In this letter a general method for expanding paraxial beams into multipolar electromagnetic fields is presented. This method is applied to the expansion of paraxial modes with orbital angular momentum (OAM), showing how the paraxial OAM is related to the general angular momentum of an electromagnetic wave. This method can be extended to quasi-paraxial beams, i.e. highly focused laser beams. Some applications to the control of electronic transitions in atoms are discussed.
We propose a framework that connects the spatial symmetries of a metasurface to its material parameter tensors and its scattering matrix. This provides a simple yet effective way to effortlessly determine properties of a metasurface scattering response, such as chirality or asymmetric transmission, and which of its effective material parameters should be taken into account in the prospect of a homogenization procedure. In contrast to existing techniques, this approach does not require any a priori knowledge of group theory or complicated numerical simulation schemes, hence making it fast, easy…
Linear scattering processes are usually described as a function of the parameters of the incident beam. The wavelength, the intensity distribution, the polarization or the phase are among them. Here, we discuss and experimentally demonstrate how the angular momentum and the helicity of light influence the light scattering of spherical particles. We measure the backscattering of a $4μm$ TiO$_2$ single particle deposited on a glass substrate. The particle is probed at different wavelengths by different beams with total angular momenta ranging from $-8$ to $+8$ units. It is observed that the spec…
There is today a growing need to accurately model the angular scattering response of metasurfaces for optical analog processing applications. However, the current metasurface modeling techniques are not well suited for such a task since they are limited to small angular spectrum transformations, as shall be demonstrated. The goal of this work is to overcome this limitation by improving the modeling accuracy of these techniques and, specifically, to provide a better description of the angular response of metasurfaces. This is achieved by extending the current methods, which are restricted to di…
Multipolar solutions of Maxwell's equations are used in many practical applications and are essential for the understanding of light-matter interactions at the fundamental level. Unlike the set of plane wave solutions of electromagnetic fields, the multipolar solutions do not share a standard derivation or notation. As a result, expressions originating from different derivations can be difficult to compare. Some of the derivations of the multipolar solutions do not explicitly show their relation to the angular momentum operators, thus hiding important properties of these solutions. In this art…
We present a theoretical study of the optical angular momentum transfer from a circularly polarized plane wave to thin metal nanoparticles of different rotational symmetries. While absorption has been regarded as the predominant mechanism of torque generation on the nanoscale, we demonstrate numerically how the contribution from scattering can be enhanced by using multipolar plasmon resonance. The multipolar modes in non-circular particles can convert the angular momentum carried by the scattered field, thereby producing scattering-dominant optical torque, while a circularly symmetric particle…
We present a new method to address multipolar resonances and to control the scattered field of a spherical scatterer. This method is based on the engineering of the multipolar content of the incident beam. We propose experimentally feasible techniques to generate light beams which contain only a few multipolar modes. The techniques uses incident beams with a well defined component of the angular momentum and appropriate focusing with aplanatic lenses. The control of the multipolar content of light beams allow for the excitation of single Mie resonances and unprecedented control of the scattere…
We present an approach to study the interaction between matter and evanescent fields. The approach is based on the decomposition of evanescent plane waves into multipoles of well-defined angular momentum transverse to both decay and propagation directions. We use the approach to identify the origin of the recently observed directional coupling of emitters into guided modes, and of the opposite Zeeman state excitation of atoms near a fiber. We explain how to rigorously quantify both effects, and show that the directionality and the difference in excitation rates grow exponentially with the mult…
The nature of light-matter interaction is governed by the spatial-temporal structures of a light field and material wavefunctions. The emergence of the light beam with transverse phase vortex, or equivalently orbital angular momentum (OAM) has been providing intriguing possibilities to induce unconventional optical transitions beyond the framework of the electric dipole interaction. The uniqueness stems from the OAM transfer from light to material, as demonstrated using the bound electron of a single trapped ion. However, many aspects of the vortex light-matter interaction are still unexplored…
Scattering of electromagnetic waves by an arbitrary nanoscale object can be characterized by a multipole decomposition of the electromagnetic field that allows to describe the scattering intensity and radiation pattern through interferences of dominating excited multipole modes. In modern nanophotonics, both generation and interference of multipole modes start to play an indispensable role, and they enable nanoscale manipulation of light with many related applications. Here we review the multipolar interference effects in metallic, metal-dielectric, and dielectric nanostructures, and suggest a…
Structured light mechanically interacts with matter via optical forces and torques. The optical torque is traditionally calculated via the flux of total angular momentum (AM) into a volume enclosing an object. In [Phys. Rev. A 92, 043843 (2015)] a powerful method was suggested to calculate optical torque separately from the flux of the spin and the orbital parts of optical AM, providing useful physical insight. However, the method predicted a new type of dipolar torque dependent on the gradient of the helicity density of the optical beam, inconsistent with prior torque calculations. In this wo…
Upper bound to optical forces through the multipolar control of optical beams
Centro de Física de Materiales (CFM), CSIC-EHU（材料物理中心）；University of the Basque Country (EHU)（巴斯克大学）；Donostia International Physics Center（圣塞巴斯蒂安国际物理中心）；LORTEK, Basque Research and Technology Alliance (BRTA)（洛尔特克，巴斯克研究与技术联盟）
Recent experiments demonstrated strongly directional coupling of light into waveguide modes. We identify here the mechanisms behind this effect. We consider emitters near a waveguide, either centered on the median plane of the waveguide, or displaced from such plane. We show that, independently of the displacement, the directionality is mostly due to a mirror symmetry breaking caused by the axial character of the angular momentum of the emitted light. The sign of the angular momentum along an axis transverse to the waveguide determines the preferential coupling direction. The degree of directi…
Electron vortex beams have been predicted to enable atomic scale magnetic information measurement, via transfer of orbital angular momentum. Research so far has focussed on developing production techniques and applications of these beams. However, methods to measure the outgoing orbital angular momentum distribution are also a crucial requirement towards this goal. Here, we use a method to obtain the orbital angular momentum decomposition of an electron beam, using a multi-pinhole interferometer. We demonstrate both its ability to accurately measure orbital angular momentum distribution, and i…
We present a scheme to measure the orbital angular momentum spectrum of light using a precisely timed optical loop and quantum non-demolition measurements. We also discuss the influence of imperfect optical components.
The interplay between spin and orbital angular momentum in the up-conversion process allows us to control the macroscopic wave front of high harmonics by manipulating the microscopic polarizations of the driving field. We demonstrate control of orbital angular momentum in high harmonic generation from both solid and gas phase targets using the selection rules of spin angular momentum. The gas phase harmonics extend the control of angular momentum to extreme-ultraviolet wavelength. We also propose a bi-color scheme to produce spectrally separated extreme-ultraviolet radiation carrying orbital a…
Light intensity control of the orbital angular momentum of the fundamental beam in a quadratic nonlinear process is theoretically and numerically presented. In particular we analyzed a seeded second harmonic generation process in presence of orbital angular momentum of the interacting beams due both to on axis and off axis optical vortices. Examples are proposed and discussed.
We investigate the dynamical properties of a type-II optical parametric oscillator pumped by a structured light beam carrying orbital angular momentum. Different dynamical regimes are theoretically derived and experimentally demonstrated, depending on the anisotropy effects imposed by the nonlinear medium. In a weakly anisotropic regime, fine-tuning of the orbital angular momentum transfer is obtained by adjusting the crystal parameters. Under strong anisotropy, orbital angular momentum transfer is not possible and a sharp dynamical behavior is observed, with abrupt switching between different…
The magnitude of the topological charge of the vortex of a ring-shaped pulse is found to be limited by the squared mean frequency of the pulse spectrum at the ring relative to its variance. This limitation implies a upper bound to the orbital angular momentum carried by a pulse, and a lower bound to the duration for a pulse to carry any orbital angular momentum.
We implement an interferometric method using two angular slits to measure the orbital angular momentum (OAM) mode spectrum of a partially coherent field. As the angular separation of the slits changes, an interference pattern for a particular OAM mode is obtained. The visibility of this interference pattern as a function of angular separation is equivalent to the angular correlation function of the field. By Fourier transforming the angular correlation function obtained from the double angular slit interference, we are able to calculate the OAM spectrum of the partially coherent field. This me…
Exploiting electro-optic effects in liquid crystals, we achieved real-time control of the retardation of liquid- crystal-based $q$-plates through an externally applied voltage. The newly conceived electro-optic $q$-plates can be operated as electrically driven converters of photon spin into orbital angular momentum, enabling a variation of the orbital angular momentum probabilities of the output photons over a time scale of milliseconds.
We introduce a new method to generate and tune the optical orbital angular momentum of a focused Gaussian beam passing through the optical superlattice under the electro-optic effect. The orbital angular momentum (OAM) arises from the curl of polarization in our calculation. We see that adjusting the external electric field, the beam waist radius and the crystal length provides dramatic variation of OAM of light across the transverse section. It is believed that this invention will find its application in optical manipulation area.
Spatiotemporal optical vortices (STOVs) are a new type of intrinsic optical orbital angular momentum (OAM) structure in which the OAM vector is orthogonal to the propagation direction [Optica 6, 1547, (2019)] and the optical phase circulates in space-time. Here, we experimentally and theoretically demonstrate, for the first time, the generation of the second harmonic of a STOV-carrying pulse along with the conservation of STOV-based OAM. Our experiments verify that individual photons can have intrinsic orbital angular momentum perpendicular to their propagation direction.
It is shown that the momentum density of free electromagnetic field splits into two parts. One has no contribution to the net momentum due to the transversality condition. The other yields all the momentum. The angular momentum that originates from the former part is spin, and the angular momentum that originates from the latter part is orbital angular momentum. Expressions for the spin and orbital angular momentum are given in terms of the electric vector in reciprocal space. The spin and orbital angular momentum defined this way are used to investigate the angular momentum of nonparaxial bea…
Many methods now exist to prepare free electrons into orbital angular momentum states, and the predicted applications of these electron states as probes of materials and scattering processes are numerous. The development of electron orbital angular momentum measurement techniques has lagged behind. We show that coupling between electron orbital angular momentum and a spatially varying magnetic field produces an angular momentum-dependent focusing effect. We propose a design for an orbital angular momentum measurement device built on this principle. As the method of measurement is non-interfero…
We demonstrate the Fourier relationship between angular position and angular momentum for a light mode. In particular we measure the distribution of orbital angular momentum states of light that has passed through an aperture and verify that the orbital angular momentum distribution is given by the complex Fourier-transform of the aperture function. We use spatial light modulators, configured as diffractive optical components, to define the initial orbital angular momentum state of the beam, set the defining aperture, and measure the angular momentum spread of the resulting beam. These measure…
Recent experiments in orbital angular momentum multiplexing have demonstrated its potential for improving the link capacity in optical interconnection networks. Meanwhile, compact photonic integrated orbital angular momentum (de-)multiplexing devices are needed to address requirements such as high scalability, fast configurability, low cost and low power consumption. Here we report on a large-scale integrated tunable orbital angular momentum mode multiplexer, which supports up to 20 multiplexed orbital angular momentum modes over 16 wavelength channels with 30 GHz channel spacing. A testbed of…
It is shown that the photon picture of the electromagnetic field enables one to determine unambiguously the splitting of the total angular momentum of the electromagnetic field into the orbital part and the spin part.
We present generalized expressions to calculate the orbital angular momentum for invariant beams using scalars potentials. The solutions can be separated into transversal electric TE, transversal magnetic TM and transversal electromagnetic TE/TM polarization modes. We show that the superposition of non-paraxial vectorial beams with axial symmetry can provide a well defined orbital angular momentum and that the modes superposition affects the angular momentum flux density. The results are illustrated and analyzed for Bessel beams.
It is shown that the momentum density of free electromagnetic field splits into two parts. One has no contribution to the net momentum due to the transversality condition. The other yields all the momentum. The angular momentum that is associated with the former part is spin, and the angular momentum that is associated with the latter part is orbital angular momentum. Expressions for the spin and orbital angular momentum are given in terms of the electric vector in reciprocal space. The spin and orbital angular momentum defined this way are used to investigate the angular momentum of nonparaxi…
We present a quantum mechanical analysis of the orbital angular momentum of a class of recently discovered elliptically-symmetric stable light fields --- the so-called Ince-Gauss modes. We study, in a fully quantum formalism, how the orbital angular momentum of these beams varies with their ellipticity and discover several compelling features, including: non-monotonic behavior, stable beams with real continuous (non-integer) orbital angular momenta, and orthogonal modes with the same orbital angular momenta. We explore, and explain in detail, the reasons for this behavior. These features may h…
We propose to use an acoustic surface wave as a memory for a photon carrying orbital angular momentum. We clarify the physical mechanism that enables the transfer of information, derive the angular momentum selection rule that must be obeyed in the process, and show how to optimize the optoacoustic coupling. We theoretically demonstrate that high fidelities can be achieved, using realistic parameters, for the transfer of a coherent optical Laguerre-Gaussian state, associated with large angular momentum, to a mechanical shear mode. Our results add a significant possibility to the ongoing effort…
From the viewpoint of classical electrodynamics, we identify the role of spin-to-orbital angular momentum conversion in spin Hall effect of light (SHE). We introduce a distinct separation between spin and orbital angular momenta to clarify the spin-orbital interaction in the SHE of light. We demonstrate that the refractive index gradient can enhance or suppress the spin-to-orbital angular momentum conversion, and thus can control the SHE of light in conventional beam refraction. We suggest that the metamaterial whose refractive index can be tailored arbitrarily may become a good candidate for …
We analyze atomic photoexcitation into the discrete states by twisted photons, or photons carrying extra orbital angular momentum along their direction of propagation. From the angular momentum and parity considerations, we are able to relate twisted-photon photoexcitation amplitudes to their plane-wave analogues, independently of the details of the atomic wave functions. We analyzed the photo-absorption cross sections of mixed-multipolarity $E2-M1$ transitions in ionized atoms and found fundamental differences coming from the photon topology. Our theoretical analysis demonstrates that it is p…
A decomposition of the angular momentum of the classical electromagnetic field into orbital and spin components that is manifestly gauge invariant and general has been obtained. This is done by decomposing the electric field into its longitudinal and transverse parts by means of the Helmholtz theorem. The orbital and spin components of the angular momentum of any specified electromagnetic field can be found from this prescription.
The expression for the total angular momentum carried by a laser optical vortex beam, splits, in the paraxial approximation, into two terms which seem to represent orbital and spin angular momentum respectively. There are, however, two very different competing versions of the formula for the spin angular momentum, one based on the use of the Poynting vector, as in classical electrodynamics, the other related to the canonical expression for the angular momentum which occurs in Quantum Electrodynamic. I analyze the possibility that a sufficiently sensitive optical measurement could decide which …
We present an optomechanical device designed to allow optical transduction of orbital angular momentum of light. An optically induced twist imparted on the device by light is detected using an integrated cavity optomechanical system based on a nanobeam slot-mode photonic crystal cavity. This device could allow measurement of the orbital angular momentum of light when photons are absorbed by the mechanical element, or detection of the presence of photons when they are scattered into new orbital angular momentum states by a sub-wavelength grating patterned on the device. Such a system allows det…
Magnetostatic modes supported by a ferromagnetic sphere have been known as the Walker modes, each of which possesses an orbital angular momentum as well as a spin angular momentum along a static magnetic field. The Walker modes with non-zero orbital angular momenta exhibit topologically non-trivial spin textures, which we call \textit{magnetic quasi-vortices}. Photons in optical whispering gallery modes supported by a dielectric sphere possess orbital and spin angular momenta forming \textit{optical vortices}. Within a ferromagnetic, as well as dielectric, sphere, two forms of vortices interac…
