We demonstrate the capability of complete thresholdless lasing operation between dressed states of a two-level atom located inside a microscopic cavity engineered in a photonic band-gap material. We distinguish between threshold and thresholdless behaves by analyzing the Mandel's Q parameter for the cavity field. We find that the threshold behave depends on whether the spontaneous emission is or is not present on the lasing transition. In the presence of the spontaneous emission, the mean photon number of the cavity field exhibits threshold behavior indicating that the system may operate as an ordinary laser. When the spontaneous emission is eliminated on the lasing transition, no threshold is observed for all values of the pumping rate indicating the system becomes a thresholdless laser. Moreover, we find that under a thresholdless operation, the mean photon number can increase nonlinearly with the pumping rate, and this process is accompanied by a sub-Poisson statistics of the field. This suggests that the nonclassical statistics can be used to distinguish a nonlinear operation of the dressed-atom laser.
We investigate spectral properties of the atomic fluorescence and the output field of the cavity-mode of a single-atom dressed-state laser in a photonic crystal. We pay a particular attention to the behavior of the spectra in the presence of the frequency dependent reservoir and search for signatures of the thresholdless lasing. Although the thresholdless behavior has been predicted by analyzing the photon statistics of the cavity field, we find that the threshold behavior still exists in the spectrum of the cavity field. We find that the structure of cavity field spectrum depends strongly on …
We identify a class of dressed atom-photon states formingat the same energy of the atom at any coupling strength. As a hallmark, their photonic component is an eigenstate of the bare photonic bath with a vacancy in place of the atom. The picture accommodates waveguide-QED phenomena where atoms behave as perfect mirrors, connecting in particular dressed bound states (BS) in the continuum or BIC with geometrically-confined photonic modes. When applied to photonic lattices, the framework provides a general criterion to predict dressed BS in lattices with topological properties by putting them in …
Making analogy with atomic physics is a powerful tool for photonic technology, witnessed by the recent development in topological photonics and non-Hermitian photonics based on parity-time symmetry. Mollow triplet is a prominent atomic effect with both fundamental and technological importance. Here we demonstrate the analogue of Mollow triplet with quantum photonic systems. Photonic entanglement is generated with spontaneous nonlinear processes in dressed photonic modes, which are introduced through coherent multimode coupling. We further demonstrate the flexibility of the photonic system to r…
In a cavity quantum electrodynamics (QED) system, where atoms coherently interact with photons in a cavity, the eigenstates of the system are the superposition states of atoms and cavity photons, the so-called dressed states of atoms. When two cavities are connected by an optical fiber with negligible loss, the coherent coupling between the cavities gives rise to photonic normal modes. One of these normal modes is the fiber-dark mode, in which photons are delocalized in the two distant cavities. Here we demonstrate the setting of coupled-cavities QED, where two nanofiber cavity-QED systems are…
Dressed states forming when quantum emitters or atoms couple to a photonic bath underpin a number of phenomena and applications, in particular dispersive effective interactions occurring within photonic bandgaps. Here, we present a compact formulation of the resolvent-based theory for calculating atom-photon dressed states built on the idea that the atom behaves as an effective impurity. This establishes an explicit connection with the standard impurity problem in condensed matter. Moreover, it allows us to formulate and settle in a model-independent context a number of properties previously k…
We discuss the properties of atom-photon bound states in waveguide QED systems consisting of single or multiple atoms coupled strongly to a finite-bandwidth photonic channel. Such bound states are formed by an atom and a localized photonic excitation and represent the continuum analog of the familiar dressed states in single-mode cavity QED. Here we present a detailed analysis of the linear and nonlinear spectral features associated with single- and multi-photon dressed states and show how the formation of bound states affects the waveguide-mediated dipole-dipole interactions between separated…
We study non-classical and spectral properties of a strongly driven single-atom laser engineered within a photonic crystal that facilitates a frequency-dependent reservoir. In these studies, we apply a dressed atom model approach to derive the master equation of the system and study the properties of the dressed laser under the frequency dependent transition rates. By going beyond the secular approximation in the dressed-atom cavity field interaction, we find that if, in addition, the non-secular terms are included into the dynamics of the system, then non-linear processes can occur that lead …
We investigate the photon induced tunneling phenomena in a photonic crystal cavity containing a strongly coupled quantum dot and describe how this tunneling can be used to generate photon states consisting mainly of a particular Fock state. Additionally, we study experimentally the photon-induced tunneling as a function of excitation laser power and frequency and show the signature of second rung of the Jaynes-Cummings Hamiltonian in the observed photon-statistics.
This paper gives an overview of recent work on three-dimensional (3D) photonic crystals with a "full and complete" 3D photonic band gap. We review five main aspects: 1) spontaneous emission inhibition, 2) spatial localization of light within a tiny nanoscale volume (aka "a nanobox for light"), 3) the introduction of a gain medium leading to thresholdless lasers, 4) breaking of the weak-coupling approximation of cavity QED, both in the frequency and in the time-domain, 5) decoherence, in particular the shielding of vacuum fluctuations by a 3D photonic bandgap. In addition, we list and evaluate …
Studying the spontaneous emission of a V-type three-level atom embedded in a photonic crystal (PC) by fractional calculus, we found that the atomic excited states in the anisotropic PC can be expressed as a superposition of four dressed states analytically. Through detuning two allowed atomic transition energies with respect to the photonic band edge, the coupling between these two transitions leads to three dynamic regimes, namely non-Markovian decay, damped quantum interference and quantum interference, classified by the numbers of contributed bounded dressed states. From the degree of quant…
The bichromatic driving of a solid state cavity quantum electrodynamics system is used to probe cavity dressed state transitions and observe coherent interaction between the system and the light field. We theoretically demonstrate the higher order cavity-dressed states, supersplitting, and AC stark shift in a solid state system comprised of a quantum dot strongly coupled to a photonic crystal cavity for on- and far off-resonant cases. For the off-resonant case, phonons mediate off-resonant coupling between the quantum dot and the photonic resonator, a phenomenon unique to solid state cavity qu…
Dressed-State Optomechanics in the Few-Photon Regime
Ulm University（乌尔姆大学）；Institute for Complex Quantum Systems and IQST, Ulm University（乌尔姆大学复杂量子系统与IQST研究所）；German Aerospace Center (DLR), Institute of Quantum Technologies（德国航空航天中心（DLR）量子技术研究所）
We present the model of one-dimensional chain of two-level artificial atoms driven with dc field and quantum light simultaneously in strong coupling regime. The interaction of atoms with light leads to entanglement of electron and photon states (dressing of the atoms). The driving via dc field leads to the Bloch oscillations (BO) in the chain of dressed atoms. We considered the mutual influence of dressing and BO and show that scenario of oscillations dramatically differs from predicted by the Jaynes-Cummings and Bloch-Zener models. We study the evolution of the population inversion, tunneling…
In this work, robustness of controlled density of optical states in doubly driven artificial atoms is studied under phonon dissipation. By using both perturbative and polaron approaches, we investigate the influence of carrier-phonon interactions on the emission properties of a two-level solid-state emitter, simultaneously coupled to two intense distinguishable lasers. Phonon decoherence effects on the emission spectra are found modest up to neon boiling temperatures ($\sim 30$ K), as compared with photon generation at the Fourier transform limit obtained in absence of lattice vibrations (zero…
Photon-mediated interactions between quantum emitters in engineered photonic baths is an emerging area of quantum optics. At the same time, non-Hermitian (NH) physics is currently thriving, spurred by the exciting possibility to access new physics in systems ruled by non-trivial NH Hamiltonians - in particular photonic lattices - which can challenge longstanding tenets such as the Bloch theory of bands. Here, we combine these two fields and study the exotic interaction between emitters mediated by the photonic modes of a lossy photonic lattice described by a NH Hamiltonian. We show in a paradi…
We propose a set of photonic crystals that realize a nonlinear quantum Rabi model equivalent to a two-level system driven by the phase of a quantized electromagnetic field. The crystals are exactly soluble in the weak-coupling regime and their dispersion relation is discrete. The system is diagonalized by normal modes equivalent to a dressed state basis. In the strong-coupling regime, we use perturbation theory and find that the dispersion relation is continuous and give the normal modes of the crystal in terms of continued fractions. We show that these photonic crystals allow state reconstruc…
The interaction of organic molecules and molecular aggregates with electromagnetic fields that are strongly confined inside optical cavities within nanoscale volumes, has allowed the observation of exotic quantum regimes of light-matter interaction at room temperature, for a wide variety of cavity materials and geometries. Understanding the universal features of such organic cavities represents a significant challenge for theoretical modelling, as experiments show that these systems are characterized by an intricate competition between coherent and dissipative processes involving entangled nuc…
We present the design of a chiral photonic quantum link, where distant atoms interact by exchanging photons propagating in a single direction in free-space. This is achieved by coupling each atom in a laser-assisted process to an atomic array acting as a quantum phased-array antenna. This provides a basic building block for quantum networks in free space, i.e. without requiring cavities or nanostructures, which we illustrate with high-fidelity quantum state transfer protocols. Our setup can be implemented with neutral atoms using Rydberg-dressed interactions.
We investigate the dynamics of a two-level atom flying through a photonic cavity when the light-matter interaction is in the ultrastrong coupling regime. We adopt a closed full quantum description that takes into account the quantization of the atom center-of-mass motion in addition to its internal degree of freedom and to the quantized photonic cavity field. We find that multiple qualitatively different dynamical regimes are achievable according to two key figures of merit: the ratio between the kinetic energy and the bare excitation energies, and the product of these bare energies with the t…
We propose a generic approach to nonresonant laser cooling of atoms/molecules in a bistable optical cavity. The method exemplifies a photonic version of Sisyphus cooling, in which the matter-dressed cavity extracts energy from the particles and discharges it to the external field as a result of sudden transitions between two stable states.
We study a two-level system (atom, superconducting qubit or quantum dot) strongly coupled to the single photonic mode of a cavity, in the presence of incoherent pumping and including detuning and dephasing. This system displays a striking quantum to classical transition. On the grounds of several approximations that reproduce to various degrees exact results obtained numerically, we separate five regimes of operations, that we term "linear", "quantum", "lasing", "quenching" and "thermal". In the fully quantized picture, the lasing regime arises as a condensation of dressed states and manifests…
We show that the dynamical Casimir effect in an optomechanical system can be achieved under incoherent mechanical pumping. We adopt a fully quantum-mechanical approach for both the cavity field and the oscillating mirror. The dynamics is then evaluated using a recently-developed master equation approach in the dressed picture, including both zero and finite temperature photonic reservoirs. This analysis shows that the dynamical Casimir effect can be observed even when the mean value of the mechanical displacement is zero. This opens up new possibilities for the experimental observation of this…
The quantum photodynamics of a simple diatomic molecule with a permanent dipole immersed within an optical cavity containing a quantized radiation field is studied in detail. The chosen molecule under study, lithium fluoride (LiF), is characterized by the presence of an avoided crossing between the two lowest $^1Σ$ potential energy curves (covalent-ionic diabatic crossing). Without field, after prompt excitation from the ground state $1\; ^1Σ$, the excited nuclear wave packet moves back and forth in the upper $2\; ^1Σ$ state, but in the proximity of the avoided crossing, the non-adiabatic coup…
We present an efficient time domain numerical scheme for computing spontaneous emission dynamics in colored vacua. Starting from first principles, we map the unitary evolution of a dressed two-level quantum emitter onto the problem of electromagnetic radiation from a complex harmonic oscillator under self-interaction conditions. This latter oscillator-field system can be efficiently integrated by using finite difference time domain method without the need for calculating the photonic eigenmodes of the surrounding environment. In contrast to earlier investigations, our computational framework p…
The fields of quantum simulation with cold atoms [1] and quantum optics [2] are currently being merged. In a set of recent pathbreaking experiments with atoms in optical cavities [3,4] lattice quantum many-body systems with both, a short-range interaction and a strong interaction potential of infinite range -mediated by a quantized optical light field- were realized. A theoretical modelling of these systems faces considerable complexity at the interface of: (i) spontaneous symmetry-breaking and emergent phases of interacting many-body systems with a large number of atoms $N\rightarrow\infty$, …
We demonstrate the ability to control the spontaneous emission from a superconducting qubit coupled to a cavity. The time domain profile of the emitted photon is shaped into a symmetric truncated exponential. The experiment is enabled by a qubit coupled to a cavity, with a coupling strength that can be tuned in tens of nanoseconds while maintaining a constant dressed state emission frequency. Symmetrization of the photonic wave packet will enable use of photons as flying qubits for transfering the quantum state between atoms in distant cavities.
Single atoms coupled to a cavity offer unique opportunities as quantum optomechanical devices because of their small mass and strong interaction with light. A particular regime of interest in optomechanics is that of "single-photon strong coupling," where motional displacements on the order of the zero-point uncertainty are sufficient to shift the cavity resonance frequency by more than its linewidth. In many cavity QED platforms, however, this is unfeasible due to the large cavity linewidth. Here, we propose an alternative route in such systems, which instead relies on the coupling of atomic …
