Emission spectra of quantum dot arrays in zero-dimensional microcavities are studied theoretically, and it is shown that they are determined by the competition between the formation of the collective superradiant mode and inhomogeneous broadening. The random sources method for the calculation of photoluminescence spectra under a non-resonant pumping is developed, and a microscopic justification of the random sources method within a framework of the standard diagram technique is given. The emission spectra of a microcavity are analyzed with allowance for the spread of exciton states energies caused by an inhomogeneous distribution of quantum dots and a tunneling between them. It is demonstrated that in the case of a strong tunneling coupling the luminescence spectra are sensitive to the geometric positions of the dots, and the collective mode can, under certain conditions, be stabilized by the random tunnel junctions.
At the occasion of the OECS conference in Madrid, we give a succinct account of some recent predictions in the spectroscopy of a quantum dot in a microcavity that remain to be observed experimentally, sometimes within the reach of the current state of the art.
We have fabricated and studied the photoluminescence from microdisks containing single, selected self-assembled quantum dots. Using two electron beam lithography exposures and a two-step selective wet etching process, the dots were positioned at the microdisks edges with sub-micron precision. The selection and positioning of quantum dots enables an optimum coupling of the dot emission to the microdisks whispering modes.
The emission properties of single quantum dots in planar microcavities are studied experimentally and theoretically. Fivefold Enhanced spontaneous emission outside the microcavity is found for dots in resonance with the cavity mode, relative to detuned dots, while their radiative lifetime is only marginally decreased. Using high power excitation we obtain the in-plane cavity dispersion. Near field images of the emission show spatial distributions of several microns for resonant dots, which decrease in size with the detuning from resonance. These experimental findings are explained using a simp…
We have recently developed a self-consistent theory of Strong-Coupling in the presence of an incoherent pumping [arXiv:0807.3194] and shown how it could reproduce quantitatively the experimental data [PRL 101, 083601 (2008)]. Here, we summarize our main results, provide the detailed analysis of the fitting of the experiment and discuss how the field should now evolve beyond merely qualitative expectations, that could well be erroneous even when they seem to be firmly established.
e study theoretically, the photoluminescence properties of a single quantum dot in a microcavity under incoherent excitation. We propose a microscopic quantum statistical approach providing a Lindblad (thus completely positive) description of pumping and decay mechanisms of the quantum dot and of the cavity mode. Our analytical results show that strong coupling (SC) and linewidths are largely independent on the pumping intensity (until saturation effects come into play), in contrast to previous theoretical findings. We shall show the reliable predicting character of our theoretical framework i…
We discuss the topical and fundamental problem of strong-coupling between a quantum dot an the single mode of a microcavity. We report seminal quantitative descriptions of experimental data, both in the linear and in the nonlinear regimes, based on a theoretical model that includes pumping and quantum statistics.
We show theoretically that the emission spectrum of a single large quantum dot strongly coupled to a single photon mode in a microcavity can be qualitatively different from the spectrum obtained with an atom in a cavity. Instead of the well-known Mollow triplet we predict appearance of multiplets with the number of peaks a function of the quantum dot size and pumping intensity. The mutiplets can appear if the quantum dot is larger than the exciton Bohr radius, so that excitons are confined as whole particles in the dot. In this case the Pauli principle is relaxed and one can accommodate more t…
We present a microscopic theory of optical initialization, control and detection for a single electron spin in a quantum dot embedded into a zero-dimensional microcavity. The strong coupling regime of the trion and the cavity mode is addressed. We demonstrate that efficient spin orientation by a single circularly polarized pulse is possible in relatively weak transverse magnetic fields. The possibilities for spin control by additional circularly polarized pulse are analyzed. Under optimal conditions the Kerr and Faraday rotation angles induced by the spin polarized electron may reach tens of d…
We show that strong-coupling (SC) of light and matter as it is realized with quantum dots (QDs) in microcavities differs substantially from the paradigm of atoms in optical cavities. The type of pumping used in semiconductors yields new criteria to achieve SC, with situations where the pump hinders, or on the contrary, favours it. We analyze one of the seminal experimental observation of SC of a QD in a pillar microcavity [Reithmaier et al., Nature (2004)] as an illustration of our main statements.
We provide a unified theory of luminescence spectra of coupled light-matter systems realized with semiconductor heterostructures in microcavities, encompassing: i) the spontaneous emission case, where the system decays from a prepared (typically pure) initial state, and ii) luminescence in the presence of a continuous, incoherent pump. While the former case has been amply discussed in the literature (albeit mainly for the case of resonance), no consideration has been given to the influence of the incoherent pump. We show how, by provoking a self-consistent quantum state, the pump considerably …
In this comment we show that there is a direct connection between coherent exchange of energy among light and matter and the emission spectrum of a microcavity quantum dot system as modeled in Phys. Rev. B 79, 235325 (2009) [arXiv:0807.3194] by F. P. Laussy, E. del Valle, and C. Tejedor. To do so, we show that in their model the necessary and sufficient conditions for having eigenvalues with non-zero imaginary parts in the propagator of the bare mode populations, are the same as for having strong coupling in the emission spectrum. This amounts to saying that, whenever there is strong coupling …
The light emission rate of a single quantum dot can be drastically enhanced by embedding it in a resonant semiconductor microcavity. This phenomenon is known as the Purcell effect, and the coupling strength between emitter and cavity can be quantified by the Purcell factor. The most natural way for probing the Purcell effect is a time-resolved measurement. However, this approach is not always the most convenient one, and alternative approaches based on a continuous-wave measurement are often more appropriate. Various signatures of the Purcell effect can indeed be observed using continuous-wave…
There exists a growing interest in the properties of the light generated by hybrid systems involving a mesoscopic number of emitters as a means of providing macroscopic quantum light sources. In this work, the quantum correlations of the light emitted by a collection of emitters coupled to a generic optical cavity are studied theoretically using an effective Hamiltonian approach. Starting from the single-emitter level, we analyse the persistence of photon antibunching as the ensemble size increases. Not only is the photon blockade effect identifiable, but photon antibunching originated from de…
The future of quantum communication systems and quantum networks heavily rely on the ability to fabricate and coherently control the conversion of photons between different modes based on a solid-state plateform. In this work, we propose and theoretically investigate a scheme to optomechanically control coherent mode conversion of optical photons by utilizing two optically coupled hybrid semiconductor microcavities containing a quantum dot (QD). One of the microcavity is pumped by an external laser and the second cavity is driven by light emitted by the QD that is embedded in the interface sep…
Measured and calculated results are presented on the emission properties of a new class of emitters operating in the cavity quantum electrodynamics regime. The structures are based on high-finesse GaAs/AlAs micropillar cavities, each with an active medium consisting of a layer of InGaAs quantum dots and distinguishing feature of having substantial fraction of spontaneous emission channeled into one cavity mode (high-beta factor). This paper shows that the usual criterion for lasing with a conventional (low-beta factor) cavity, a sharp nonlinearity in an input-output curve accompanied by notice…
In this chapter we will discuss the technology and experimental techniques to realize quantum dot (QD) single photon sources combining high outcoupling efficiencies and highest degrees of non-postselected photon indistinguishability. The system, which is based on ultra low density InAs QDs embedded in a quasi planar single sided microcavity with natural photonic traps is an ideal testbed to study quantum light emission from single QDs. We will discuss the influence of the excitation conditions on the purity of the single photon emission, and in particular on the degree of indistinguishability …
We investigate coupling of localized spins in a semiconductor quantum dot embedded in a microcavity with a finite quality factor. The lowest cavity mode and the quantum dot exciton are coupled forming a polariton, whereas excitons interact with localized spins via exchange. The finite quality of the cavity Q is incorporated in the model Hamiltonian by adding an imaginary part to the photon frequency. The Hamiltonian, which treats photons, spins and excitons quantum mechanically, is solved exactly. Results for a single polariton clearly demonstrate the existence of a resonance, sharper as the t…
We discuss the luminescence spectra of coupled light-matter systems realized with semiconductor heterostructures in microcavities in the presence of a continuous, incoherent pumping, when the matter field is Fermionic. The linear regime--which has been the main topic of investigation both experimentally and theoretically--converges to the case of coupling to a Bosonic material field, and has been amply discussed in the first part of this work. We address here the nonlinear regime, and argue that, counter to intuition, it is better observed at low pumping intensities. We support our discussion …
We compare three different notions of concurrence to measure the polarization entanglement of two-photon states generated by the biexciton cascade in a quantum dot embedded in a microcavity. We focus on the often-discussed situation of a dot with finite biexciton binding energy in a cavity tuned to the two-photon resonance. Apart from the time-dependent concurrence, which can be assigned to the two-photon density matrix at any point in time, we study single- and double-time integrated concurrences commonly used in the literature that are based on different quantum state reconstruction schemes.…
Collective (elementary) excitations of quantum bosonic condensates, including condensates of exciton polaritons in semiconductor microcavities, are a sensitive probe of interparticle interactions. In anisotropic microcavities with momentum-dependent TE-TM splitting of the optical modes, the excitations dispersions are predicted to be strongly anisotropic, which is a consequence of the synthetic magnetic gauge field of the cavity, as well as the interplay between different interaction strengths for polaritons in the singlet and triplet spin configurations. Here, by directly measuring the disper…
Recent photoabsorption measurements have revealed a rich fine structure in the collective charge-density excitation spectrum of few-electron quantum dots in the presence of magnetic fields. We have performed systematic computational studies of the far-infrared density response of quantum dots, using time-dependent density-functional theory in the linear regime and treating the dots as two-dimensional disks. It turns out that the main characteristics observed in the experiment can be understood in terms of the electronic shell structure of the quantum dots. However, new features arise if a brea…
The emission spectrum of exciton complexes formed in individual self-assembled quantum dots (QDs) embedded into a p-n junction is theoretically studied using an effective mass model. We calculate the particle Coulomb interactions, eletron-hole overlaps and transition energies of exciton complexes for the different strength and direction of electric field. Both redshifts and blueshifts are observed in exciton, trions and biexciton. The Stark effect may be applied to manipulate the spontaneous emission rate of individual QDs embedded in microcavities.
A theory of optical emission of quantum dot arrays in quantum microcavities is developed. The regime of the strong coupling between the quantum dots and photonic mode of the cavity is considered. The quantum dots are modeled as two-level systems. In the low pumping (linear) regime the emission spectra are mainly determined by the superradiant mode where the effective dipoles of the dots oscillate in phase. In the non-linear regime the superradiant mode is destroyed and the emission spectra are sensitive to the parity of quantum dot number. Further increase of the pumping results in the line wi…
Most optical quantum devices require deterministic single-photon emitters. Schemes so far demonstrated in the solid state imply an energy relaxation which tends to spoil the coherent nature of the time evolution, and with it the photon indistinguishability. We focus our theoretical investigation on semiconductor quantum dots embedded in microcavities. Simple and general relations are identified between the photon indistinguishability and the collection efficiency. The identification of the key parameters and of their interplay provides clear indications for the device optimization.
A theoretical investigation is presented of the statistics of excitons in quantum dots (QDs) of different sizes. A formalism is developed to build the exciton creation operator in a dot from the single exciton wavefunction and it is shown how this operator evolves from purely fermionic, in case of a small QD, to purely bosonic, in case of large QDs. Nonlinear optical emission spectra of semiconductor microcavities containing single QDs are found to exhibit a peculiar multiplet structure which reduces to Mollow triplet and Rabi doublet in fermionic and bosonic limits, respectively.
We demonstrate non-perturbative coupling between a single self-assembled InGaAs quantum dot and an external fiber-mirror based microcavity. Our results extend the previous realizations of tunable microcavities while ensuring spatial and spectral overlap between the cavity-mode and the emitter by simultaneously allowing for deterministic charge control of the quantum dots. Using resonant spectroscopy, we show that the coupled quantum dot cavity system is at the onset of strong coupling, with a cooperativity parameter of 2. Our results constitute a milestone towards the realization of a high eff…
We study the collective interaction of excitons in closely spaced artificial molecules and arrays of nearly identical quantum dots with the electromagnetic modes. We discuss how collective fluorescence builds up in the presence of a small mismatch of the transition energy. We show that a superradiant state of a single exciton in a molecule of two dots with realistic energy mismatch undergoes a two-rate decay. We analyze also the stability of subdecoherent states for non-identical systems.
We study the spontaneous emission from a coherently delocalized exciton state in a double quantum dot as a function of the distance between the dots, focusing on the similarities and differences between the cases of radiative (long-range, dipole) and tunnel coupling between the excitons in the dots. We show that there may be no qualitative difference between the collective emission induced by these two coupling types in spite of their essentially different physical properties.
Polariton emission from optical cavities integrated with various luminophores has been extensively studied recently due to the wide variety of possible applications in photonics, particularly promising in terms of fabrication of low-threshold sources of coherent emission. Tuneable microcavities allow extensive investigation of the photophysical properties of matter placed inside the cavity by deterministically changing the coupling strength and controllable switching from weak to strong and ultra-strong coupling regimes. Here we demonstrate room temperature strong coupling of exciton transitio…
We investigate different types of collective excitations in a quantum dot containing finite number of electrons at zero magnetic field. To estimate the excitation energies analytically we follow the energy weighted sum-rule approach. We consider the most general multipole excitation with angular momentum l, and the breathing mode excitation (monopole excitation) of a large quantum dot, for three different types of effective electron-electron interaction. These are the logarithmic interaction, the short range pseudopotential and the coulomb interaction. The ground state density of the many-body…
We study the evolution of a quantum state of a double quantum dot system interacting with the electromagnetic environment and with the lattice modes, in the presence of a coupling between the two dots. We propose a unified approach to the simulation of the system evolution under joint impact of the two reservoirs. We discuss the sub- and superradiant radiative decay of the system, the phonon-induced decay of entanglement between the dots, and the transfer of excitation between them.
A theory of non-linear emission of quantum dot ensembles coupled to the optical mode of the microcavity is presented. Numerical results are compared with analytical approaches. The effects of exciton-exciton interaction within the quantum dots and with the reservoir formed by nonresonant pumping are considered. It is demonstrated, that the nonlinearity due to the interaction strongly affects the shape of the emission spectra. The collective superradiant mode of the excitons is shown to be stable against the non-linear effects.
We discuss the properties of few electrons and electron-hole pairs confined in coupled semiconductor quantum dots, with emphasis on correlation effects and the role of tunneling. We shall discuss, in particular, exact diagonalization results for biexciton binding energy, electron-hole localization, magnetic-field induced Wigner molecules, and spin ordering.
In the regime of strong coupling between molecular excitons and confined optical modes, the intra-molecular degrees of freedom are profoundly affected, leading to a reduced vibrational dressing of polaritons compared to bare electronically excited states. However, existing models only describe a single vibrational mode in each molecule, while actual molecules possess a large number of vibrational degrees of freedom and additionally interact with a continuous bath of phononic modes in the host medium in typical experiments. In this work, we investigate a small ensemble of molecules with an arbi…
Narrow line-widths and the possibility of enhanced spontaneous emission via coupling to microcavities make semiconductor quantum dots ideal for harnessing coherent quantum phenomena at the single photon level. So far, however, all approaches have relied on incoherent pumping, which limits the desirable properties of the emission. In contrast, coherent excitation was recognized to be necessary for providing both improved photon indistinguishability and high efficiency, and offers the quantum control capabilities required for basic qubit manipulations. Here we achieve, for the first time, resona…
We report a full (3D) micromagnetic simulation of a set of 100 ferrite (Fe$_3$O$_4$) cylindrical dots, arranged in a 10 by 10 square (planar) array of side 3.27 $μ$m, excited by an external in-plane magnetic field. The resulting power spectrum of magnetic excitations and the dynamical magnetization field at the resulting resonance modes were investigated. The absorption spectrum deviates considerably from that of a single particle reference simulation, presenting a mode-shifting and splitting effect. We found an inversion symmetry through the center of the array, in the sense that each particl…
We propose that an optically excited heavy hole in a quantum dot can drive the surrounding nuclear spins into a quiescent collective state, leading to significantly prolonged coherence time for the electron spin qubit. This provides a general paradigm to combat decoherence by environmental control without involving the active qubit in quantum information processing. It also serves as a unified solution to some open problems brought about by two recent experiments [X. Xu et al., Nature 459, 1105 (2009) and C. Latta et al., Nature Phys. 5, 758 (2009)].
We present a theoretical analysis of the intensity autocorrelation for the spontaneous emission from a planar ensemble of self-assembled quantum dots. Using the quantum jump approach, we numerically simulate the evolution of the system and construct photon-photon delay time statistics that approximates the second order correlation function of the field. The form of this correlation function in the case of collective emission from a highly homogeneous ensemble qualitatively differs form that characterizing an ensemble of independent emitters (inhomogeneous ensemble of uncoupled dots). The signa…
We analyse the ground state properties of vertical double quantum dots in the lowest Landau level regime for filling factor ν=2. This analysis follow two lines: on the one hand, we study the dispersion relation of different collective excitations and look for the roton-type minima that signal some type of order within the ground state. On the other hand, we calculate expected values of the antiferremagnetic order operator defined as <S_x^RS_x^L>. We conclude that of the three existing types of ground state at ν=2 the canted and symmetric states show spin order on the plane of the dots. In the …
We theoretically investigate the nonlinear effects in a hybrid quantum optomechanical system consisting of two optically coupled semiconductor microcavities containing a quantum dot and a Kerr nonlinear substrate.The steady state behavior of the mean intracavity optical field demonstrates that the system can be used as an all optical switch. We further investigate the spectrum of small fluctuations in the mechanical displacement of the movable distributed Bragg reflectors (DBR) and observe that normal mode splitting (NMS) takes place for high Kerr nonlinearity and pump power. In addition, we h…
The spectral and dispersive emission properties are analytically determined for the two-dimensional system of exciton-polaritons in microcavities excited by a resonant and coherent optical pump. New collective excitations result from the anomalous coupling between one generic polariton state and its idler, created by the scattering of two pumped polaritons. The corresponding parametric correlation is stimulated by the emitter and idler populations and drives very efficiently the luminescence. The intrinsic properties of the collective excitations determine a peculiar emission pattern.
Site-controlled growth of semiconductor quantum dots (QDs) represents a major advancement to achieve scalable quantum technology platforms. One immediate benefit is the deterministic integration of quantum emitters into optical microcavities. However, site-controlled growth of QDs is usually achieved at the cost of reduced optical quality. Here, we show that the buried-stressor growth technique enables the realization of high-quality site-controlled QDs with attractive optical and quantum optical properties. This is evidenced by performing excitation power dependent resonance fluorescence expe…
Deviations from the uniform oscillator spacing, related to the shape of the confining potential, have a strong influence on few-electron states in quantum dots when Coulomb effects are included. Distinct signatures are found for level spacings increasing (pot shape) and decreasing (cone shape) with energy. Cone deformations affect the levels near the ground state, such that observable effects are predicted. Pot deformations partially negate the effect of the Coulomb force, thus their spectra are similar to those of a perfect oscillator with a smaller Coulomb repulsion. The Coulomb force is tre…
The large arrays of magnetic dots are the building blocks of magnonic crystals and the emerging bit patterned media for future recording technology. In order to fully utilize the functionalities of high density magnetic nanodots, a method for the selective reversal of a single nanodot in a matrix of dots is desired. We have proposed a method for magnetization reversal of a single nanodot with microwave excitation in a matrix of magneto-statically interacting dots. The method is based on the excitation of collective modes and the spatial anomaly in the microwave power absorption. We perform num…
For a scalable photonic device producing entangled photons, it is desirable to have multiple quantum emitters in an ensemble that can be collectively excited, despite their spectral variability. For quantum dots, Rabi rotation, the most popular method for resonant excitation, cannot assure a universal, highly efficient excited state preparation, because of its sensitivity to the excitation parameters. In contrast, Adiabatic Rapid Passage (ARP), relying on chirped optical pulses, is immune to quantum dot spectral inhomogeneity. Here, we advocate the robustness of ARP for simultaneous excitation…
Entangled photon sources are crucial for quantum optics, quantum sensing and quantum communication. Semiconductor quantum dots generate on-demand entangled photon pairs via the biexciton-exciton cascade. However, the pair of photons are emitted isotropically in all directions, thus limiting the collection efficiency to a fraction of a percent. Moreover, strain and structural asymmetry in quantum dots lift the degeneracy of the intermediate exciton states in the cascade, thus degrading the measured entanglement fidelity. Here, we propose an approach for generating a pair of entangled photons fr…
The possibility of steady-state population inversion in a small sample of strongly driven two-level emitters like quantum dots (QDs) in micro-cavities, and its utilization towards amplification of light and acoustic waves is investigated theoretically. We find that inversion and absorption spectrum of photons, and phonons crucially depend on the interplay between the intrinsic vacuum and phonon environments. The absorption profiles of photons and phonons show marked novel features like gain instead of transparency and absorption reversed to gain, respectively. Furthermore, we report collectivi…
Motivated by recent developments on the fabrication and control of semiconductor-based quantum dot qubits, we theoretically study a finite system of tunnel-coupled quantum dots with the electrons interacting through the long-range Coulomb interaction. When the inter-electron separation is large and the quantum dot confinement potential is weak, the system behaves as an effective Wigner crystal with a period determined by the electron average density with considerable electron hopping throughout the system. For stronger periodic confinement potentials, however, the system makes a crossover to a…
Lattice vibration modes are collective excitations in periodic arrays of atoms or molecules. These modes determine novel transport properties in solid crystals. Analogously, in periodical arrangements of magnetic vortex-state disks, collective vortex motions have been predicted. Here, we experimentally observe wave modes of collective vortex gyration in one-dimensional (1D) chains of periodic disks using time-resolved scanning transmission x-ray microscopy. The observed modes are interpreted based on micromagnetic simulation and numerical calculation of coupled Thiele equations. Dispersion of …
Spin rotations induced by an AC electric field in a two-electron double quantum dot are studied by an exact numerical solution of the time dependent Schroedinger equation in the context of recent electric dipole spin resonance experiments based on the Pauli blockade. We demonstrate that the splitting of the main resonance line by the spin exchange coupling is accompanied by the appearance of fractional resonances and that both these effects are triggered by interdot tunnel coupling. We find that the AC driven system generates residual but distinct harmonics of the driving frequency which are a…
A theoretical investigation has been made of the magnetoplasmon excitations in a quasi-one-dimensional electron system comprised of vertically stacked, self-assembled InAs/GaAs quantum dots. The smaller length scales involved in the experiments impel us to consider a perfectly periodic system of two-dimensionally confined InAs quantum dot layers separated by GaAs spacers. Subsequent system is subjected to a two-dimensional confining (harmonic) potential in the x-y plane and an applied magnetic field (B) in the symmetric gauge. This scheme defines virtually a system of quantum wire comprised of…
We report on the theoretical investigation of the elementary electronic excitations in a quantum wire made up of vertically stacked self-assembled InAs/GaAs quantum dots. The length scales (of a few nanometers) involved in the experimental setups prompt us to consider an infinitely periodic system of two-dimensionally confined (InAs) quantum dot layers separated by GaAs spacers. The the Bloch functions and the Hermite functions together characterize the whole system. We then make use of the Bohm-Pines' (full) random-phase approximation in order to derive a general nonlocal, dynamic dielectric …
