We revisit the approach proposed by Mukamel and coworkers to describe interacting excitons through infinite series of composite-boson operators for both, the system Hamiltonian and the exciton commutator -- which, in this approach, is properly kept different from its elementary boson value. Instead of free electron-hole operators, as used by Mukamel's group, we here work with composite-exciton operators which are physically relevant operators for excited semiconductors. This allows us to get \emph{all} terms of these infinite series explicitly, the first terms of each series agreeing with the ones obtained by Mukamel's group when written with electron-hole pairs. All these terms nicely read in terms of Pauli and interaction scatterings of the composite-exciton many-body theory we have recently proposed. However, even if knowledge of these infinite series now allows to tackle $N$-body problems, not just 2-body problems like third order nonlinear susceptibility $χ^{(3)}$, the necessary handling of these two infinite series makes this approach far more complicated than the one we have developed and which barely relies on just four commutators.
We derive the closure relation for $N$ polaritons made of three different types of excitons: bosonized excitons, Frenkel or Wannier excitons. In the case of polaritons made of Wannier excitons, we show how this closure relation, which appears as non-diagonal, may reduce to the one of $N$ elementary bosons, the photons, with its $1/N!$ prefactor, or to the one of $N$ Wannier excitons, with its $(1/N!)^2$ prefactor. Widely different forms of closure relations are thus found depending on the composite bosons at hand. Comparison with closure relations of excitons, either bosonized or kept composit…
This paper introduces a new quantum object, the ``coboson'', for composite particles, like the excitons, which are made of two fermions. Although commonly dealed with as elementary bosons, these composite bosons -- ``cobosons'' in short -- differ from them due to their composite nature which makes the handling of their many-body effects quite different from the existing treatments valid for elementary bosons. Due to this composite nature, it is not possible to correctly describe the interaction between cobosons as a potential $V$. Consequently, the standard Fermi golden rule, written in terms …
We have recently constructed a many-body theory for composite excitons, in which the possible carrier exchanges between $N$ excitons can be treated exactly through a set of dimensionless ``Pauli scatterings'' between two excitons. Many-body effects with excitons turn out to be rather simple because excitons are the exact one-electron-hole-pair eigenstates of the semiconductor Hamiltonian, thus forming a complete orthogonal set for one-pair states. It can however be of interest to extend this new many-body theory to more complicated composite bosons, \emph{i. e.}, ``cobosons'', which are not ne…
We present a many-body theory for Frenkel excitons which takes into account their composite nature exactly. Our approach is based on four commutators similar to the ones we previously proposed for Wannier excitons. They allow us to calculate any physical quantity dealing with $N$ excitons in terms of "Pauli scatterings" for carrier exchange in the absence of carrier interaction and "interaction scatterings" for carrier interaction in the absence of carrier exchange. We show that Frenkel excitons have a novel "transfer assisted exchange scattering", specific to these excitons. It comes from ind…
We here consider an exciton $i$ embedded in a sea of $N$ identical excitons 0. If the excitons are bosonized, a bosonic enhancement factor, proportional to $N$, is found for $i=0$. If the exciton composite nature is kept, this enhancement not only exists for $i=0$, but also for any exciton having a center of mass momentum equal to the sea exciton momentum. This physically comes from the fact that an exciton with such a momentum can be transformed into a sea exciton by ``Pauli scattering'', \emph{i}. \emph{e}., carrier exchange with the sea, making this $i$ exciton not so much different from a …
Charged excitons of composite fermions (CFs) are considered in the fractional quantum Hall effect. Energies of the charged CF excitons are computed at $ν=1/3$ as a function of the size of exciton. We show that the charged CF exciton with size of roton is lower in energy than the unbound state of a neutral roton and a lone charge. Therefore we propose that the lowest-energy excitation of the fractional quantum Hall effect is in fact due to the charged excitons of composite fermions composed of two CF-particles and one CF-hole. We believe that charged excitons of composite fermions shed new ligh…
By using the composite many-body theory for Frenkel excitons we have recently developed, we here derive the ground state energy of $N$ Frenkel excitons in the Born approximation through the Hamiltonian mean value in a state made of $N$ identical $\mathbf{Q=0}$ excitons. While this quantity reads as a density expansion in the case of Wannier excitons, due to many-body effects induced by fermion exchanges between $N$ composite particles, we show that the Hamiltonian mean value for $N$ Frenkel excitons only contains a first order term in density, just as for elementary bosons. Such a simple resul…
The aim of this paper is to clarify the conceptual difference which exists between the interactions of composite bosons and the interactions of elementary bosons. A special focus is made on the physical processes which are missed when composite bosons are replaced by elementary bosons. Although what is here said directly applies to excitons, it is also valid for bosons in other fields than semiconductor physics. We in particular explain how the two basic scatterings -- Coulomb and Pauli -- of our many-body theory for composite excitons can be extended to a pair of fermions which is not an Hami…
We present a quantitative microscopic analysis of the formation of exciton-polaritons, the composite particles possessing light and material components, polariton-polariton interactions, and resonant pumping dynamics in cylindrical semiconductor micropillars. We discuss how the redistribution effect can be used in devices generating photons with non zero orbital angular momenta.
We present a new exciton-based formalism for calculating the coherent response of asymmetric semiconductor multiple quantum well structures to ultra-short optical pulses valid to infinite order in the optical field and including the self-generated intraband fields. We use these equations to calculate and explain the oscillations with time delay of peaks in the spectrally-resolved degenerate four wave mixing signals from biased semiconductor superlattices, obtaining good agreement with experiment.
We consider a nanostructure consisting of a semiconductor quantum dot coupled to a metal nanoparticle, and show with numerical simulations that the exciton state of the quantum dot can be robustly generated from the ground state even for small interparticle distances, using conventional chirped pulses with Gaussian and hyperbolic secant envelopes. The asymmetry observed in the final exciton population with respect to the chirp sign of the applied pulses is explained using the nonlinear density matrix equations describing the system, and is attributed to the real part of the parameter emerging …
Half-filled Landau levels admit the theoretically powerful fermion-vortex duality but longstanding puzzles remain in their experimental realization as $ν_T=1$ quantum Hall bilayers, further complicated by Zheng et al's recent numerical discovery of an unknown phase at intermediate layer spacing. Here we propose that half-filled quantum Hall bilayers ($ν_T=1$) at intermediate values of the interlayer distance $d/\ell_B$ enter a phase with \textit{paired exciton condensation}. This phase shows signatures analogous to the condensate of interlayer excitons (electrons bound to opposite-layer holes)…
Exact diagonalization studies have revealed that the energy spectrum of interacting electrons in the lowest Landau level splits, non-perturbatively, into bands, which is responsible for the fascinating phenomenology of this system. The theory of nearly free composite fermions has been shown to be valid for the lowest band, and thus to capture the low temperature physics, but it over-predicts the number of states for the excited bands. We explain the state counting of higher bands in terms of composite fermions with an infinitely strong short range interaction between an excited composite-fermi…
We compute the exciton transfer (ET) rate between semiconducting single-wall carbon nanotubes (SWNTs). We show that the main reasons for the wide range of measured ET rates reported in the literature are 1) exciton confinement in local quantum wells stemming from disorder in the environment and 2) exciton thermalization between dark and bright states due to intratube scattering. The SWNT excitonic states are calculated by solving the Bethe-Salpeter equation using tight-binding basis functions. The ET rates due to intertube Coulomb interaction are computed via Fermi's golden rule. In pristine s…
Although excitons are not exact bosons, they are commonly treated as such provided that their composite nature is included in effective scatterings dressed by exchange. We here \emph{prove} that, \emph{whatever these scatterings are}, they cannot give both the scattering rates $T_{ij}^{-1}$ and the exciton lifetime $τ_0$, correctly: A striking factor 1/2 exists between $τ_0^{-1}$ and the sum of $T_{ij}^{-1}$'s, which originates from the composite nature of excitons, irretrievably lost when they are bosonized. This result, which appears as very disturbing at first, casts major doubts on bosoniz…
The X$^-$ trion is essentially an electron bound to an exciton. However, due to the composite nature of the exciton, there is no way to write an exciton-electron interaction potential. We can overcome this difficulty by using a commutation technique similar to the one we introduced for excitons interacting with excitons, which allows to take exactly into account the close-to-boson character of the excitons. From it, we can obtain the X$^-$ trion creation operator in terms of exciton and electron. We can also derive the X$^-$ trion ladder diagram between an exciton and an electron. These are th…
We here give a brief survey of our new many-body theory for composite excitons, as well as some of the results we have already obtained using it. In view of them, we conclude that, in order to fully trust the results one finds, interacting excitons should not be bosonized: Indeed, all effective bosonic Hamiltonians (even the hermitian ones !) can miss terms as large as the ones they generate; they can even miss the dominant term, as in problems dealing with optical nonlinearities.
We call "proteons" -- from the ever-changing greek sea-god $Πρωτε\upsilonς$ -- composite particles made of two fermions. Among them, are the semiconductor excitons, but also various atoms and molecules, like the giant molecules made of two $^{40}$K or $^6$Li atoms which have recently Bose condensed. In addition to their indistinguishability, these composite particles are ``ever-changing'' in the sense that there is no way to know with which fermions they are precisely made. As direct consequences, (i) the proteons are not true bosons, (ii) the basis made with proteon states is \emph{overcomple…
We study the interlayer coherent incompressible phase in Trilayer Quantum Hall systems (TLQH) at total filling factor $ ν_{T}=1 $ from three approaches: Mutual Composite Fermion (MCF), Composite Boson (CB) and wavefunction approach. Just like in Bilayer Quantum Hall system, CB approach is superior than MCF approach in studying TLQH with broken symmetry. The Hall and Hall drag resistivities are found to be quantized at $ h/e^{2} $. Two neutral gapless modes with linear dispersion relations are identified and the ratio of the two velocities is close to $ \sqrt{3} $. The novel excitation spectra …
The mean field (MF) composite Fermion (CF) picture successfully predicts low lying states of fractional quantum Hall systems. This success cannot be attributed to a cancellation between Coulomb and Chern-Simons interactions beyond the mean field and solely depends on the short range (SR) of the Coulomb pseudopotential in the lowest Landau level (LL). The class of pseudopotentials for which the MFCF picture can be applied is defined. The success or failure of the MFCF picture in various systems (electrons in excited LL's, Laughlin quasiparticles, charged magneto-excitons) is explained.
We study the effect of a uniform pseudomagnetic field, induced by a strain in a monolayer and double layer of gapped graphene, acting on excitons. For our analysis it is crucial that the pseudomagnetic field acts on the charges of the constituent particles of the excitons, i.e., the electrons and holes, the same way in contrast to a magnetic field. Moreover, using a circularly polarized laser field, the electrons and the holes can be excited only in one valley of the honeycomb lattice of gapped graphene. This breaks the time-reversal symmetry and provides the possibility to observe the various…
Although semiconductor Bloch equations have been widely used for decades to address ultrafast optical phenomena in semiconductors, they have a few important drawbacks: (i) Coulomb terms between free electron-hole pairs require Hartree-Fock treatment which, in its usual form, preserves excitonic poles but loses biexcitonic resonances. (ii) Solving the resulting coupled differential equations imposes heavy numerics which completely hide the physics. This can be completely avoided if, instead of free electron-hole pairs, we use correlated pairs, i.e., excitons. Their interactions are easy to hand…
The mean field (MF) composite Fermion (CF) picture successfully predicts the band of low lying angular momentum multiplets of fractional quantum Hall systems for any value of the magnetic field. This success cannot be attributed to a cancellation between Coulomb and Chern--Simons interactions between fluctuations beyond the mean field. It results instead from the short range behavior of the Coulomb pseudopotential in the lowest Landau level (LL). The class of pseudopotentials for which the MFCF picture is successful can be defined, and used to explain the success or failure of the picture in d…
Excitons in monolayer transition metal dichalcogenide (TMD) provide a paradigm of composite Boson in 2D system. This letter reports a photoluminescence and reflectance study of excitons in monolayer molybdenum diselenide (MoSe2) with electrostatic gating. We observe the repulsive and attractive Fermi polaron modes of the band edge exciton, its excited state and the spin-off excitons. Our data validate the polaronic behavior of excitonic states in the system quantitatively where the simple three-particle trion model is insufficient to explain.
We consider the effect of a magnetic field $B$ on the transport of neutral composite particles, excitons, in weakly disordered 2D systems. In the case of classical transport, when the interference of different paths is neglected, the magnetic field suppresses exciton transport, and the static diffusion constant $D(B)$ monotonically drops with $B$. When quantum-mechanical corrections due to weak localization are taken into account, $D(B)$ becomes a nonmonotonic function of $B$. In weak magnetic fields, where the magnetic length is much larger than the exciton Bohr radius, $l_B >> a_B$, a positi…
We present a fully microscopic approach to the transition rate of two exciton-photon polaritons. The non-trivial consequences of the polariton composite nature -- here treated exactly through a development of our composite-exciton many-body theory -- lead to results noticeably different from the ones of the conventional approaches in which polaritons are mapped into elementary bosons. Our work reveals an appealing fundamental scattering which corresponds to a photon-assisted exchange -- in the absence of Coulomb process. This scattering being dominant when one of the scattered polaritons has a…
A cavity-polariton, formed due to the strong coupling between exciton and cavity mode, is one of the most promising composite bosons for realizing macroscopic spontaneous coherence at high temperature. Up to date, most of polariton quantum degeneracy experiments were conducted in the complicated two-dimensional (2D) planar microcavities. The role of dimensionality in coherent quantum degeneracy of a composite bosonic system of exciton polaritons remains mysterious. Here we report the first experimental observation of a one-dimensional (1D) polariton condensate in a ZnO microwire at room temper…
The quantum nature of matter lies in the wave function phases that accumulate while particles move along their trajectories. A prominent example is the Aharonov-Bohm phase, which has been studied in connection with the conductance of nanostructures. However, optical response in solids is determined by neutral excitations, for which no sensitivity to magnetic flux would be expected. We propose a new mechanism for the topological phase of a neutral particle, a polarized exciton confined to a semiconductor quantum ring. We predict that this magnetic-field induced phase may strongly affect exciton…
The optical exciton Aharonov-Bohm effect, i. e. an oscillatory component in the energy of optically active (bright) states, is investigated in nanorings. It is shown that a small effective electron mass, strong confinement of the electron, and high barrier for the hole, achieved e. g. by an InAs nanoring embedded in an AlGaSb quantum well, are favorable for observing the optical exciton Aharonov-Bohm effect. The second derivative of the exciton energy with respect to the magnetic field is utilized to extract Aharonov-Bohm oscillations even for the lowest bright state unambiguously. A connectio…
We propose a trial wave function for the quantum Hall bilayer system of total filling factor $ν_T=1$ at a layer distance $d$ to magnetic length $\ell$ ratio $d/\ell=κ_{c1}\approx1.1$, where the lowest charged excitation is known to have a level crossing. The wave function has two-particle correlations which fit well with those in previous numerical studies, and can be viewed as a Bose-Einstein condensate of free excitons formed by composite bosons and anti-composite bosons in different layers. We show the free nature of these excitons indicating an emergent SU(2) symmetry for the composite bos…
In organic semiconductors working under ambient circumstance, there are remarkable quantum effects lack of comprehensive understanding, and an exotic composite particle named charge transfer (CT) exciton is normally regarded as the key ingredient. Another essential substance is the phonons stemming from intra- and inter-molecular vibrations, and the relevant diagonal electron-phonon couplings give rise to spatial localization and the off-diagonal couplings refer to the dispersion of electron wavefunctions. In this work, we first propose a toy model based upon the fracton physics to phenomenolo…
The quantum Hall effect is studied by introducing two different matrix variables for electrons and holes, having Chern-Simons type interactions. By generalizing the constraint condition proposed by Susskind to realize the Pauli's exclusion principle in this two component matrix model, the classical exciton solution having excitation of both quasi-electron and quasi-hole is obtained. The constraint condition is also solved quantum mechanically in the infinite-sized matrix case, giving the examples of the physical states. Using these quantum states, the corrections of the exciton energy, coming …
We apply the fermion commutation technique for composite bosons to polariton-polariton scattering in semiconductor planar microcavities. Derivations are presented in a simple and physically transparent fashion. A procedure of orthogonolization of the initial and final two-exciton state wavefunctions is used to calculate the effective scattering matrix elements and the scattering rates. We show how the bosonic stimulation of the scattering appears in this full fermionic approach whose equivalence to the bosonization method is thus demonstrated in the regime of low exciton density. We find an ad…
We explore the mechanism for the long-lived quantum coherence by considering the discrete phonon modes: these vibrational modes effectively weaken the exciton-environment interaction, due to the new composite (polaron) formed by excitons and vibrons. This subsequently demonstrates the role of vibrational coherence which greatly contributes to long-lived feature of the excitonic coherence that has been observed in femtosecond experiments. The estimation of the timescale of coherence elongated by vibrational modes is given in an analytical manner. To test the validity of our theory, we study the…
