We describe a simple strontium vapor cell for laser spectroscopy experiments. Strontium vapor is produced using an electrically heated commercial dispenser source. The sealed cell operates at room temperature, and without a buffer gas or vacuum pump. The cell was characterised using laser spectroscopy, and was found to offer stable and robust operation, with an estimated lifetime of >10,000 hours. By changing the dispenser, this technique can be readily extended to other alkali and alkaline earth elements.
Alkali metal dispensers have become an indispensable tool in the production of atomic vapors for magnetometry, alkali vapor cell clocks, and laser cooling experiments. A primary advantage of these dispensers is that they contain alkali metal in an inert form that can be exposed to air without hazard. However, their high temperature of operation (>600 C) is undesirable for many applications, as it shifts the atomic speed distribution to higher values and presents a radiative heat source that can raise the temperature of its surroundings. For this reason, dispensers are typically not used in lin…
Here, we report our studies on the continuous loading of a U-magneto-optical trap (U-MOT) on atom-chip from background rubidium (Rb) vapor generated using a dispenser source in ultra high vacuum (UHV) environment. Using the U-MOT loading curves, the partial pressure due to Rb vapor and pressure due to background gas have been estimated near the MOT cloud position. The estimated pressure due to Rb vapor increased from $\sim \; 1.4 \times 10^{-10}$ Torr to $ \sim \; 4.1 \times 10^{-9} $ Torr as Rb-dispenser current was increased from 2.8 to 3.4 A. The increase in dispenser current also resulted …
We report the construction of a simple, light weight and compact atomic beam spectroscopy cell for Strontium atoms. The cell is built using glass blowing technique and includes a simple Titanium Sublimation Pump for active pumping of the residual and background gases to maintain ultra-high vacuum. Commercially available and electrically heated dispenser source is used to generate the beam of Sr atoms. We perform spectroscopy on the $5s^2\ ^1S_0\longrightarrow 5s\ 5p\ ^1P_1$ transition to obtain a well resolved Doppler free spectroscopic signal for frequency stabilization of the laser source. T…
A dichroic atomic vapor laser lock (DAVLL) system exploiting buffer-gas-filled millimeter-scale vapor cells is presented. This system offers similar stability as achievable with conventional DAVLL system using bulk vapor cells, but has several important advantages. In addition to its compactness, it may provide continuous stabilization in a multi-gigahertz range around the optical transition. This range may be controlled either by changing the temperature of the vapor or by application of a buffer gas under an appropriate pressure. In particular, we experimentally demonstrate the ability of th…
We demonstrate a compact (0.25 L) system for laser cooling and trapping atoms from a heated dispenser source. Our system uses a nanofabricated diffraction grating to generate a magneto-optical trap (MOT) using a single input laser beam. An aperture in the grating allows atoms from the dispenser to be loaded from behind the chip, increasing the interaction distance of atoms with the cooling light. To take full advantage of this increased distance, we extend the magnetic field gradient of the MOT to create a Zeeman slower. The MOT traps approximately $10^6$ $^7$Li atoms emitted from an effusive …
The knowledge of the frequency noise spectrum of a diode laser is of interest in several high resolution experiments. Specifically, in laser-pumped vapor cell clocks, it is well established that the laser frequency noise plays a role in affecting the clock performances. It is then important to characterize the frequency noise of a diode laser, especially since such measurements are rarely found in the literature and hardly ever provided by vendors. In this paper, we describe a technique based on a frequency-to-voltage converter that transforms the laser frequency fluctuations into voltage fluc…
We have studied the temporal behavior of the atomic absorption signal under resonant excitation with a continuous-wave laser radiation. Measurements done for D2 line of 85Rb with ~ 1 ns temporal resolution have shown irregular oscillatory behavior of the transmission signal, which becomes well pronounced for high laser power, and disappears when the laser is tuned off-resonance. Application of the fast Fourier transform analysis of the transmission signal reveals power-dependent frequency peaks, which are shown to be associated with Rabi frequency. Possible linkage of the observed results with…
We report a robust method of stabilizing a laser to the frequency of an atomic transition using a hollow cathode lamp. In contrast to the standard dichroic atomic vapor laser lock (DAVLL) method, which uses dichroism induced by a longitudinal magnetic field, we employ birefringence induced by a transversal magnetic field. We applied this method to the $(5s^2)\ {}^{1}S_{0} - (5s5p)\ {}^{1}P_{1}$ transition (461 nm) of Sr. Although the hollow cathode is made of ferromagnetic material, we successfully applied a magnetic field of sufficient strength to obtain an error signal with a theoretical max…
We have developed and implemented a compact transparent nozzle for use in laser vaporization sources. This nozzle eliminates the need for an ablation aperture, allowing for a more intense molecular beam. We use this nozzle to prepare a molecular beam of aluminum monohydride (AlH) suitable for ion trap loading of AlH$^+$ via photoionization in ultra-high vacuum. We demonstrate stable AlH production over hour time scales using a liquid ablation target. The long-term stability, low heat load and fast ion production rate of this source are well-suited to molecular ion experiments employing destruc…
We demonstrate the single-photon excitation spectra of cesium Rydberg atoms by means of a Doppler-free purely all-optical detection with a room-temperature vapor cell and a 319 nm ultra-violet (UV) laser. We excite atoms directly from 6S1/2 ground state to 71P3/2 Rydberg state with a narrow-linewidth 319 nm UV laser. The detection of Rydberg states is performed by monitoring the absorption of an 852 nm probe beam in a V-type three-level system. With a strong coupling light, we observe the Autler-Townes doublet and investigate experimentally the dependence of the separation and linewidth on the…
We report the fabrication of alkali-metal vapor cells using femtosecond laser machining. This laser-written vapor-cell (LWVC) technology allows arbitrarily-shaped 3D interior volumes and has potential for integration with photonic structures and optical components. We use non-evaporable getters both to dispense rubidium and to absorb buffer gas. This enables us to produce cells with sub-atmospheric buffer gas pressures without vacuum apparatus. We demonstrate sub-Doppler saturated absorption spectroscopy and single beam optical magnetometry with a single LWVC. The LWVC technology may find appl…
Generation of nonclassical light is an essential tool for quantum optics research and applications in quantum information technology. We present realization of the source of nonclassically correlated photon pairs based on the process of spontaneous four-wave-mixing in warm atomic vapor. Atoms are excited only by a single laser beam in retro-reflected configuration and narrowband frequency filtering is employed for selection of correlated photon pairs. Nonclassicality of generated light fields is proved by analysis of their statistical properties. Measured parameters of the presented source pro…
We investigate a solid-state, reversible, alkali-ion battery (AIB) capable of regulating the density of alkali atoms in a vacuum system used for the production of laser-cooled atoms. The cold-atom sample can be used with in-vacuum chronoamperometry as a diagnostic for the voltage-controlled electrochemical reaction that sources or sinks alkali atoms into the vapor. In a combined reaction-diffusion-limited regime, we show that the number of laser-cooled atoms in a magneto-optical trap can be increased both by initially loading the AIB from the vapor for longer, and by using higher voltages acro…
A comprehensive study of three-photon electromagnetically-induced transparency (EIT) and absorption (EIA) on the rubidium cascade $5S_{1/2} \rightarrow 5P_{3/2}$ (laser wavelength 780~nm), $5P_{3/2} \rightarrow 5D_{5/2}$ (776~nm), and $5D_{5/2}\rightarrow 28F_{7/2}$ (1260~nm) is performed. The 780-nm probe and 776-nm dressing beams are counter-aligned through a Rb room-temperature vapor cell, and the 1260-nm coupler beam is co- or counter-aligned with the probe beam. Several cases of EIT and EIA, measured over a range of detunings of the 776-nm beam, are studied. The observed phenomena are mod…
We demonstrate a single-photon Rydberg excitation spectroscopy of cesium (Cs) atoms in a room-temperature vapor cell. Cs atoms are excited directly from 6S1/2 ground state to nP3/2 (n = 70 - 100) Rydberg states with a 318.6 nm ultraviolet (UV) laser,and Rydberg excitation spectra are obtained by transmission enhancement of a probe beam resonant to Cs 6S1/2, F = 4 - 6P3/2, F' = 5 transition as partial population on F = 4 ground state are transferred to Rydberg state .Analysis reveals that the observed spectra are velocity-selective spectroscopy of Rydberg state, from which the amplitude and lin…
Magnetic resonance of sodium fluorescence is studied with varying laser intensity, duty cycle, and field strength. A magnetometer based on sodium vapor cell filled with He buffer gas is demonstrated, which uses a single amplitude-modulated laser beam. With a 589 nm laser tuned at D1 or D2 line, the magnetic field is inferred from the variation of fluorescence. A magnetic field sensitivity of 150 pT per Hz square root is achieved at D1 line. The work is a step towards sensitive remote magnetometry with mesospheric sodium.
We study $Λ$-type Electromagnetically Induced Transparency (EIT) on the Rb D2 transition in a buffer-gas-free thermal vapor cell without anti-relaxation coating. Experimental data show distinguished features of velocity-selective optical pumping and one EIT resonance. The Zeeman splitting of the EIT line in magnetic fields up to 12 Gauss is investigated. One Zeeman component is free of the first-order shift and its second-order shift agrees well with theory. The full width at half maximum (FWHM) of this magnetic-field-insensitive EIT resonance is reduced due to Doppler narrowing, scales linear…
A nanometer-thin-cell (in the direction of laser beam propagation) has been elaborated with the thickness of the atomic vapor column varying smoothly in the range of $L = \unit[50-1500]{nm}$. The cell allows one to study the behavior of the resonance absorption over the $D_1$ line of potassium atoms by varying the laser intensity and the cell thickness from $L = λ/ 2$ to $L = 2 λ$ with the step $λ/2$ ($λ=\unit[770]{nm}$ is the resonant wavelength of the laser). It is shown that despite the huge Doppler broadening ($>\unit[0.9]{GHz}$ at the cell temperature $\unit[170]{^{\circ}C}$), at low lase…
We demonstrate a high-performance coherent-population-trapping (CPT) Cs vapor cell atomic clock using the push-pull optical pumping technique (PPOP) in the pulsed regime, allowing the detection of high-contrast and narrow Ramsey-CPT fringes. The impact of several experimental parameters onto the clock resonance and short-term fractional frequency stability, including the laser power, the cell temperature and the Ramsey sequence parameters, has been investigated. We observe and explain the existence of a slight dependence on laser power of the central Ramsey-CPT fringe line-width in the pulsed …
Experimental measurements and calculations of STIRAP transfer efficiencies were made on a sodium gas starting from the $3^2{\rm S}_{1/2}$ electronic ground state, passing through the $3^2{\rm P}_{1/2}$ and/or the $3^2{\rm P}_{3/2}$ to the $5^2{\rm S}_{1/2}$ state. The lasers used in the experiments had a pulse width of several picoseconds and were close to the Fourier transform limit. Although the linewidth of the laser was much smaller than the spin orbit splitting between the $3^2{\rm P}_{1/2}$ and $3^2{\rm P}_{3/2}$ states, Experiments and calculations reveal that both 3p states play a role…
DEVCOM Army Research Laboratory South（美国陆军研发司令部南实验室）；Department of Physics, The American University（美国大学物理系）；General Technical Services（通用技术服务公司）；Department of Physics, Center for Complex Quantum Systems, The University of Texas at Austin（德克萨斯大学奥斯汀分校复杂量子系统中心物理系）；DEVCOM Army Research Laboratory（美国陆军研发司令部实验室）
Spontaneous emission from individual atoms in vapor lasts nanoseconds, if not microseconds, and beatings in this emission involve only directly excited energy sublevels. In contrast, the superfluorescent emissions burst on a much-reduced timescale and their beatings involve both directly and indirectly excited energy sublevels. In this work, picosecond and femtosecond superfluorescent beatings are observed from a dense cesium atomic vapor. Cesium atoms are excited by 60-femtosecond long, 800 nm laser pulses via two-photon processes into their coherent superpositions of the ground 6S and excite…
Chip-scale atomic devices built around micro-fabricated alkali vapor cells are at the forefront of compact metrology and atomic sensors. We demonstrate a micro-fabricated vapor cell that is actively-pumped to ultra-high-vacuum (UHV) to achieve laser cooling. A grating magneto optical trap (GMOT) is incorporated with the 4 mm-thick Si/glass vacuum cell to demonstrate the feasibility of a fully-miniaturized laser cooling platform. A two-step optical excitation process in rubidium is used to overcome surface-scatter limitations to the GMOT imaging. The unambiguous miniaturization and form-customi…
We present Rydberg-state electromagnetically-induced-transparency (EIT) measurements examining the effects of laser polarization, magnetic fields, laser intensities, and the optical density of the thermal $^{87}$Rb medium. Two counter-propagating laser beams with wavelengths of 480 nm and 780 nm were employed to sweep the spectrum across the Rydberg states $|33D_{3/2}\rangle$ and $|33D_{5/2}\rangle$. An analytic transmission expression well fits the Rydberg-EIT spectra with multiple transitions under different magnetic fields and laser polarization after accounting for the relevant Clebsch-Gor…
We optically excite $^{85}$Rb atoms in a heated vapor cell to a low-lying Rydberg state 10D$_{5/2}$ and observe directional terahertz (THz) beams at 3.3 THz and 7.8 THz. These THz fields are generated by amplified spontaneous emission from the 10D$_{5/2}$ state to the 11P$_{3/2}$ and 8F$_{7/2}$ states, respectively. In addition, we observe ultraviolet (UV) light produced by four-wave mixing of optical pump lasers and the 3.3 THz field. We characterize the generated THz power over the detuning and power of pump lasers, and identify experimental conditions favoring THz and UV generation, respect…
Rydberg-atom-enabled atomic vapor cell technologies show great potentials in developing devices for quantum enhanced sensors. In this paper, we demonstrate laser induced DC electric fields in an all-glass vapor cell without bulk or thin film electrodes. The spatial field distribution is mapped by Rydberg electromagnetically induced transparency spectroscopy. We explain the measured with a boundary-value electrostatic model. This work may inspire new ideas for DC electric field control in designing miniaturized atomic vapor cell devices. Limitations and other charge effects are also discussed.
We demonstrate matterwave interference in a warm vapor of rubidium atoms. Established approaches to light pulse atom interferometry rely on laser cooling to concentrate a large ensemble of atoms into a velocity class resonant with the atom optical light pulse. In our experiment, we show that clear interference signals may be obtained without laser cooling. This effect relies on the Doppler selectivity of the atom interferometer resonance. This interferometer may be configured to measure accelerations, and we demonstrate that multiple interferometers may be operated simultaneously by addressing…
We have characterized the molecular tellurium (Te$_2$) spectrum in the vicinity of the 423nm $^1S_0-^1P_1$ and the 431nm $^3P_1-^3P_0$ transitions in neutral calcium. These transitions are relevant to optical clocks for atomic-beam characterization and cooling (423nm) and enhanced detection (431nm). The use of a Te$_2$ vapor cell as a frequency reference has many advantages over other laser stabilization techniques, and we discuss an application to measuring the instability due to the second-order Doppler shift in a calcium beam clock.
We study telecom-wavelength spectra of a Rydberg state in an atomic vapor with a three-photon excitation scheme. Two lasers of 780 nm and 776 nm are used to pump Rubidium-85 atoms in a vapor cell to the $5D_{\mathrm{5/2}}$ state, from which a probe beam of 1292 nm in the O-band telecommunication wavelength drives a transition to the $21F_{\mathrm{7/2}}$ Rydberg state. We investigate the probe spectra over the power of pump lasers. The simulation based on a 4-level theoretical model captures the main features of the experimental results. This spectroscopic study paves the way for future experim…
We use two continuous-wave (CW) laser beams of 780 nm and 515 nm to optically drive $^{85}$Rb atoms in a heated vapor cell to a low-lying Rydberg state 10D$_{5/2}$. We observe a collimated ultraviolet (UV) beam at 311 nm, corresponding to the transition frequency from the 11P$_{3/2}$ state to the 5S$_{1/2}$ state. This indicates the presence of a coherent four-wave mixing process, built up by two input laser fields as well as a terahertz (THz) radiation of 3.28 THz that is generated by amplified spontaneous emission between the 10D$_{5/2}$ and the 11P$_{3/2}$ states. We characterize the 311 nm…
Recent experimental observations of laser-induced adsorption at the interface between an alkali vapor and a dielectric surface have demonstrated the possibility of growing metallic films of nanometric thickness on dielectric surfaces, with arbitrary shapes determined by the intensity profile of the light. The mechanisms directly responsible for the accumulation of atoms at the irradiated surface have been shown to involve photo-ionization of atoms very close to the surface. However, the existence of a vapor-pressure threshold for initiating the film growth still raises questions on the process…
We demonstrate backward-directed continuous-wave (cw) emission at 2.21 μm generated on the 4P3/2-4S1/2 population-inverted transition in Na vapors two-photon excited with resonant laser light at 589 and 569 nm. Our study of power and atom-number-density threshold characteristics shows that lasing occurs at sub-10 mW total power of the applied laser light. The observed 6 mrad divergence is defined mainly by the aspect ratio of the gain region. We find that mirrorless lasing at 2.21 μm is magnetic field and polarization dependent that may be useful for remote magnetometry. The presented results …
Atomic devices such as atomic clocks and optically-pumped magnetometers rely on the interrogation of atoms contained in a cell whose inner content has to meet high standards of purity and accuracy. Glass-blowing techniques and craftsmanship have evolved over many decades to achieve such standards in macroscopic vapor cells. With the emergence of chip-scale atomic devices, the need for miniaturization and mass fabrication has led to the adoption of microfabrication techniques to make millimeter-scale vapor cells. However, many shortcomings remain and no process has been able to match the qualit…
