Spatiotemporal optical vortices (STOVs) are a new type of intrinsic optical orbital angular momentum (OAM) structure in which the OAM vector is orthogonal to the propagation direction [Optica 6, 1547, (2019)] and the optical phase circulates in space-time. Here, we experimentally and theoretically demonstrate, for the first time, the generation of the second harmonic of a STOV-carrying pulse along with the conservation of STOV-based OAM. Our experiments verify that individual photons can have intrinsic orbital angular momentum perpendicular to their propagation direction.
Recently, a spatiotemporal optical vortex (STOV) with a transverse orbital angular momentum (OAM) has been generated from coherent ultrafast pulses using mode-locked lasers. In contrast, we demonstrate theoretically and experimentally that a STOV can be generated from a light source with partial temporal coherence with fluctuating temporal phase. By eliminating the need of mode-locked laser sources, the partially coherent STOV will serve as a convenient and cost-effective transverse OAM source.
As a new degree of freedom for optical manipulation, recently spatiotemporal optical vortices (STOVs) carrying transverse orbital angular momentums have been experimentally demonstrated with pulse shapers. Here a spatiotemporal differentiator is proposed to generate STOVs with transverse orbital angular momentum. In order to create phase singularity in the spatiotemporal domain, the spatiotemporal differentiator is designed by breaking spatial mirror symmetry. In contrast to pulse shapers, the device proposed here is a simple one-dimensional periodic nanostructure and thus it is much more comp…
In this study, we demonstrate the concept of combining optical combs with optical vortices for the first time. By combining the advantages of the both light sources, we realize an optical vortex comb technology for arbitrary spatiotemporal phase manipulation. This idea corresponds to simultaneous control of the longitudinal and transverse modes of light based on the high controllability of the optical comb. As a proof-of-concept experiment, we applied an optical vortex comb to the generation and rotational control of a ring-shaped optical lattice. Furthermore, to demonstrate the utility of thi…
We introduce a model for spatiotemporal modelocking in multimode fiber lasers, which is based on the (3+1)-dimensional cubic-quintic complex Ginzburg-Landau equation (cGLE) with conservative and dissipative nonlinearities and a 2-dimensional transverse trapping potential. Systematic numerical analysis reveals a variety of stable nonlinear modes, including stable fundamental solitons and breathers, as well as solitary vortices with winding number $n=1$, while vortices with $n=2$ are unstable, splitting into persistently rotating bound states of two unitary vortices. A characteristic feature of …
Shenzhen University（深圳大学）；East China Normal University（华东师范大学）；University of Shanghai for Science and Technology（上海理工大学）；Northwestern Polytechnical University（西北工业大学）
Using an example of a Raman active medium we describe how a common nonlinear process of four-wave mixing can be used to induce strong coupling between the spatial and temporal degrees of freedom in optical waves. This coupling produces several unexpected effects. Amongst those are cascaded excitation of multiply charged optical vortices, spatial focusing in a nonlinearly defocusing medium and generation of helically shaped spatio-temporal optical solitons.
Generation of few-cycle optical vortex pulses is challenging due to the large spectral bandwidths, as most vortex generation techniques are designed for monochromatic light. In this work, we use a spiral phase plate to generate few-cycle optical vortices from an ultrafast titanium:sapphire oscillator, and characterize them in the spatiotemporal domain using a recently introduced technique based on spatially resolved Fourier transform spectrometry. The performance of this simple approach to the generation of optical vortices is analyzed from a wavelength dependent perspective, as well as in the…
Light with spatiotemporal orbital angular momentum (ST-OAM) is a recently discovered type of structured and localized electromagnetic field. This field carries characteristic space-time spiral phase structure and transverse intrinsic OAM. In this work, we present the generation and characterization of the second-harmonic of ST-OAM pulses. We uncovered the conservation of transverse OAM in a second-harmonic generation process, where the space-time topological charge of the fundamental field is doubled along with the optical frequency. Our experiment thus suggests a general ST-OAM nonlinear scal…
Orbital angular momentum of spatiotemporal vortices: a ray-mechanical analogy
The Institute of Optics, University of Rochester（罗切斯特大学光学研究所）；Donostia International Physics Center (DIPC)（圣塞巴斯蒂安国际物理中心）；IKERBASQUE, Basque Foundation for Science（伊卡巴斯基克，巴斯克科学基金会）；Centre of Excellence ENSEMBLE3 Sp. z o.o.（卓越中心 ENSEMBLE3 有限责任公司）；Aix Marseille Univ, CNRS, Centrale Med, Institut Fresnel, UMR 7249（艾克斯-马赛大学、法国国家科学研究中心、中央理工学院马赛分校、菲涅耳研究所）
Scaling law from orbital angular momentum conservation in harmonic and high-order harmonic generation driven by spatiotemporal light fields
Universidad Politécnica de Madrid（马德里理工大学）；Instituto de Fusión Nuclear “Gillermo Velarde”, Universidad Politécnica de Madrid (ETSII)（马德里理工大学（ETSII）核聚变研究所“吉列尔莫·贝尔德”）；Universidad de Salamanca（萨拉曼卡大学）
Optical parametric amplification of spatiotemporal optical vortices
Zhejiang Key Laboratory of 3D Micro/Nano Fabrication and Characterization, Department of Electronic and Information Engineering, School of Engineering, Westlake University（西湖大学工程学院电子信息工程系三维微纳加工与表征浙江省重点实验室）；School of Optical and Electronic Information and Wuhan National Laboratory for Optoelectronics, Huazhong University of Science and Technology（华中科技大学光学与电子信息学院/武汉光电国家研究中心）；Westlake-Kromoson Joint Laboratory of Light-Field Intelligence, School of Engineering, Westlake University（西湖大学工程学院光场智能西湖-科慕森联合实验室）
Vortex solitons (dark solitons) are described in self-defocusing Kerr media whose phase line singularity is not parallel to the propagation direction, but is perpendicular or tilted almost arbitrary angles, depending on the medium linear dispersion. These solitons broaden the so-called spatiotemporal optical vortices recently observed in experiments to the nonlinear realm, opening new perspectives in practical applications of optical vortices.
Vortices are whirling disturbances commonly found in nature ranging from tremendously small scales in Bose-Einstein condensates to cosmologically colossal scales in spiral galaxies. An optical vortex, generally associated with a spiral phase, can carry orbital angular momentum (OAM). The optical OAM can either be in the longitudinal direction if the spiral phase twists in the spatial domain or in the transverse direction if the phase rotates in the spatiotemporal domain. In this article, we demonstrate the intersection of spatiotemporal vortices and spatial vortices in a wave packet. As a resu…
Spatiotemporal Optical Vortices From All-Dielectric Bilayer Metagratings
The Hong Kong University of Science and Technology (Guangzhou)（香港科技大学（广州））；University of Electronic Science and Technology of China（电子科技大学）；Chinese Academy of Sciences（中国科学院）；Wuhan University of Technology（武汉理工大学）
In any form of wave propagation, strong spatiotemporal coupling appears when non-elementary, three-dimensional wave-packets are composed by superimposing pure plane waves, or spontaneously generated by light-matter interaction and nonlinear processes. Ultrashort pulses with orbital angular momentum (OAM), or ultrashort vortices, furnish a critical paradigm in which the analysis of the spatiotemporal coupling in the form of temporal-OAM coupling can be carried out accurately by analytical tools. By generalizing and unifying previously reported results, we show that universal and spatially heter…
Probing Internal Dynamics of Spatiotemporal Optical Vortex Strings: Spatiotemporal Attraction and Filament Stretching
Shanghai Institute of Optics and Fine Mechanics, Chinese Academy of Sciences（中国科学院上海光学精密机械研究所）；University of Chinese Academy of Sciences（中国科学院大学）；Tianjin University（天津大学）；Chongqing University of Technology（重庆理工大学）
Spatiotemporal optical vortices (STOVs) carrying transverse orbital angular momentum (OAM) are of rapidly growing interest for the field of optics due to the new degree of freedom that can be exploited. In this paper, we propose cylindrical vector two dimensional STOVs (2D-STOVs) containing two orthogonal transverse OAMs in both x-t and y-t planes for the first time, and investigate the tightly focusing of such fields using the Richards-Wolf vectorial diffraction theory. Highly confined spatiotemporal wavepackets with polarization structure akin to toroidal topology is generated, whose spatiot…
We present the first experimental evidence, supported by theory and simulation, of spatiotemporal optical vortices (STOVs). Quantized STOVs are a fundamental element of the nonlinear collapse and subsequent propagation of short optical pulses in material media. A STOV consists of a ring-shaped null in the electromagnetic field about which the phase is spiral, forming a dynamic torus which is concentric with and tracks the propagating pulse. Depending on the sign of the material dispersion, the local electromagnetic energy flow is saddle or spiral about the STOV. STOVs are born and evolve conse…
Stony Brook University（石溪大学）；Donostia International Physics Center (DIPC)（多诺斯蒂亚国际物理中心）；IKERBASQUE, Basque Foundation for Science（伊克巴萨奎，巴斯克科学基金会）；Centre of Excellence ENSEMBLE3 Sp. z o.o.（卓越中心 ENSEMBLE3 有限公司）
Magnetostatic modes supported by a ferromagnetic sphere have been known as the Walker modes, each of which possesses an orbital angular momentum as well as a spin angular momentum along a static magnetic field. The Walker modes with non-zero orbital angular momenta exhibit topologically non-trivial spin textures, which we call \textit{magnetic quasi-vortices}. Photons in optical whispering gallery modes supported by a dielectric sphere possess orbital and spin angular momenta forming \textit{optical vortices}. Within a ferromagnetic, as well as dielectric, sphere, two forms of vortices interac…
Spatio-temporal optical vortices (STOVs) are a new type of optical orbital angular momentum (OAM) with optical phase circulation in space-time. In prior work [N. Jhajj et al., Phys. Rev X 6, 031037 (2016)], we demonstrated that a STOV is a universal structure emerging from the arrest of self-focusing collapse leading to nonlinear self-guiding in material media. Here, we demonstrate linear generation and propagation in free space of STOV-carrying pulses. Our measurements and simulations demonstrate STOV mediation of space-time energy flow within the pulse and conservation of OAM in space-time. …
We investigate twisted electrons with a well defined orbital angular momentum, which have been ionised via a strong laser field. By formulating a new variant of the well-known strong field approximation, we are able to derive conservation laws for the angular momenta of twisted electrons in the cases of linear and circularly polarised fields. In the case of linear fields, we demonstrate that the orbital angular momentum of the twisted electron is determined by the magnetic quantum number of the initial bound state. The condition for the circular field can be related to the famous ATI peaks, an…
We demonstrate the creation of vortices in a macroscopically occupied polariton state formed in a semiconductor microcavity. A weak external laser beam carrying orbital angular momentum (OAM) is used to imprint a vortex on the condensate arising from the polariton optical parametric oscillator (OPO). The vortex core radius is found to decrease with increasing pump power, and is determined by polariton-polariton interactions. As a result of OAM conservation in the parametric scattering process, the excitation consists of a vortex in the signal and a corresponding anti-vortex in the idler of the…
Isolated attosecond spatio-temporal optical vortices: Interplay between the topological charge and orbital angular momentum scaling in high harmonic generation
Nonlinear Nanophotonic Chip-space Interfaces: On-chip Generation of Structured, Topological and Spatiotemporal Lights Via Nonlinear Čerenkov Radiation
State Key Laboratory of Optoelectronic Materials and Technologies, School of Physics, Sun Yat-sen University（中山大学物理学院光电材料与技术国家重点实验室）；CAS Key Laboratory of Quantum Information, University of Science and Technology of China（中国科学技术大学量子信息重点实验室）；CAS Center for Excellence in Quantum Information and Quantum Physics, University of Science and Technology of China（中国科学技术大学量子信息与量子物理学前沿卓越创新中心）
A ferromagnetic sphere can support \textit{optical vortices} in forms of whispering gallery modes and \textit{magnetic quasi-vortices} in forms of magnetostatic modes with non-trivial spin textures. These vortices can be characterized by their orbital angular momenta. We experimentally investigate Brillouin scattering of photons in the whispering gallery modes by magnons in the magnetostatic modes, zeroing in on the exchange of the orbital angular momenta between the optical vortices and the magnetic quasi-vortices. We find that the conservation of the orbital angular momentum results in diffe…
Single-shot 3D characterization the spatiotemporal optical vortex via a spatiotemporal wavefront sensor (STWFS)
Key Laboratory of High Power Laser and Physics, Shanghai Institute of Optics and Fine Mechanics, Chinese Academy of Sciences（中国科学院上海光学精密机械研究所高功率激光物理重点实验室）；Center of Materials Science and Optoelectronics Engineering, University of Chinese Academy of Sciences（中国科学院大学材料科学与光电技术研究中心）；School of Physics, Xi'an Jiaotong University（西安交通大学物理学院）；College of Information Science and Technology, Donghua University（东华大学信息科学与技术学院）
