It has been recently pointed out that the presence of a nonmagnetic impurity in a Heisenberg antiferromagnet generates an alternating order of the surrounding spins which is independent of temperature in a wide range. Quantum Monte Carlo simulations in the two-dimensional $S=1/2$ case confirmed this picture, but showed a counterintuitive enhancement of the alternating order around the Kosterlitz-Thouless transition. We propose here an explanation in terms of the effect of vortex excitations.
Controlled doping of SrCu$_2$(BO$_3$)$_2$, a faithful realization of the Heisenberg spin-1/2 antiferromagnet on the Shastry-Sutherland lattice, with non-magnetic impurities generates bound-states below the spin gap. These bound-states and their symmetry properties are investigated by exact diagonalisation of small clusters and within a simple effective model describing a spinon submitted to an attractive extended potential. It is shown that Raman spectroscopy is a unique technique to probe these bound-states. Quantitative theoretical Raman spectra are numerically obtained.
Is Herbertsmithite far from an ideal antiferromagnet? Ab-initio answer including in-plane Dzyaloshinskii-Moriya interactions and coupling with extra-plane impurities
The effect of nonmagnetic impurities on the phase diagram of the classical Heisenberg antiferromagnet on a triangular lattice is investigated. We present analytical arguments confirmed by numerical calculations that at zero temperature vacancies stabilize a conical state providing an example of "order by quenched disorder" effect. Competition between thermal fluctuations and the site disorder leads to a complicated H-T phase diagram, which is deduced from the classical Monte Carlo simulations for a representative vacancy concentration. For the XY triangular-lattice antiferromagnet with in-plan…
Impurities in triangular lattice spin 1/2 antiferromagnet
我们研究了自旋1/2受抑三角形反铁磁体中杂质的影响，目的是了解在有机自旋液体材料$κ$ -（ET）$_2$ Cu $_2$（CN）$_3$中观察到的$^{13}$ C NMR谱线的增宽。在高温下，我们计算了最近邻Heisenberg模型在$J/3$附近和晶界附近的局域磁化率。我们发现，在几个晶格间距的局部磁化率衰减到均匀的，和低密度的杂质，我们将无法解释的线加宽的实验中已经在升高的温度。在低温下，我们假设一个无带隙自旋液体的费米表面的自旋。利用Gutzwiller投影计算了平均场中的局域极化率，并在平均场之外进行了计算。零温局域磁化率按幂律衰减，并在$2 k_F$处振荡。正如在高温分析中，我们发现低密度的杂质不能解释观察到的谱线加宽。因此，我们得出结论，在系统中有更多的混乱。我们发现，一个大密度的点状无序给加宽，这是一致的实验下降到约5 K，但低于这个温度下，可能需要额外的机制。
In conventional quasi-one-dimensional antiferromagnets with quantum spins, magnetic excitations are carried by either magnons or spinons in different energy regimes: they do not coexist independently, nor could they interact with each other. In this Letter, by combining inelastic neutron scattering, quantum Monte Carlo simulations and Random Phase Approximation calculations, we report the discovery and discuss the physics of the coexistence of magnons and spinons and their interactions in Botallackite-Cu2(OH)3Br. This is a unique quantum antiferromagnet consisting of alternating ferromagnetic …
We theoretically study a spin-spin correlation enhanced by non-magnetic impurities in a frustrated two-leg spin ladder. The frustration is introduced by the next-nearest-neighbor antiferromagnetic interaction in the leg direction in the antiferromagnetic two-leg spin ladder. The spin-spin correlation function around impurity site is calculated by the density-matrix renormalization-group method. We find that the spin-spin correlation is enhanced around impurity site with the wavenumber reflecting the frustration. As increasing the frustration, the wavenumber is shifted from commensurate to inco…
X-ray photon correlation spectroscopy (XPCS) enables us to study dynamics of antiferromagnets. Using coherent soft X-ray diffraction, we resonantly probe Mn and Co Bragg peaks in the frustrated magnetic chain compound Lu2CoMnO6 significantly below the Neel temperature. Bragg peaks of incommensurate order slide towards commensurate 'up up down down' order with decreasing temperature. Antiferromagnetic inhomogeneities produce speckle within the Bragg peaks, whose dynamics are probed by XPCS and compared to the classic Axial Next-Nearest Neighbor Interaction model of frustration. The data support…
We consider the effects of local impurities in highly frustrated diamond lattice antiferromagnets, which exhibit large but non-extensive ground state degeneracies. Such models are appropriate to many A-site magnetic spinels. We argue very generally that sufficiently dilute impurities induce an ordered magnetic ground state, and provide a mechanism of degeneracy breaking. The states which are selected can be determined by a "swiss cheese model" analysis, which we demonstrate numerically for a particular impurity model in this case. Moreover, we present criteria for estimating the stability of t…
Dissipationless dynamics of spin supersolid states in a spin-1/2 triangular antiferromagnet with impurities
RIKEN Center for Emergent Matter Science (CEMS)（理化学研究所物质结构理论研究中心）；School of Physics, Beihang University（北京航空航天大学物理学院）；Institute of Theoretical Physics, Chinese Academy of Sciences（中国科学院理论物理研究所）；Peng Huanwu Collaborative Center for Research and Education, Beihang University（北京航空航天大学彭桓武研究中心）；RIKEN Center for Computational Science (R-CCS)（理化学研究所计算科学中心）；RIKEN Center for Quantum Computing (RQC)（理化学研究所量子计算中心）；RIKEN Pioneering Research Institute (PRI)（理化学所先锋研究本部）；Advanced Science Research Center, Japan Atomic Energy Agency（日本原子力研究机构先进科学研究中心）
Impurities, which are inherently present in any real material, may play an important role in the magnetism of frustrated spin systems with spin-liquid ground states. We address the impurity issue in quantum kagome antiferromagnets by investigating ZnCu$_3$(OH)$_6$SO$_4$ (Zn-brochantite) by means of muon spin spectroscopy. We show that muons couple to the impurity magnetism, originating from Cu-Zn intersite disorder, and that the impurities are highly correlated with the kagome spins, allowing us to probe the intrinsic kagome physics via a Kondo-like effect. The low-temperature plateau in local…
The doping of quantum Heisenberg antiferromagnets on the kagome lattice by non-magnetic impurities is investigated within the framework of a generalized quantum dimer model (QDM) describing a) the valence bond crystal (VBC), b) the dimer liquid and c) the critical region on equal footing. Following the approach by Ralko et al. [Phys. Rev. Lett. 101, 117204 (2008)] for the square and triangular lattices, we introduce the (minimal) extension of the QDM on the Kagome lattice to account for spontaneous creation of mobile S=1/2 spinons at finite magnetic field. Modulations of the dimer density (at …
By using the coupled cluster method, the numerical exact diagonalization method, and the numerical density matrix renormalization group method, we investigated the properties of the one-dimensional Heisenberg chain with alternating antiferromagnetic and ferromagnetic next nearest neighbor interactions. In the classical limit, the ground state is in the collinear Neel state if a<1/2, while for a>1/2, there is an noncollinear canted state. For the quantum case, we found that, although the classical Neel state is absent, the canted state exists if the frustration parameter a exceeds a critical po…
Low energy inelastic neutron scattering on single crystals of the kagome spin liquid compound ZnCu3(OD)6Cl2 (Herbertsmithite) reveals antiferromagnetic correlations between impurity spins for energy transfers E < 0.8 meV (~J/20). The momentum dependence differs significantly from higher energy scattering which arises from the intrinsic kagome spins. The low energy fluctuations are characterized by diffuse scattering near wavevectors (1 0 0) and (0 0 3/2), which is consistent with antiferromagnetic correlations between pairs of nearest neighbor Cu impurities on adjacent triangular (Zn) interlay…
We study the effect of anisotropy of spin-$S$ impurities on an antiferromagnetic SU(2) Heisenberg chain. The magnetic impurities are assumed to have an XXZ-type anisotropic exchange with its neighboring sites. First, using density-matrix renormalization group technique. we examine spin-spin correlation function, instability of Néel order, and local spin susceptibility in the presence of a single spin-$S$ impurity. Based on the results, we find that the types of spin-$S$ impurities are classified into two groups: $\rm(\hspace{.18em}i\hspace{.18em})$ nonmagnetic and $S=1$ impurities enhance only…
Magnetic polarization induced by nonmagnetic impurities in high Tc cuprates
采用变分蒙特卡罗模拟方法研究了高T_c铜酸盐化合物中锌等非磁性杂质引起的磁极化。由二维t-J模型的Bogoliubov de Gennes平均场哈密顿量得到的本征态构造了变分波函数。引入Jastrow因子来解释感应磁矩和空穴与杂质之间的排斥。通过在杂质周围形成覆盖4或5个晶格位置的反铁磁极化，获得了相当大的能量增益。我们还发现了与实验一致的诱导磁矩的掺杂依赖性。
We study a quenched disordered d=3 tJ Hamiltonian with static vacancies as a model of nonmagnetic impurities in high-Tc materials. Using a position-space renormalization-group approach, we calculate the evolution of the finite-temperature phase diagram with impurity concentration p, and find several features with close experimental parallels: away from half-filling we see the rapid destruction of a spin-singlet phase (analogous to the superconducting phase in cuprates) which is eliminated for p > 0.05; in the same region for these dilute impurity concentrations we observe an enhancement of ant…
Ordered State in a Haldane Material PbNi$_2$V$_2$O$_8$ Doped with Magnetic and Non-Magnetic Impurities
通过直流、交流磁化率和热容测量，系统地研究了掺杂卤化物Pb（Ni $_{1-x}$ $M_x$）$_2$ V $_2$ O $_8$（$M$ = Mn，Co，Cu，Mg）的杂质效应.对所有杂质普遍观察到三维有序态的出现，并得到了与其它自旋带隙材料定性相似的完整的温度-浓度相图。的独特之处是发现在激烈的依赖性的转变温度上的物种的杂质。基于VBS模型对有效哈密顿量的考虑表明，杂质与边自旋之间的铁磁次近邻相互作用和反铁磁最近邻相互作用是导致这种独特性的关键.
We theoretically investigate the Heisenberg antiferromagnet on a triangular lattice doped with nonmagnetic impurities. Two nontrivial effects resulting from collective impurity behavior are predicted. The first one is related to presence of uncompensated magnetic moments localized near vacancies as revealed by the low-temperature Curie tail in the magnetic susceptibility. These moments exhibit an anomalous growth with the impurity concentration, which we attribute to the clustering mechanism. In an external magnetic field, impurities lead to an even more peculiar phenomenon lifting the classic…
We consider the effects of impurities on the enigmatic hidden order (HO) state of the heavy-fermion material URu2Si2. In particular, we focus on local effects of Rh impurities as a tool to probe the suppression of the HO state. To study local properties we introduce a lattice free energy, where the time invariant HO order parameter "psi" and local antiferromagnetic (AFM) order parameter M are competing orders. Near each Rh atom the HO order parameter is suppressed, creating a hole in which local AFM order emerges as a result of competition. These local holes are created in the fabric of the HO…
