We have used an electromigration technique to fabricate a $\rm{C_{60}}$ single-molecule transistor (SMT). Besides describing our electromigration procedure, we focus and present an experimental study of a single molecule quantum dot containing an even number of electrons, revealing, for two different samples, a clear out-of-equilibrium Kondo effect. Low temperature magneto-transport studies are provided, which demonstrates a Zeeman splitting of the finite bias anomaly.
Tunnelling conductances observed for mesoscopic Kondo systems exhibit a zero-bias peak and two coherent side peaks. The former peak is usually understood as a Kondo effect and the latter side peak is recently clarified as the effect of inter-reservoir coherence. However, fitting the experimental $dI/dV$ line shapes, where $I$ and $V$ denote the current and bias voltage, respectively, has not been performed theoretically. Here, we fit the entire line shape range of the tunnelling conductance observed for a quantum dot, quantum point contact, and magnetized atom adsorbed on an insulating layer c…
In a single-walled carbon nanotube, we observe the spin-1/2 Kondo effect. The energy of spin-resolved Kondo peaks is proportional to magnetic field at high fields, contrary to recent reports. At lower fields, the energy falls below this linear dependence, in qualitative agreement with theoretical expectations. For even electron occupancy, we observe a spin-1 Kondo effect due to the degeneracy of the triplet ground states. Tuning gate voltage within the same Coulomb diamond drives a transition to a singlet ground state. We also independently tune the energy difference between singlet and triple…
We investigate theoretically and experimentally the singlet-triplet Kondo effect induced by a magnetic field in a molecular junction. Temperature dependent conductance, $G(T)$, is calculated by the numerical renormalization group, showing a strong imprint of the relevant low energy scales, such as the Kondo temperature, exchange and singlet-triplet splitting. We demonstrate the stability of the singlet-triplet Kondo effect against weak spin anisotropy, modeled by an anisotropic exchange. Moderate spin anisotropy manifests itself by lowering the Kondo plateaus, causing the $G(T)$ to deviate fro…
From our theoretical studies of resonant Raman transitions in two-electron quantum dots (artificial helium atoms) we show that in this system, the singlet-triplet Raman transitions are allowed (in polarized configuration) only in the presence of spin-orbit interactions. With an increase of the applied magnetic field this transition dominates over the singlet-singlet and triplet-triplet transitions. This intriguing effect can therefore be utilized to tune Raman transitions as well as the spin-orbit coupling in few-electron quantum dots.
We apply an elementary measurement scheme to calculate the electronic triplet-singlet transition mediated by hyperfine interaction in a double quantum dot. We show how the local character of the hyperfine interaction and the nuclear back-action process (flip-flop) are crucial to cancel destructive interferences of the triplet-singlet transition probability. It is precisely this cancellation which differentiates the hyperfine interaction from an anisotropic magnetic field which mixes the triplet and the singlet eigenstates.
The tunneling conductances of a quantum point contact and a magnetized atom adsorbed on an insulating layer above a metallic substrate are obtained by considering the coherent transport of the entangled and nonentangled Kondo singlets, and these are compared with the experimental results. Spins of the entangled Kondo singlet flow unidirectionally in a sequential up-and-down manner. This transport does not follow linear response theory. The nonentangled Kondo singlet performs resonant tunneling through a coherent transport channel and yields coherent side peaks at a finite bias. The coherent tr…
We present a study of spin 1/2 Kondo singlets in single electron transistors under a microwave frequency bias excitation. We compare time-averaged conductance $G$ to predicted universal response with respect to microwave frequency, oscillation amplitude and the Kondo temperature and find a non-adiabatic response when the microwave photon energy $hf$ is comparable to the Kondo temperature $k_B T_K$. We show that our measurements are qualitatively consistent with the predictions for the radiation-induced decoherence rate of the Kondo spin.
Transition metal dichalcogenides (TMDCs) heterostructure with a type II alignment hosts unique interlayer excitons with the possibility of spin-triplet and spin-singlet states. However, the associated spectroscopy signatures remain elusive, strongly hindering the understanding of the Moire potential modulation of the interlayer exciton. In this work, we unambiguously identify the spin-singlet and spin-triplet interlayer excitons in the WSe2/MoSe2 hetero-bilayer with a 60-degree twist angle through the gate- and magnetic field-dependent photoluminescence spectroscopy. Both the singlet and tripl…
An artifcial two-atomic molecule, also called a double quantum dot (DQD), is an ideal system for exploring few electron physics. Spin-entanglement between just two electrons can be explored in such systems where singlet and triplet states are accessible. These two spin-states can be regarded as the two states in a quantum two-state system, a so-called singlet-triplet qubit. A very attractive material for realizing spin based qubits is the carbon nanotube (CNT), because it is expected to have a very long spin coherence time. Here we show the existence of a gate-tunable singlet-triplet qubit in …
In a GaAs single quantum dot, the relaxation time T_{1} between spin triplet and singlet states has been measured for the last few even number of electrons. The singlet-triplet energy separation E_{ST} is tuned as a control parameter for the comparison of T_{1} between different electron numbers. T_{1} shows a steady decrease from 2-electrons, 4-electrons, to 6-electrons, and we found this implies an enhancement of the spin-orbital coupling strength in a multi-electron quantum dot.
In double quantum dot singlet-triplet qubits, the exchange interaction is used in both quantum gate operation and the measurement of the state of the qubit. The exchange can be controlled electronically by applying gate voltage pulses. We simulate the exchange induced charge state transitions in one and two singlet-triplet qubit systems using the exact diagonalization method. We find that fast detuning pulses may result in leakage between different singlet charge states. The leakage could cause measurement errors and hinder quantum gate operation for example in the case of the two-qubit Coulom…
We discuss pure dephasing of singlet-triplet superpositions in two-electron double quantum dots due to elastic phonon scattering. We generalize our previous results to a system built of two non-identical dots. We show that the asymmetry must be very strong in order to considerably affect the dephasing rate.
A pulsed-gate technique with charge sensing is used to measure the singlet-triplet relaxation time for nearly-degenerate spin states in a two-electron double quantum dot. Transitions from the (1,1) charge occupancy state to the (0,2) state, measured as a function of pulse cycle duration and magnetic field, allow the (1,1) singlet-triplet relaxation time (~70 microseconds) and the (0,2) singlet-triplet splitting to be measured. The use of charge sensing rather than current measurement allows long relaxation times to be readily probed.
Embedding a WS$_2$ monolayer in flakes of hexagonal boron nitride allowed us to resolve and study the photoluminescence response due to both singlet and triplet states of negatively charged excitons (trions) in this atomically thin semiconductor. The energy separation between the singlet and triplet states has been found to be relatively small reflecting rather weak effects of the electron-electron exchange interaction for the trion triplet in a WS$_2$ monolayer, which involves two electrons with the same spin but from different valleys. Polarization-resolved experiments demonstrate that the h…
The Kondo effect, a hallmark of strong correlation physics, is characterized by the formation of an extended cloud of singlet states around magnetic impurities at low temperatures. While many implications of the Kondo cloud's existence have been verified, the existence of the singlet cloud itself has not been directly demonstrated. We suggest a route for such a demonstration by considering an observable that has no classical analog, but is still experimentally measurable: "singlet weights", or projections onto particular entangled two-particle states. Using approximate theoretical arguments, w…
We study theoretically phonon-induced spin dynamics of two electrons confined in a self-assembled double quantum dot. We calculate the transition rates and time evolution of occupations for the spin-triplet and spin-singlet states. We characterize the relative importance of various relaxation channels as a function of the electric and magnetic fields. The simulations are based on a model combining the eight-band k.p method and configuration-interaction approach. We show that the electron g-factor mismatch between the Zeeman doublets localized on different dots opens a relatively fast triplet-s…
We study double quantum dots in a Ge/SiGe heterostructure and test their maturity towards singlet-triplet ($S-T_0$) qubits. We demonstrate a large range of tunability, from two single quantum dots to a double quantum dot. We measure Pauli spin blockade and study the anisotropy of the $g$-factor. We use an adjacent quantum dot for sensing charge transitions in the double quantum dot at interest. In conclusion, Ge/SiGe possesses all ingredients necessary for building a singlet-triplet qubit.
We investigate various aspects of the Kondo singlet in a quantum dot (QD) electrostatically coupled to a mesoscopic detector. The two subsystems are represented by an entangled state between the Kondo singlet and the charge-dependent detector state. We show that the phase-coherence of the Kondo singlet is destroyed in a way that is sensitive to the charge-state information restored both in the magnitude and in the phase of the scattering coefficients of the detector. We also introduce the notion of the `conditional evolution' of the Kondo singlet under projective measurement on the detector. O…
We report the first theoretical calculations of excited state absorptions (ESAs) from the singlet and triplet excitons, as well as the key intermediate in the singlet fission (SF) process, the spin singlet multiexciton triplet-triplet state, for solid pentacene with herringbone crystal structure. Our goal is to compare theoretical results against ultrafast transient photoinduced absorption (PA) measurements and their interpretations, which have remained controversial. We show that the elusive triplet-triplet state absorbs both in the visible and near infrared (NIR), at or close to the PA energ…
We present a theoretical study of the spectrum of electrons confined in triple concentric rings. An unusual ordering and rich variety of angular momentum transitions are found that depend on the coupling between the rings and the confinement potential of the rings. Using the Configuration Interaction (CI) method, we calculated the two electron energy spectrum. Spin singlet to spin triplet transitions of the electron ground state are predicted and a fractional Aharonov-Bohm effect is found. We show that both the period and amplitude of the spin singlet - triplet energy gap depend strongly on th…
We estimate the triplet-singlet relaxation rate due to spin-orbit coupling assisted by phonon emission in weakly-confined quantum dots. Our results for two and four electrons show that the different triplet-singlet relaxation trends observed in recent experiments under magnetic fields can be understood within a unified theoretical description, as the result of the competition between spin-orbit coupling and phonon emission efficiency. Moreover, we show that both effects are greatly affected by the strength of the confinement and the external magnetic field, which may give access to very long-l…
In the present work we provide an easily accessible way to achieve the singlet-triplet Kondo effect in a hybrid system consisting of a quantum point contact (QPC) coupled to an electronic cavity. We show that by activating the coupling between the QPC and cavity, a zero-bias anomaly occurs in a low conductance regime, a coexistence of zero-bias and finite-bias anomaly (FBA) in a medium conductance regime, and a FBA-only anomaly in a high conductance regime. The latter two observations are due to the singlet-triplet Kondo effect.
We investigate the enhancement of the Kondo effect in quantum dots with an even number of electrons, using a scaling method and a mean field theory. We evaluate the Kondo temperature $T_K$ as a function of the energy difference between spin-singlet and triplet states in the dot, $Δ$, and the Zeeman splitting, $E_Z$. If the Zeeman splitting is small, $E_Z \ll T_K$, the competition between the singlet and triplet states enhances the Kondo effect. $T_K$ reaches its maximum around $Δ=0$ and decreases with $Δ$ obeying a power law. If the Zeeman splitting is strong, $E_Z \gg T_K$, the Kondo effect o…
We observe mixing between two-electron singlet and triplet states in a double quantum dot, caused by interactions with nuclear spins in the host semiconductor. This mixing is suppressed by applying a small magnetic field, or by increasing the interdot tunnel coupling and thereby the singlet-triplet splitting. Electron transport involving transitions between triplets and singlets in turn polarizes the nuclei, resulting in striking bistabilities. We extract from the fluctuating nuclear field a limitation on the time-averaged spin coherence time T2* of 25 ns. Control of the electron-nuclear inter…
We report implementation of a resonantly driven singlet-triplet spin qubit in silicon. The qubit is defined by the two-electron anti-parallel spin states and universal quantum control is provided through a resonant drive of the exchange interaction at the qubit frequency. The qubit exhibits long $T_2^*$ exceeding 1 $μ$s that is limited by dephasing due to the $^{29}$Si nuclei rather than charge noise thanks to the symmetric operation and a large micro-magnet Zeeman field gradient. The randomized benchmarking shows 99.6 % single gate fidelity which is the highest reported for singlet-triplet qu…
We have evaluated hyperfine-induced electron spin dynamics for two electrons confined to a double quantum dot. Our quantum solution accounts for decay of a singlet-triplet correlator even in the presence of a fully static nuclear spin system, with no ensemble averaging over initial conditions. In contrast to an earlier semiclassical calculation, which neglects the exchange interaction, we find that the singlet-triplet correlator shows a long-time saturation value that differs from 1/2, even in the presence of a strong magnetic field. Furthermore, we find that the form of the long-time decay un…
Spin-orbit mediated phonon relaxation in a two-dimensional quantum dot is investigated using different confining potentials. Elliptical harmonic oscillator and cylindrical well results are compared to each other in the case of a two-electron GaAs quantum dot subjected to a tilted magnetic field. The lowest energy set of two-body singlet and triplet states are calculated including spin-orbit and magnetic effects. These are used to calculate the phonon induced transition rate from the excited triplet to the ground state singlet for magnetic fields up to where the states cross. The roll of the cu…
We consider a quantum dot embedded in a three-dimensional nanowire with tunable aspect ratio a. A configuration interaction theory is developed to calculate the energy spectra of the finite 1D quantum dot systems charged with two electrons in the presence of magnetic fields B along the wire axis. Fruitful singlet-triplet transition behaviors are revealed and explained in terms of the competing exchange interaction, correlation interaction, and spin Zeeman energy. In the high aspect ratio regime, the singlet-triplet transitions are shown designable by tuning the parameters a and B. The transiti…
Kondo effect in the vicinity of a singlet-triplet transition in a vertical quantum dot is considered. This system is shown to map onto a special version of the two-impurity Kondo model. At any value of the control parameter, the system has a Fermi-liquid ground state. Explicit expressions for the linear conductance as a function of the control parameter and temperature $T$ are obtained. At T=0, the conductance reaches the unitary limit $\sim 4e^2/h$ at the triplet side of the transition, and decreases with the increasing distance to the transition at the singlet side. At finite temperature, th…
Heavy fermion systems represent a prototypical setting to study magnetic quantum phase transitions. A particular focus has been on the physics of Kondo destruction, which captures quantum criticality beyond the Landau framework of order-parameter fluctuations. In this context, we study the spin one-half Kondo-Heisenberg model on a honeycomb lattice at half filling. The problem is approached from the Kondo destroyed, antiferromagnetically ordered insulating phase. We describe the local moments in terms of a coarse grained quantum non-linear sigma model, and show that the skyrmion defects of the…
The magnetic-field evolution of Coulomb blockade peaks in lateral InGaAs/InAlAs quantum dots in the few-electron regime is reported. Quantum dots are defined by gates evaporated onto a 60 nm-thick hydrogen silsesquioxane insulating film. A gyromagnetic factor of 4.4 is measured via zero-bias spin spectroscopy and a transition from singlet to triplet spin configuration is found at an in-plane magnetic field B = 0.7 T. This observation opens the way to the manipulation of singlet and triplet states at moderate fields and its relevance for quantum information applications will be discussed.
We investigate the effect of the charge state measurement of the Kondo singlet for a quantum dot transistor via a capacitively coupled quantum point contact detector. By employing the variational ansatz for the singlet ground state of the quantum dot combined with the density matrix formulation for the coupled system, we show that the coherent Kondo singlet is destroyed by the phase-sensitive as well as the magnitude-sensitive detection in the transmission/reflection coefficients at the quantum point contact. We argue that the phase-sensitive component of the decoherence rate may explain the a…
We study two tunnel-coupled quantum dots each with a spin 1/2 and attached to leads in the Coulomb blockade regime. We study the interplay between Kondo correlations and the singlet-triplet exchange splitting $K$ between the two spins. We calculate the cotunneling current with elastic and inelastic contributions and its renormalization due to Kondo correlations, away and at the degeneracy point K=0. We show that these Kondo correlations induce pronounced peaks in the conductance as function of magnetic field $B$, inter-dot coupling $t_0$, and temperature. Moreover, the long-range part of the C…
We address a recent theoretical discrepancy concerning the Kondo effect in quantum dots with an even number of electrons where spin-singlet and -triplet states are nearly degenerate. We show that the discrepancy arises from the fact that the Kondo scaling involves many parameters, which makes the results depend on concrete microscopic models. We illustrate this by the scaling calculations of the Kondo temperature, $T_K$, as a function of the energy difference between the singlet and triplet states $Δ$. $T_K(Δ)$ decreases with increasing $Δ$, showing a crossover from a power law with a universa…
Spin relaxation from a triplet excited state to a singlet ground state in a semiconductor quantum dot is studied by employing an electrical pump-and-probe method. Spin relaxation occurs via cotunneling when the tunneling rate is relatively large, confirmed by a characteristic square dependence of the relaxation rate on the tunneling rate. When cotunneling is suppressed by reducing the tunneling rate, the intrinsic spin relaxation is dominated by spin-orbit interaction. We discuss a selection rule of the spin-orbit interaction based on the observed double-exponential decay of the triplet state.
We study the magnetic field induced singlet/triplet transition for two electrons in vertically coupled quantum dots by exact diagonalization of the Coulomb interaction. We identify the different mechanisms occurring in the transition, involving either in-plane correlations or localization in opposite dots, depending on the field direction. Therefore, both spin and orbital degrees of freedom can be manipulated by field strength and direction. The phase diagram of realistic devices is determined.
We study transport and zero frequency shot noise properties of a normal metal-superconductor-normal metal (NSN) junction, with the superconductor having mixed singlet and chiral triplet pairings. We show that in the subgapped regime when the chiral triplet pairing amplitude dominates over that of the singlet, a resonance phenomena emerges out at zero energy where all the quantum mechanical scattering probabilities acquire a value of 0.25. At the resonance, crossed Andreev reflection mediating through such junction, acquires a zero energy peak. This reflects as a zero energy peak in the conduct…
The linear and nonlinear transport through a multi-level lateral quantum dot connected to two leads is investigated using a generalized finite-$U$ slave-boson mean field approach. For a two-level quantum dot, our calculation demonstrates a substantial conductance enhancement near the degeneracy point of the spin singlet and triplet states, a non-monotonic temperature-dependence of conductance and a sharp dip and nonzero bias maximum of the differential conductance. These agree well with recent experiment observations. This two-stage Kondo effect in an out-of-equilibrium situation is attributed…
We demonstrate singlet-triplet readout and parity readout allowing to distinguish T0 and the polarized triplet states. We achieve high fidelity spin readout with an average fidelity above $99.9\%$ for a readout time of $20~μ$s and $99\%$ for $4~μ$s at a temperature of $0.5~K$. We initialize a singlet state in a single dot with a fidelity higher than $99\%$ and separate the two electrons while keeping the same spin state with $a \approx 95.6\%$ fidelity.
The spin-orbit interaction is the key element for electrically tunable spin qubits. Here we probe the effect of cubic Rashba spin-orbit interaction on mixing of the spin states by investigating singlet-triplet oscillations in a planar Ge hole double quantum dot. By varying the magnetic field direction we find an intriguing transformation of the funnel into a butterfly-shaped pattern. Landau-Zener sweeps disentangle the Zeeman mixing effect from the spin-orbit induced coupling and show that large singlet-triplet avoided crossings do not imply a strong spin-orbit interaction. Our work emphasizes…
A strong coupling between an electronic cavity and a quantum dot has been recently demonstrated [Phys. Rev. Lett. 115, 166603 (2015)] and described in a comprehensive theoretical framework [Phys. Rev. B 96, 235431 (2017)]. Here, we focus on the signatures that demonstrate the cavity's impact on inelastic singlet-triplet transport through the dot. We find the same transport signatures in the experiment as predicted by the model that describes the coupled dot--cavity system. Interestingly, a lowest-order treatement of the coupling to the electronic leads on top of an exact diagonalisation of the…
We report a successful measurement of the magnetic field-induced spin singlet-triplet transition in silicon-based coupled dot systems. Our specific experimental scheme incorporates a lateral gate-controlled Coulomb-blockaded structure in Si to meet the proposed scheme of Loss and DiVincenzo [1], and a non-equilibrium single-electron tunneling technique to probe the fine energy splitting between the spin singlet and triplet, which varies as a function of applying magnetic fields and interdot coupling constant. Our results, exhibiting the singlet-triplet crossing at a magnetic field for various …
Wavefunction and interaction effects in the addition spectrum of a Coulomb blockaded many electron quantum ring are investigated as a function of asymmetrically applied gate voltages and magnetic field. Hartree and exchange contributions to the interaction are quantitatively evaluated at a crossing between states extended around the ring and states which are more localized in one arm of the ring. A gate tunable singlet-triplet transition of the two uppermost levels of this many electron ring is identified at zero magnetic field.
The magnetic character of the ground-state of two electrons on a double quantum dot, connected in series to left and right single-channel leads, is considered. By solving exactly for the spectrum of the two interacting electrons, it is found that the coupling to the continuum of propagating states on the leads, in conjunction with the electron-electron interactions, may result in a delocalization of the bound state of the two electrons. This, in turn, reduces significantly the range of the Coulomb interaction parameters over which singlet-triplet transitions can be realized. It is also found t…
We study the effect of charge and spin noise on singlet-triplet qubits in Si quantum dots. We set up a theoretical framework aimed at enabling experiment to efficiently identify the most deleterious defects, and complement it with the knowledge of defects gained in decades of industrial and academic work. We relate the dephasing rates $Γ_ϕ$ due to various classes of defects to experimentally measurable parameters such as charge dipole moment, spin dipole moment and fluctuator switching times. We find that charge fluctuators are more efficient in causing dephasing than spin fluctuators.
When a cerocene molecule is chemisorbed on metallic substrate, or when an asymmetric double dot is hybridized with itinerant electrons, its singlet ground state crosses its lowly excited triplet state, leading to a competition between the Zhang-Rice mechanism of singlet-triplet splitting in a confined cluster and the Kondo effect (which accompanies the tunneling through quantum dot under a Coulomb blockade restriction). The rich physics of an underscreened S=1 Kondo impurity in the presence of low-lying triplet/singlet excitations is exposed. Estimates of the magnetic susceptibility and the el…
We study spin relaxation in a two-electron quantum dot in the vicinity of the singlet-triplet crossing. The spin relaxation occurs due to a combined effect of the spin-orbit, Zeeman, and electron-phonon interactions. The singlet-triplet relaxation rates exhibit strong variations as a function of the singlet-triplet splitting. We show that the Coulomb interaction between the electrons has two competing effects on the singlet-triplet spin relaxation. One effect is to enhance the relative strength of spin-orbit coupling in the quantum dot, resulting in larger spin-orbit splittings and thus in a s…
The singlet-triplet relaxation in nanowire-based quantum dots induced by confined phonons is investigated theoretically. Due to the quasi-one-dimensional nature of the confined phonons, the singlet-triplet relaxation rates exhibit multi-peaks as function of magnetic field and the relaxation rate between the singlet and the spin up triplet state is found to be enhanced at the vicinity of the singlet-triplet anti-crossing. We compare the effect of the deformation-potential coupling and the piezoelectric coupling and find that the deformation-potential coupling dominates the relaxation rates in m…
We study the low energy spectrum of a correlated quantum dot embedded between the normal conducting and superconducting reservoirs and hybridized with the topological superconducting nanowire, hosting the Majorana end-modes. We investigate the leaking Majorana quasiparticle and inspect its interplay with the proximity induced on-dot pairing and correlations. In particular, we focus on the subgap Kondo effect near the quantum phase transition/crossover from the spinfull (doublet) to the spinless (BCS-type singlet) configurations. Treating the correlations perturbatively and within the NRG appro…
We investigate the Kondo effect in a quantum dot with almost degenerate spin-singlet and triplet states for an even number of electrons. We show that the Kondo temperature as a function of the energy difference between the states Delta reaches its maximum around Delta=0 and decreases with increasing Delta. The Kondo effect is thus enhanced by competition between singlet and triplet states. Our results explain recent experimental findings. We evaluate the linear conductance in the perturbative regime.
The search of a sweet spot, locus in qubit parameters where quantum control is first-order insensitive to noises, is key to achieve high-fidelity quantum gates. Efforts to search for such a sweet spot in conventional double-quantum-dot singlet-triplet qubits where each dot hosts one electron ("two-electron singlet-triplet qubit"), especially for two-qubit operations, have been unsuccessful. Here we consider singlet-triplet qubits allowing each dot to host more than one electron, with a total of four electrons in the double quantum dots ("four-electron singlet-triplet qubit"). We theoretically …
We analyze two pairs of doublet states for the two Anderson impurity problem. We found that for short interimpurity distances they have a lower energy than the ferro triplet and the antiferro singlet. For medium to long distances between the impurities, the doublets also have a lower energy than the two decoupled Kondo-singlet state for most of the range of interest. The mechanism behind their energy gain is an coherence enhanced Kondo-like interaction.
We study a pair of capacitively coupled singlet-triplet spin qubits. We characterize the two-qubit decoherence through two complementary measures, the decay time of coupled-qubit oscillations and the fidelity of entangled state preparation. We provide a quantitative map of their dependence on charge noise and field noise, and we highlight the magnetic field gradient across each singlet-triplet qubit as an effective tool to suppress decoherence due to charge noise.
We consider two interacting electrons in a semiconductor quantum dot structure which consists of a small dot within a larger dot, and demonstrate a singlet-triplet filtering mechanism which involves spin-dependent resonances and can generate entanglement. By studying the exact time evolution of singlet and triplet states we show how the degree of both filtering and spin entanglement can be tuned using a time-dependent gate voltage.
Singlet-triplet states in double quantum dots are promising realizations of qubits, and capacitive coupling can be used to create entanglement between these qubits. We propose an entangling three-qubit gate of singlet-triplet qubits in a triangular setup. Our simulations using a realistic microscopic model show that a maximally entangled Greenberger-Horne-Zeilinger state can be generated as the qubits are evolved under exchange. Furthermore, our analysis for the gate operation can be used to extract the actual experimental pulse sequence needed to realize this.
We discuss transport through a lateral quantum dot in the vicinity of a singlet-triplet spin transition in its ground state. Extracting the scattering phase shifts from the numerical renormalization group spectra, we determine the linear conductance at zero temperature as a function of a Zeeman field and the splitting of the singlet and triplet states. We find reduced low-energy transport, and a non-monotonic magnetic field dependence both in the singlet and the triplet regime. For a generic set of dot parameters and no Zeeman splitting, the singlet-triplet transition may be identified with th…
We measure singlet-triplet mixing in a precision fabricated double donor dot comprising of 2 and 1 phosphorus atoms separated by $16{\pm}1$ nm. We identify singlet and triplet-minus states by performing sequential independent spin readout of the two electron system and probe its dependence on magnetic field strength. The relaxation of singlet and triplet states are measured to be $12.4{\pm}1.0$ s and $22.1{\pm}1.0$ s respectively at $B_z{=}2.5$ T.
In the singlet-triplet qubit architecture, the two-qubit interactions required in universal quantum computing can be implemented by capacitative coupling, by exploiting the charge distribution differences of the singlet and triplet states. The efficiency of this scheme is limited by decoherence, that can be mitigated by stronger coupling between the qubits. In this paper, we study the capacitative coupling of singlet-triplet qubits in different geometries of the two-qubit system. The effects of the qubit-qubit distance and the relative orientation of the qubits on the capacitative coupling str…
We study the triplet-singlet relaxation in two-electron semiconductor quantum dots. Both single dots and vertically coupled double dots are discussed. In our work, the electron-electron Coulomb interaction, which plays an important role in the electronic structure, is included. The spin mixing is caused by spin-orbit coupling which is the key to the triplet-singlet relaxation. We show that the selection rule widely used in the literature is incorrect unless near the crossing/anticrossing point in single quantum dots. The triplet/singlet relaxation in double quantum dots can be markedly changed…
