Light-shift tomography in an optical-dipole trap for neutral atoms
Jean-Philippe Brantut, Jean-François Clément, Martin Robert De Saint Vincent, Gael Varoquaux, Robert A. Nyman, Alain Aspect, Thomas Bourdel, Philippe Bouyer
We report on light-shift tomography of a cloud of 87 Rb atoms in a far-detuned optical-dipole trap at 1565 nm. Our method is based on standard absorption imaging, but takes advantage of the strong light-shift of the excited state of the imaging transition, which is due to a quasi-resonance of the trapping laser with a higher excited level. We use this method to (i) map the equipotentials of a crossed optical-dipole trap, and (ii) study the thermalisation of an atomic cloud by following the evolution of the potential-energy of atoms during the free-evaporation process.
We report on an investigation of loading characteristics of deep microscopic dipole traps. The dipole trap is loaded from a low density magneto optical trap (MOT) containing $\approx 5\times 10^{6}$ atoms. We determine the loading parameters that maximize the trapped atom number for a trap of waist 5 μm with trap depths ranging from 3.5 mK to 10 mK. We determine the optimal trap loading conditions and the loading rates, loss coefficients and temperature of the trapped atoms under these conditions. We show that it is possible to load a few hundred to thousand atoms in dipole traps of depth 3.5 …
One important factor which determines efficiency of loading cold atoms into an optical dipole trap from a magneto-optical trap is the distance between the trap centers. By studying this efficiency for various optical trap depths (2--110 mK) we find that for optimum dipole trap loading, longitudinal displacements up to 15 mm are necessary. An explanation for this observation is presented and compared with other work and a simple analytical formula is derived for the optimum distance between the trap centers.
We report an optical dipole trap for calcium. The trap is created by focusing a 488 nm argon-ion laser beam into a calcium magneto-optical trap. The argon-ion laser photo-ionizes atoms in the trap because of a near-resonance with the 4s4f 1F3 level. By measuring the dipole trap decay rate as a function of argon-ion laser intensity, we determine the 1F3 photo-ionization cross section at our wavelength to be approximately 230 Mb.
It has been shown in an earlier publication that magnetic field gradients applied to particles in traps can induce Larmor frequency shifts that may falsely be interpreted as electric-dipole moment (EDM) signals. This study has now been extended to include nonuniform magnetic field gradients due to the presence of a local magnetic dipole. It is found that, in the high orbit-frequency regime, the magnitude of the shifts can be enhanced beyond the simple expectation of proportionality to the volume-averaged magnetic-field gradient.
We explore the classical dynamics of atoms in an optical dipole trap formed by two identical Gaussian beams propagating in perpendicular directions. The phase space is a mixture of regular and chaotic orbits, the later becoming dominant as the energy of the atoms increases. The trapping capabilities of these perpendicular Gaussian beams are investigated by considering an atomic ensemble in free motion. After a sudden turn on of the dipole trap, a certain fraction of atoms in the ensemble remains trapped. The majority of these trapped atoms has energies larger than the escape channels, which ca…
The parity of atomic wave functions prevents neutral atoms from having permanent electric-dipole moment. Electric-dipole moment is induced in an atom when exposed to strong light, the electric field of the light. Hence the optical trapping of neutral atoms relies on the induced dipole moment. Here we present the calculated numerical values of the detuning, potential depth, minimum laser power required to trap $^{87}$Rb ($D_2$ line) atoms using lasers of wavelength 1064 nm, 850 nm, 820 nm and 800 nm and beam waists 50$μ$m, 100$μ$m and 200$μ$m.
Quantum gases of rare-earth elements are of interest due to the large magnetic moment of many of those elements, leading to strong dipole-dipole interactions, as well as an often nonvanishing orbital angular momentum in the electronic ground state, with prospects for long coherence time Raman manipulation, and state-dependent lattice potentials. We report on the realization of a Bose-Einstein condensate of erbium atoms in a quasielectrostatic optical dipole trap generated by a tightly focused midinfrared optical beam derived from a $\textrm{CO}_2$ laser near 10.6$μ$m in wavelength. The quasist…
We report an apparatus and method capable of producing Bose-Einstein condensates (BECs) of ~1x10^6 87Rb atoms, and ultimately designed for sympathetic cooling of 133Cs and the creation of ultracold RbCs molecules. The method combines several elements: i) the large recapture of a magnetic quadrupole trap from a magneto-optical trap, ii) efficient forced RF evaporation in such a magnetic trap, iii) the gain in phase-space density obtained when loading the magnetically trapped atoms into a far red-detuned optical dipole trap and iv) efficient evaporation to BEC within the dipole trap. We demonstr…
We describe a model of inelastic and elastic collisional dynamics of atoms in an optical dipole trap that utilizes numerical evaluation of statistical mechanical quantities and numerical solution of equations for the evolution of number and temperature of trapped atoms. It can be used for traps that possess little spatial symmetry and when the ratio of trap depth to sample temperature is relatively small. We compare simulation results with experiments on $^{88}$Sr and $^{84}$Sr, which have well-characterized collisional properties.
We consider the practical feasibility of using the direct, electric dipole-dipole interaction between co-trapped molecular ions for robust quantum logic without the need for static polarizing fields. The use of oscillating dipole moments, as opposed to static electric dipoles, dynamically decouples the dipoles from laboratory fields, including the electric fields of the trap itself. Further, this implementation does not require quantum control of motion, potentially removing a major roadblock to ion trap quantum computing scalability. Since the polarizing field is electromagnetic radiation, ev…
The influence of large permanent dipoles on molecular orbital tomography via high-order harmonic generation (HHG) is investigated in this work. It is found that, owing to the modification of the angle-dependent ionization rate resulting from the Stark shift, the one-side-recollision condition for the tomographic imaging can not be satisfied even with the few-cycle driving pulses. To overcome this problem, we employ a tailored driving pulse by adding a weak low-frequency pulse to the few-cycle laser pulse to control the HHG process and the recollision of the continuum electrons are effectively …
We have trapped cesium atoms over many minutes in the focus of a CO$_2$-laser beam employing an extremely simple laser system. Collisional properties of the unpolarized atoms in their electronic ground state are investigated. Inelastic binary collisions changing the hyperfine state lead to trap loss which is quantitatively analyzed. Elastic collisions result in evaporative cooling of the trapped gas from 25 $μ$K to 10 $μ$K over a time scale of about 150 s.
We demonstrate loading of SrF molecules into an optical dipole trap (ODT) via in-trap $Λ$-cooling. We find that this cooling can be optimized by a proper choice of relative ODT and $Λ$ beam polarizations. In this optimized configuration, we observe molecules with temperatures as low as 14(1) $μ$K in traps with depths up to 570 $μ$K. With optimized parameters, we transfer $\!\sim\!5$% of molecules from our radio-frequency magneto-optical trap into the ODT, at a density of $\sim\!2\times 10^{9}$ cm$^{-3}$, a phase space density of $\sim\!2\times 10^{-7}$, and with a trap lifetime of $\!\sim\!1$ …
We present quantitative measurements of the photoassociation of cesium molecules inside a far-detuned optical dipole trap. A model of the trap depletion dynamics is derived which allows to extract absolute photoassociation rate coefficients for the initial single-photon photoassociation step from measured trap-loss spectra. The sensitivity of this approach is demonstrated by measuring the Franck-Condon modulation of the weak photoassociation transitions into the low vibrational levels of the outer well of the 0g- state that correlates to the 6s+6p3/2 asymptote. The measurements are compared to…
We experimentally study the breakdown of hyperfine coupling for an atom in a deep optical-dipole trap. One-color laser spectroscopy is performed at the resonance lines of a single $^{87}$Rb atom for a trap wavelength of 1064 nm. Evidence of hyperfine breakdown comes from three observations, namely a nonlinear dependence of the transition frequencies on the trap intensity, a splitting of lines which are degenerate for small intensities, and the ability to drive transitions which would be forbidden by selection rules in the absence of hyperfine breakdown. From the data, we infer the hyperfine in…
The effect of the dipole-dipole interaction on the far-off-resonance optical dipole trapping scheme is calculated by a mean-field approach. The trapping laser field polarizes the atoms and the accompanying dipole-dipole energy shift deepens the attractive potential minimum in a pancake-shaped cloud. At high density the thermal motion cannot stabilize the gas against self-contraction and an instability occurs. We calculate the boundary of the stable and unstable equilibrium regions on a two-dimensional phase diagram of the atom number and the ratio of the trap depth to the temperature. We discu…
We demonstrate a novel optical dipole trap which is based on the enhancement of the optical power density of a Nd:YAG laser beam in a resonator. The trap is particularly suited for experiments with ultracold gases, as it combines a potential depth of order 1 mK with storage times of several tens of seconds. We study the interactions in a gas of fermionic lithium atoms in our trap and observe the influence of spin-changing collisions and off-resonant photon scattering. A key element in reaching long storage times is an ultra-low noise laser. The dependence of the storage time on laser noise is …
We propose a novel Sisyphus cooling scheme for atoms confined in a far off resonance optical dipole trap. Utilizing the differential trap-induced AC Stark shift, two electronic levels of the atom are resonantly coupled by a cooling laser preferentially near the trap bottom. After absorption of a cooling photon, the atom loses energy by climbing the steeper potential, and then spontaneously decays preferentially away from the trap bottom. The proposed method is particularly suited to cooling alkaline-earth-like atoms where two-level systems with narrow electronic transitions are present. Numeri…
We have measured the AC-Stark shift of the $14D_{5/2}$ Rydberg state of rubidium 87 in an optical dipole trap formed by a focussed CO$_2$-laser. We find good quantitative agreement with the model of a free electron experiencing a ponderomotive potential in the light field. In order to reproduce the observed spectra we take into account the broadening of the Rydberg state due to photoionization. The extracted cross-section is compatible with previous measurements on neighboring Rydberg states.
We present the first simultaneous trapping of two different ultracold atomic species in a conservative trap. Lithium and cesium atoms are stored in an optical dipole trap formed by the focus of a CO$_2$ laser. Techniques for loading both species of atoms are discussed and observations of elastic and inelastic collisions between the two species are presented. A model for sympathetic cooling of two species with strongly different mass in the presence of slow evaporation is developed. From the observed Cs-induced evaporation of Li atoms we estimate a cross section for cold elastic Li-Cs collision…
Dipolar atoms have unique properties, making them interesting for laser cooling and quantum simulations. But, due to relatively large orbital momentum in the ground state these atoms may have large dynamic tensor and vector polarizabilities in the ground state. This enables the formation of spin-dependent optical traps. In this paper real part of tensor and vector dynamic polarizability was experimentally measured and compared to theoretical simulation. For an optical dipole trap operating around 532.07 nm tensor, polarizability was found to be $ - 145 \pm 53\,\,{\rm{a}}{\rm{.u}}{\rm{.}}$ and …
We study the quantum properties of Rydberg atoms in a magnetic Ioffe-Pritchard trap which is superimposed by a homogeneous electric field. Trapped Rydberg atoms can be created in long-lived electronic states exhibiting a permanent electric dipole moment of several hundred Debye. The resulting dipole-dipole interaction in conjunction with the radial confinement is demonstrated to give rise to an effectively one-dimensional ultracold Rydberg gas with a macroscopic interparticle distance. We derive analytical expressions for the electric dipole moment and the critical linear density of Rydberg at…
We present studies of strong coupling in single-photon photoassociation of cesium dimers using an optical dipole trap. A thermodynamic model of the trap depletion dynamics is employed to extract absolute rate coefficents. From the dependence of the rate coefficient on the photoassociation laser intensity, we observe saturation of the photoassociation scattering probability at the unitarity limit in quantitative agreement with the theoretical model by Bohn and Julienne [Phys. Rev. A, 60, 414 (1999)]. Also the corresponding power broadening of the resonance width is measured. We could not observ…
Recently thulium has been condensed to Bose-Einstein condensate. Machine learning was used to avoid a detailed study of all obstacles making cooling difficult. This paper analyses the atomic loss mechanism for the 532 nm optical trap, used in the Bose-condensation experiment, and compares it with the alternative and more traditional micron-range optical dipole trap. We also measured the scalar and tensor polarizability of thulium at 1064 nm and was found to be $167\pm 25$ a.u. ($275\pm 41\times {{10}^{-41}}\text{F }\cdot \text{ }{\text{m}^{\text{2}}}$) and $-4\pm 1$ a.u. ($7\pm 2\times {{10}^{…
We present the simultaneous cooling and trapping of an isotopic mixture in a magneto-optical trap and we describe the transfer of the mixture into a conservative, far-off resonant dipole trap. The mixture is prepared with a new technique that applies to intermediate and heavy alkaline earth like atoms. In this work, 88Sr and 86Sr are simultaneously loaded first into the magneto-optical trap operated on the 1S0-3P1 spin-forbidden line at 689 nm, and then transferred into the dipole trap. We observe fast inter-species thermalization in the dipole trap which allows one to set a lower bound on the…
The absolute photodetachment cross section of OH- anions at a rotational and translational temperature of 170K is determined by measuring the detachment-induced decay rate of the anions in a multipole radio-frequency ion trap. In comparison with previous results, the obtained cross section shows the importance of the initial rotational state distribution. Using a tomography scan of the photodetachment laser through the trapped ion cloud, the derived cross section is model-independent and thus features a small systematic uncertainty. The tomography also yields the column density of the OH- anio…
The evanescent field surrounding nano-scale optical waveguides offers an efficient interface between light and mesoscopic ensembles of neutral atoms. However, the thermal motion of trapped atoms, combined with the strong radial gradients of the guided light, leads to a time-modulated coupling between atoms and the light mode, thus giving rise to additional noise and motional dephasing of collective states. Here, we present a dipole force free scheme for coupling of the radial motional states, utilizing the strong intensity gradient of the guided mode and demonstrate all-optical coupling of the…
Ion-atom interactions are a comparatively recent field of research that has drawn considerable attention due to its applications in areas including quantum chemistry and quantum simulations. In first experiments, atomic ions and neutral atoms have been successfully overlapped by devising hybrid apparatuses combining established trapping methods, Paul traps for ions and optical or magneto-optical traps for neutral atoms, respectively. Since then, the field has seen considerable progress, but the inherent presence of radiofrequency (rf) fields in such hybrid traps was found to have a limiting im…
We report loading of laser-cooled caesium atoms into a hollow-core photonic-bandgap fiber and confining the atoms in the fiber's 7 $μm$ diameter core with a magic-wavelength dipole trap at $\sim$935 nm. The use of the magic wavelength removes the AC-Stark shift of the 852nm optical transition in caesium caused by the dipole trap in the fiber core and suppresses the inhomogeneous broadening of the atomic ensemble that arises from the radial distribution of the atoms. This opens the possibility to continuously probe the atoms over time scales of a millisecond -- approximately 1000 times longer t…
Heavy polar molecules can be used to measure the electric dipole moment of the electron, which is a sensitive probe of physics beyond the Standard Model. The value is determined by measuring the precession of the molecule's spin in a plane perpendicular to an applied electric field. The longer this precession evolves coherently, the higher the precision of the measurement. For molecules in a trap, this coherence time could be very long indeed. We evaluate the sensitivity of an experiment where neutral molecules are trapped electrically, and compare this to an equivalent measurement in a molecu…
Single atoms are interesting candidates for studying quantum optics and quantum information processing. Recently, trapping and manipulation of single atoms using tight optical dipole traps have generated considerable interest. Here we report an experimental investigation of the dynamics of atoms in a modified optical dipole trap with a backward propagating dipole trap beam, where a change in the two-atom collision rate by six times has been achieved. The theoretical model presented gives a prediction of high probabilities of few-atom loading rates under proper experimental conditions. This wor…
We report on highly effective trapping of cold atoms by a new method for a stable single optical trap in the near-optical resonant regime. An optical trap with the near-optical resonance condition consists of not only the dipole but also the radiative forces, while a trap using a far-off resonance dominates only the dipole force. We estimate a near-optical resonant trap for ultracold rubidium atoms in the range between -0.373 and -2.23 THz from the resonance. The time dependence of the trapped atoms indicates some difference of the stable center-of-mass positions in the near-optical resonant t…
We present a combined computational and experimental study to optimize the efficiency of evaporative cooling for atoms in optical dipole traps. By employing a kinetic model of evaporation, we provide a strategy for determining the optimal relation between atom temperature, trap depth, and average trap frequency during evaporation given experimental initial conditions. We then experimentally implement a highly efficient evaporation process in an optical dipole trap, showing excellent agreement between the theory and experiment. This method has allowed the creation of pure Bose-Einstein condensa…
In the present work, the effect of AC-Stark shift (i.e. light-shift) in optical dipole trap on in-situ absorption probe imaging of the trapped atoms has been investigated. We have calculated the light-shift of various energy levels of $^{87}$Rb atoms relevant for trapping in an optical dipole trap (ODT). The spatial varying intensity of the ODT beam results in position dependent light-shift (i.e. AC-Stark shift). Such modifications in the energy levels of the atom result in modification in the absorption cross-section, which finally modifies the optical density (OD) in in-situ absorption imagi…
We investigate fluorescence detection using a standing wave of blue-detuned light of one or more atoms held in a deep, microscopic dipole trap. The blue-detuned standing wave realizes a Sisyphus laser cooling mechanism so that an atom can scatter many photons while remaining trapped. When imaging more than one atom, the blue detuning limits loss due to inelastic light-assisted collisions. Using this standing wave probe beam, we demonstrate that we can count from one to the order of 100 atoms in the microtrap with sub-poissonian precision.
We experimentally investigate $σ^+$-$σ^-$ polarization gradient cooling~(PGC) of a single $^{87}$Rb atom in a tightly focused dipole trap and show that the cooling limit strongly depends on the polarization of the trapping field. For optimized cooling light power, the temperature of the atom reaches~$10.4(6)\,μ$K in a linearly polarized trap, approximately five times lower than in a circularly polarized trap. The inhibition of PGC is qualitatively explained by the fictitious magnetic fields induced by the trapping field. We further demonstrate that switching the trap polarization from linear t…
Optical trapping of selected species of radioactive atoms has great potential in precision measurements for testing fundamental physics such as EDM, PNC and parity violating beta-decay asymmetry correlation coefficients. We report trapping of 10^4 radioactive ^{82}Rb atoms (t_{1/2}=75 s) with a trap lifetime of ~55 seconds in an optical dipole trap. Transfer efficiency from the magneto-optical trap was ~14%. We further report the evidence of spontaneous spin polarization of the atoms in optical dipole trap loading. This advancement is an important step towards a new generation of precision J-b…
We report on the achieving of Bose-Einstein condensation of a dilute atomic gas based on trapping atoms in tightly confining CO_2-laser dipole potentials. Quantum degeneracy of rubidium atoms is reached by direct evaporative cooling in both crossed and single beam trapping geometries. At the heart of these all-optical condensation experiments is the ability to obtain high initial atomic densities in quasistatic dipole traps by laser cooling techniques. Finally, we demonstrate the formation of a condensate in a field insensitive m_F=0 spin projection only. This suppresses fluctuations of the ch…
We report a simple method for the creation of Bose-Einstein condensates of $^{85}$Rb by direct evaporation in a crossed optical dipole trap. The independent control of the trap frequencies and magnetic bias field afforded by the trapping scheme permits full control of the trapped atomic sample, enabling the collision parameters to be easily manipulated to achieve efficient evaporation in the vicinity of the 155 G Feshbach resonance. We produce nearly pure condensates of up to $4\times10^4$ atoms and demonstrate the tunable nature of the atomic interactions.
The electric dipole moments of various neutral elementary particles, such as neutron, neutrinos, certain hypothetical dark matter particles and others, are predicted to exist by the standard model of high energy physics and various extensions of it. However, the predicted values are beyond the present experimental capabilities. We propose to simulate and emulate the electric dipole moment of neutral relativistic particles and the ensuing effects in the presence of electrostatic field by emulation of an extended Dirac equation in ion traps.
We present the experimental realization of a compressible blue detuned crossed dipole trap for cold atoms allowing for fast dynamical compression (~ 5 - 10 ms) of 5x10^7 Rubidium atoms up to densities of ~ 10^13 cm^-3. The dipole trap consists of two intersecting tubes of blue-detuned laser light. These tubes are formed using a single, rapidly rotating laser beam which, for sufficiently fast rotation frequencies, can be accurately described by a quasi-static potential. The atomic cloud is compressed by dynamically reducing the trap volume leading to densities close to the Ioffe-Reggel criterio…
We demonstrate a simple scheme to reach Bose-Einstein condensation (BEC) of metastable triplet helium atoms using a single beam optical dipole trap with moderate power of less than 3 W. Our scheme is based on RF-induced evaporative cooling in a quadrupole magnetic trap and transfer to a single beam optical dipole trap that is located below the magnetic trap center. We transfer 1x10^6 atoms into the optical dipole trap, with an initial temperature of 14 μK, and observe efficient forced evaporative cooling both in a hybrid trap, in which the quadrupole magnetic trap operates just below the levit…
The capture of a moving atom by a non-dissipative trap, such as an optical dipole trap, requires the removal of the excessive kinetic energy of the atom. In this article we develop a mechanism to harvest ultra cold atoms from a guided atom beam into an optical dipole trap by removing their directed kinetic energy. We propose a continuous loading scheme where this is accomplished via deceleration by a magnetic potential barrier followed by optical pumping to the energetically lowest Zeeman sublevel. We theoretically investigate the application of this scheme to the transfer of ultra cold chromi…
The subject of this review are atom traps based on optical dipole forces in laser fields, along with their unique features as storage devices at ultralow energies. The basic physics of the dipole interaction is discussed, and the experimental background of dipole trapping experiments is explained. Specific trapping schemes and experiments are presented, where the wide range of applications of dipole traps is explored considering particular examples.
We measure the AC-Stark shifts of the 5S{1/2}, F=2 to 5P{3/2}, F'=3 transitions of individual optically trapped 87Rb atoms using a non-destructive detection technique that allows us to measure the fluorescent signal of one-and-the-same atom for over 60 seconds. These measurements allow efficient and rapid characterization of single atom traps that is required for many coherent quantum information protocols. Although this method is demonstrated using a single atom trap, the concept is readily extended to resolvable atomic arrays.
We report the all-optical production of a Rb87 Bose-Einstein condensate (BEC) in a simple 1.06 micron dipole trap experiment. We load a single beam dipole trap directly from a magneto-optic trap (MOT) using an optimized loading sequence. After evaporation in the single beam, a second crossed beam is used for compression. The intensity in both beams is then reduced for evaporation to BEC. We obtain a BEC with 3.5E4 atoms after 3 seconds of total evaporation time. We also give a detailed account of the thermal distribution in cross beam traps. This account highlights the possible difficulties in…
A dynamic blue-detuned optical dipole trap with stable $^{87}Rb$ atoms produces a differential ac Stark shift of 18 Hz in the ground state hyperfine transition, and it preserves the ground state hyperfine superpositions for a long coherence time of 180 ms. The trapped atoms undergoing microwave Rabi oscillations are sensitive to a small signal, artificially generated with a second microwave source, phase locked to the first allow- ing a simple and effective method for determining signal-to-noise ratio limits through interference techniques. This provides an excellent means of calibrating sensi…
In recent years, cold atoms could prove their scientific impact not only on ground but in microgravity environments such as the drop tower in Bremen, sounding rockets and parabolic flights. We investigate the preparation of cold atoms in an optical dipole trap, with an emphasis on evaporative cooling under microgravity. Up to $ 1\times10^{6} $ rubidium-87 atoms were optically trapped from a temporarily dark magneto optical trap during free fall in the droptower in Bremen. The efficiency of evaporation is determined to be equal with and without the effect of gravity. This is confirmed using num…
The quadrupole interaction between the Rydberg electronic states of a Rydberg ion and the radio frequency electric field of the ion trap is analyzed. Such a coupling is negligible for the lowest energy levels of a trapped ion but it is important for a trapped Rydberg ion due to its large electric dipole moment. This coupling cannot be neglected by the standard rotating-wave approximation because it is comparable to the frequency of the trapping electric field. We investigate the effect of the quadrupole coupling by performing a suitable effective representation of the Hamiltonian. For a single…
An integrated optical dipole trap uses two-color (red and blue-detuned) traveling evanescent wave fields for trapping cold neutral atoms. To achieve longitudinal confinement, we propose using an integrated optical waveguide coupler, which provides a potential gradient along the beam propagation direction sufficient to confine atoms. This integrated optical dipole trap can support an atomic ensemble with a large optical depth due to its small mode area. Its quasi-TE0 waveguide mode has an advantage over the HE11 mode of a nanofiber, with little inhomogeneous Zeeman broadening at the trapping re…
