We use exact diagonalization techniques to study the interplay between strong correlations, superconductivity, and disorder in a model system. We study an extension of the t-J model by adding an infinite-range d-wave superconductivity inducing term and disorder. Our work shows that in the clean case the magnitude of the order parameter is surprisingly small for low-hole filling, thus implying that mean-field theories might be least accurate in that important regime. We demonstrate that substantial disorder is required to destroy a d-wave superconducting state for low-hole doping. We provide the first bias free numerical results for the local density of states of a strongly correlated d-wave superconducting model, relevant for STM measurements at various fillings and disorders.
We study the low-energy density of states of Dirac fermions in disordered d-wave superconductor. At zero energy, a finite density of states is obtained via the mechanism of dynamical mass generation in an effective (1+1)-dimensional relativistic field theory.
We show that strong correlations play a vital role in protecting low energy excitations in disordered high temperature superconductors. The impurity-induced low-energy density of states (DOS) is greatly reduced in the strongly correlated superconductor compared to d-wave Bogoliubov-deGennes theory. The gapless nodal quasiparticles, and the resulting `V' in the low-energy DOS, are much more robust against disorder compared to the large-gap antinodal excitations. We discuss the relevance of our results to angle-resolved photoemission and scanning tunneling spectroscopy experiments.
The paramagnon contribution to the quasiparticle inelastic scattering rate in disordered superconductors is presented. Using Anderson's exact eigenstate formalism, it is shown that the scattering rate is Stoner enhanced and is further enhanced by the disorder relative to the clean case in a manner similar to the disorder enhancement of the long-range Coulomb contribution. The results are discussed in connection with the possibility of conventional or unconventional superconductivity in the borocarbides. The results are compared to recent tunneling experiments on LuNi$_{2}$B$_{2}$C.
Through a detailed study of scaling near the magnetic field-tuned superconductor-to-insulator transition in strongly disordered films, we find that results for a variety of materials can be collapsed onto a single phase diagram. The data display two clear branches, one with weak disorder and an intervening metallic phase, the other with strong disorder. Along the strongly disordered branch, the resistance at the critical point approaches $R_Q = h/4e^2$ and the scaling of the resistance is consistent with quantum percolation, and therefore with the predictions of the dirty boson model.
The robustness against local perturbations, as long as the symmetry of the system is preserved, is a distinctive feature of topological quantum states. Magnetic impurities and defects break time-reversal invariance and, consequently, time-reversal invariant (TRI) topological superconductors are fragile against this type of disorder. Non-magnetic impurities, however, preserve time-reversal symmetry and one naively expects a TRI topological superconductor to persist in the presence of non-magnetic impurities. In this work, we study the effect of non-magnetic disorder on a TRI topological superco…
We show, using a simple model, how ordinary disorder can gap an extended-$s$ ($A_{1g}$) symmetry superconducting state with nodes. The concommitant crossover of thermodynamic properties, particularly the $T$-dependence of the superfluid density, from pure power law behavior to an activated one is exhibited. We discuss applications of this scenario to experiments on the ferropnictide superconductors.
Effects of non-magnetic disorder on the critical temperature T_c and on diamagnetism of quasi-one-dimensional superconductors are reported. The energy of Josephson-coupling between wires is considered to be random, which is typical for dirty organic superconductors. We show that this randomness destroys phase coherence between wires and that T_c vanishes discontinuously at a critical disorder-strength. The parallel and transverse components of the penetration-depth are evaluated. They diverge at different critical temperatures T_c^{(1)} and T_c, which correspond to pair-breaking and phase-cohe…
The understanding of disorder has profoundly influenced the development of condensed matter physics, explaining such fundamental effects as, for example, the transition from ballistic to diffusive propagation, and the presence of quantized steps in the quantum Hall effect. For superconductors, the response to disorder reveals crucial information about the internal gap symmetries of the condensate, and thereby the pairing mechanism itself. The destruction of superconductivity by disorder is traditionally described by Abrikosov-Gor'kov (AG) theory, which however ignores spatial modulations and c…
We study the basic features of the local density of states (LDOS) observed in STM experiments on high-T$_c$ d-wave superconductors in the context of a minimal model of a d-wave superconductor which has {\it weakly} modulated off-diagonal disorder. We show that the low and high energy features of the LDOS are consistent with the observed experimental patterns and in particular, the anisotropic local domain features at high energies. At low energies, we obtain not only the scattering peaks predicted by the octet model, but also weak features that should be experimentally accessible. Finally, we …
The density of states of the organic superconductor $κ$-(BEDT-TTF)$_2$Cu[N(CN)$_2$]Br, measured by scanning tunneling spectroscopy on \textit{in-situ} cleaved surfaces, reveals a logarithmic suppression near the Fermi edge persisting above the critical temperature $T_\mathrm{c}$. A soft Hubbard gap as predicted by the Anderson-Hubbard model for systems with disorder exactly describes the experimentally observed suppression. The electronic disorder also explains the diminished coherence peaks of the quasiparticle density of states below $T_\mathrm{c}$.
The effect of disorder on the superconducting transition temperature $T_{c}$ of cuprate superconductors is examined. Disorder is introduced into the cation sites in the plane adjacent to the CuO$_{2}$ planes of two single-layer systems, Bi$_{2.0}$Sr$_{1.6}$Ln$_{0.4}$CuO$_{6+δ}$ and La$_{1.85-y}$Nd$_{y}$Sr$_{0.15}$CuO$_{4}$. Disorder is controlled by changing rare earth (Ln) ions with different ionic radius in the former, and by varying the Nd content in the latter with the doped carrier density kept constant. We show that this type of disorder works as weak scatterers in contrast to the in-pla…
When periodicity of crystal is disturbed by atomic disorder, its electronic state becomes inhomogeneous and band dispersion is obscured. In case of Fe-based superconductors, disorder of chalcogen/pnictogen height causes disorder of Fe 3d level splitting. Here, we report an angle-resolved photoemission spectroscopy study on FeSe_1-xTe_x with the chalcogen height disorder, showing that the disorder affects the Fe 3d band dispersions in an orbital-selective way instead of simple obscuring effect. The reverse of the Fe 3d level splitting due to the chalcogen height difference causes the splitting …
Recent experimental and theoretical studies have highlighted the possible role of a electronic nematic liquid in underdoped cuprate superconductors. We calculate, within a model of d-wave superconductor with Hubbard correlations, the spin susceptibility in the case of a small explicitly broken rotational symmetry of the underlying lattice. We then exhibit how the induced spin response asymmetry is strongly enhanced by correlations as one approaches the instability to stripe order. In the disorder-induced stripe phase, impurities become spin nematogens with a C_2 symmetric impurity resonance st…
We propose a mechanism whereby disorder can enhance the transition temperature Tc of an unconventional superconductor with pairing driven by exchange of spin fluctuations. The theory is based on a self-consistent real space treatment of pairing in the disordered one-band Hubbard model. It has been demonstrated before that impurities can enhance pairing by softening the spin fluctuations locally; here, we consider the competing effect of pair-breaking by the screened Coulomb potential also present. We show that, depending on the impurity potential strength and proximity to magnetic order, this …
Non-magnetic impurities are known as strong pair breakers in superconductors with pure d-wave pairing symmetry. Here we discuss d-wave states under the combined influence of impurities and competing instabilities, such as pairing in a secondary channel as well as lattice symmetry breaking. Using the self-consistent T-matrix formalism, we show that disorder can strongly modify the competition between different pairing states. For a d-wave superconductor in the presence of a subdominant local attraction, Anderson's theorem implies that disorder always generates an s-wave component in the gap at …
The low-energy quasiparticle states of a disordered d-wave superconductor are investigated theoretically. A class of such states, formed via tunneling between the Andreev bound states that are localized around extended impurities (and result from scattering between pair-potential lobes that differ in sign) is identified. Its (divergent) contribution to the total density of states is determined by taking advantage of connections with certain one-dimensional random tight-binding models. The states under discussion should be distinguished from those associated with nodes in the pair potential.
Effects of non-magnetic randomness on the critical temperature T_c and diamagnetism are studied in a class of quasi-one dimensional superconductors. The energy of Josephson-coupling between wires is considered to be random, which is typical for dirty organic superconductors. We show that this randomness destroys phase coherence between the wires and T_c vanishes discontinuously when the randomness reaches a critical value. The parallel and transverse components of the penetration depth are found to diverge at different critical temperatures T_c^{(1)} and T_c, which correspond to pair-breaking …
On the basis of the Hubbard model, we extend the fluctuation-exchange (FLEX) approach to investigating the properties of antiferromagnetic (AF) phase in electron-doped cuprate superconductors. Furthermore, by incorporating the effect of scatterings due to the disordered dopant-atoms into the FLEX formalism, our numerical results show that the antiferromagnetic transition temperature, the onset temperature of pseudogap due to spin fluctuations, the spectral density of the single particle near the Fermi surface, and the staggered magnetization in the AF phase as a function of electron doping can…
We study analytically the effects of inhomogeneous pairing interactions in short coherence length superconductors, using a spatially varying Bogoliubov-deGennes model. Within the Born approximation, it reproduces all of the standard Abrikosov-Gor'kov pairbreaking and gaplessness effects, even in the absence of actual magnetic impurities. For pairing disorder on a single site, the T-matrix gives rise to bound states within the BCS gap. Our results are compared with recent scanning tunneling microscopy measurements on Bi$_2$Sr$_2$CaCu$_2$O$_{8+δ}$ with Zn or Ni impurities.
We study the insulating phase of disordered indium oxide films that undergo a field-tuned superconductor-insulator transition. The transport measurements in a perpendicular magnetic field show distinct regimes of strongly fluctuating order-parameter amplitude and phase, and reveal a wide range of insulator strength in samples with differing disorder, despite the similarity in behavior near the SIT. We characterize the strength of the insulating phase and compare it to the superconducting strength. We find that the films do not return to the expected normal state even at high perpendicular magn…
We investigate the influence of disorders in terminal ethylene groups of BEDT-TTF molecules (ethylene-disorders) on the vortex pinning of the organic superconductor $κ$-(BEDT-TTF)$_2$Cu[N(CN)$_2$]Br. Magnetization measurements are performed under different cooling-processes. The second peak in the magnetization hysteresis curve is observed for all samples studied, and the hysteresis width of the magnetization becomes narrower by cooling faster. In contradiction to the simple pinning effect of disorder, this result shows the suppression of the vortex pinning force by introducing more ethylene-d…
We study the Fulde-Ferrel-Larkin-Ovchinnikov (FFLO) superconducting state in the disordered systems. We analyze the microscopic model, in which the d-wave superconductivity is stabilized near the antiferromagnetic quantum critical point, and investigate two kinds of disorder, namely, box disorder and point disorder, on the basis of the Bogoliubov-deGennes (BdG) equation. The spatial structure of modulated superconducting order parameter and the magnetic properties in the disordered FFLO state are investigated. We point out the possibility of "FFLO glass" state in the presence of strong point d…
We calculate superfluid density for a dirty d-wave superconductor. The effects of impurity scattering are treated within the self-consistent t-matrix approximation, in weak-coupling BCS theory. Working from a realistic tight-binding parameterization of the Fermi surface, we find a superfluid density that is both correlated with T_c and linear in temperature, in good correspondence with recent experiments on overdoped La2-xSrxCuO4.
The Aharonov-Casher effect is the analogue of the Aharonov-Bohm effect that applies to neutral particles carrying a magnetic moment. This can be manifested by vortices or fluxons flowing in trajectories that encompass an electric charge. These have been predicted to result in a persistent voltage which fluctuates for different sample realizations. Here we show that disordered superconductors exhibit reproducible voltage fluctuation, antisymmetrical with respect to magnetic field, as a function of various parameters such as magnetic field amplitude, field orientations and gate voltage. These re…
The most profound effect of disorder on electronic systems is the localization of the electrons transforming an otherwise metallic system into an insulator. If the metal is also a superconductor then, at low temperatures, disorder can induce a dramatic transition from a superconducting into an insulating state. An outstanding question is whether the route to insulating behavior proceeds via the direct localization of Cooper pairs or, alternatively, by a two-step process in which the Cooper pairing is first destroyed followed by the standard localization of single electrons. Here we address thi…
The influence of static magnetic correlations on the temperature-dependent superfluid density ρ_s(T) is calculated for d-wave superconductors. In self-consistent calculations, itinerant holes form incommensurate spin density waves (SDW) which coexist with superconductivity. In the clean limit, the density of states is gapped, and ρ_s(T << T_c) is exponentially activated. In inhomogeneously-doped cases, the SDW are disordered and both the density of states and ρ_s(T) obtain forms indistinguishable from those in dirty but pure d-wave superconductors, in accordance with experiments. We conclude t…
Using model calculations of a disordered d-wave superconductor with on-site Hubbard repulsion, we show how dopant disorder can stabilize novel states with antiferromagnetic order. We find that the critical strength of correlations or impurity potential necessary to create an ordered magnetic state in the presence of finite disorder is reduced compared to that required to create a single isolated magnetic droplet. This may explain why in cuprates like LSCO low-energy probes have identified a static magnetic component which persists well into the superconducting state, whereas in cleaner systems…
We investigate the role of disorder on the superconducting (SC) fluctuation in short coherence length d-wave superconductors. The particular intetest is focused on the disorder-induced microscopic inhomogeneity of SC fluctuation and its effect on the pseudogap phenomena. We formulate the self-consistent 1-loop order theory for the SC fluctuation in inhomogeneous systems and analyze the disordered $t$-$t'$-$V$ model. The SC correlation function, electronic DOS and the critical temperature are estimated. The SC fluctuation is localized like a nanoscale granular structure when the coherence lengt…
A model for high-temperature superconductors incorporating antiferromagnetism, d-wave superconductivity, and no double lattice-site occupancy can give energy surfaces exquisitely balanced between antiferromagnetic and superconducting order for specific ranges of doping and temperature. The resulting properties can reconcile a universal cuprate phase diagram with rich inhomogeneity, relate that inhomogeneity to pseudogaps, give a fundamental rationale for giant proximity effects and other emergent behavior, and provide an objective framework for separating essential from peripheral in the super…
We investigate the effect of site-disorder on the superconducting (SC) state in the attractive Hubbard model within the framework of dynamical mean field theory. For a fixed interaction strength ($U$), the SC order parameter (OP) decreases monotonically with increasing disorder ($x$), while the single-particle spectral gap (SG) decreases for small $x$, reaches a minimum and keeps increasing for larger $x$. Thus, the system remains gapped beyond the destruction of the superconducting state, indicating a disorder-driven superconductor-insulator transition. We investigate this transition in depth…
Strongly disordered superconductors in a magnetic field display many characteristic properties of type-II superconductivity--- except at low temperatures where an anomalous linear $T$-dependence of the resistive critical field $B_{c2}$ is routinely observed. This behavior violates the conventional theory of superconductivity, and its origin remains a long-standing puzzle. Here we report on systematic measurements of the critical magnetic field and current on amorphous indium oxide films of various levels of disorder. Surprisingly, our measurements show that the $B_{c2}$ anomaly near zero-tempe…
A powerful approach to analysing quantum systems with dimensionality $d>1$ involves adding a weak coupling to an array of one-dimensional (1D) chains. The resultant quasi-one-dimensional (q1D) systems can exhibit long-range order at low temperature, but are heavily influenced by interactions and disorder due to their large anisotropies. Real q1D materials are therefore ideal candidates not only to provoke, test and refine theories of strongly correlated matter, but also to search for unusual emergent electronic phases. Here we report the unprecedented enhancement of a superconducting instabili…
We explore the role of phase fluctuations in a 3-dimensional s-wave superconductor, NbN, as we approach the critical disorder for the destruction of the superconducting state. Scanning tunneling spectroscopy measurements reveal that in the presence of strong disorder, a finite gap in the electronic spectrum continues to persist at temperatures above Tc. With increase in disorder, the superfluid density is strongly suppressed at low temperatures and evolves towards a linear-T variation at higher temperatures. These observations provide strong evidence that phase fluctuation leads to the formati…
We implement the effects of disorder on a holographic superconductor by introducing a random chemical potential on the boundary. We demonstrate explicitly that increasing disorder leads to the formation of islands where the superconducting order is enhanced and subsequently to the transition to a metal. We study the behavior of the superfluid density and of the conductivity as a function of the strength of disorder. We find explanations for various marked features in the conductivities in terms of hydrodynamic quasi-normal modes of the holographic superconductors. These identifications plus a …
We study the effect of disorder symmetry in a disordered s-wave superconductor. We begin with an attractive Hubbard model on a two-dimensional square lattice in the presence of diagonal- and off-diagonal disorder. The model is studied numerically using Bogoliubov-deGennes mean-field approach. We find that the off-diagonal disorder is much more efficient in destroying superconducting order. A detailed analysis brings out very distinct qualitative pictures in the two cases: diagonal disorder leads to formation of small scale isolated superconducting islands separated by large region of normal me…
In this paper we present a method to compute the exact density of states induced by $N$ non magnetic impurities in a system of two dimensional Dirac fermions in the unitarity limit. We review the case of the $π$-flux phase of the Heisenberg model and also treat the disordered d-wave superconductor. In both case we find additional states in the gap with $δρ(ω) \simeq n_i/ |ω(\ln^2 |ω/Δ_0| + (π/2)^2)|$.
Disorder in Weyl semimetals and superconductors is surprisingly subtle, attracting attention and competing theories in recent years. In this brief review, we discuss the current theoretical understanding of the effects of short-ranged, quenched disorder on the low energy-properties of three-dimensional, topological Weyl semimetals and superconductors. We focus on the role of non-perturbative rare region effects on destabilizing the semimetal phase and rounding the expected semimetal-to-diffusive metal transition into a cross over. Furthermore, the consequences of disorder on the resulting natu…
Isolated islands in two-dimensional strongly-disordered and strongly-coupled superconductors become optically active inducing sub-gap collective excitations in the ac conductivity. Here, we investigate the fate of these excitations as a function of the disorder strength in the experimentally relevant case of weak electron-phonon coupling. An explicit calculation of the ac conductivity, that includes vertex corrections to restore gauge symmetry, reveals the existence of collective sub-gap excitations, related to phase fluctuations and therefore identified as the Goldstone modes, for intermediat…
We make the first testable predictions for the local two-particle spectral function of a disordered s-wave superconductor, probed by scanning Josephson spectroscopy (sjs), providing complementary information to scanning tunneling spectroscopy (sts). We show that sjs provides a direct map of the local superconducting order parameter that is found to be anticorrelated with the gap map obtained by sts. Furthermore, this anticorrelation increases with disorder. For the momentum resolved spectral function, we find the Higgs mode shows a non-dispersive subgap feature at low momenta, spectrally separ…
As a prototype of a disordered superconductor we consider the attractive Hubbard model with on-site disorder. We solve the Bogoljubov-de-Gennes equations on two-dimensional finite clusters at zero temperature and evaluate the electromagnetic response to a vector potential. We find that the standard decoupling between transverse and longitudinal response does not apply in the presence of disorder. Moreover the superfluid density is strongly reduced by the relaxation of the phase of the order parameter already at mean-field level when disorder is large. We also find that the anharmonicity of the…
The notion of spontaneous formation of an inhomogeneous superconducting state is at the heart of most theories attempting to understand the superconducting state in the presence of strong disorder. Using scanning tunneling spectroscopy and high resolution scanning transmission electron microscopy, we experimentally demonstrate that under the competing effects of strong homogeneous disorder and superconducting correlations, the superconducting state of a conventional superconductor, NbN, spontaneously segregates into domains. Tracking these domains as a function of temperature we observe that t…
More than fifty years old "Anderson's theorem" suggests disorder-independent pair-amplitude and critical temperature at low to moderate strength of disorders. In spite of the extension of this paradigm and several subsequent theoretical proposals, mechanism for the superconductor-insulator transition (SIT) at large disorder is still an open problem. The understanding of experimental data at intermediate disorder is also lacking. Here, we proceed beyond "Anderson's theorem" by calculating disorder-averaged two-point pair-amplitude fluctuations. We find this correlation to be finite and long-ran…
Motivated by recent proposals of correlation induced insensitivity of d-wave superconductors to impurities, we develop a simple pairing theory for these systems for up to a moderate strength of disorder. Our description implements the key ideas of Anderson, originally proposed for disordered s-wave superconductors, but in addition takes care of the inherent strong electronic repulsion in these compounds, as well as disorder induced inhomogeneities. We first obtain the self-consistent one-particle states, that capture the effects of disorder exactly, and strong correlations using Gutzwiller app…
Spectroscopic evidence of disorder-induced quantum phase transitions in monolayer Fe(Te,Se) superconductor
Peking University（北京大学）；ShanghaiTech University（上海科技大学）；Quantum Science Center of Guangdong-Hong Kong-Macao Greater Bay Area (Guangdong)（粤港澳大湾区量子科学中心（广东））；Renmin University of China（中国人民大学）；The Ohio State University（俄亥俄州立大学）；Hefei National Laboratory（合肥国家实验室）；Collaborative Innovation Center of Quantum Matter（量子物质协同创新中心）
In a recent Letter Balatsky and Salkola made their conclusion about the absence of localization in disordered d-wave superconductors exploiting the idea that strongly overlapping impurity states formed a network capable to provide the transport. We present here the correct estimate of hopping matrix elements between two impurities which were the basic quantities for the subsequent consideration in the abovementioned Letter. We conclude, that the picture of the impurity-impurity potential acting only within the slowly broadening tails claimed by Balatsky and Salkola as well as all the physical …
We implement the effects of disorder on a holographic p-wave superconductor by introducing a random chemical potential which defines the local energy of the charge carriers. Since there are various possibilities for the orientation of the vector order parameter, we explore the behavior of the condensate in the parallel and perpendicular directions to the introduced disorder. We clarify the nature of various branches representing competing solutions and construct the disordered phase diagram. We find that moderate disorder enhances superconductivity as determined by the value of the condensate.…
We study a simple model of a two-dimensional s-wave superconductor in the presence of a random potential in the regime of large disorder. We first use the Bogoliubov-de Gennes (BdG) approach to show that, with increasing disorder the pairing amplitude becomes spatially inhomogeneous, and the system cannot be described within conventional approaches for studying disordered superconductors which assume a uniform order parameter. In the high disorder regime, we find that the system breaks up into superconducting islands (with large pairing amplitude) separated by an insulating sea. We show that t…
