as to…
We analyze the strongly correlated regime of a two-component trapped ultracold fermionic gas in a synthetic non-Abelian U(2) gauge potential, that consists of both a magnetic field and a homogeneous spin-orbit coupling. This gauge potential deforms the Landau levels (LLs) with respect to the Abelian case and exchanges their ordering as a function of the spin-orbit coupling. In view of experimental realizations, we show that a harmonic potential combined with a Zeeman term, gives rise to an angular momentum term, which can be used to test the stability of the correlated states obtained through …
