We report on a scheme for the creation of time-bin entangled states out of two subsequent single photons. Both photons arrive on the same input port of a beamsplitter and the situation in which the photons leave the beamsplitter on different output ports is post-selected. We derive a full quantum mechanical analysis of such time-bin entanglement for emitters subject to uncorrelated dephasing processes and apply this model to sequential single photons emerging from a single semiconductor quantum dot. Our results indicate that the visibility of entanglement is degraded by decoherence effects in the quantum dot, but can be restored by use of CQED effects, namely the Purcell effect.
We propose and analyse the use of a three-well Bose-Hubbard model for the creation of two spatially separated entangled atomic samples. Our three wells are in a linear configuration, with all atoms initially in the middle well, which gives some spatial separation of the two end wells. The evolution from the initial quantum state allows for the development of entanglement between the atomic modes in the two end wells. Using inseparability criteria developed by Hillery and Zubairy, we show how the detected entanglement is time dependent, oscillating with the well occupations. We suggest and anal…
We present an experiment testing quantum correlations with frequency shifted photons. We test Bell inequality with 2-photon interferometry where we replace the beamsplitters by acousto-optic modulators, which are equivalent to moving beamsplitters. We measure the 2-photon beatings induced by the frequency shifts, and we propose a cryptographic scheme in relation. Finally, setting the experiment in a relativistic configuration, we demonstrate that the quantum correlations are not only independent of the distance but also of the time ordering between the two single-photon measurements.
We propose a simple probabilistic optical gate to expand polarization entangled W states. The gate uses one polarization-dependent beamsplitter and a horizontally polarized single photon as an ancilla. The gate post-selectively expands $N$-photon W states to $(N+1)$-photon W states. A feasibility analysis considering the realistic experimental conditions show that the scheme is within the reach of the current quantum optical technologies.
A one-dimensional waveguide enables a single two-level emitter to route the propagation of a single photon, as to provide a quantum mirror or a quantum beamsplitter. Here we present a fully-quantum Mach-Zehnder interferometer (QMZ) for single-photon pulses comprised of two quantum beamsplitters. We theoretically show how nonlinearities of the QMZ due to photon-emitter detunings and to the spectral linewidth of the pulse contribute to the versatility of the device with respect to the classical-beamsplitters scenario. We employ a quantum dynamics framework to obtain analytical expressions for th…
A linear 50/50 beamsplitter, together with a coincidence measurement, has been widely used in quantum optical experiments, such as teleportation, dense coding, etc., for interferometrically distinguishing, measuring, or projecting onto one of the four two-photon polarization Bell-states $|ψ^{(-)}>$. In this paper, we demonstrate that the coincidence measurement at the output of a beamsplitter cannot be used as an absolute identifier of the input state $|ψ^{(-)}>$ nor as an indication that the input photons have projected to the $|ψ^{(-)}>$ state.
In spontaneous emission an atom in an excited state undergoes a transition to the ground state and emits a single photon. Associated with the emission is a change of the atomic momentum due to photon recoil. Photon emission can be modified close to surfaces and in cavities. For an ion, localized in front of a mirror, coherence of the emitted resonance fluorescence has been reported. In free space experiments demonstrated that spontaneous emission destroys motional coherence. Here we report on motional coherence created by a single spontaneous emission event close to a mirror surface. The coher…
We report an interference experiment in which the two-photon entangled state interference cannot be pictured in terms of the overlap and bunching of two individual photons on a beamsplitter. We also demonstrate that two-photon interference, or photon bunching effect on a beamsplitter, does not occur if the two-photon Feynman amplitudes are distinguishable, even though individual photons do overlap on a beamsplitter. Therefore, two-photon interference cannot be viewed as interference of two individual photons, rather it should be viewed as two-photon or biphoton interfering with itself. The res…
The visibility of the quantum interference "dip" seen in the Hong-Ou-Mandel experiment is optimized when a symmetric 50/50 beamsplitter is used in the interferometer. Here we show that the reduction in visibility caused by an asymmetric beamsplitter can be compensated by manipulating the polarization states of the two input photons. We experimentally demonstrate this by using a highly asymmetric 10/90 beamsplitter, and converting an initial dip visibility of 22% to a compensated value of 99%.
We demonstrated the first-order interference between coherent light at 1580 nm and 795 nm by using frequency-domain Mach-Zehnder interferometer (MZI). The MZI is implemented by two frequency-domain BSs based on a second-order nonlinear optical effect in a periodically-poled lithium niobate waveguide with a strong pump light. We achieved the visibility of over 0.99 at 50% conversion efficiencies of the BSs. Toward photonic quantum information processing, sufficiently small background photon rate is necessary. From the measurement results with a superconducting single photon detector, we discuss…
We analyze the ultimate bounds on the phase sensitivity of an interferometer, given the constraint that the state input to the interferometer's initial 50:50 beamsplitter $B$ is a product state of the two input modes. Requiring a product state is a natural restriction: if one were allowed to input an arbitrary, entangled two-mode state $|Ξ\rangle$ to the beamsplitter, one could generally just as easily input the state $B|Ξ\rangle$ directly into the two modes after the beamsplitter, thus rendering the beamsplitter unnecessary. We find optimal states for a fixed photon number and for a fixed mea…
When a one-photon state is mixed with a (separate) weak coherent state at a beamsplitter the probability for detecting one photon in each beamsplitter output approaches zero due to destructive interference. We demonstrate this non-classical interference effect using pulse-gated single photons and weak mode-locked laser pulses.
Fourth-order interference is an information processing primitive for photonic quantum technologies. When used in conjunction with post-selection, it forms the basis of photonic controlled logic gates, entangling measurements, and can be used to produce quantum correlations. Here, using classical weak coherent states as inputs, we study fourth-order interference in novel $4 \times 4$ multi-port beam splitters built within multi-core optical fibers. Using two mutually incoherent weak laser pulses as inputs, we observe high-quality fourth order interference between photons from different cores, a…
The well-known Hong-Ou-Mandel effect is revisited. Two physical reasons are discussed for the effect to be less pronounced or even to disappear: differing polarizations of photons coming to the beamsplitter and delay time of photons in one of two channels. For the latter we use the concepts of biphoton frequency and temporal wave functions depending, correspondingly, on two frequency continuous variables of photons and on two time variables $t_1$ and $t_2$ interpreted as the arrival times of photons to the beamsplitter. Explicit expressions are found for the probability densities and total pro…
The implementation of a fully integrated Hadamard gate on one single chip is currently one of the major goals in the quantum computation and communication community. Prerequisites for such a chip are the integration of single-photon sources and detectors into waveguide structures such as photonic crystals or slab and ridge waveguide. Here, we present an implementation of a single-photon on-chip experiment based on a III-V semiconductor platform. Individual semiconductor quantum dots were used as pulsed single-photon sources integrated in ridge waveguides, and on-chip waveguide-beamsplitter ope…
We demonstrate a monolithic III-V photonic circuit combining a heralded single photon source with a beamsplitter, at room temperature and telecom wavelength. Pulsed parametric down-conversion in an AlGaAs waveguide generates counterpropagating photons, one of which is used to herald the injection of its twin into the beamsplitter. We use this configuration to implement an integrated Hanbury-Brown and Twiss experiment, yielding a heralded second-order correlation $g^{(2)}_{\rm her}(0)=0.10 \pm 0.02$ that confirms single-photon operation. The demonstrated generation and manipulation of quantum s…
We generalize a new approach to entanglement conditions for light of undefined photons numbers given in [Phys. Rev. A {\bf 95}, 042113 (2017)] for polarization correlations to a broader family of interferometric phenomena. Integrated optics allows one to perform experiments based upon multiport beamsplitters. To observe entanglement effects one can use multi-mode parametric down-conversion emissions. When the structure of the Hamiltonian governing the emissions has (infinitely) many equivalent Schmidt decompositions into modes (beams), one can have perfect EPR-like correlations of numbers of p…
Here, we numerically simulate probabilistic elementary entangling operations between rail-encoded photons for the purpose of scalable universal quantum computation or communication. We propose grouping logical qubits into single-photon blocks wherein single-qubit rotations and the CNOT gate are fully deterministic and simple to implement. Inter-block communication is then allowed through said probabilistic entangling operations. We find a promising trend in the increasing probability of successful inter-block communication as we increase the number of optical modes operated on by our elementar…
We propose an approach to optical quantum computation in which a deterministic entangling quantum gate may be performed using, on average, a few hundred coherently interacting optical elements (beamsplitters, phase shifters, single photon sources, and photodetectors with feedforward). This scheme combines ideas from the optical quantum computing proposal of Knill, Laflamme and Milburn [Nature 409 (6816), 46 (2001)], and the abstract cluster-state model of quantum computation proposed by Raussendorf and Briegel [Phys. Rev. Lett. 86, 5188 (2001)].
We derive the maximum success probability of the circuits with passive linear optics for expanding an N-photon W state to an (N + n)-photon W state, by accessing only one photon of the initial W state and adding n photons in a Fock state. We show that the maximum success probability is achieved by a polarization-dependent beamsplitter and n-1 polarization-independent beamsplitters.
We demonstrate unambiguous entangling operation of a photonic quantum-logic gate driven by an ultrabright solid-state single-photon source. Indistinguishable single photons emitted by a single semiconductor quantum dot in a micropillar optical cavity are used as target and control qubits. For a source brightness of 0.56 collected photons-per-pulse, the measured truth table has an overlap with the ideal case of 68.4%, increasing to 73.0% for a source brightness of 0.17 photons- per-pulse. The gate is entangling: at a source brightness of 0.48, the Bell-state fidelity is above the entangling thr…
Exceptional points (EPs) are degeneracies of non-Hermitian operators where, in addition to the eigenvalues, corresponding eigenmodes become degenerate. Classical and quantum photonic systems with EPs have attracted tremendous attention due to their unusual properties, topological features, and an enhanced sensitivity that depends on the order of the EP, i.e. the number of degenerate eigenmodes. Yet, experimentally engineering higher-order EPs in classical or quantum domains remains an open challenge due to the stringent symmetry constraints that are required for the coalescence of multiple eig…
We describe a simple entangling principle based on the scattering of photons off single emitters in one-dimensional waveguides (or extremely-lossy cavities). The scheme can be applied to photonic qubits encoded in polarization or time-bin, and features a filtering mechanism that works effectively as a built-in error-correction directive. This automatically maps imperfections from weak couplings, atomic decay into undesired modes, frequency mismatches, or finite bandwidths of the incident photonic pulses, into heralded losses instead of infidelities. The scheme is thus adequate for high-fidelit…
A method is proposed for generating and discriminating Bell states of high fidelity from consecutive single-photons generated in a semiconductor quantum dot. The use of a non-symmetric beam splitter is found to be essential and sufficient, and no nonlinear optical process such as SPDC is required at any stage. This should be of considerable importance for testing the foundations of quantum mechanics.
Significant experimental advances in single-electron silicon spin qubits have opened the possibility of realizing long-range entangling gates mediated by microwave photons. Recently proposed iSWAP gates, however, require tuning qubit energies into resonance and have limited fidelity due to charge noise. We present a novel photon-mediated cross-resonance gate that is consistent with realistic experimental capabilities and requires no resonant tuning. Furthermore, we propose gate sequences capable of suppressing errors due to quasistatic noise for both the cross-resonance and iSWAP gates.
In continuous-variable quantum computing with qubits encoded in the infinite-dimensional Hilbert space of bosonic modes, it is a difficult task to realize strong and on-demand interactions between the qubits. One option is to engineer a beamsplitter interaction for photons in two superconducting cavities by driving an intermediate superconducting circuit with two continuous-wave drives, as demonstrated in a recent experiment. Here, we show how quantum optimal control theory (OCT) can be used in a systematic way to improve the beamsplitter interaction between the two cavities. We find that repl…
A scheme is proposed here to achieve swapping and entangling of photonic and atomic qubits with high fidelity. The mechanism is based on the scattering of a single photon from a $Λ$-type three-level atom. The evolution of the coupled system is analyzed by projecting the quantum state onto a `bright' and a `dark' state. Quantum interference of these two states, which is determined by a frequency-dependent phase angle, can be exploited to perform various two-qubit transformations. It is remarkable that the probability of success of such transformations can approach unity in the strong coupling c…
Bosonic quantum error correction has proven to be a successful approach for extending the coherence of quantum memories, but to execute deep quantum circuits, high-fidelity gates between encoded qubits are needed. To that end, we present a family of error-detectable two-qubit gates for a variety of bosonic encodings. From a new geometric framework based on a "Bloch sphere" of bosonic operators, we construct $ZZ_L(θ)$ and $\text{eSWAP}(θ)$ gates for the binomial, 4-legged cat, dual-rail and several other bosonic codes. The gate Hamiltonian is simple to engineer, requiring only a programmable be…
We propose a scheme for entangling two photons via the quantum Zeno effect, which describes the inhibition of quantum evolution by frequent measurements and is based on the difference between summing amplitudes and probabilities. For a given error probability $P_{\rm error}$, our scheme requires that the one-photon loss rate $ξ_{1γ}$ and the two-photon absorption rate $ξ_{2γ}$ in some medium satisfy $ξ_{1γ}/ξ_{2γ}=2P_{\rm error}^2/π^2$, which is significantly improved in comparison to previous approaches. Again based on the quantum Zeno effect, as well as coherent excitations, we present a pos…
In 1994, Reck et al. showed how to realize any unitary transformation on a single photon using a product of beamsplitters and phaseshifters. Here we show that any single beamsplitter that nontrivially mixes two modes, also densely generates the set of unitary transformations (or orthogonal transformations, in the real case) on the single-photon subspace with m>=3 modes. (We prove the same result for any two-mode real optical gate, and for any two-mode optical gate combined with a generic phaseshifter.) Experimentally, this means that one does not need tunable beamsplitters or phaseshifters for…
We report an experimental test of complementarity using clock-triggered single-photon pulses emitted by an individual N-V color center in a diamond nanocrystal. The single photons are sent into a Mach-Zehnder interferometer with an output beamsplitter of adjustable reflection coefficient R. In addition, the choice of introducing or removing this beamsplitter is random and relativistically space-like separated from the entering of the photon inside the interferometer, as required for the Wheeler's delayed-choice regime. Each set value of R allows us to observe interference with visibility V and…
Bose-Einstein coalescence of independent photons at the surface of a beam splitter is the physical process that allows linear optical quantum gates to be built. When distinct parametric down-conversion events are used as an independent photon source, distinguishability arises form the energy correlation of each photon with its twin. We find that increasing the pump bandwidth may help in improving the visibility of non-classical interference and reaching a level of near perfect indistinguishability. PACS: 03.67.Mn, 42.65.Lm, 42.50.St.
Fock states are a fundamental resource for many quantum technologies such as quantum metrology. While much progress has been made in single-photon source technologies, preparing Fock states with large photon number remains challenging. We present and analyze a bootstrapped approach for non-deterministically preparing large photon-number Fock states by iteratively fusing smaller Fock states on a beamsplitter. We show that by employing state recycling we are able to exponentially improve the preparation rate over conventional schemes, allowing the efficient preparation of large Fock states. The …
We propose a feasible scheme to realize the optical entanglement of single-photon-added coherent state (SPACS) and show that, besides the Sanders entangled coherent state, the entangled SPACS also leads to new forms of hybrid entanglement of quantum Fock state and classical coherent state. We probe the essential difference of two types of hybrid entangled state (HES). This HES provides a novel link between the discrete- and the continuous-variable entanglement in a natural way.
Heralded entangling quantum gates are an essential element for the implementation of large-scale optical quantum computation. Yet, the experimental demonstration of genuine heralded entangling gates with free-flying output photons in linear optical system, was hindered by the intrinsically probabilistic source and double-pair emission in parametric down-conversion. Here, by using an on-demand single-photon source based on a semiconductor quantum dot embedded in a micro-pillar cavity, we demonstrate a heralded controlled-NOT (CNOT) operation between two single photons for the first time. To cha…
We report experimental realization of high-fidelity photonic quantum gates for frequency-encoded qubits and qutrits based on electro-optic modulation and Fourier-transform pulse shaping. Our frequency version of the Hadamard gate offers near-unity fidelity ($0.99998\pm0.00003$), requires only a single microwave drive tone for near-ideal performance, functions across the entire C-band (1530-1570 nm), and can operate concurrently on multiple qubits spaced as tightly as four frequency modes apart, with no observable degradation in the fidelity. For qutrits we implement a $3\times 3$ extension of …
We present two novel schemes to generate photon polarization entanglement via single electron spins confined in charged quantum dots inside microcavities. One scheme is via entangled remote electron spins followed by negatively-charged exciton emissions, and another scheme is via a single electron spin followed by the spin state measurement. Both schemes are based on giant circular birefringence and giant Faraday rotation induced by a single electron spin in a microcavity. Our schemes are deterministic and can generate an arbitrary amount of multi-photon entanglement. Following similar procedu…
For a thought experiment concerning the mixing of two classical gases, Gibbs concluded that the work that can be extracted from mixing is determined by whether or not the gases can be distinguished by a semi-permeable membrane; that is, the mixing work is a discontinuous function of how similar the gases are. Here we describe an optomechanical setup that generalises Gibbs' thought experiment to partially distinguishable quantum gases. Specifically, we model the interaction between a polarising beamsplitter, that plays the role of a semi-permeable membrane, and two photon gases of non-orthogona…
Entanglement is a fundamental property of quantum mechanics, and is a primary resource in quantum information systems. Its manipulation remains a central challenge in the development of quantum technology. In this work, we demonstrate a device which can generate, manipulate, and analyse two-qubit entangled states, using miniature and mass-manufacturable silicon photonics. By combining four photon-pair sources with a reconfigurable six-mode interferometer, embedding a switchable entangling gate, we generate two-qubit entangled states, manipulate their entanglement, and analyse them, all in the …
We report an experimental realisation of a quantum random number generator using a plasmonic beamsplitter. Free-space single photons are converted into propagating single surface plasmon polaritons on a gold stripe waveguide via a grating. The surface plasmons are then guided to a region where they are scattered into one of two possible outputs. The presence of a plasmonic excitation in a given output determines the value of a random bit generated from the quantum scattering process. Using a stream of single surface plasmons injected into the beamsplitter we achieve a quantum random number gen…
Semiconductor quantum dots (known as artificial atoms) hold great promise for solid-state quantum networks and quantum computers. To realize a quantum network, it is crucial to achieve light-matter entanglement and coherent quantum-state transfer between light and matter. Here we present a robust photon-spin entangling gate with high fidelity and high efficiency (up to 50 percent) using a charged quantum dot in a double-sided microcavity. This gate is based on giant circular birefringence induced by a single electron spin, and functions as an optical circular polariser which allows only one ci…
A paradigm for universal quantum information processing with integrated acousto-optic frequency beamsplitters
Purdue University（普渡大学）；Oak Ridge National Laboratory（橡树岭国家实验室）；Northern Arizona University（北亚利桑那大学）；Sandia National Laboratories（桑迪亚国家实验室）；Qunnect Inc.（Qunnect公司）
Generalised quantum measurements go beyond the textbook concept of a projection onto an orthonormal basis in Hilbert space. They are not only of fundamental relevance but have also an important role in quantum information tasks. However, it is highly demanding to certify that a generalised measurement is indeed required to explain the results of a quantum experiment in which only the degrees of freedom are assumed to be known. Here, we use state-of-the-art multicore optical fiber technology to build multiport beamsplitters and faithfully implement a seven-outcome generalised measurement in a f…
Deterministic sources of multi-photon entanglement are highly attractive for quantum information processing but are challenging to realize experimentally. In this paper, we demonstrate a route towards a scaleable source of time-bin encoded Greenberger-Horne-Zeilinger and linear cluster states from a solid-state quantum dot embedded in a nanophotonic crystal waveguide. By utilizing a self-stabilizing double-pass interferometer, we measure a spin-photon Bell state with $(67.8\pm0.4)\%$ fidelity and devise steps for significant further improvements. By employing strict resonant excitation, we dem…
We consider a system consisting of a $Λ$-type atom and a V-type atom, which are individually trapped in two spatially separated cavities that are connected by an optical fibre. We show that an extremely entangled state of the two atoms can be deterministically generated through both photon emission of the $Λ$-type atom and photon absorption of the V-type atom in an ideal situation. The influence of various decoherence processes such as spontaneous emission and photon loss on the fidelity of the entangled state is also investigated. We find that the effect of photon leakage out of the fibre on …
A single photon can be made to entangle simultaneously in its different internal degrees of freedom (DoF) -- polarization, orbital angular momentum (OAM), and frequency -- as well as in its external DoF -- path. Such entanglement in multiple DoF is known as hyperentanglement and provide additional advantage for quantum information processing. We propose a passive optical setup using $q$-plates and polarization beamsplitters to hyperentangle an incoming single photon in polarization, OAM, and path DoF. By mapping polarization DoF to a two-dimensional coin state, and path and OAM DoF to two spat…
Two-photon anti-bunching at a beamsplitter is only possible if the photons are entangled in a specific state, anti-symmetric in the spatial modes. Thus, observation of anti-bunching is an indication of entanglement in a degree of freedom which might not be easily accessible in an experiment. We experimentally demonstrate this concept in the case of the interference of two frequency entangled photons with continuous frequency detunings. The principle of anti-symmetrisation of the spatial part of a wavefunction and subsequent detection of hidden entanglement via anti-bunching at a beamsplitter m…
The effects of a beamsplitter are frequently described mathematically as a matrix acting on a two input ports vector. This might be comprehensive for a scalar field but certainly insufficient in case of photons which are vector fields. In this paper we discuss theoretical grounds to define elements of a 4x4 matrix to more accurately represent the beamsplitter, fully accounting for transverse polarization modes. We also provide experimental evidence confirming this matrix representation. From an educational point of view the paper addresses a new applicability of Hilbert space description of ve…
We show how entanglement between two optically levitated nanoparticles can be generated and detected by coherent scattering of tweezer photons into a single cavity mode. Triggered by the detection of a Stokes photon, the tweezer detuning is switched from the blue to the red; entanglement is then verified by the conditioned anti-Stokes photon flux, which oscillates with the mechanical beat frequency. The proposed setup is realizable with near-future technology and opens the door to the first experimental observation of non-classical center-of-mass correlations between two or more levitated nano…
