We experimentally analyze the complete photon number statistics of parametric downconversion and ascertain the influence of multimode effects. Our results clearly reveal a difference between single mode theoretical description and the measured distributions. Further investigations assure the applicability of loss-tolerant photon number reconstruction and prove strict photon number correlation between signal and idler modes.
We address parametric-downconversion seeded by multimode pseudo-thermal fields. We show that this process may be used to generate multimode pairwise correlated states with entanglement properties that can be tuned by controlling the seed intensities. Multimode pseudo-thermal fields seeded parametric-downconversion represents a novel source of correlated states, which allows one to explore the classical-quantum transition in pairwise correlations and to realize ghost imaging and ghost diffraction in regimes not yet explored by experiments.
We report generation of near-infrared photon pairs in fundamental spatial modes via type-II spontaneous parametric down-conversion in a periodically poled potassium titanyl phosphate (KTiOPO4) nonlinear waveguide supporting multiple transverse modes. This demonstrates experimentally a versatile scheme for controlling the spatial characteristics of the produced nonclassical light based on exploitation of intermodal dispersion. The down-converted photons are characterized by the measurement of the beam quality factors in the heralded regime.
We present a multimode treatment of the optical parametric oscillator, which is valid for both pulsed and continuous-wave pump fields. The two-time correlation functions of the output field are derived, and we apply the theory to analyze a scheme for heralded production of non-classical field states that may be subsequently stored in an atomic quantum memory.
Phase-sensitive optical parametric amplification of squeezed states helps to overcome detection loss and noise and thus increase the robustness of sub-shot-noise sensing. Because such techniques, e.g., imaging and spectroscopy, operate with multimode light, multimode amplification is required. Here we find the optimal methods for multimode phase-sensitive amplification and verify them in an experiment where a pumped second-order nonlinear crystal is seeded with a Gaussian coherent beam. Phase-sensitive amplification is obtained by tightly focusing the seed into the crystal, rather than seeding…
We describe the realization of multimode phononic correlations that arise from nonlinear interactions in a mechanical nondegenerate parametric amplifier. The nature of these correlations differs qualitatively depending on the strength of the driving field in relation to the threshold for parametric instability. Below this threshold, the correlations are manifest in a combined quadrature of the coupled mechanical modes. In this regime, the system is amenable to back-action evading measurement schemes for the detection of weak forces. Above threshold, the correlations are manifest in the amplitu…
We address the intrinsic multimode nature of the quantum state of light obtained by pulsed spontaneous parametric downconversion and develop a theoretical model based only on experimentally accessible quantities. We exploit the pairwise entanglement as a resource for conditional multimode measurements and derive closed formulas for the detection probability and the density matrix of the conditional states. We present a set of experiments performed to validate our model in different conditions that are in excellent agreement with experimental data. Finally, we evaluate nonGaussianity of the con…
In this Letter, we demonstrate the generation of multimode entangled states of propagating microwaves. The entangled states are generated by parametrically pumping a multimode superconducting cavity. By combining different pump frequencies, applied simultaneously to the device, we can produce different entanglement structures in a programable fashion. The Gaussian output states are fully characterized by measuring the full covariance matrices of the modes. The covariance matrices are absolutely calibrated using an in situ microwave calibration source, a shot noise tunnel junction. Applying a v…
We study the quantum correlations induced by spontaneous parametric down-conversion (SPDC) of a frequency comb. We derive a theoretical method to find the output state corresponding to a pump with an arbitrary spectral profile. After applying it to the relevant example of a spectrally chirped pump, we run an optimization algorithm to numerically find the pump profiles maximizing some target functions. These include the number of independently squeezed modes and the variances of nullifiers defining cluster states used in many continuous-variable quantum information protocols. To assess the adva…
Spectro-temporal modes of light can be exploited for the generation of high-dimensional Gaussian quantum states. Such states are at the basis of continuous variable quantum information protocols where they have to support mode-selective non-Gaussian operations. We develop a general framework for single-photon addition on multimode states of light via parametric down conversion processes. We identify the analytical conditions for single-mode and mode-selective photon addition. We show that spectral mode selectivity can be achieved in the Type-II collinear down conversion, while single-mode cond…
Coherent temporal filtering of multimode parametric down-conversion using a quantum pulse gate
Integrated Quantum Optics Group, Institute for Photonic Quantum Systems (PhoQS), Paderborn University（帕德博恩大学光子量子系统研究所）；School of Mathematics and Physics, University of Queensland（昆士兰大学数学与物理学院）
We report measurements of two-photon interference using a cw-pumped type-II spontaneous parametric down-conversion source based on a multimode perodically poled potassium titanyl phosphate waveguide. We have used the recently demonstrated technique of controlling the spatial characteristics of the down-conversion process via intermodal dispersion to generate photon pairs in fundamental transverse modes, thus ensuring their spatial indistinguishability. Good spatial overlap of photon modes within pairs has been verified using the Hong-Ou-Mandel interferometer and the preparation of polarization…
We study the process of multimode Spontaneous Parametric Down--Conversion (SPDC) in the lossy, one dimensional waveguide. We propose a description using first order Correlation Functions (CF) in the fluorescence fields, as a very fruitful and easy approach providing us with a complete information about the final multimode state. We formulate the equation of the evolution of the multimode CF along the crystal using four characteristic length scales. We solve it analytically in the one mode case and numerically in the multimode case. We capture simultaneous effects of three wave mixing with ultr…
We experimentally demonstrate the conversion of a Gaussian beam to an approximate Bessel-Gauss mode by making use of a non-collinear four-wave mixing process in hot atomic vapor. The presence of a strong, spatially non-Gaussian pump both converts the probe beam into a non-Gaussian mode, and generates a conjugate beam that is in a similar non-Gaussian mode. The resulting probe and conjugate modes are compared to the output of a Gaussian beam incident on an annular aperture that is then spatially filtered according to the phase-matching conditions imposed by the four-wave mixing process. We find…
We analyze theoretically spontaneous parametric down-conversion in a multimode nonlinear waveguide as a source of entangled pairs of spatial qubits, realized as superpositions of a photon in two orthogonal transverse modes of the waveguide. It is shown that by exploiting intermodal dispersion, down-conversion into the relevant pairs of spatial modes can be selected by spectral filtering, which also provides means to fine-tune the properties of the generated entangled state. We also discuss an inverting interferometer detecting the spatial parity of the input beam as a versatile tool to charact…
An oscillatory correlation function has been observed by the coincidence counting of multimode two-photon pairs produced with a degenerate optical parametric oscillator far below threshold. The coherent superposition of the multimode two-photon pairs provides the oscillation in the intensity correlation function. The experimental data are well fitted to a theoretical curve.
We address the reconstruction of the full photon distribution of multimode fields generated by seeded parametric down-conversion (PDC). Our scheme is based on on/off avalanche photodetection assisted by maximum-likelihood (MaxLik) estimation and does not involve photon counting. We present a novel constrained MaxLik method that incorporates the request of finite energy to improve the rate of convergence and, in turn, the overall accuracy of the reconstruction.
Two-photon interference of multimode two-photon pairs produced by an optical parametric oscillator has been observed for the first time with an unbalanced interferometer. The time correlation between the multimode two photons has a multi-peaked structure. This property of the multimode two-photon state induces two-photon interference depending on delay time. The nonclassicality of this interference is also discussed.
We review some recent experiments based upon multimode two-photon interference of photon pairs created by spontaneous parametric down-conversion. The new element provided by these experiments is the inclusion of the transverse spatial profiles of the pump, signal and idler fields. We discuss multimode Hong-Ou-Mandel interference, and show that the transverse profile of the pump beam can be manipulated in order to control two-photon interference. We present the basic theory and experimental results as well as several applications to the field of quantum information.
The 'Ghost' interference experiment is analyzed when the source of entangled photons is a multimode Optical Parametric Amplifier(OPA) whose weak limit is the two-photon Spontaneous Parametric Downconversion(SPDC) beam. The visibility of the double-slit pattern is calculated, taking the finite coincidence time window of the photon counting detectors into account. It is found that the coincidence window and the bandwidth of light reaching the detectors play a crucial role in the loss of visibility on coincidence detection, not only in the 'Ghost' interference experiment but in all experiments in…
We propose and demonstrate experimentally a new method based on the spatial entanglement for the absolute calibration of analog detector. The idea consists on measuring the sub-shot-noise intensity correlation between two branches of parametric down conversion, containing many pairwise correlated spatial modes. We calibrate a scientific CCD camera and a preliminary evaluation of the statistical uncertainty indicates the metrological interest of the method.
We discuss the possible cooling of different phonon modes via three wave mixing interactions of vibrational and optical modes. Since phonon modes exhibit a variety of dispersion relations or frequency spectra with diverse spatial structures, depending on the shape and size of the sample, we formulate our theory in terms of relevant spatial mode functions for the interacting fields in any given geometry. We discuss the possibility of Dicke like collective effects in phonon cooling and present explicit results for simultaneous cooling of two phonon modes via the anti-Stokes up conversions. We sh…
We consider multimode two-photon interference at a beam splitter by photons created by spontaneous parametric down-conversion. The resulting interference pattern is shown to depend upon the transverse spatial symmetry of the pump beam. In an experiment, we employ the first-order Hermite-Gaussian modes in order to show that, by manipulating the pump beam, one can control the resulting two-photon interference behavior. We expect these results to play an important role in the engineering of quantum states of light for use in quantum information processing and quantum imaging.
We experimentally observe the two-photon interference of multimode photon pairs produced by an optical parametric oscillator far below threshold via a michelson interferometer, which shows a multipeaked structure. We find that the correlation function when the interferometer is unbalanced is clearly dependent on the path difference and phase between two interfering beams, but the shape of correlation function in balanced case is independent on the small path difference and phase beside the height. All experimental results are well agreed with the theoretical prediction.
We report experimental determination of the phase-matching function for type-II three-wave mixing in a periodically poled KTiOPO_4 waveguide in the 792-815 nm spectral region. The measurement was performed by sum-frequency generation of spectrally tuned fundamental components. Strong dependence of the observed signal on the excited spatial modes in the waveguide has been observed and fully interpreted. These results indicate a route to employ the waveguide for spontaneous parametric down-conversion producing photon pairs in well-defined spatial modes.
The theory of parametric down conversion of the vacuum, based on a real zeropoint, or "vacuum" electromagnetic field, has been treated in earlier articles. The same theory predicts a hitherto unsuspected phenomenon - parametric up conversion of the vacuum. This article describes how the phenomenon may be demonstrated experimentally.
We present a first experimental test of the existence of Spontaneus Parametric Up Conversion, predicted by a specific local realistic model based on Wigner function formalism. The measurement has been made using a ccd camera on the emission of a LiIO3 crystal pumped by a 351 nm and/or a 789 (1064) nm lasers. We obtain an upper limit of 160 times on the ratio between intensity of Spontaneus Parametric Up Conversion and Spontaneous Parametric Down conversion.
We use photon counters to obtain the joint photon counting statistics from twin-beam non-degenerate parametric down conversion, and we demonstrate directly, and with no auxiliary assumptions, that these twin beams are nonclassical.
We show that an Optical Parametric Oscillator which is simultaneously resonant for several modes, either spatial or temporal, generates both below and above threshold a multimode non-classical state of light consisting of squeezed vacuum states in all the non-oscillating modes. We confirm this prediction by an experiment dealing with the degenerate TEM$_{01}$ and TEM$_{10}$ modes. We show the conservation of non-classical properties when the threshold is crossed. The experiment is made possible by the implementation of a new method to lock the relative phase of the pump and the injected beam.
Coincidence-structures in the transverse plane of Type-II spontaneous parametric down-conversion carrying orbital angular momentum are obtained. Azimuthal symmetry breaking around the pump beam direction reveals itself on these quantum images. Analytical expressions for the amplitude probability of the down conversion process are shown including the nonlinear polarizability components.
We present an experiment of preparing Werner state via spontaneous parametric down-conversion and controlled decoherence of photons in this paper. In this experiment two independent BBO (beta-barium borate) crystals are used to produce down-conversion light beams, which are mixed to prepare Werner state.
Recent work using spontaneous parametric down-conversion (SPDC) has made possible investigations of the Einstein-Podolsky-Rosen paradox in its original (position-momentum) form. We propose an experiment that uses SPDC photon pairs to measure through which slit a photon passes while simultaneously observing double-slit interference.
Surface spontaneous parametric down-conversion is predicted as a consequence of continuity requirements for electric- and magnetic-field amplitudes at a discontinuity of chi2 nonlinearity. A generalization of the usual two-photon spectral amplitude is suggested to describe this effect. Examples of nonlinear layered structures and periodically-poled nonlinear crystals show that surface contributions to spontaneous down-conversion can be important.
We propose a novel scheme to generate polarization entanglement from spatially-correlated photon pairs. We experimentally realized a scheme by means of a spatial correlation effect in a spontaneous parametric down-conversion and a modified Michelson interferometer. The scheme we propose in this paper can be interpreted as a conversion process from spatial correlation to polarization entanglement.
We implement experimentally a method to generate photon-number$-$path and polarization entangled photon pairs using ``beamlike'' type-II spontaneous parametric down-conversion (SPDC), in which the signal-idler photon pairs are emitted as two separate circular beams with small emission angles rather than as two diverging cones.
High-gain parametric down-conversion (PDC) is a source of bright squeezed vacuum, which is a macroscopic nonclassical state of light and a promising candidate for quantum information applications. Here we study its properties, such as the intensity spectral width and the spectral width of pairwise correlations.
Photon-added coherent states have been realized in optical parametric down-conversion by Zavatta {\em et al} [Science 306 (2004) 660-662]. In this report, it is established that the states generated in the process are {\em ideal} photon-added coherent states. It is shown that the scheme can generate higher order photon-added coherent states. A comparative study of the down-conversion process and atom-cavity interaction in generating the photon-added coherent states is presented.
Spontaneous parametric down-conversion (SPDC) sources are an important technology for quantum sensing and imaging. We demonstrate a general simulation method, based on modeling from first principles, reproducing the spectrally and spatially resolved absolute counts of a SPDC experiment. By simulating additional processes and effects we accomplish good agreement with the experimental results. This method is broadly applicable and allows for the separation of contributing processes, virtual characterization of SPDC sources, and enables the simulation of many quantum based applications.
We analyze the long-time quantum dynamics of degenerate parametric down-conversion from an initial sub-harmonic vacuum (spontaenous down-conversion). Standard linearization of the Heisenberg equations of motions fails in this case, since it is based on an expansion around an unstable classical solution and neglects pump depletion. Introducing a mean-field approximation we find a periodic exchange of energy between the pump and subharmonic mode goverened by an anharmonic pendulum equation. From this equation the optimum interaction time or crystal length for maximum conversion can be determined…
In this paper we report our systematic study of a promising absolute calibration technique of analog photo-detectors, based on the properties of parametric down conversion. Our formal results and a preliminary uncertainty analysis show that the proposed method can be effectively developed with interesting applications to metrology.
The phenomenon of parametric down conversion from the vacuum may be understood as a process in classical electrodynamics, in which a nonlinear crystal couples the modes of the pumping field with those of the zeropoint, or "vacuum" field. This is an entirely local theory of the phenomenon, in contrast with the presently accepted nonlocal theory. The new theory predicts a hitherto unsuspected phenomenon - parametric up conversion from the vacuum.
We experimentally investigate electromagnetically-induced transparency (EIT) created on an inhomogeneously broadened 5S_1/2-5P_1/2 transition in rubidium vapor using a control field of a complex temporal shape. A comb-shaped transparency spectrum enhances the delay-bandwidth product and the light storage capacity for a matched probe pulse by a factor of about 50 compared to a single EIT line [D. D. Yavuz, Phys. Rev. A 75, 031801 (2007)]. If the temporal mode of the control field is slowly changed while the probe is propagating through the EIT medium, the probe will adiabatically follow, provid…
We study the two-photon detection amplitude of the down-converted beams in spontaneous parametric down-conversion when the physical variable of orbital angular momentum is involved, taking into account both conservation and non-conservation of angular momentum. Agreeing with experimental observations, our theoretical calculation shows that spatial structure of the two-photon detection amplitude of the down-converted beams carries important information about conservation or non-conservation of orbital angular momentum in spontaneous parametric down-conversion.
We introduce an effective numerical method of density matrix determination of fiber coupled single photon generated in process of spontaneous parametric down conversion in type I non-collinear configuration. The presented theory has been successfully applied in case of source exploited in Phys. Rev. Lett. 99, 123601 (2007) to demonstrate the experimental characterization of spectral state of single photon.
We solve analytically master equations that describe a cavity filled with a kerr medium, taking into account the dissipation induced by the environment, and parametric down conversion processes. We use superoperator techniques.
We show how stimulated parametric processes can be employed in experiments on beyond the diffraction limit to overcome the problem of low visibility obtained by using spontaneous down conversion operating in the high gain regime. We further show enhancement of the count rate by several orders when stimulated parametric processes are used. Both the two photon counts and the visibility can be controlled by the phase of the stimulating coherent beam.
A theory of spontaneous parametric down-conversion, which gives rise to a quantum state that is entangled in multiple parameters, such as three-dimensional wavevector and polarization, allows us to understand the unusual characteristics of fourth-order quantum interference in many experiments, including ultrafast type-II parametric down-conversion, the specific example illustrated in this paper. The comprehensive approach provided here permits the engineering of quantum states suitable for quantum information schemes and new quantum technologies.
We describe parametric down conversion process in a two-level atomic gas, where the atoms are in a superposition state of relevant energy levels. This superposition results in splitting of the phase matching condition into three different conditions. Another, more important, peculiarity of the system under discussion is the nonsaturability of amplification coefficients with increasing pump wave intensity, under "sideband" generation conditions.
An experimental scheme for preparing a polarization entangled W states from four photons emitted by parametric down-conversion is proposed. We consider two different configurations and a method of improving the yield by using single photon sources. In the proposed scheme, one uses only linear optical elements and photon detectors, so that this scheme is feasible by current technologies.
Using a basic Mach-Zehnder interferometer, we demonstrate experimentally the measurement of the photonic de Broglie wavelength of an entangled photon pair (a biphoton) generated by spontaneous parametric down-conversion. The observed interference manifests the concept of the photonic de Broglie wavelength. The result also provides a proof-of-principle of the quantum lithography that utilizes the reduced interferometric wavelength.
