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arXiv 0809.0666cond-mat.str-el
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KCuF3在Neel温度以上对称性变化的光学证据

Optical evidence for symmetry changes above the Neel temperature in KCuF3

J. Deisenhofer, I. Leonov, M. V. Eremin, Ch. Kant, P. Ghigna, F. Mayr, V. V. Iglamov, V. I. Anisimov, D. van der Marell

摘要:

我们报告的光学测量的一维海森堡反铁磁体KCuF3。晶体场激发的Cu 2+离子已被观察到,其温度依赖性可以理解的磁性和交换诱导的偶极机制和振动相互作用。在T_N以上,我们观察到一个新的温标T_S,其特征是出现了与Paolasini等人[Phys.Rev.Lett. 88,106403(2002)]。这些光学跃迁的出现为Neel温度以上的对称性变化提供了证据,该对称性变化影响轨道有序并为反铁磁有序铺平了道路。

英文摘要:

We report on optical measurements of the 1D Heisenberg antiferromagnet KCuF3. The crystal-field excitations of the Cu2+ ions have been observed and their temperature dependence can be understood in terms of magnetic and exchange-induced dipole mechanisms and vibronic interactions. Above T_N we observe a new temperature scale T_S characterized by the emergence of narrow absorption features that correlate with changes of the orbital ordering as observed by Paolasini et al. [Phys. Rev. Lett. 88, 106403 (2002)]. The appearance of these optical transitions provides evidence for a symmetry change above the Neel temperature that affects the orbital ordering and paves the way for the antiferromagnetic ordering.

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