We studied the possibility of the spin pump in a S=1/2 antiferromagnetic chain. The spin chain is mapped into a fermion system and bosonization is utilized to transform the equation of motion to a sine-Gordon equation. The sine-Gordon equation on a finite chain with different boundary conditions is solved. Among numerous solutions, the static soliton is compatible with the original physical system. By varying adiabatically a angle in the phase space composed of applied electric and magnetic fields, the spin states change between the Neel state and dimer state and a quantized spin is transported by the bulk state from one end of the system to the other.
In this paper, we propose the quantum spin pumping in quantum spin systems where an applied electric field ($E$) and magnetic field ($H$) cause a finite spin gap to its critical ground state. When these systems are subject to alternating electromangetic fields; $(E,H)=(\sin\frac{2πt}{T},\cos\frac{2πt}{T})$ and travel along the {\it{loop}} $Γ_{\rm{loop}}$ which encloses their critical ground state in this $E$-$H$ phase diagram, the locking potential in the sine-Gordon model slides and changes its minimum. As a result, the phase operator acquires $2π$ holonomy during one cycle along $Γ_{\rm{loop…
The notion of topological (Thouless) pumping in topological phases is traditionally associated with Laughlin's pump argument for the quantization of the Hall conductance in two-dimensional (2D) quantum Hall systems. It relies on magnetic flux variations that thread the system of interest without penetrating its bulk, in the spirit of Aharonov-Bohm effects. Here we explore a different paradigm for topological pumping induced, instead, by magnetic flux variations $δχ$ inserted through the bulk of topological phases. We show that $δχ$ generically controls the analog of a topological pump, accompa…
We study the quantum spin pumping of an antiferromagnetic spin-1/2 chain with competing exchange interactions. We show that spatially periodic potential modulated in space and time acts as a quantum spin pump. In our model system, an applied electric field causes a spin gap to its critical ground state by introducing bond-alternation exchange interactions. We study quantum spin pumping at different quantized magnetization states and also explain physically the presence and absence of quantum spin pumping at different fractionally quantized magnetization states.
We report optical spectroscopy and ultrafast pump-probe measurements on the antiferromagnetic heavy fermion compound CePt$_2$In$_7$, a member showing stronger two dimensionality than other compounds in CeIn$_3$-derived heavy-fermion family. We identify clear and typical hybridization spectral structures at low temperature from the two different spectroscopy probes. However, the strength and related energy scale of the hybridization are much weaker and smaller than that in the superconducting compounds CeCoIn$_5$ and CeIrIn$_5$. The features are more similar to observations on the antiferromagn…
Ultrafast optical excitation of magnons in 2D antiferromagnetic semiconductors via spin torque mediated by unbound electron-hole pairs and excitons: Signatures in magnonic charge pumping
Department of Physics and Astronomy, University of Delaware（特拉华大学物理与天文学系）
We have performed angle-resolved photoemission spectroscopy on EuIn2As2 which is predicted to be an axion insulator in the antiferromagnetic state. By utilizing soft-x-ray and vacuum-ultraviolet photons, we revealed a three-dimensional hole pocket centered at the Gamma point of bulk Brillouin zone together with a heavily hole-doped surface state in the paramagnetic phase. Upon entering the antiferromagnetic phase, the band structure exhibits a marked reconstruction characterized by the emergence of a "M"-shaped bulk band near the Fermi level. The qualitative agreement with first-principles ban…
An extended Bose-Hubbard model (EBHM) with three- and four-body constraints can be feasible in cold atoms in an optical lattice. A rich phase structure including various symmetry-protected topological (SPT) phases is obtained numerically with suitable parameter settings and particle filling. The SPT phase is characterized by the Berry phase as a local topological order parameter and the structure of the entanglement spectrum (ES). Based on the presence of various topological phases, separated by gapless phase boundaries, the EBHM exhibits various bosonic topological pumps, which are constructe…
Recent studies suggest that an exemplary Kondo insulator SmB6 belongs to a new class of topological insulators (TIs), in which non-trivial spin-polarized metallic states emerge on surface upon the formation of Kondo hybridization gap in the bulk. Remarkably, the bulk resistivity reaches more than 20 Ohm cm at 4 K, making SmB6 a candidate for a so-called bulk-insulating TI. We here investigate optical-pulse responses of SmB6 by pump-and-probe photoemission spectroscopy. Surface photovoltage effect is observed below ~90 K. This indicates that an optically-active band bending region develops bene…
The bulk-boundary correspondence relates quantized edge states to bulk topological invariants in topological phases of matter. In one-dimensional symmetry-protected topological systems (SPTs), quantized topological Thouless pumps directly reveal this principle and provide a sound mathematical foundation. Symmetry-protected higher-order topological phases of matter (HOSPTs) also feature a bulk-boundary correspondence, but its connection to quantized charge transport remains elusive. Here we show that quantized Thouless pumps connecting $C_4$-symmetric HOSPTs can be described by a tuple of four …
Within the framework of the QED3 theory of cuprates it is argued that bulk antiferromagnetic (AF) order can coexist with d-wave superconductivity in the underdoped region, in agreement with recent experiments. The AF order arises from the phase fluctuating d-wave superconductor via the mechanism of spontaneous chiral symmetry breaking, provided that fluctuations are sufficiently strong. The phase diagram for this coexistence is mapped out by means of analytical and numerical solutions of the underlying Dyson-Schwinger equation in the large N limit.
Establishing the relation between the ubiquitous antiferromagnetism in the non-superconducting parent compounds of unconventional superconductors and their superconducting phase is believed to be important for the understanding of the complex physics in these materials. Going from the bulk systems to thin films strongly affects the phase diagram of unconventional superconductors. For Fe$_{1+y}$Te, the parent compound of the Fe$_{1+y}$Se$_{1-x}$Te$_x$ superconductors, bulk sensitive neutron diffraction has revealed an in-plane oriented bicollinear antiferromagnetic structure. Here, we show by s…
We propose a one-dimensional electron model with parameters modulated adiabatically in closed cycles, which can continuously pump spin to leads. By defining the spin-polarized Wannier functions, we show that the spin pump is protected by the spin Chern numbers, so that it is stable to perturbations violating the time-reversal symmetry and spin conservation. Our work demonstrates the possibility and principle to realize topological spin pumps independent of any symmetries, and also suggests a possible way to experimentally observe the bulk topological invariants.
When adiabatically varied in time, certain one-dimensional band insulators allow for the quantized noiseless pumping of spin even in the presence of strong spin orbit scattering. These spin pumps are closely related to the quantum spin Hall system, and their properties are protected by a time-reversal restriction on the pumping cycle. In this paper we study pumps formed of one-dimensional insulators with a time-reversal restriction on the pumping cycle and a bulk energy gap which arises due to interactions. We find that the correlated gapped phase can lead to novel pumping properties. In parti…
We have performed unpolarized and polarized neutron diffraction experiments on monodisperse 8 nm and 13 nm antiferromagnetic MnO nanoparticles. For the 8 nm sample, the antiferromagnetic transition temperature $T_N$ (114 K) is suppressed compared to the bulk material (119 K) while for the 13 nm sample $T_N$ (120 K) is comparable to the bulk. The neutron diffraction data of the nanoparticles is well described using the bulk MnO magnetic structure but with a substantially reduced average magnetic moment of 4.2$\pm$0.3 $μ_B$/Mn for the 8 nm sample and 3.9$\pm$0.2 $μ_B$/Mn for the 13 nm sample. An…
We propose a electron-pumping mechanism called Chern pump to explain the integer quantum Hall effect(IQHE) in the Chern insulator. By using the parallel transport gauge in the hybrid Wannier representation we establish the bulk and edge states correspondence in the Chern insulator. The same correspondence can also be established in two dimensional(2D) topological insulator(TI). So we can consider 2D TI as two time reversal(TR) related CIs put together. The quantum spin Hall effect(QSHE) can be viewed as two TR related Chern pumps pumping electrons to opposite directions. Compared with the Z2 s…
In this paper, we study the localized states of a generic quadratic fermionic chain with finite-range couplings and an inhomogeneity in the hopping (defect) that breaks translational invariance. When the hopping of the defect vanishes, which represents an open chain, we obtain a simple bulk-edge correspondence: the zero-energy modes localized at the ends of the chain are related to the roots of a polynomial determined by the couplings of the Hamiltonian of the bulk. From this result, we define an index that characterizes the different topological phases of the system and can be easily computed…
Applying a symmetric bulk bipartition to one-dimensional Affleck-Kennedy-Lieb-Tasaki valence bond solid (VBS) states for the integer spin-S Haldane gapped phase, we can create an array of fractionalized spin-S/2 edge states with the super unit cell $l$ in the reduced bulk system, and the topological properties encoded in the VBS wave functions can be revealed. The entanglement Hamiltonian (EH) with $l=even$ corresponds to the quantum antiferromagnetic Heisenberg spin-S/2 model. For the even integer spins, the EH still describes the Haldane gapped phase. For the odd integer spins, however, the …
We revisit bulk FeSe through the systematic first-principles electronic structure calculations. We find that there are a series of staggered $n$-mer antiferromagnetic (AFM) states with corresponding energies below that of the collinear AFM state which is the ground state for the parent compounds of most iron-based superconductors. Here the staggered $n$-mer ($n$ any integer $>1$) means that a set of $n$ adjacent spins parallel on a line along $b$-axis with spins in antiparallel between $n$-mers and along $a$-axis. Among them, the lowest energy states are quasi-degenerate staggered dimer and st…
Using the recently introduced adaptive density-matrix renormalization-group method, we study the many spin-spin correlations of the spin-$1/2$ antiferromagnetic Heisenberg chain with random coupling constants, namely, the mean value of the bulk and of the end-to-end correlations, the typical value of the bulk correlations, and the distribution of the bulk correlations. Our results are in striking agreement with the predictions of the strong-disorder renormalization group method. We do not find any hint of logarithmic corrections neither in the bulk average correlations, which were recently rep…
Electronic orderings of charges, orbitals and spins are observed in many strongly correlated electron materials, and revealing their dynamics is a critical step toward understanding the underlying physics of important emergent phenomena. Here we use time-resolved resonant soft x-ray scattering spectroscopy to probe the dynamics of antiferromagnetic spin ordering in the manganite Pr$_{0.7}$Ca$_{0.3}$MnO$_3$ following ultrafast photo-exitation. Our studies reveal a glass-like recovery of the spin ordering and a crossover in the dimensionality of the restoring interaction from quasi-1D at low pum…
Using density functional calculations we have examined the evolution of the electronic structure of SrRuO3 films grown on SrTiO3 substrates as a function of film thickness. At the ultrathin limit of two monolayers (RuO2-terminated surface) the films are found to be at the brink of a spin-state transition which drives the system to an antiferromagnetic and insulating state. Increasing the film thickness to four monolayers, one finds the surprising result that two entirely different solutions coexist. An antiferromagnetic insulating solution coexists with a metallic solution corresponding to an …
We propose a realization of the electric-field-induced antiferromagnetic resonance. We consider three-dimensional antiferromagnetic insulators with spin-orbit coupling characterized by the existence of a topological term called the $θ$ term. By solving the Landau-Lifshitz-Gilbert equation in the presence of the $θ$ term, we show that, in contrast to conventional methods using ac magnetic fields, the antiferromagnetic resonance state is realized by ac electric fields along with static magnetic fields. This mechanism can be understood as the inverse process of the dynamical chiral magnetic effec…
We use a non-equilibrium many-body theory that engages the elements of transient coherence, correlation, and nonlinearity to describe changes in the magnetic and electronic phases of strongly correlated systems induced by femtosecond nonlinear photoexcitation. Using a generalized tight--binding mean field approach based on Hubbard operators and including the coupling of the laser field, we describe a mechanism for simultaneous insulator--to--metal and anti-- to ferro--magnetic transition to a transient state triggered by non-thermal ultrafast spin and charge coupled excitations. We demontrate,…
We study the low-energy excitations of the spin-1/2 antiferromagnetic Heisenberg chain and $N$-leg ($N$=2, 3, 4) ladders in a staggered magnetic field $h_s$. We show that $h_s$ induces gap and midgap states in all the cases and examine their field scaling behavior. A modified boundary scheme is devised to extract accurate bulk excitation behavior. The gap values converge rapidly as $N$ increases, leading to a field scaling exponent $γ=1/2$ for both the longitudinal and transverse gaps of the square lattice ($N \to \infty$). The midgap states induced by the boundary edge effects share the bulk …
Magnetic properties of monolayer, multilayer, and bulk CrTe$_2$
Moscow Institute of Physics and Technology（莫斯科物理技术学院）；M. N. Mikheev Institute of Metal Physics of the Ural Branch of the Russian Academy of Sciences（俄罗斯科学院乌拉尔分校 M.N. 米凯耶夫金属物理研究所）；Ludwig-Maximilians-Universität München（慕尼黑大学）；Technical University of Munich（慕尼黑工业大学）
Motivated by the recent development of time-resolved resonant-inelastic x-ray scattering (TRRIXS) in photoexcited antiferromagnetic Mott insulators, we numerically investigate momentum-dependent transient spin dynamics in a half-filled Hubbard model on a square lattice. After turning off a pumping photon pulse, the intensity of a dynamical spin structure factor temporally oscillates with frequencies determined by the energy of two magnons in the antiferromagnetic Mott insulator. We find an antiphase behavior in the oscillations between two orthogonal momentum directions, parallel and perpendic…
We theoretically study the dynamic time evolution following laser pulse pumping in an antiferromagnetic insulator Cr$_{2}$O$_{3}$. From the photoexcited high-spin quartet states to the long-lived low-spin doublet states, the ultrafast demagnetization processes are investigated by solving the dissipative Schrödinger equation. We find that the demagnetization times are of the order of hundreds of femtosecond, in good agreement with recent experiments. The switching times could be strongly reduced by properly tuning the energy gaps between the multiplet energy levels of Cr$^{3+}$. Furthermore, th…
It has recently been established that cluster-like states -- states that are in the same symmetry-protected topological phase as the cluster state -- provide a family of resource states that can be utilized for Measurement-Based Quantum Computation. In this work, we ask whether it is possible to prepare cluster-like states in finite time without breaking the symmetry protecting the resource state. Such a symmetry-preserving protocol would benefit from topological protection to errors in the preparation. We answer this question in the positive by providing a Hamiltonian in one higher dimension …
Nd_0.5 Ca_0.5 MnO_3 (NCMO) nanoparticles (average diameter ~ 20 and 40 nm) are synthesized by polymeric precursor sol-gel method and characterized by X- ray diffraction, transmission electron microscopy (TEM), selective area electron diffraction (SAED), superconducting quantum interference device (SQUID) magnetometery and resistivity measurements. Both single crystalline and polycrystalline particles are present in the samples and they are found to retain the orthorhombic structure of the bulk NCMO. However, most strikingly, in the 20 nm particles, the charge ordered (CO) and the antiferromagn…
