One of considered nowadays scenarios of proton - nucleus reaction is spallation. Its motivation is based on experimental final-state observations of one heavy nucleus, a small number of light fragments and numerous individual nucleons. It is theoretically described as two step process involving energy deposition in the target nucleus and subsequent evaporation. Several models, based on different assumptions, have been constructed in order to describe the spallation process. The main subject of this work is description of global average properties of proton induced spallation reactions in wide range of projectile energy (0.1 - 10 GeV) and mass of target nuclei. This is investigated within Hadron String Dynamics (HSD) model, based on Boltzmann - Uehling - Uhlenbeck (BUU) equation, supplemented by a statistical evaporation model for the second stage of the reaction. It has been shown that spallation is the most probable scenario of proton - nucleus reaction. Proton induced reactions, in considered here incident energy range, are visibly non-invasive processes. Properties of residual nuclei after the first stage of the reaction are weakly dependent on incident energy, but strongly dependent on mass of target. The second stage of the reaction is a competition of evaporation and fission. Results obtained from the HSD model vary smoothly as function of proton incident energy and mass of target, so interpolation of the results is quite feasible.
The dynamics of high-energy proton-induced spallation reactions on target nuclides of $^{136}$Xe, $^{59}$Ni, $^{56}$Fe, $^{208}$Pb, $^{184}$W, $^{181}$Ta, $^{197}$Au and $^{112}$Cd, are investigated with the quantum molecular dynamics transport model. The production mechanism of light nuclides and fission fragments is thoroughly analyzed. The statistical code GEMINI is employed in conjunction to the model for managing the decay of primary fragments. For the treatment of cluster emission during the preequilibrium stage, a surface coalescence model is implemented into the model. It is found that…
We have used an extended version of the Cascade-Exciton Model (CEM) to analyze more than 600 excitation functions for proton induced reactions on 19 targets ranging from C-12 to Au-197, for incident energies ranging from 10 MeV to 5 GeV. We have compared the calculations to available data, to calculations using approximately two dozen other models, and to predictions of several phenomenological systematics. We present here our conclusions concerning the relative roles of different reaction mechanisms in the production of specific final nuclides. We comment on the strengths and weaknesses of th…
We have investigated the influence of different non-linear relativistic mean field models ($NL$, $NLρ$ and $NLρδ$) on spallation neutrons for p+Fe and Pb reactions at 0.8, 1.2 and 1.6 GeV by means of a relativistic Boltzmann Uehling Uhlenbeck (RBUU) approach plus a statistical multifragmentation (SM) decay model. We find that the "evaporation shoulder", i.e. the neutron energy spectrum from 3 to 30 MeV, almost for any emission angle is quite sensitive to the isospin part of the mean field. For the more neutron-rich Pb-target the evaporation component can be directly related to the low density …
Fragments productions in spallation reactions are key infrastructure data for various applications. Based on the empirical parameterizations {\sc spacs}, a Bayesian-neural-network (BNN) approach is established to predict the fragment cross sections in the proton induced spallation reactions. A systematic investigation have been performed for the measured proton induced spallation reactions of systems ranging from the intermediate to the heavy nuclei and the incident energy ranging from 168 MeV/u to 1500 MeV/u. By learning the residuals between the experimental measurements and the {\sc spacs} …
We studied the complete dynamics of the proton-induced spallation process with the microscopic framework of the Constrained Molecular Dynamics (CoMD) Model. We performed calculations of proton-induced spallation reactions on 181Ta, 208Pb, and 238U targets with the CoMD model and compared the results with a standard two-step approach based on an intranuclear cascade model (INC) followed by a statistical deexcitation model. The calculations were also compared with recent experimental data from the literature. Our calculations showed an overall satisfactory agreement with the experimental data an…
The Bayesian neural network (BNN) method is used to construct a predictive model for fragment prediction of proton induced spallation reactions with the guidance of a simplified EPAX formula. Compared to the experimental data, it is found that the BNN + sEPAX model can reasonably extrapolate with less information compared with BNN method. The BNN + sEPAX method provides a new approach to predict the energy-dependent residual cross sections produced in proton-induced spallation reactions from tens of MeV/u up to several GeV/u.
The ratio of pairing-energy coefficient to temperature ($a_{p}/T$) of neutron-rich fragments produced in spallation reactions has been investigated by adopting an isobaric yield ratio method deduced in the framework of a modified Fisher model. A series of spallation reactions, 0.5$A$ and 1$A$ GeV $^{208}$Pb + $p$, 1$A$ GeV $^{238}$U + $p$, 0.5$A$ GeV $^{136}$Xe + $d$, 0.2$A$, 0.5$A$ and 1$A$ GeV $^{136}$Xe + $p$, and $^{56}$Fe + $p$ with incident energy ranging from 0.3$A$ to 1.5$A$ GeV, has been analysed. An obvious odd-even staggering is shown in the fragments with small neutron excess ($I\e…
We present a statistical-model description of fission, in the framework of compound-nucleus decay, which is found to simultaneously reproduce data from both heavy-ion-induced fusion reactions and proton-induced spallation reactions at around 1 GeV. For the spallation reactions, the initial compound-nucleus population is predicted by the Liège Intranuclear Cascade Model. We are able to reproduce experimental fission probabilities and fission-fragment mass distributions in both reactions types with the same parameter sets. However, no unique parameter set was obtained for the fission probability…
The spatial and energy distribution of spallation neutrons have an effect on the performance of Accelerator Driven Subcritical systems. In this work, the spatial, energy distribution of spallation neutrons and the effect of these factors on proton efficiency was studied. When the radius of spallation region increases, backward neutrons were found to have a rather big ratio and have a positive effect on proton efficiency. By making better use of these neutrons, we may increase the radius of target to satisfy some other requirements in the design of subcritical core.
A qualitative and quantitative comparison of the recent GSI measurements of the nuclide yields from 208Pb and 238U at 1 GeV/nucleon and 197Au at 800 MeV/nucleon interactions with protons with the codes LAHET (with both ISABEL and Bertini options), CEM95, CEM97, CEM2k, CASCADE, CASCADE/INPE, YIELDX, HETC, and INUCL is presented. The predictive power of these codes is reasonable for nuclides in the near spallation region but is worse for deep spallation and much worse in the fission region. None of these codes agree well with the data in the whole mass region of product nuclides and all must be …
We use particle-transport simulations to show that secondary pions play a crucial role for the development of the hadronic cascade and therefore for the production of neutrons and photons from thick spallation targets. In particular, for the n_TOF lead spallation target, irradiated with 20 GeV/c protons, neutral pions are involved in the production of ~90% of the high-energy photons; charged pions participate in ~40% of the integral neutron yield. Nevertheless, photon and neutron yields are shown to be relatively insensitive to large changes of the average pion multiplicity in the individual s…
In the future several Spallation Source facilities will be available worldwide. Spallation Sources produce large amount of neutrinos from decay-at-rest muons and thus can be well adapted to accommodate state-of-the-art neutrino experiments. In this paper low energy neutrino scattering experiments that can be performed at such facilities are reviewed. Estimation of expected event rates are given for several nuclei, electrons and protons at a detector located close to the source. A neutrino program at Spallation Sources comprises neutrino-nucleus cross section measurements relevant for neutrino …
The LAQGSM code has been recently developed at Los Alamos National Laboratory to simulate nuclear reactions for proton radiography applications. We have benchmarked our code against most available measured data both for proton-nucleus and nucleus-nucleus interactions at incident energies from 10 MeV to 800 GeV and have compared our results with predictions of other current models used by the nuclear community. Here, we present a brief description of our code and show illustrative results obtained with LAQGSM for neutron spectra measured recently by Nakamura's groups for reactions induced by li…
Use of deuteron-induced spallation reactions at intermediate energies has recently been proposed for transmutation of several long-lived fission products (LLFPs). In the design study of a transmutation system using a deuteron primary beam, accurate cross section data of deuteron-induced reactions on the LLFPs are indispensable. Reliable model predictions play an important role in completing the necessary cross section data since currently available experimental data are very limited. Under the circumstances, we have been developing a code system dedicated for deuteron-induced reactions, which …
Based on the Boltzmann-Uehling-Uhlenbeck (BUU) transport model coupled with a phase-space coalescence afterburner, spallation reaction of $p+^{197}Au$ at the incident beam energy of E$_{beam}$= 800 MeV/nucleon is studied. We find that the number of test particles per nucleon has minor effects on the neutron to proton ratio (n/p) of the produced heavier fragments while it affects much on their yields. The external strong magnetic field affects the production of heavier fragments much than the n/p of produced fragments. The n/p of free nucleons is greatly affected by the strong magnetic field, e…
We investigate the prompt emission of few intermediate-mass fragments in spallation reactions induced by protons and deuterons in the 1 GeV range. Such emission has a minor contribution to the total reaction cross section, but it may overcome evaporation and fission channels in the formation of light nuclides. The role of mean-field dynamics and phase-space fluctuations in these reactions is investigated through the Boltzmann-Langevin transport equation. We found that a process of frustrated fragmentation and re-aggregation is a prominent mechanism of production of IMFs which can not be assimi…
Rules for in-medium complex particle production in nuclear reactions are proposed. These rules have been implemented in two models to simulate nucleon-nucleus and nucleus-nucleus reactions around the Fermi energy. Our work emphasizes the effect of randomness in cluster formation, the importance of the nucleonic Fermi motion as well as the role of conservation laws. The concepts of total available phase-space and explored phase-space under constraint imposed by the reaction are clarified. The compatibility of experimental observations with a random clusterization is illustrated in a schematic s…
The ability to describe production of light fragments (LF) is important for many applications, such as cosmic-ray-induced single event upsets (SEUs), radiation protection, and cancer therapy with proton and heavy-ion beams. The Cascade-Exciton Model (CEM) and the Los Alamos version of the Quark-Gluon String Model (LAQGSM) event generators in the LANL transport code MCNP6, describe quite well the spectra of fragments with sizes up to 4He across a broad range of target masses and incident energies (up to ~ 5 GeV for CEM and up to ~ 1 TeV/A for LAQGSM). However, they do not predict the high-energ…
A simple model based on relativistic geometry and final-state hadronic rescattering is used to predict pion source parameters extracted in two-pion femtoscopy studies of proton-proton collisions at s**(1/2) = 200 GeV. From studying the momentum and particle multiplicity dependences of these parameters in the context of this model and assuming a very short hadronization time, flow-like behavior is seen which resembles the flow behavior commonly observed in relativistic heavy-ion collisions.
The production of strange particles (kaons, hyperons) and hypernuclei in light charged particle induced reactions in the energy range of a few GeV (2-15 GeV) has become a topic of active research in several facilities (e.g., HypHI and PANDA at GSI and/or FAIR (Germany), JLab (USA), and JPARC (Japan)). This energy range represents the low-energy limit of the string models (degree of freedom: quark and gluon) or the high-energy limit of the so-called spallation models (degree of freedom: hadrons). A well known spallation model is INCL, the Liège intranuclear cascade model (combined with a de-exc…
The CEM2k and LAQGSM codes have been recently developed at Los Alamos National Laboratory to simulate nuclear reactions induced by particles and nuclei for a number of applications. We have benchmarked our codes against most available measured data at projectile energies from 10 MeV/A to 800 GeV/A and have compared our results with predictions of other current models used by the nuclear community. Here, we present a brief description of our codes and show illustrative results obtained with CEM2k and LAQGSM for A+p and A+A spallation, fission, and fragmentation reactions measured recently at GS…
A combined analysis of the existing data on the reactions $γp \to p η^\prime $ and $pp \to ppη^\prime $, based on a relativistic meson exchange model of hadronic interactions, is presented.
The induced-activity investigations in off-line analysis performed in different experiments, concerning pre-actinide and actinide nuclei, are here presented and discussed. Generalized expressions for the determination of independent yields/cross sections of radioactive nuclei, formed in the targets, are derived and analysed. The fragment mass distribution from U-238, Th-232 and Ta-181 photofission at the bremsstrahlung end-point energies of 50 and 3500 MeV, and from Am-241, U-238 and Np-237 fission induced by 660-MeV protons, are scrutinized from the point of view of the multimodal fission app…
Different reaction mechanisms contribute to the production of light fragments (LF) from nuclear reactions. Available models cannot accurately predict emission of LF from arbitrary reactions. However, the emission of LF is important for many applications, such as cosmic-ray-induced single event upsets, radiation protection, and cancer therapy with proton and heavy-ion beams, to name just a few. The cascade-exciton model (CEM) and the Los Alamos version of the quark-gluon string model (LAQGSM), as implemented in the CEM03.03 and LAQGSM03.03 event generators used in the Los Alamos transport code …
Two NaI (85% 129-I and 15% 127-I) targets were exposed to a beam of 660-MeV protons. Cross sections for formation of 76 residual nuclei were obtained by the induced activity method. The results are compared with other experimental data on 127-I and theoretical calculations by eleven models contained in the codes LAHET3 (using the Bertini+Dresner, ISABEL+Dresner, INCL+Dresner, and INCL+ABLA options), CASCADE, CEM95, CEM2K, LAQGSM+GEM2, CEM2k+GEM2, LAQGSM+GEMINI, and CEM2k+GEMINI. Most of the models describe spallation products with masses close to the target reasonably well while the reliabilit…
A large set of data on proton-proton differential cross sections, analyzing powers and the double polarization parameter A_NN is analyzed employing the Regge formalism. We find that the data available at proton beam momenta from 3 GeV/c to 50 GeV/c exhibit features that are very well in line with the general characteristics of Regge phenomenology and can be described with a model that includes the rho, omega, f_2, and a_2 trajectories and single Pomeron exchange. Additional data, specifically for spin-dependent observables at forward angles, would be very helpful for testing and refining our R…
113 residual product nuclide yields in a 1.0 GeV proton-irradiated thin monoisotopic 208-Pb sample and 107 residual product nuclide yields in a 2.6 GeV proton-irradiated nat-W sample have been measured and simulated by 8 different codes. The irradiations were made using proton beams extracted from the ITEP synchrotron. The nuclide yields were gamma-spectrometered directly using a high-resolution Ge-detector. The gamma-spectra were processed by the GENIE-2000 code. The ITEP-developed SIGMA code was used together with the PCNUDAT nuclear decay database to identify the gamma-lines and to determin…
We comment on the statement by Kuznetsov et al. that the structure around W=1.72 GeV seen in the beam asymmetry in Compton scattering off the proton is not observed in the total cross section of $η$ photoproduction on the neutron.
We compare calculations for the production of charged pions by pion or proton beams off nuclei calculated within our coupled channel transport model (GiBUU) with recent data of the HARP collaboration for beam energies from 3 up to 13 GeV. Predictions for the 30 GeV data for pions and kaons from the NA61/SHINE experiment are included.
The ITEP proton synchrotron U10 was used to irradiate isotopically-enriched 208Pb and natU thin targets with 1.0 GeV protons and 197Au thin targets with 0.8 GeV protons. More than 400 cross sections of the nuclides produced were measured using the direct spectrometry method with a high-resolution Ge detector. The measured cross sections are compared with similar data obtained at GSI for kinematically inverse reactions of 1 GeV/nucleon 208Pb, 1 GeV/nucleon 238U, and 0.8 GeV/nucleon 197Au interacting with a hydrogen target and with the ZSR data on natPb and 197Au irradiated with 1 and 0.8 GeV pr…
We discuss three different cases of hard inclusive spectra in proton-proton collisions: high $p_T$ single hadron production at $\sqrt{s}\approx$ 20 GeV and at $\sqrt{s}$ = 62.4 GeV, and direct photon production at $\sqrt{s}$ = 200 GeV; with regard to their relevance for the search of Quark Gluon Plasma signals in A+A collisions at SPS and RHIC energies.
