We report on transport characteristics of quantum dot devices etched entirely in graphene. At large sizes, they behave as conventional single-electron transistors, exhibiting periodic Coulomb blockade peaks. For quantum dots smaller than 100 nm, the peaks become strongly non-periodic indicating a major contribution of quantum confinement. Random peak spacing and its statistics are well described by the theory of chaotic neutrino (Dirac) billiards. Short constrictions of only a few nm in width remain conductive and reveal a confinement gap of up to 0.5eV, which demonstrates the in-principle possibility of molecular-scale electronics based on graphene.
We calculate the density P(τ) of the eigenvalues of the Wigner-Smith time delay matrix for two-dimensional rectangular and circular billiards with one opening. For long times, the density of these so-called "proper delay times" decays algebraically, in contradistinction to chaotic quantum billiards for which P(τ) exhibits a long-time cut-off.
We perform numerical studies of the wave packet propagation through open quantum billiards whose classical counterparts exhibit regular and chaotic dynamics. We show that for t less or similar to tau (tau being the Heisenberg time), the features in the transmitted and reflected currents are directly related to specific classical trajectories connecting the billiard leads. In contrast, the long-time asymptotics of the wave packet dynamics is qualitatively different for classical and quantum billiards. In particularly, the decay of the quantum system obeys a power law that depends on the number …
We present realistic simulations of quantum confinement effects in ballistic graphene quantum dots with linear dimensions of 10 to 40 nm. We determine wavefunctions and energy level statistics in the presence of disorder resulting from edge roughness, charge impurities, or short-ranged scatterers. Marked deviations from a simple Dirac billiard for massless fermions are found. We find a remarkably stable dependence of the nearest-neighbor level spacing on edge roughness suggesting that the roughness of fabricated devices can be potentially characterized by the distribution of measured Coulomb b…
We present analytical and numerical results that demonstrate the presence of anomalous entanglement behavior on the Dirac Billiards. We investigate the statistical distribution of the characteristic entangled measures, focusing on the mean, on the variance and on the quantum interference terms. We show a quite distinct behavior of the Dirac Billiard compared with the non-relativist (Schrodinger) ones. Particularly, we show a very plausible Bell state and a sharp amplitude of quantum interference term on entangled electrons left from the Dirac Billiards. The results have remarkable relevance to…
In previous work we have found a regime in ballistic quantum dots where interelectron interactions can be treated asymptotically exactly as the Thouless number $g$ of the dot becomes very large. However, this work depends on some assumptions concerning the renormalization group and various properties of the dot obeying Random Matrix Theory predictions at scales of the order of the Thouless energy. In this work we test the validity of those assumptions by considering a particular ballistic dot, the Robnik-Berry billiard, numerically. We find that almost all of our predictions based on the earli…
This article reports on a joint theoretical and experimental study of the Pauli quantum-mechanical stress tensor $T_{αβ}(x,y)$ for open two-dimensional chaotic billiards. In the case of a finite current flow through the system the interior wave function is expressed as $ψ= u+iv$. With the assumption that $u$ and $v$ are Gaussian random fields we derive analytic expressions for the statistical distributions for the quantum stress tensor components $T_{αβ}$. The Gaussian random field model is tested for a Sinai billiard with two opposite leads by analyzing the scattering wave functions obtained …
We study the statistical properties of wavefunctions in a chaotic billiard that is opened up to the outside world. Upon increasing the openings, the billiard wavefunctions cross over from real to complex. Each wavefunction is characterized by a phase rigidity, which is itself a fluctuating quantity. We calculate the probability distribution of the phase rigidity and discuss how phase rigidity fluctuations cause long-range correlations of intensity and current density. We also find that phase rigidities for wavefunctions with different incoming wave boundary conditions are statistically correla…
In this work, we perform a statistical study on Dirac Billiards in the extreme quantum limit (a single open channel on the leads). Our numerical analysis uses a large ensemble of random matrices and demonstrates the preponderant role of dephasing mechanisms in such chaotic billiards. Physical implementations of these billiards range from quantum dots of graphene to topological insulators structures. We show, in particular, that the role of finite crossover fields between the universal symmetries quickly leaves the conductance to the asymptotic limit of unitary ensembles. Furthermore, we show t…
We investigate the effective field theory of a quantum chaotic billiard from a new perspective of quantum anomalies, which result from the absence of continuous spectral symmetry in quantized systems. It is shown that commutators of composite operators on the energy shell acquire anomalous part. The presence of the anomaly allows one to introduce effective dual fields as phase variables without any additional coarse-graining nor ensemble averaging in a ballistic system. The spectral Husimi function plays a role as the corresponding amplitude.
An effective random matrix theory description is developed for the universal gap fluctuations and the ensemble averaged density of states of chaotic Andreev billiards for finite Ehrenfest time. It yields a very good agreement with the numerical calculation for Sinai-Andreev billiards. A systematic linear decrease of the mean field gap with increasing Ehrenfest time $τ_E$ is observed but its derivative with respect to $τ_E$ is in between two competing theoretical predictions and close to that of the recent numerical calculations for Andreev map. The exponential tail of the density of states is …
We consider chaotic billiards in d dimensions, and study the matrix elements M_{nm} corresponding to general deformations of the boundary. We analyze the dependence of |M_{nm}|^2 on ω= (E_n-E_m)/\hbar using semiclassical considerations. This relates to an estimate of the energy dissipation rate when the deformation is periodic at frequency ω. We show that for dilations and translations of the boundary, |M_{nm}|^2 vanishes like ω^4 as ω-> 0, for rotations like ω^2, whereas for generic deformations it goes to a constant. Such special cases lead to quasi-orthogonality of the eigenstates on the bo…
A semiclassical theory is developed for the appearance of an excitation gap in a ballistic chaotic cavity connected by a point contact to a superconductor. Diffraction at the point contact is a singular perturbation in the limit $\hbar\to 0$, which opens up a gap $E_{\rm gap}$ in the excitation spectrum. The time scale $\hbar/E_{\rm gap}\proptoα^{-1}\ln\hbar$ (with $α$ the Lyapunov exponent) is the Ehrenfest time, the characteristic time scale of quantum chaos.
Quantum cavities or dots have markedly different properties depending on whether their classical counterparts are chaotic or not. Connecting a superconductor to such a cavity leads to notable proximity effects, particularly the appearance, predicted by random matrix theory, of a hard gap in the excitation spectrum of quantum chaotic systems. Andreev billiards are interesting examples of such structures built with superconductors connected to a ballistic normal metal billiard since each time an electron hits the superconducting part it is retroreflected as a hole (and vice-versa). Using a semic…
This is a review of recent advances in our understanding of how Andreev reflection at a superconductor modifies the excitation spectrum of a quantum dot. The emphasis is on two-dimensional impurity-free structures in which the classical dynamics is chaotic. Such Andreev billiards differ in a fundamental way from their non-superconducting counterparts. Most notably, the difference between chaotic and integrable classical dynamics shows up already in the level density, instead of only in the level--level correlations. A chaotic billiard has a gap in the spectrum around the Fermi energy, while in…
The persistent current of ballistic chaotic billiards is considered with the help of the Gutzwiller trace formula. We derive the semiclassical formula of a typical persistent current $I^{typ}$ for a single billiard and an average persistent current $<I>$ for an ensemble of billiards at finite temperature. These formulas are used to show that the persistent current for chaotic billiards is much smaller than that for integrable ones. The persistent currents in the ballistic regime therefore become an experimental tool to search for the quantum signature of classical chaotic and regular dynamics.
The stability properties of the classical trajectories of charged particles are investigated in a two dimensional stadium-shaped inverse magnetic domain, where the magnetic field is zero inside the stadium domain and constant outside. In the case of infinite magnetic field the dynamics of the system is the same as in the Bunimovich billiard, i.e., ergodic and mixing. However, for weaker magnetic fields the phase space becomes mixed and the chaotic part gradually shrinks. The numerical measurements of the Lyapunov exponent (performed with a novel method) and the integrable/chaotic phase space v…
The quantum dynamics of a chaotic billiard with moving boundary is considered in this work. We found a shape parameter Hamiltonian expansion which enables us to obtain the spectrum of the deformed billiard for deformations so large as the characteristic wave length. Then, for a specified time dependent shape variation, the quantum dynamics of a particle inside the billiard is integrated directly. In particular, the dispersion of the energy is studied in the Bunimovich stadium billiard with oscillating boundary. The results showed that the distribution of energy spreads diffusively for the firs…
We investigate the Schrödinger (non-relativistic) and the Dirac (``relativistic") billiards in the universal regime. The study is based on a non-ideal quantum resonant scattering numerical simulation. We show universal results that reveal anomalous behavior on the conductance, on the shot-noise power and on the respective eigenvalues distributions. In particular, we demonstrate the Klein's paradox in the graphene and tunable suppression/amplification transitions on the typical observables of the quantum dots.
The connection of a superconductor to a chaotic ballistic quantum dot leads to interesting phenomena, most notably the appearance of a hard gap in its excitation spectrum. Here we treat such an Andreev billiard semiclassically where the density of states is expressed in terms of the classical trajectories of electrons (and holes) that leave and return to the superconductor. We show how classical orbit correlations lead to the formation of the hard gap, as predicted by random matrix theory in the limit of negligible Ehrenfest time $\tE$, and how the influence of a finite $\tE$ causes the gap to…
We investigate the local electronic structure of a Sinai-like, quadrilateral graphene quantum billiard with zigzag and armchair edges using scanning tunneling microscopy at room temperature. It is revealed that besides the $(\sqrt{3}\times\sqrt{3})R30$° superstructure, which is caused by the intervalley scattering, its overtones also appear in the STM measurements, which are attributed to the Umklapp processes. We point out that these results can be well understood by taking into account the Coulomb interaction in the quantum billiard, accounting for both the measured density of state values a…
We investigate the properties of eigenstates and local density of states (LDOS) for a periodic 2D rippled billiard, focusing on their quantum-classical correspondence in energy representation. To construct the classical counterparts of LDOS and the structure of eigenstates (SES), the effects of the boundary are first incorporated (via a canonical transformation) into an effective potential, rendering the one-particle motion in the 2D rippled billiard equivalent to that of two-interacting particles in 1D geometry. We show that classical counterparts of SES and LDOS in the case of strong chaotic…
We report on the experimental realization of a flat, superconducting microwave resonator, a microwave billiard, with partially violated time-reversal (T ) invariance, induced by inserting a ferrite into the cavity and magnetizing it with an external magnetic field perpendicular to the resonator plane. In order to prevent its expulsion caused by the Meissner-Ochsenfeld effect we used a cavity of which the top and bottom plate were made from niobium, a superconductor of type II, and cooled it down to liquid-helium temperature T LHe ' 4 K. The Cavity had the shape of a chaotic Afrivca billiard. S…
When a quantum-chaotic normal conductor is coupled to a superconductor, random-matrix theory predicts that a gap opens up in the excitation spectrum which is of universal size $E_g^{\rm RMT}\approx 0.3 \hbar/t_D$, where $t_D$ is the mean scattering time between Andreev reflections. We show that a scarred state of long lifetime $t_S\gg t_D$ suppresses the excitation gap over a window $ΔE\approx 2 E_g^{\rm RMT}$ which can be much larger than the narrow resonance width $Γ_S=\hbar/t_S$ of the scar in the normal system. The minimal value of the excitation gap within this window is given by $Γ_S/2\l…
Thermodynamic Uncertainty Relations in Chaotic Andreev Billiards
Universidade Estadual Paulista（圣保罗州立大学）；Laboratório Nacional de Luz Síncrotron, Centro Nacional de Pesquisa em Energia e Materiais（巴西国家同步辐射光源实验室，国家能源与材料研究中心）；Universidade Federal da Paraíba（帕拉伊巴联邦大学）
We investigate statistical aspects of the entanglement production for open chaotic mesoscopic billiards in contact with superconducting parts, known as Andreev billiards. The complete distributions of concurrence and entanglement of formation are obtained by using the Altland-Zirnbauer symmetry classes of circular ensembles of scattering matrices, which complements previous studies in chaotic universal billiards belonging to other classes of random matrix theory. Our results show a unique and very peculiar behavior: the realization of entanglement in a Andreev billiard always results in non-se…
Using the supersymmetry technique, we calculate the joint distribution of local densities of electron wavefunctions in two coupled disordered or chaotic quantum billiards. We find novel spatial correlations that are absent in a single chaotic system. Our exact result can be interpreted for small coupling in terms of the hybridization of eigenstates of the isolated billiards. We show that the presented picture is universal, independent of microscopic details of the coupling.
We consider two particles hopping on a chain with a contact interaction between them. At strong interaction, there is a molecular bound state separated by a direct gap from a continuous band of atomic states. Introducing weak disorder in the interaction, the molecular state becomes Anderson localized. At stronger disorder, part of the molecular band delocalizes and dissociates due to its hybridization to the atomic band. We characterize these different regimes by computing the density of states, the inverse participation ratio, the level-spacing statistics and the survival probability of an in…
Conductance fluctuations have been studied in a soft wall stadium and a Sinai billiard defined by electrostatic gates on a high mobility semiconductor heterojunction. These reproducible magnetoconductance fluctuations are found to be fractal confirming recent theoretical predictions of quantum signatures in classically mixed (regular and chaotic) systems. The fractal character of the fluctuations provides direct evidence for a hierarchical phase space structure at the boundary between regular and chaotic motion.
Recent works have established universal entanglement properties and demonstrated validity of single-particle eigenstate thermalization in quantum-chaotic quadratic Hamiltonians. However, a common property of all quantum-chaotic quadratic Hamiltonians studied in this context so far is the presence of random terms that act as a source of disorder. Here we introduce tight-binding billiards in two dimensions, which are described by non-interacting spinless fermions on a disorder-free square lattice subject to curved open (hard-wall) boundaries. We show that many properties of tight-binding billiar…
We study matrix element fluctuations of the two-body screened Coulomb interaction and of the one-body surface charge potential in ballistic quantum dots, comparing behavior in actual chaotic billiards with analytic results previously obtained in a normalized random wave model. We find that the matrix element variances in actual chaotic billiards typically exceed by a factor of 3 or 4 the predictions of the random wave model, for dot sizes commonly used in experiments. We discuss dynamical effects that are responsible for this enhancement. These dynamical effects have an even more striking effe…
We present a computational scheme based on classical molecular dynamics to study chaotic billiards in static external magnetic fields. The method allows to treat arbitrary geometries and several interacting particles. We test the scheme for rectangular single-particle billiards in magnetic fields and find a sequence of regularity islands at integer aspect ratios. In the case of two Coulomb-interacting particles the dynamics is dominated by chaotic behavior. However, signatures of quasiperiodicity can be identified at weak interactions, as well as regular trajectories at strong magnetic fields.…
The elastic mean free path of carriers in a recently introduced model of quantum chaotic billiards in two and three dimensions is calculated. The model incorporates surface roughness at a microscopic scale by randomly choosing the atomic levels at the surface sites between -W/2 and W/2. Surface roughness yields a mean free path l that decreases as L/W^2 as W increases, L being the linear size of the system. But this diminution ceases when the surface layer begins to decouple from the bulk for large enough values of W, leaving more or less unperturbed states on the bulk. Consequently, the mean …
We study quantum localization phenomena in chaotic systems with a parameter. The parametric motion of energy levels proceeds without crossing any other and the defined avoided crossings quantify the interaction between states. We propose the elimination of avoided crossings as the natural mechanism to uncover localized structures. We describe an efficient method for the elimination of avoided crossings in chaotic billiards and apply it to the stadium billiard. We find many scars of short periodic orbits revealing the skeleton on which quantum mechanics is built. Moreover, we have observed stro…
