We have studied the noise spectra in a nonlinear magneto-optical rotation experiment in a rubidium vapor. We observed the reduction of noise in the intensity difference of two orthogonally polarized components of the laser beam. The dependence of the noise level on both the frequency and the longitudinal magnetic field has been studied. We found that the optimal condition for the noise reduction is to work around zero longitudinal magnetic field, where the intensity correlation between the two orthogonally polarized components is maximum. Our results can be used to reduce or eliminate the atomic excess noise, therefore improving the sensitivity of nonlinear magneto-optical rotation magnetometers and other atom-optical based applications.
We report the generation of optical squeezed vacuum states by means of polarization self-rotation in rubidium vapor following a proposal by Matsko et al. [Phys. Rev. A 66, 043815 (2002)]. The experimental setup, involving in essence just a diode laser and a heated rubidium gas cell, is simple and easily scalable. A squeezing of 0.85+-0.05 dB was achieved.
Sub-wavelength diameter tapered optical fibers surrounded by rubidium vapor can undergo a substantial decrease in transmission at high atomic densities due to the accumulation of rubidium atoms on the surface of the fiber. Here we demonstrate the ability to control these changes in transmission using light guided within the taper. We observe transmission through a tapered fiber that is a nonlinear function of the incident power. This effect can also allow a strong control beam to change the transmission of a weak probe beam.
Nonlinear optical effects can be enhanced in tapered optical fibers with diameters less than the wavelength of the propagating light. Here we report on the observation of two-photon absorption using tapered fibers in rubidium vapor at power levels of less than 150 nW. Transit-time broadening produces two-photon absorption spectra with sharp peaks that are very different from conventional line shapes.
The realization of quantum memory using warm atomic vapor cells is appealing because of their commercial availability and the perceived reduction in experimental complexity. In spite of the ambiguous results reported in the literature, we demonstrate that quantum memory can be implemented in a single cell with buffer gas using the geometry where the write and read beams are nearly co-propagating. The emitted Stokes and anti-Stokes photons display cross-correlation values greater than 2, characteristic of quantum states, for delay times up to 4 microseconds.
We present an experimental demonstration of simultaneous above-threshold oscillations of the Stokes and anti-Stokes fields together with the single pumping beam with rubidium atoms inside an optical standing-wave cavity. The triple resonant conditions can be achieved easily by making use of the large dispersions due to two-photon transitions in the three-level atomic system. This work provides a way to achieve high efficient nonlinear frequency conversion and the generated bright Stokes and anti-Stokes cavity output beams are potential resource for applications in quantum information science.
We have observed CW lasing without inversion in a gas of hot rubidium atoms in an optical cavity under conditions of electromagnetically-induced transparency (EIT). The medium is pumped coherently and resonantly by a single ``coupling'' beam which also produces EIT in the lasing transition. The steady-state intensity exhibits thresholds as a function of the atomic density and the strength of the coupling beam. A theoretical model for an effective three-level lambda system indicates that gain without inversion is possible in this system if the two ground states are coupled by depolarizing colli…
Entangled multi-spatial-mode fields have interesting applications in quantum information, such as parallel quantum information protocols, quantum computing, and quantum imaging. We study the use of a nondegenerate four-wave mixing process in rubidium vapor at 795 nm to demonstrate generation of quantum-entangled images. Owing to the lack of an optical resonator cavity, the four-wave mixing scheme generates inherently multi-spatial-mode output fields. We have verified the presence of entanglement between the multi-mode beams by analyzing the amplitude difference and the phase sum noise using a …
The use of sub-wavelength diameter tapered optical fibers (TOF's) in warm rubidium vapor has recently been identified as a promising system for realizing ultra-low-power nonlinear optical effects. However, at the relatively high atomic densities needed for many of these experiments, rubidium atoms accumulating on the TOF surface can cause a significant loss of overall transmission through the fiber. Here we report direct measurements of the time-scale associated with this transmission degradation for various rubidium density conditions. Transmission is affected almost immediately after the int…
The orbital angular momentum (OAM) of light is a quantity explored for communication and quantum technology, its key strength being a wide set of values offering a large basis for q-working. In this context we have studied the vortex conversion from a red optical vortex to a blue one, for OAMs ranging -30 to +30. The conversion is realized in a rubidium vapor, via the $5S_{1/2}-5D_{5/2}$ $^{85} Rb$ two-photon transition done with a Gaussian beam at 780 nm plus a Laguerre-Gaussian beam at 776 nm with the OAM $\ell$, producing a radiation at 420 nm. With co-propagating input beams, we demonstrat…
We experimentally investigate ultralow-power saturation of the rubidium D2 transitions using a tapered optical fiber (TOF) suspended in a warm Rb vapor. A direct comparison of power-dependent absorption measurements for the TOF system with those obtained in a standard free-space vapor cell system highlights the differences in saturation behavior for the two systems. The effects of hyperfine pumping in the TOF system are found to be minimized due to the short atomic transit times through the highly confined evanescent optical mode guided by the TOF. The TOF system data is well-fit by a relative…
Quantum correlations and entanglement shared among multiple quantum modes are important for both fundamental science and the future development of quantum technologies. This development will also require an efficient quantum interface between multimode quantum light sources and atomic ensembles, which makes it necessary to implement multimode quantum light sources that match the atomic transitions. Here we report on such a source that provides a method for generating quantum correlated beams that can be extended to a large number of modes by using multiple four-wave mixing (FWM) processes in h…
We use weak-value amplification to enhance the polarization-sensitive fast-light effect from induced Raman absorption in hot rubidium vapor. We experimentally demonstrate that projecting the output signal into an appropriate polarization state enables a pulse advancement of 4.2 μs, which is 15 times larger than that naturally caused by dispersion. More significantly, we show that combining weak-value amplification with the dispersive response of an atomic system provides a clear advantage in terms of the maximum pulse advancement achievable for a given value of loss. This technique has potenti…
It is clearly important to pursue atomic standards for quantities like electromagnetic fields, time, length and gravity. We have recently shown, using Rydberg states, that Rb atoms in a vapor cell can serve as a practical, compact standard for microwave electric field strength. Here, we demonstrate, for the first time, that Rb atoms excited in a vapor cell can also be used for vector microwave electrometry by using Rydberg atom electromagnetically induced transparency. We describe the measurements necessary to obtain an arbitrary microwave electric field polarization at a resolution of $0.5^\c…
We study ultra-broadband slow light in a warm Rubidium vapor cell. By working between the D1 and D2 transitions, we find a several-nm window centered at 788.4 nm in which the group index is highly uniform and the absorption is small (<1%). We demonstrate that we can control the group delay by varying the temperature of the cell, and observe a tunable fractional delay of 18 for pulses as short as 250 fs (6.9 nm bandwidth) with a fractional broadening of only 0.65 and a power leakage of 55%. We find that a simple theoretical model is in excellent agreement with the experimental results. Using th…
We demonstrate a tunable, narrow-band filter based on optical-pumping-induced circular dichroism in rubidium vapor. The filter achieves a peak transmission of 14.6%, a linewidth of 80 MHz, and an out-of-band extinction >35 dB. The transmission peak can be tuned within the range of the Doppler linewidth of the D1 line of atomic rubidium at 795 nm. While other atomic filters work at frequencies far from absorption, the presented technique provides light resonant with atomic media, useful for atom-photon interaction experiments. The technique could readily be extended to other alkali atoms.
We apply collective Raman scattering to create, store and retrieve spatially multimode light in warm rubidium-87 vapors. The light is created in a spontaneous Stokes scattering process. This is accompanied by the creation of counterpart collective excitations in the atomic ensemble -- the spin waves. After a certain storage time we coherently convert the spin waves into the light in deterministic anti-Stokes scattering. The whole process can be regarded as a delayed four-wave mixing which produces pairs of correlated, delayed random images. Storage of higher order spatial modes up to microseco…
Diffusion is the main limitation of storage time in spatially multimode applications of warm atomic vapors. Precise knowledge of diffusional decoherence in the system is desired for designing most of vapor memory setups. Here we present a novel, efficient and direct method of measuring unbiased diffusional decoherence, clearly distinguished from all other decoherence sources. We found the normalized diffusion coefficients of rubidium atoms in noble gases to be as follows: neon 0.20 cm$^{2}$/s, krypton 0.068 cm$^{2}$/s and we are the first to give an experimental result for rubidium in xenon: 0…
We investigate the transient response of the generated light from Four-Wave Mixing (FWM) in the diamond configuration using a step-down field excitation. The transients show fast decay times and oscillations that depend on the detunings and intensities of the fields. A simplified model taking into account the thermal motion of the atoms, propagation, absorption and dispersion effects shows qualitative agreement with the experimental observations with the energy levels in rubidium (5S1/2, 5P1/2, 5P3/2 and 6S1/2). The atomic polarization comes from all the contributions of different velocity cla…
We study quantum intensity correlations produced using four-wave mixing in a room-temperature rubidium vapor cell. An extensive study of the effect of the various parameters allows us to observe very large amounts of non classical correlations.
We report on the observation of a Zeeman shift (order of 100 MHz) of the Doppler-broadened D2 transition of both 85Rb and 87Rb isotopes via transmission through a tapered optical nanofiber in the presence of a DC magnetic field. Linearly-polarized light propagating in the nanofiber is analyzed as a superposition of two orthogonally circularly-polarized orientations, σ+ and σ-. In the absence of the magnetic field, the absorption of these polarizations by the atomic vapor, via the evanescent field at the waist of the nanofiber, is degenerate. When a weak magnetic field is applied parallel to th…
We report an experimental realization of an atomic vapor quantum memory for the photonic po- larization qubit. The performance of the quantum memory for the polarization qubit, realized with electromagnetically-induced transparency in two spatially separated ensembles of warm Rubidium atoms in a single vapor cell, has been characterized with quantum process tomography. The process fidelity better than 0.91 for up to 16 μs of storage time has been achieved.
We experimentally investigate the optical storage of perfect optical vortex (POV) and spatially multimode perfect optical vortex (MPOV) beams via electromagnetically induced transparency (EIT) in a hot vapor cell. In particular, we study the role that phase gradients and phase singularities play in reducing the blurring of the retrieved images due to atomic diffusion. Three kinds of manifestations are enumerated to demonstrate such effect. Firstly, the suppression of the ring width broadening is more prominent for POVs with larger orbital angular momentum (OAM). Secondly, the retrieved double-…
We experimentally demonstrate a quantum communication protocol that enables frequency conversion and routing of quantum optical information in an adiabatic and thus robust way. The protocol is based on electromagnetically-induced transparency in systems with multiple excited levels: transfer and/or distribution of optical states between different signal modes is implemented by adiabatically changing the control fields. The proof-of-principle experiment is performed using the hyperfine levels of the rubidium D1 line.
We realize a combined trap for bosonic chromium 52Cr and rubidium 87Rb atoms. First experiments focus on exploring a suitable loading scheme for the combined trap and on studies of new trap loss mechanisms originating from simultaneous trapping of two species. By comparing the trap loss from the 87Rb magneto-optical trap (MOT) in absence and presence of magnetically trapped ground state 52Cr atoms we determine the scattering cross section of sigma_{inelRbCr}=(5.0+-4.0)*10^{-18}m^2 for light induced inelastic collisions between the two species. Studying the trap loss from the Rb magneto-optical…
We report slowed propagation and storage and retrieval of thermal light in warm rubidium vapor using the effect of electromagnetically-induced transparency (EIT). We first demonstrate slowed-propagation of the probe thermal light beam through an EIT medium by measuring the second-order correlation function of the light field using the Hanbury-Brown$-$Twiss interferometer. We also report an experimental study on the effect of the EIT slow-light medium on the temporal coherence of thermal light. Finally, we demonstrate the storage and retrieval of thermal light beam in the EIT medium. The direct…
We study the generation of intensity quantum correlations using four-wave mixing in a rubidium vapor. The absence of cavity in these experiments allows to deal with several spatial modes simultaneously. In the standard, amplifying, configuration, we measure relative intensity squeezing up to 9.2 dB below the standard quantum limit. We also theoretically identify and experimentally demonstrate an original regime where, despite no overall amplification, quantum correlations are generated. In this regime a four-wave mixing set-up can therefore play the role of a photonic beam splitter with non--c…
We present evidence for Rydberg-Rydberg interaction in a gas of rubidium atoms above room temperature. Rabi oscillations on the nanosecond timescale to different Rydberg states are investigated in a vapor cell experiment. Analyzing the atomic time evolution and comparing to a dephasing model we find a scaling with the Rydberg quantum number n that is consistent with van der Waals interaction. Our results show that the interaction strength can be larger than the kinetic energy scale (Doppler width) which is the requirement for realization of thermal quantum devices in the GHz regime.
We demonstrate ladder-type electromagnetically induced transparency (EIT) using an optical nanofiber suspended in a warm rubidium vapor. The signal and control fields are both guided along the nanofiber, which enables strong nonlinear interactions with the surrounding atoms at relatively low powers. Transit-time broadening is found to be a significant EIT decoherence mechanism in this tightly-confined waveguiding geometry. Nonetheless, we observe significant EIT and controlled polarization rotation using control-field powers of only a few microWatts in this relatively robust warm-atom nanofibe…
We report on the observation of Rabi oscillations to a Rydberg state on a timescale below one nanosecond in thermal rubidium vapor. We use a bandwidth-limited pulsed excitation and observe up to 6 full Rabi cycles within a pulse duration of ~ 4 ns. We find good agreement between the experiment and numerical simulations based on a surprisingly simple model. This result shows that fully coherent dynamics with Rydberg states can be achieved even in thermal atomic vapor thus suggesting small vapor cells as a platform for room temperature quantum devices. Furthermore the result implies that previou…
We demonstrate continuous-frequency electric field measurements of high-intensity microwaves via optical spectroscopy in a small atomic vapor cell. The spectroscopic response of a room-temperature rubidium atomic vapor in a glass cell is investigated and employed for absolute measurements of K$_a$-band microwave electric fields from $\sim$200 V/m to $>$1 kV/m over a continuous frequency range of $\pm $1 GHz (15% band coverage). It is established that in strong microwave fields frequency-specific spectral features allow for electric field measurements over a large continuous frequency range.
Using a blue detuned laser shaped in a Laguerre-Gaussian donut mode we highly collimate the output of a two dimensional magneto-optical trap. The resulting atomic beam has a 1 mm diameter, its divergence is reduced from 40 down to 3 mrad and the atomic density is increased by a factor of 200. The collimation effect has been studied versus the order of the Laguerre-Gaussian mode (up to 10) and the laser atom frequency detuning (2 to 120 GHz). The 2D-colli-MOT study allows us to determine the best conditions which minimize the atom heating due to residual light absorption and optimize the collim…
Hot atomic vapors are widely used in non-linear and quantum optics due to their large Kerr non-linearity. While the linear refractive index and the transmission are precisely measured and well modeled theoretically, similar characterization remains partial for the $χ^{(3)}$ non-linear part of the susceptibility. In this work, we present a set of tools to measure and estimate numerically the non-linear index of hot atomic vapors both in the steady state and during the transient response of the medium. We apply these techniques for the characterization of a hot vapor of rubidium and we evidence …
Strongly interacting atom-cavity systems within a network with many nodes constitute a possible realization for a quantum internet which allows for quantum communication and computation on the same platform. To implement such large-scale quantum networks, nanophotonic resonators are promising candidates because they can be scalably fabricated and interconnected with waveguides and optical fibers. By integrating arrays of ring resonators into a vapor cell we show that thermal rubidium atoms above room temperature can be coupled to photonic cavities as building blocks for chip-scale hybrid circu…
We report the fabrication of alkali-metal vapor cells using femtosecond laser machining. This laser-written vapor-cell (LWVC) technology allows arbitrarily-shaped 3D interior volumes and has potential for integration with photonic structures and optical components. We use non-evaporable getters both to dispense rubidium and to absorb buffer gas. This enables us to produce cells with sub-atmospheric buffer gas pressures without vacuum apparatus. We demonstrate sub-Doppler saturated absorption spectroscopy and single beam optical magnetometry with a single LWVC. The LWVC technology may find appl…
We present experimental studies on the generation and detection of pulsed, relative-intensity squeezed light in a warm rubidium vapor. The noise correlations between a pulsed probe beam and its conjugate -generated through nearly-degenerate four-wave mixing in a double-lambda system- are studied via time-resolved balanced detection. We observe -0.96 dB of time-resolved relative intensity squeezing with 50 nanosecond pulses at 1 MHz repetition rate. (-1.34 dB corrected for loss).
We present an experimental study of energy transfer in a thermal vapor of atomic rubidium. We measure the fluorescence spectrum in the visible and near infra-red as a function of atomic density using confocal microscopy. At low density we observe energy transfer consistent with the well-known energy pooling process. In contrast, above a critical density we observe a dramatic enhancement of the fluorescence from high-lying states that is not to be expected from kinetic theory. We show that the density threshold for excitation on the D1 and D2 resonance line corresponds to the value at which the…
We demonstrate the phenomenon of blockade in two-photon excitations to the Rydberg state in thermal vapor. A technique based on optical heterodyne is used to measure the dispersion of a probe beam far off resonant to the D2 line of rubidium in the presence of a strong laser beam that couples to the Rydberg state via two-photon resonance. Density dependent suppression of the dispersion peak is observed while coupling to the Rydberg state with principal quantum number, n = 60. The experimental observation is explained using the phenomenon of Rydberg blockade. The blockade radius is measured to b…
We study an integrated silicon photonic chip, composed of several sub-wavelength ridge waveguides, and immersed in a micro-cell with rubidium vapor. Employing two-photon excitation, including a telecom wavelength, we observe that the waveguide transmission spectrum gets modified when the photonic mode is coupled to rubidium atoms through its evanescent tail. Due to the enhanced electric field in the waveguide cladding, the atomic transition can be saturated at a photon number $\approx$ 80 times less than a free-propagating beam case. The non-linearity of the atom-clad Si-waveguide is about 4 o…
With the help of Stokes operator S2 squeezed state (also called polarization squeezed state (PSS)) of 795-nm light, rubidium-87 (87Rb) atomic magnetometer based on Faraday rotation has been implemented and characterized.The PSS of Stokes operator S2 of 795-nm light has been prepared by means of coherently combining the polarization coherent state (PCS) of a linearly p-polarized bright 795-nm light beam and a linearly s-polarized squeezed vacuum state (SVS) generated by a 397.5-nm ultraviolet laser pumped sub-threshold optical parametric oscillator (OPO) with a PPKTP bulk crystal inside the OPO…
We exploit the effect of light-induced atomic desorption to produce high atomic densities ($n\gg k^3$) in a rubidium vapor cell. An intense off-resonant laser is pulsed for roughly one nanosecond on a micrometer-sized sapphire-coated cell, which results in the desorption of atomic clouds from both internal surfaces. We probe the transient atomic density evolution by time-resolved absorption spectroscopy.With a temporal resolution of $\approx1\,\mathrm{ns}$, we measure the broadening and line shift of the atomic resonances. Both broadening and line shift are attributed to dipole-dipole interact…
Rydberg-assisted atomic electrometry using alkali-metal atoms contained inside a vacuum environment for detecting external electric fields (E-fields) at frequencies $<$ a few kHz has been quite challenging due to the low-frequency E-field screening effect that is caused by the alkali-metal atoms adsorbed on the inner surface of the container. We report a very slow E-field screening phenomenon with a time scale up to $\sim$ second on a rubidium (Rb) vapor cell that is made of monocrystalline sapphire. Using this sapphire-made Rb vapor cell with optically induced, internal bias E-field, we demon…
We report on an experimental test of the spin selection rule for two-photon transitions in atoms. In particular, we demonstrate that the $5S_{1/2}\to 6S_{1/2}$ transition rate in a rubidium gas follows a quadratic dependency on the helicity parameter linked to the polarization of the excitation light. For excitation via a single Gaussian beam or two counterpropagating beams in a hot vapor cell, the transition rate scales as the squared degree of linear polarization. The rate reaches zero when the light is circularly polarized. In contrast, when the excitation is realized via an evanescent fiel…
We present a spectral analysis of Rydberg atoms in strong microwave fields using electromagnetically induced transparency (EIT) as an all-optical readout. The measured spectroscopic response enables optical, atom-based electric field measurements of high-power microwaves. In our experiments, microwaves are irradiated into a room-temperature rubidium vapor cell. The microwaves are tuned near the two-photon 65D-66D Rydberg transition and reach an electric field strength of 230V/m, about 20% of the microwave ionization threshold of these atoms. A Floquet treatment is used to model the Rydberg lev…
This article is designed as a step-by-step guide to optically pumped magnetometers based on alkali atomic vapor cells. We begin with a general introduction to atomic magneto-optical response, as well as expected magnetometer performance merits and how they are affected by main sources of noise. This is followed by a brief comparison of different magnetometer realizations and an overview of current research, with the aim of helping readers to identify the most suitable magnetometer type for specific applications. Next, we discuss some practical considerations for experimental implementations, u…
We experimentally demonstrate hyperfine optical pumping of rubidium atoms probed by an evanescent electromagnetic field at a dielectric-vapor interface. This light-atom interaction at the nanoscale is investigated using a right angle prism integrated with a vapor cell and excited by evanescent wave under total internal reflection. An efficient hyperfine optical pumping, leading to a complete suppression of absorption on the probed evanescent signal, is observed when a pump laser beam is sent at normal incidence to the interface. In contrast, when the pump and probe beams are co-propagating in …
